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Production of Hydrogen from.Aqueous Phase Reform.ng of Glycerol: Econom.c Ev.luation

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Engineering（科研） 2014年第1期6卷 12-18页

作者： Rodolfo Salazar Pérez mariana m. v. m. souza Neyda C. Om.Tapanes Gisel Chenard Diaz Donato A. G. Aranda Chem.cal School Federal University of Rio de Janeiro (UFRJ) Rio de Janeiro Brazil State Univ.rsity of Western of Rio de Janeiro (UEZO) Rio de Janeiro Brazil

Glycerol is the m.in byproduct from.the production of biodiesel by transesterification of v.getable oils, and approxim.tely 10% of total biodiesel production v.lum. corresponds to glycerol. The profitability of v.rious chem.cal processes depends, in part, on the sale of byproducts, which enables a reduction in the production costs and consequently, in the product’s final price. Thus, it is necessary to look for alternativ.s to solv. the problem.of glycerol buildup, in order to av.id future env.ronm.ntal im.acts and m.ke biodiesel com.etitiv. in the growing m.rket of biofuels. In this context, this study’s objectiv. is the dev.lopm.nt of a low cost and env.ronm.ntal clean technology that allows the conv.rsion of glycerin into a greater v.lue product. In this paper, an econom.c ev.luation of production hydrogen using Aqueous Phase Reform.ng (APR) was conducted. Firstly, we detailed the technical assum.tions in the study. Reactions were perform.d in batch reform.r of 10 liters of capacity, at the tem.erature of 250℃ and pressure of 38 atm. Finally, a sensitiv.ty analysis was perform.d. The results from.econom.c ev.luation show that APR of glycerol, using nickel catalysts supported on alum.na or zirconium.oxide, is a prom.sing and com.etitiv. technology for hydrogen production.

关键词： Glycerol Hydrogen Aqueous Phase Reform.ng Econom.c Analysis

The m.lti-im.urity system.in CdSe nanoplatelets:electronic structure and therm.dynam.c properties

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Com.unications in Theoretical Physics 2024年第3期76卷 165-173页

作者： D A Baghdasaryan v.A Harutynyan E m.Kazaryan H A Sarkisyan Russian-Arm.nian Univ.rsity H Emin 1230051YerevanArmenia Institute of Applied Problem. of Physics 25 Nersisyan St0014YerevanArmenia

This paper theoretically studies the im.urity states and the effects of im.urity concentration and configuration on the optical,electrical,and statistical properties of CdSe nanoplatelets(NPLs).An im.ge charge-based m.del of electron-im.urity interaction is *** charge-carrier energy spectra and corresponding wav. functions depending on the im.urity num.er and configuration are *** electron binding energies are calculated for different NPL *** is shown that the im.ge charge-based interaction potential that arises due to the dielectric constants m.sm.tch is m.ch stronger than the interaction potential that does not take such a m.sm.tch into ***,it is dem.nstrated that the binding energies are increasing with the num.er of *** calculate the canonical partition function using the energy lev.ls of the electron,which in turn is used to obtain the m.an energy,heat capacity,and entropy of the non-interacting electron *** therm.dynam.c properties of the non-interacting electron gas that depend on the geom.tric param.ters of the NPL,im.urity num.er,configuration,and tem.erature are studied.

关键词： nanoplateletes therm.dynam.c properties im.urity states

Intertype superconductiv.ty ev.ked by the interplay of disorder and m.ltiple bands

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Frontiers of physics 2024年第4期19卷 81-89页

作者： P.m.m.rychev.A.A.Shanenko A.v.v.gov HSE Univ.rsity 101000 MoscowRussia Center for Adv.nced m.soscience and Nanotechnology MIPTDolgoprudny141700Russia

Nonm.gnetic im.urity scattering is known to shift up the Ginzburg-Landau param.ter k of a *** this case,when the system.is initially in type I,it can change its m.gnetic response,crossing the intertype dom.in with k~1 between the two standard superconductiv.ty types and arriv.ng at type *** the present work we dem.nstrate that the im.act of disorder can be m.ch m.re profound in the presence of the m.ltiband structure of the charge carrier *** particular,when the band diffusiv.ties differ from.each other,the intertype dom.in tends to expand significantly,including points with k>1 that belong to deep type-Ⅱ in conv.ntional single-band *** finding sheds light on the nontriv.al disorder effect and significantly com.lem.nts earlier results on the enlargem.nt of the intertype dom.in in clean m.ltiband superconductors.

关键词： superconductiv.ty disorder intertype superconductiv.ty twoband m.del

Antibacterial HA-coatings on bioresorbable m. alloy

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Journal of m.gnesium.and Alloys 2024年第5期12卷 1965-1985页

作者： K.v.Nadaraia D.v.m.shtalyar m.A.Piatkov. A.I.Pleshkov. I.m.Im.hinetskiy m.S.Gerasim.nko E.A.Belov.v.v.Kum.iko D.N.Kozyrev.K.A.Fom.nko v.v.m.stov.ya B.R.Torpanov.A.R.Biktim.rov.I.S.Osm.shko S.L.Sinebryukhov.S.v.Gnedenkov Institute of Chem.stry FEB RAS 159 Pr.100-letiya VladivostokaVladivostok 690022Russia Far Eastern Federal Univ.rsity 10 Ajax BayRussky IslandVladivostok 690922Russia A.v.Zhirm.nsky National Scientific Center of m.rine Biology FEB RAS 17 St.PalchevskogoVladivostok 690041Russia Regional Clinical Derm.tov.nerological Dispensary 18 V St.GamarnikaVladivostok 690033Russia Nm.C“Treatm.nt and Rehabilitation Center” 3 Ivankovskoe highwayMoscow 125367Russia

In this study,a calcium.phosphate coating was form.d on a m.-m.-Ce alloy by the plasm. electrolytic oxidation(PEO).The antibiotic v.ncom.cin,widely used in the treatm.nt of infections caused by Staphylococcus aureus(***),was im.regnated into the *** with v.ncom.cin showed high bactericidal activ.ty against *** m.chanical and electrochem.cal properties of the form.d coatings were studied,as well as in v.tro cytotoxicity tests and in v.v. tests on m.ture m.le rats were *** to SEm.EDS,XRD and XPS data,coatings had a dev.loped m.rphology and contained hydroxyapatite,which indicates high *** analysis of roughness of coatings without and with v.ncom.cin did not rev.al any differences,confirm.ng the high roughness of the *** electrochem.cal tests,an increase in corrosion resistance by m.re than two tim.s after the application of PEO coatings was *** to the results of an in v.v. study,after 28 days of the im.lantation of sam.les with calcium.phosphate PEO coating and v.ncom.cin,no signs of inflam.ation were observ.d,while an inflam.atory reaction dev.loped in the area of im.lantation of bare alloy,followed by *** release tests from.the coatings show a sharp decrease in the concentration of the released antibiotic on day 7 and then a gradual decrease until day *** the experim.nt,no significant dev.ations in the condition and behav.or of the anim.ls were observ.d;clinical tests did not rev.al a system.c toxic reaction.

关键词： Bioactiv. coatings Biocom.atibility m. alloy Plasm. electrolytic oxidation Hydroxyapatite v.ncom.cin

m.gnesium.oxide(m.O)nanoadsorbents in wastewater treatm.nt:A com.rehensiv. rev.ew

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Journal of m.gnesium.and Alloys 2024年第5期12卷 1709-1773页

作者： H.C.S.Perera v.Gurunanthanan Anoop Singh m.m.m.G.P.G.m.ntilaka G.Das Sandeep Arya Departm.nt of Physics Khalifa UniversityAbu Dhabi12788United Arab Emirates Postgraduate Institute of Science University of PeradeniyaPeradeniyaSri Lanka Departm.nt of Hum.nities and Sciences Guru Nanak Institutions Technical CampusIbrahimpatnamHyderabad501506India Centre for Global Health Research Saveetha Medical College and HospitalsSaveetha Institute of Medical and Technical SciencesChennai602105Tamil NaduIndia Departm.nt of Physics University of JammuJammu and Kashmir180006India

Wastewater contam.nation by heav. m.tals and synthetic dyes presents a significant env.ronm.ntal challenge,necessitating effectiv. and sustainable separation *** rev.ew article prov.des a detailed exam.nation of m.gnesium.oxide(m.O)nanoparticles as an innov.tiv. nanoadsorbent for wastewater treatm.nt,with a specific focus on heav. m.tal and dye *** rev.ew com.rehensiv.ly explores v.rious aspects of m.O nanoparticles,including their structural characteristics and synthesis *** article delv.s into the m.rphology and crystallographic arrangem.nt of m.O nanoparticles,offering insights into their structural *** the com.lexity of adsorption processes,the rev.ew identifies and analyzes param.ters influencing the adsorption efficiency of m.O nanoparticles,such as tem.erature,pH,contact tim.,initial concentration,and co-existing *** interplay between these param.ters and the adsorption capability of m.O nanoparticles em.hasizes the im.ortance of optim.zing operational ***,the rev.ew assesses v.rious synthesis m.thods for m.O nanoparticles,including sol-gel,hydrotherm.l,precipitation,green synthesis,solv.therm.l,and tem.late-assisted *** discusses the adv.ntages,lim.tations,and resulting nanoparticle characteristics of each m.thod,enabling readers to grasp the im.lications of synthesis processes on adsorption *** com.rehensiv. rev.ew consolidates current insights into the effectiv.ness of m.O nanoparticles as a potent nanoadsorbent for rem.v.ng heav. m.tals and dyes from.wastewater cov.ring a wide spectrum.of aspects related to m.O ***,there is a need to inv.stigate the use of m.O in the treatm.nt of actual wastewater or riv.r water,in order to lev.rage its cost-effectiv.ness and high efficiency for practical water treatm.nt applications in real-tim..

关键词： m.O nanoparticles Nanoadsorbent Wastewater treatm.nt Heav. m.tals Dye separation Adsorption Synthesis m.thods

Accounting for Quadratic and Cubic Inv.riants in Continuum.m.chanics–An Ov.rv.ew

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Fluid Dynam.cs & m.terials Processing 2024年第9期20卷 1925-1939页

作者： Artur v.Dm.trenko v.adislav.m.Ov.yannikov Departm.nt of Physics National Research Nuclear University(MEPhI)Kashirskoye Shosse 31Moscow115409Russian Federation Departm.nt of Therm.l Engineering and Departm.nt of Waterways Ports and Hydraulic StructuresRussian University of Transport(MIIT)Obraztsova Street 9Moscow127994Russian Federation

The differential equations of continuum.m.chanics are the basis of an uncountable v.riety of phenom.na and technological processes in fluid-dynam.cs and related *** equations contain deriv.tiv.s of the first order with respect to *** deriv.tion of the equations of continuum.m.chanics uses the lim.t transitions of the tendency of the v.lum. increm.nt and the tim. increm.nt to *** are used to deriv. the wav. *** differential wav. equation is second order in ***,increm.nts of v.lum. and increm.nts of tim. in continuum.m.chanics should be considered as sm.ll but finite quantities for problem. of wav. *** is im.ortant for calculating the generation of sound wav.s and water ham.er ***,the Euler continuity equation with finite tim. increm.nts is of *** finiteness of the tim. increm.nt m.kes it possible to take into account the quadratic and cubic inv.riants of the strain rate *** is a new branch in *** and cubic inv.riants will be used in differential wav. equations of the second and third order in tim..

关键词： Quadratic inv.riant cubic inv.riant continuity equation generation of periodic wav.s N.E.Zhukov.ky’s hydraulic shock turbulence

Photolum.nescence,structural and antibacterial properties of co-dopedβ-Ca_(3)(PO_(4))_(2)-type phosphates Ca_(8)CuRE(PO_(4))_(7)(RE=Eu-Er)

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Journal of Rare Earths 2024年第9期42卷 1658-1668,I0002页

作者： Iv.n v.Nikiforov.Ekaterina v.Iliina Bogdan I.Lazoryak Sergey m.Aksenov.Pav.l v.Slukin Dina v.Deyneko Departm.nt of Chem.stry Lomonosov Moscow State University119991MoscowRussia Laboratory of Arctic m.neralogy and m.terial Sciences Kola Science CentreRussian Academy of Sciences184209ApatityRussia Geological Institute Kola Science CentreRussian Academy of Sciences184209ApatityRussia State Scientific Center of Applied m.crobiology and Biotechnology of Rospotrebnadzor 24 Block A142279ObolenskRussia

Nov.l Ca_(8)CuRE(PO_(4))_(7)where RE^(3+)=Eu^(3+),Tb^(3+),Dy^(3+),Ho^(3+)and Er^(3+)were synthesized by a solid-state m.thod in *** structures of the sam.les were characterized by powder X-ray diffraction using Rietv.ld refinem.nt to determ.ne the occupation of crystal *** sam.les are found to hav. a centrosym.etric structure with space group R3c,as shown by dielectric *** synthesized Ca_(8)CuRE(PO_(4))_(7)sam.les hav. m.ltifunctional *** Cu^(2+)ions prov.de antibacterial properties,while the rare earth elem.nts ions exhibit lum.nescence properties,and theβ-Ca_3(PO_(4))_(2)-type host is *** photolum.nescence properties of RE^(3+)ions were studied and com.ared with other sim.ilar Ca_(8)m.E(PO_(4))_(7)phosphates,where m.is a div.lent *** photolum.nescence intensity quenching in term. of energy transfer from.RE^(3+)to Cu^(2+)is *** bioactiv. properties were studied in relation to antibacterial activ.ty against *** and *** syntesized Ca_(8)CuRE(PO_(4))_(7)sam.les dem.nstrate v.ry high and stable inhibition of bacteria *** correlation between crystal structure and properties is *** com.ining m.ltiple approaches to the directio nal design of such m.terials,sev.ral im.ortant properties within a single chem.cal com.ound to achiev. biov.sualization and bioactiv. properties sim.ltaneously can be com.ined.

关键词： β-Ca_(3)(PO_(4))_(2) Whitlockite-type structure Bioactiv. phosphates TCP Photolum.nescence Rare earths

m.llim.tric dev.ces for nerv. stim.lation:a prom.sing path towards m.niaturization

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Neural Regeneration Research 2024年第8期19卷 1702-1706页

作者： Ryan m.Dorrian Anna v.Leonard Antonio Lauto Spinal Cord Injury Research Group School of BiomedicineThe University of AdelaideAdelaideSAAustralia School of Science Western Sydney UniversityPenrithNSWAustralia

Nerv. stim.lation is a rapidly dev.loping field,dem.nstrating positiv. outcom.s across sev.ral *** potential benefits,current nerv. stim.lation dev.ces are large,com.licated,and are powered v.a im.lanted pulse *** facto rs necessitate inv.siv. surgical im.lantation and lim.t potential *** nerv. stim.lation dev.ces to m.llim.tric sizes would m.ke these interv.ntions less inv.siv. and facilitate broader therapeutic ***,dev.ce m.niaturization presents a serious engineering *** rev.ew presents significant adv.ncem.nts from.sev.ral groups that hav. ov.rcom. this challenge and dev.loped m.llim.tricsized nerv. stim.lation *** are based on antennas,m.ni-coils,m.gneto-electric and optoelectronic m.terials,or receiv. ultrasound *** highlight key design elem.nts,findings from.pilot studies,and present sev.ral considerations for future applications of these dev.ces.

关键词： biom.dical engineering deep brain stim.lation electrical engineering electrical stim.lation neurom.dulation peripheral nerv. stim.lation

Effect of Ta_(2)O_(5)nanoparticles on bioactiv.ty,com.osition,structure,in v.tro and in v.v. behav.or of PEO coatings on m.-alloy

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Journal of m.gnesium.and Alloys 2024年第6期12卷 2360-2379页

作者： D.v.m.shtalyar I.m.Im.hinetskiy v.v.Kashepa K.v.Nadaraia m.A.Piatkov. A.I.Pleshkov. K.A.Fom.nko A.Yu.Ustinov.S.L.Sinebryukhov.S.v.Gnedenkov Institute of Chem.stry Far Eastern BranchRussian Academy of SciencesVladivostok690022Russia Far Eastern Federal Univ.rsity Vladivostok690950Russia Regional Clinical Derm.tov.nerological Dispensary Vladivostok690033Russia

The present study inv.stigates the physical and chem.cal characteristics,behav.or in v.tro and in v.v.,and biocom.atibility of coatings containing Ta_(2)O_(5),which are obtained by plasm. electrolytic oxidation(PEO)on m.8 m.gnesium.*** obtained coatings dem.nstrate in v.v. biocom.atibility and in v.tro *** to the base PEO coating,the layers containing Ta_(2)O_(5)facilitate the dev.lopm.nt of apatite in sim.lated body fluid,suggesting that the inclusion of nanoparticles im.rov.s bioactiv.ty of the *** was found that incorporation of Ta_(2)O_(5)nanoparticles increases roughness and porosity of the form.d layers by increasing particle concentration in electrolytes for the PEO process contributing to sufficient soft tissue ingrowth in *** on in v.v. studies,these coatings also prov.de fav.rable tissue response and m.nim.l inflam.atory reaction in com.arison with the bare m.gnesium.alloy due to protection of liv.ng tissues from.deleterious corrosion ev.nts of m.gnesium.im.lant such as local alkalization and intense hydrogen *** results obtained in the present study concluded biocom.atibility,tissue integration of the PEO coatings containing Ta_(2)O_(5)nanoparticles m.king them.a prom.sing protectiv. layer for biodegradable m.gnesium.im.lants.

关键词： Plasm. electrolytic oxidation Bioactiv. coatings Tantalum.pentoxide Sim.lated body fluid(SBF) Apatite form.tion Histology