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large ferro-pyro-phototronic effect in 0.5Ba(Zr_(0.2)Ti_(0.8))O_(3)-0.5(Ba_(0.7)Ca_(0.3))TiO_(3)thin films integrated on silicon for photodetection

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Carbon Energy 2023年第6期5卷 1-10页

作者： JoséP.B.Silva Katarzyna Gwozdz luís S.Marques Mario Pereira maria J.M.Gomes Judith l.MacManus‐Driscoll Robert l.Z.Hoye Centre of Physics of Universities of Minho and Porto(CF‐UM‐UP) University of MinhoBragaPortugal laboratory of Physics for Materials and Emergent Technologies LapMETUniversity of MinhoBragaPortugal Department of Quantum Technologies Faculty of Fundamental Problems of TechnologyWroclaw University of Science and TechnologyWroclawPoland Department of Materials Science and Metallurgy CambridgeUK Inorganic Chemistry laboratory Department of ChemistryUniversity of OxfordOxfordUK Department of Materials Imperial College LondonLondonUK

Coupling together the ferroelectric,pyroelectric,and photovoltaic characteristics within a single material is a novel way to improve the performance of *** this work,we take advantage of the triple multifunctionality shown by 0.5Ba(Zr_(0.2)Ti_(0.8))O_(3)-0.5(Ba_(0.7)Ca_(0.3))TiO_(3)(BCZT),as demonstrated in an Al/Si/SiOx/BCZT/ITO thin-film *** Si/SiOx acts as an n-type layer to form a metal-ferroelectric-insulator-semiconductor heterostructure with the BCZT,and with Al and ITO as *** photo-response of the device,with excitation from a violet laser(405 nm wavelength),is carefully investigated,and it is shown that the photodetector performance is invariant with the chopper frequency owing to the pyro-phototronic effect,which corresponds to the coupling together of the pyroelectric and photovoltaic ***,the photodetector performance was significantly better than that of the devices operating based only on the pyro-phototronic effect by a factor of 4,due to the presence of ferroelectricity in the ***,after a poling voltage of−15 V,for a laser power density of 230mW/cm^(2)and at a chopper frequency of 400Hz,optimized responsivity,detectivity,and sensitivity values of 13.1mA/W,1.7×10^(10)Jones,and 26.9,respectively,are ***,ultrafast rise and fall times of 2.4 and 1.5μs,respectively,are obtained,which are 35,000 and 36,000 times faster rise and fall responses,respectively,than previous reports of devices with the ferro-pyro-phototronic *** is understood based on the much faster ferroelectric switching in ferroelectric thin films owing to the predominant 180°domains in a single direction out of plane.

关键词： ferroelectric ferro-pyro-phototronic effect photodetector polarization-controlled response

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Micro-arc oxidation of magnesium alloys:A review

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Journal of Materials Science & Technology 2022年第23期118卷 167-189页

作者： Wenhui Yao liang Wu Jingfeng Wang Bin Jiang Dingfei Zhang maria Serdechnova Tatsiana Shulha Carsten Blawert Mikhail l.Zheludkevich Fusheng Pan College of Materials Science and Engineering Chongqing UniversityChongqing 400044China National Engineering Research Center for Magnesium Alloys Chongqing UniversityChongqing 400044China Institute of Surface Science Helmholtz-Zentrum HereonMax-Planck Str.1Geesthacht 21502Germany Institute of Materials Science Faculty of EngineeringCAU Kiel UniversityKaiser Str.2Kiel 24143Germany

Magnesium(Mg)and its alloys present great potential to be extensively applied in different ***,the relatively poor resistance to corrosion and wear significantly restricts their applications in *** one of strategies of surface treatment,micro-arc oxidation(MAO)process attracts a lot of attention,since it does not use neither expensive equipment,nor complicated *** review systematically discusses MAO mechanism and some typical models,which still need to be further developed to provide a better understanding and guide for future ***,main influencing factors of MAO process are analyzed in ***,some popular applications of MAO coatings are respectively reviewed,including biomedical application,decoration,thermal control,corrosion and wear resistance,and industrial applications in *** existing issues and future perspectives are finally discussed to further accelerate extensive applications of Mg alloys.

关键词： Micro-arc oxidation Magnesium alloys Review Main MAO applications Existing issues and future perspective

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A DNA sensor based on upconversion nanoparticles and two-dimensional dichalcogenide materials

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Frontiers of Chemical Science and Engineering 2021年第4期15卷 935-943页

作者： Konstantina Alexaki Davide Giust maria-Eleni Kyriazi Afaf H.El-Sagheer Tom Brown Otto l.Muskens Antonios G.Kanaras School of Physics and Astronomy Faculty of Engineering and Physical SciencesUniversity of SouthamptonSouthampton SO171BJUK Department of Chemistry University of OxfordChemistry Research LaboratoryOxford OX13TAUK Chemistry Branch Department of Science and MathematicsFaculty of Petroleum and Mining EngineeringSuez UniversitySuez 43721Egypt Institute for life Sciences University of SouthamptonSouthampton SO171BJUK

We demonstrate the fabrication of a new DNA sensor that is based on the optical interactions occurring between oligonucleotide-coated NaYF4:Yb^(3+);Er^(3+) upconversion nanoparticles and the two-dimensional dichalcogenide materials,MoS_(2) and WS_(2).Monodisperse upconversion nanoparticles were functionalized with single-stranded DNA endowing the nanoparticles with the ability to interact with the surface of the two-dimensional materials via van der Waals interactions leading to subsequent quenching of the upconversion *** contrast,in the presence of a complementary oligonucleotide target and the formation of double-stranded DNA,the upconversion nanoparticles could not interact with MoS_(2) and WS_(2),thus retaining their inherent fluorescence *** this sensor we were able to detect target oligonucleotides with high sensitivity and specificity whilst reaching a concentration detection limit as low as 5 mol·l^(-1),within minutes.

关键词： upconversion nanoparticles DA sensor two-dimensional materials MoS_(2) WS_(2)

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Predetermination of potential plastic hinges on reinforced concrete frames using GFRP reinforcement

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Frontiers of Structural and Civil Engineering 2022年第5期16卷 624-637页

作者： Dominik KUERES Dritan TOPUZI maria Anna POlAK Department of Civil and Environmental Engineering University of WaterlooWaterlooON N2L 3G1Canada Schoeck Canada Inc. OttawaON K1P 5G3Canada

In the past,glass fiber-reinforced polymer(GFRP)-reinforcement has been successfully applied in reinforced concrete(RC)structures where corrosion resistance,electromagnetic neutrality,or cuttability were *** investigations suggest that the application of GFRP in RC structures could be advantageous in areas with seismic activity due to their high deformability and ***,especially the low modulus of elasticity of GFRP limited its wide application as GFRP-reinforced members usually exhibit considerably larger deformations under service loads than comparable steel-reinforced *** overcome the aforementioned issues,the combination of steel and GFRP reinforcement in hybrid RC sections has been investigated in the *** on this idea,this paper presents a novel concept for the predetermination of potential plastic hinges in RC frames using GFRP *** analyze the efficiency of the concept,nonlinear finite element simulations were *** results underscore the high efficiency of hybrid steel-GFRP RC sections for predetermining potential plastic hinges on RC *** results also indicate that the overall seismic behavior of RC structures could be improved by means of GFRP as both the column base shear force during the seismic activity as well as the plastic deformations after the earthquake were considerably less pronounced than in the steel-reinforced reference structure.

关键词： glass fiber-reinforced polymer GFRP hybrid section plastic hinge seismic design reinforced concrete

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How many subductions in the Variscan orogeny?Insights from numerical models

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Geoscience Frontiers 2020年第3期11卷 1025-1052页

作者： Alessandro Regorda Jean-Marc lardeaux Manuel Roda Anna maria Marotta maria Iole Spalla Universita Degli Studi di Milano Dipartimento di Scienze Della Terra'A.Desio’Via Mangiagalli 34I-20133MilanoItaly Universite Nice Sophia-Antipolis UMR Geoazur250 Rue A.EinsteinSophia-Antipolis06560ValbonneFrance

We developed a 2 D numerical model to simulate the evolution of two superposed ocean-continent-ocean subduction cycles with opposite vergence,both followed by continental collision,aiming to better understand the evolution of the Variscan *** models with different velocities of the first oceanic subduction have been *** differences in the thermo-mechanical evolution between the first subduction,which activates in an unperturbed system,and the second subduction,characterised by an opposite vergence,have been enlighten,in particular regarding the temperature in the mantle wedge and in the interior of the *** and temperature(P-T) conditions predicted by one cycle and two cycles models have been compared with natural P-T estimates of the Variscan metamorphism from the Alps and from the French Massif Central(FMC).The comparative analysis supports that a slow and hot subduction well reproduces the P-T conditions compatible with data from the FMC,while P-T conditions compatible with data of Variscan metamorphism from the Alps can be reproduced by either a cold or hot oceanic subduction *** the agreement of both double and single subduction models with natural P-T estimates,we observed that polycyclic models better describe the evolution of the Variscan orogeny.

关键词： Alps Double subduction French Massif Central Numerical modelling Variscan orogeny

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Physics, chemistry, and Hirshfeld surface analyses of gamma-irradiated thalidomide to evaluate behavior under sterilization doses

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Journal of Pharmaceutical Analysis 2018年第3期8卷 194-201页

作者： Valner A.F.S.N.Mussel Max R Ferreira maria B.E Marques maria I.Yoshida mariana R.Almeida Bernardo l.Rodrigues Wagner N.Mussel Departamento de Quimica ICExUniversidade Federal de Minas Gerais-UFMGAv.Antonio Carlos 662731270-901 Belo HorizonteMGBrazil CNEN-CDTN Comissao Nacional de Energia Nuclear-Centro de Desenvolvimento da Tecnologia NuclearAv.Antonio Carlos6627 Belo HorizonteMGBrazil

Thalidomide was indicated as a sedative and antiemetic and prescribed for pregnant women. Its tragic teratogenic effects culminated in withdrawal from the market. Since the discovery of its anti-angiogenic and anti-inflammatory actions, thalidomide has been used in the treatment of leprosy and multiple myeloma, which justify studies of its stability. We investigated the effects of irradiation of thalidomide up to 100 kGy （fourfold the usual sterilizing dose for pharmaceutics）. The polymorph of thalidomide was obtained in an isothermal experiment at 270℃. All samples underwent gamma irradiation for specific times. At different doses, decomposition of the pharmaceutical was not observed up to 100 kGy. The observed effect was angle turning between the phthalimide and glutarimide rings modulated by repulsion towards the carbonyl group, leading to a stable energetic configuration, as measured by the equilibrium in the torsion angle after irradiation. The thalidomide molecule has a center of symmetry, so a full turn starting from 57.3° will lead to an identical molecule. Further irradiation will start the process again. Samples irradiated at 30 and 100 kGy have more compact unit cells and a lower volume, which leads to an increase in the intermolecular hydrogen interaction within the unit cell, resulting in higher thermal stability for polymorph α.

关键词： Thalidomide Thermal stability Polymorphs Gamma irradiation Hirshfeld

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Thermal and microstructural characterization of a novel ductile cast iron modified by aluminum addition

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International Journal of Minerals,Metallurgy and Materials 2020年第2期27卷 190-199页

作者： Gülsah Aktas Celik maria-Ioanna TTzini Seyda Polat SHakan Atapek Gregory NHaidemenopoulos Department of Metallurgical and Materials Engineering Kocaeli UniversityKocaeli 41001Turkey laboratory of Materials Department of Mechanical EngineeringUniversity of ThessalyVolos 38334Greece Department of Mechanical Engineering Khalifa University of Science and TechnologyAbu Dhabi 127788UAE

In high-temperature applications,like exhaust manifolds,cast irons with a ferritic matrix are mostly ***,the increasing demand for higher-temperature applications has led manufacturers to use additional expensive materials such as stainless steels and Ni-resist austenitic ductile cast ***,in order to meet the demand while using low-cost materials,new alloys with improved high-temperature strength and oxidation resistance must be *** this study,thermodynamic calculations with Thermo-Calc software were applied to study a novel ductile cast iron with a composition of 3.5wt%C,4wt%Si,1wt%Nb,0‒4wt%*** designed compositions were cast,and thermal analysis and microstructural characterization were performed to validate the *** lowest critical temperature of austenite to pearlite eutectoid transformation,i.e.,A1,was calculated,and the solidification sequence was *** calculations and experimental data revealed the importance of aluminum addition,as the A1 increased by increasing the aluminum content in the alloys,indicating the possibility of utilizing the alloys at higher *** experimental data validated the transformation temperature during solidification and at the solid state and confirmed the equilibrium phases at room temperature as ferrite,graphite,and MC-type carbides.

关键词： ductile cast iron alloy design Thermo-Calc high-temperature material

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In vitro antioxidant,antilipoxygenase and antimicrobial activities of extracts from seven climbing plants belonging to the Bignoniaceae

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Journal of Integrative Medicine 2018年第4期16卷 255-262页

作者： Carola Analla Torres Cristina Marisel Perez Zamora maria Beatriz Nunez Ana maria Gonzalez laboratory of Microbiology and Pharmaceutical Technology Department of Basic and Applied SciencesNational University of Chaco AustralPresidencia Roque Saenz Pena 3700ChacoArgentina National Council for Scientific and Technical Research(CONICET) Godoy Cruz 2290Buenos Aires C1425FQBArgentina Institute of Botany of the Northeast(IBONE-CONICET) Sargento Juan Bautista Cabral 2131CorrientesArgentina

Objectives： This study aimed to evaluate the in vitro antioxidant capacity, to determine the anti-inflammatory effect due to lipoxygenase inhibition and to test the antimicrobial activity of ethanolic extracts from leaves of seven climbing species belonging to the Bignoniaceae family. These species are Adenocalyrnrna rnarginatum （Cham.） DC., Amphilophium vauthieri DC., Cuspidaria convoluta （VEIl） A. H. Gentry, Dolichandra dentata （K. Schum.） l. G. lohmann, Fridericia caudigera （S. Moore） l. G. lohmann, Fridericia chica （Bonpl.） l. G. lohmann and Tanaecium selloi （Spreng.） l. G. lohmann. Methods： The antioxidant activity was evaluated using three methods, 2,2＇-azino-bis（3-ethylbenzothiazo line-6-sulfonic acid）（ABTS）, 2,2-diphenyl-l-picrylhydrazyl （DPPH）, and ferric reducing antioxidant power. lipoxygenase-inhibiting activity was assayed spectrophotometrically; the result was expressed as percent inhibition. The antimicrobial activity was assessed using the agar disk diffusion method. Minimal inhibitory concentration （MIC） and minimal bactericidal]fungicidal concentration were also determined for each extract against 12 pathogenic bacterial strains of Staphylococcus aureus and seven fungal strains of the Candida genus. The identification of the major compounds present in the most promising extract was established by high-performance liquid chromatography-tandem mass spectrometry. Results： C convoluta, F. caudigera, and F. chica exhibited the best antioxidant activity by scavenging DPPH and ABTS~ radicals and reducing Fe3＋ ion. These extracts showed a notable inhibition of lipnxygenase. F. caudigera was found to have the lower MIC value against S. aureus strains and six Candida species. The extracts of F. caudigera and C. convoluta were active even against methicillin-resistant S. aureus. C convoluta had higher total phenol content, better antioxidant activity and superior anti- inflammatory and antimicrobial activity. The main phenolic compounds found in this extract

关键词： Cuspidaria Fridericia Antioxidants lipoxygenase Antimicrobials Herbal drugs Free radical scavengers

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The effects of temperature and resource availability on denitrification and relative N_(2)O production in boreal lake sediments

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Journal of Environmental Sciences 2016年第9期28卷 82-90页

作者： maria Myrstener Anders Jonsson Ann-Kristin Bergstrom Department of Ecology and Environmental Science Umea University90187 UmeaSweden

Anthropogenic environmental stressors（like atmospheric deposition,land use change,and climate warming） are predicted to increase inorganic nitrogen and organic carbon loading to northern boreal lakes,with potential consequences for denitrification in ***,our ability to predict effects of these changes is currently limited as northern boreal lakes have been largely neglected in denitrification *** aim of this study was therefore to assess how maximum potential denitrification and N_2O production rates,and the relationship between the two（relative N_2O production）,is controlled by availability of nitrate（NO_3^-）,carbon（C）,phosphorus（P）,and *** were performed using the acetylene inhibition technique on sediments from a small,nutrient poor boreal lake in northern Sweden in *** potential denitrification and N_2O production rates at 4°C were reached already at NO_3^-additions of 106–120 μg NO_3^-–N/l,and remained unchanged with higher NO_3 *** incubation temperatures increased maximum potential denitrification and N_2O production rates,and Q10 was somewhat higher for N_2O production（1.77） than for denitrification（1.69）.The relative N_2O production ranged between 13% and 64%,and was not related to NO_3^-concentration,but the ratio increased when incubations were amended with C and P（from a median of 16% to 27%）.Combined,our results suggests that unproductive northern boreal lakes currently have low potential for denitrification but are susceptible to small changes in NO_3 loading especially if these are accompanied by enhanced C and P availability,likely promoting higher N_2O production relative to N_2.

关键词： Acetylene NO3 Carbon DOC Nitrous oxide ratio Sediment

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Assessment of Climate Change in Nicaragua: Analysis of Precipitation and Temperature by Dynamical Downscaling over a 30-Year Horizon

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Atmospheric and Climate Sciences 2016年第3期6卷 445-474页

作者： Josep maria Solé raúl Arasa Miquel Picanyol Mª Ángeles González Anna Domingo-Dalmau Marta Masdeu Ignasi Porras Bernat Codina Technical Department Meteosim S.L. Barcelona Spain Department of Astronomy and Meteorology University of Barcelona Barcelona Spain

The present study has generated and analyzed Climate Change projections in Nicaragua for the period 2010-2040. The obtained results are to be used for evaluating and planning more resilient transport infrastructures in the next decades. This study has focused its efforts to pay attention into the effect of Climate Change on precipitation and temperature from a mean and extreme event perspective. Dynamical Downscaling approach on a 4 km resolution grid has been chosen as the most appropriate methodology for the estimation of the projected climate, being able to account for local-scale factors like complex topography or local land uses properly. We selected MPI-ESM-MR as the global climate model with the best skill scores in terms of precipitation and temperature in Nicaragua. MPI-ESM-MR was coupled to a mesoscale model. We chose WRF mesoescale model as the most appropriate regional model and we optimized their physical and dynamical options in order to minimize the model uncertainty in Nicaragua. For this, model output against the available in-situ measurements from the national meteorological station network and satellite data were compared. Climate change signal was estimated by comparing the different climate statistics calculated from a model run over an historical period, 1980-2009, with a model run over a projected period, 2010-2040. The obtained results from the projected climate show an increase of the mean temperature between 0.6°C and 0.8°C and an increase of the number of days per year with maximum daily temperatures higher than 35°C. Regarding precipitation, annual projected amounts do not change remarkably with respect to the historical period. However, significant changes in the distribution of the precipitation within the wet period (May-October) were observed. Moreover, an increment between 5% and 10% of the number of days without precipitation is expected. Finally, Intensity-Duration-Frequency (IDF) projected curves show an increment of the rainfall

关键词： WRF Climate Change Global Warming Dynamical Downscaling Precipitation Projections IDF

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