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Selective biomass conversion over novel designed tandem catalyst

Journal of Bioresources and Bioproducts 2024年第4期9卷 508-517页

作者： Fatima-Zahra Azar Achraf el Kasmi mariaánge.e. lillo-róde.as maria del Carmen román-Martínez Haichao Liu department of Inorganic Chemistry and Materials Institute Faculty of SciencesUniversity of Alicante.Alicante E-03080Spain Sustainable Materials research Center University of Mohammed Ⅵ PolytechnicBenguerir 43150Morocco Laboratory LSIA ENSAHAbdelmalek Essaadi UniversityTetouan 93030Morocco College of Chemistry and Molecular engineering Peking UniversityBeijing 100871China

Selective conversion of biomass into targeted molecules like polyols, especially, from cellulosic compounds, is being widely investigated as a sustainable process to produce biodiesel and bio- additives. The known process involves two steps, namely hydrolysis and hydrogenation. Thus, it requires two different catalytic materials or bifunctional catalysts. In this context, the present work reports a new catalytic approach based on the use of tandem catalysts, consisting of the combination of an acid solid catalyst (active for hydrolysis) and a supported metal catalyst (active for hydrogenation). Two different functionalized activated carbons and the resin Amberlyst 15 have been tested as solid acid catalysts, and ru nanoparticles supported on the original activated carbon (SA) are the metal catalyst part of the tandem. All the tested tandem catalysts exhibited higher activity than the supported ru catalyst did. The highest cellulose conversion and selectivity to sorbitol (70% and 86%, respectively) have been obtained over a novel tandem catalyst, which resulted from a physical mixture between a sulfuric acid modified SA carbon (SASu) and ru loaded SA (ru/SA), leading to a tandem catalyst (ru/SA + SASu). This novel-designed tandem catalyst is reusable. Based on tandem catalysts with a solid-solid system combination, the adopted novel- designed catalytic approach is cost-efficient and sustainable, and can be considered promising for the green production of high-added-value chemicals.

关键词： Biomass Tandem catalysts Carbon materials One-pot conversion Sustainability

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Photovoltaic energy balance estimation based on the building integration level

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建筑节能（中英文） 2023年第3期51卷 36-36页

作者： I.lillo-Bravo Anton Lopez-roman Sara Moreno-Tejera J.M.Delgado-SanchezArticle 112786

The photovoltaic module building integration level affects the module temperature and,consequently,its output *** this work,a methodology has been proposed to estimate the influence of the level of architectural photovoltaic integration on the photovoltaic energy balance with natural ventilation or with forced cooling *** developed methodology is applied for five photovoltaic module technologies(m⁃Si,p⁃Si,a⁃Si,CdTe,and CIGS)on four characteristic locations(Athens,Davos,Stockholm,and Würzburg).To this end,a photovoltaic module thermal radiation parameter,PVj,is introduced in the characterization of the PV module technology,rendering the correlations suitable for building⁃integrated photovoltaic(BIPV)applications,with natural ventilation or with forced cooling *** results show that PVj has a significant influence on the energy balances,according to the architectural photovoltaic integration and climatic ***:Photovoltaic cooling;BIPV;Photovoltaic;Ventilation;Photovoltaic integration level in building【OA】(2)Graph⁃Based methodology for Multi⁃Scale generation of energy analysis models from IFC,by Asier Mediavilla,Peru elguezabal,Natalia Lasarte,Article 112795 Abstract:Process digitalisation and automation is unstoppable in all industries,including ***,its widespread adoption,even for non⁃experts,demands easy⁃to⁃use tools that reduce technical *** to BeM(Building energy Models)workflows are a clear example,where ad⁃hoc prepared models are *** paper describes a methodology,based on graph techniques,to automate it by highly reducing the input BIM requirements found in similar approaches,being applicable to almost any *** is especially relevant in retrofitting,where reality capture tools(e.g.,3D laser scanning,object recognition in drawings)are prone to create geometry clashes and other inconsistencies,posing higher challenges for *** innovation presented is its multi⁃scale nature,e

关键词： Open BIM BeM Multiscale models Building graphs Process automation IFC gbXML energy Plus

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Fungal diversity notes 253-366:taxonomic and phylogenetic contributions to fungal taxa

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Fungal Diversity 2016年第3期78卷 1-237页

作者： Guo Jie Li Kevin D.Hyde rui Lin Zhao Sinang Hongsanan Faten Awad Abdel-Aziz Mohamed A.Abdel-Wahab Pablo Alvarado Genivaldo Alves-Silva Joseph F.Ammirati Hiran A.Ariyawansa Abhishek Baghela Ali Hassan Bahkali Michael Beug D.Jayarama Bhat Dimitar Bojantchev Thitiya Boonpratuang Timur S.Bulgakov erio Camporesi Marcela CBoro Oldriska Ceska Dyutiparna Chakraborty Jia Jia Chen K.W.Thilini Chethana Putarak Chomnunti Giovanni Consiglio Bao Kai Cui Dong Qin Dai Yu Cheng Dai Dinushani A.Daranagama Kanad Das Monika C.Dayarathne eske de Crop rafael J.V.de Oliveira Carlos Alberto Fragoso de Souza JoséIde Souza Bryn T.M.dentinger Asha J.Dissanayake Mingkwan Doilom e.ricardo Drechsler-Santos Masoomeh Ghobad-Nejhad Sean P.Gilmore Aristóteles Góes-Neto MichałGorczak Charles H.Haitjema Kalani Kanchana Hapuarachchi Akira Hashimoto Mao Qiang He John K.Henske Kazuyuki Hirayama maria J.Iribarren Subashini C.Jayasiri ruvishika S.Jayawardena Sun Jeong Jeon Gustavo H.Jerônimo Ana L.Jesus e.B.Gareth Jones Ji Chuan Kang Samantha C.Karunarathna Paul M.Kirk Sirinapa Konta eric Kuhnert ewald Langer Haeng Sub Lee Hyang Burm Lee Wen Jing Li Xing Hong Li Kare Liimatainen Diogo Xavier Lima Chuan Gen Lin Jian Kui Liu Xings Zhong Liu Zuo Yi Liu J.Jennifer Luangsa-ard robert Lücking H.Thorsten Lumbsch Saisamorn Lumyong eduardo M.Leaño Agostina V.Marano Misato Matsumura eric H.C.McKenzie Suchada Mongkolsamrit Peter e.Mortimer Thi Thuong Thuong Nguyen Tuula Niskanen Chada Norphanphoun Michelle A.O’Malley Sittiporn Parnmen Julia Pawłowska rekhani H.Perera rungtiwa Phookamsak Chayanard Phukhamsakda Carmen L.A.Pires-Zottarelli Olivier raspé Mateus A.reck Sarah C.O.rocha AndréL.C.M.Ade Santiago Indunil C.Senanayake Ledo Setti Qiu Ju Shang Sanjay K.Singh esteban B.Sir Kevin V.Solomon Jie Song Prasert Srikitikulchai Marc Stadler Satinee Suetrong Hayato Takahashi Takumasa Takahashi Kazuaki Tanaka Li Ping Tang Kasun M.Thambugala Donnaya Thanakitpipattana Michael K.Theodorou Benjarong Thongbai Tuksaporn Thummarukcharoen Qing Tian Saowaluck Tibpromma Annemieke State Key Laboratory of Mycology Institute of MicrobiologyChinese Academy of SciencesNo 31st West Beichen RoadChaoyang DistrictBeijing 100101People’s Republic of China Centre of excellence in Fungal research and School of Science Mae Fah Luang UniversityChiang Rai 57100Thailand Key Laboratory for Plant Diversity and Biogeography of east Asia Kunming Institute of BotanyChinese Academy of ScienceKunming 650201YunnanPeople’s Republic of China department of Botany and Microbiology College of ScienceKing Saud UniversityP.O.Box:2455Riyadh 1145Saudi Arabia department of Botany and Microbiology Faculty of ScienceSohag UniversitySohag 82524Egypt ALVALAB C/La Rochela nº47E-39012 SantanderSpain Micolab Programa de Pós-Graduação em Biologia de FungosAlgas e PlantasDepartamento de BotânicaUniversidade Federal de Santa CatarinaCampus Universitário TrindadeCEP:88040-900 FlorianópolisSanta CatarinaBrazil department of Biology University of WashingtonBox 351800SeattleWA 98195-1800USA Guizhou Key Laboratory of Agricultural Biotechnology Guizhou Academy of Agricultural SciencesGuiyang 550006GuizhouPeople’s Republic of China National Fungal Culture Collection of India(NFCCI) Biodiversity and Palaeobiology GroupMACS’Agharkar Research InstituteG.G.Agarkar RoadPune 411004India PO Box 116 HusumWA 98623-0116USA Formerly Department of BotanyGoa UniversityGoaIndia No.128/1-J Azad Housing SocietyCurcaP.O.Goa Velha 403108India *** 345 Shipwatch LaneHerculesCA 94547USA Microbe Interaction Laboratory(BMIT) BIOTECNational Science and Technology Development Agency(NSTDA)113 Thailand Science ParkThanon PhahonyothinTombon Khlong NuengAmphoeKhlong LuangPathum Thani 12120Thailand Academy of Biology and Biotechnology Southern Federal UniversityRostov-on-Don 344090Rostov regionRussia A.M.B.Gruppo Micologico Forlivese BAntonio“Cicognani” Via Roma Forlì Italy 18 A.M.B.Circolo Micologico“Giovanni Carini”C.P.314BresciaItaly Societàper gli Studi Naturalistici della romagna C.P.144Bagnacavallo

Notes on 113 fungal taxa are compiled in this paper,including 11 new genera,89 new species,one new subspecies,three new combinations and seven reference *** geographic and taxonomic range of fungal taxa are *** the Ascomycota the new genera Angustospora(Testudinaceae),Camporesia(Xylariaceae),Clematidis,Crassiparies(Pleosporales genera incertae sedis),Farasanispora,Longiostiolum(Pleosporales genera incertae sedis),Multilocularia(Parabambusicolaceae),Neophaeocryptopus(Dothideaceae),Parameliola(Pleosporales genera incertae sedis),and Towyspora(Lentitheciaceae)are *** introduced species are Angustospora nilensis,Aniptodera aquibella,Annulohypoxylon albidiscum,Astrocystis thailandica,Camporesia sambuci,Clematidis italica,Colletotrichum menispermi,***,Comoclathris pimpinellae,Crassiparies quadrisporus,Cytospora salicicola,Diatrype thailandica,Dothiorella rhamni,Durotheca macrostroma,Farasanispora avicenniae,Halorosellinia rhizophorae,Humicola koreana,Hypoxylon lilloi,Kirschsteiniothelia tectonae,Lindgomyces okinawaensis,Longiostiolum tectonae,Lophiostoma pseudoarmatisporum,Moelleriella phukhiaoensis,***,Mucoharknessia anthoxanthi,Multilocularia bambusae,Multiseptospora thysanolaenae,Neophaeocryptopus cytisi,Ocellularia arachchigei,***,Ochronectria thailandica,Ophiocordyceps karstii,Parameliola acaciae,***,Parastagonospora cumpignensis,Pseudodidymosphaeria phlei,Polyplosphaeria thailandica,Pseudolachnella brevifusiformis,Psiloglonium macrosporum,rhabdodiscus albodenticulatus,rosellinia chiangmaiensis,Saccothecium rubi,Seimatosporium pseudocornii,***,Sigarispora ononidis and Towyspora *** combinations are provided for eutiarosporella dactylidis(sexual morph described and illus trated)and Pseudocamarosporium ***,illustrations and/or reference specimens are designated for Aposphaeria corallinolutea,Cryptovalsa ampelina,Dothiorella vidmadera,Ophiocordyceps formosana,P

关键词： Ascomycota Basidiomycota Neocallimastigomycota Oomycota.Zygomycota Phylogeny Taxonomy New genus New species

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Phytochemical Composition and Antioxidant Capacity of Psidium guajava Fresh Fruits and Flour

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Food and Nutrition Sciences 2014年第8期5卷 725-732页

作者： M.Alejandra Moreno I.Catiana Zampini Milena Costamagna Jorge e.Sayago roxana M.Ordonez María I.Isla Instituto de Química del Noroeste Argentino(INQUINOA) CONICETSan Miguel de TucumánArgentina Cátedra de elementos de Química Orgánica y Biológica Facultad de Ciencias Naturales e Instituto Miguel LilloUniversidad Nacional de TucumánSan Lorenzo 1469San Miguel de TucumánArgentina Cátedra de Fitoquímica Facultad de BioquímicaQuímica y FarmaciaUniversidad Nacional de TucumánAyacucho 471San Miguel de TucumánArgentina Fundación Miguel lillo San Miguel de TucumánArgentina

Psidium guajava fruits are consumed fresh or processed (beverages, syrup, ice cream, jams and jellies). Guayaba is a fruit highly perishable and susceptible to damage during the postharvest. One strategy to overcome this problem is its processing by using techniques that preserve its organoleptic, nutritive and functional properties and allow getting food with added value. The purpose of this study was to obtain flour from fresh fruits cultivated in Argentina Northwestern by lyophilization and to determine the antioxidant activity and the main phytochemicals present in fresh fruits and flour. Nutritional composition (sugar, protein and fat) and the bioactive phytochemicals (total phenolic compounds, flavonoid phenolic, condensed and hydrolizable tannin, ascorbic acid, pigments such as anthocyanin and carotenoids) as well as fiber content, were evaluated. The flour preserved flavor, aroma and color of pulp from fresh fruits. The flour contained around 30% of sugar, 20% of total protein, 0.5% of fat and high level of crude fiber. Carotenoids and ascorbic acid were the dominant phytochemicals in flour as well as in fresh fruits. The guayaba flour showed antioxidant activity with SC50 values similar to fresh fruits. The flour showed nutraceutical characteristics that are demanded by functional food and could be used as a dietary supplement.

关键词： Fresh Fruit Flour Psidium guajava Nutritional Properties Functional Properties

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Nutritional,Antioxidant and Anti-Inflammatory Properties of Cyclanthera pedata,an Andinean Fruit and Products derived from Them

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Food and Nutrition Sciences 2013年第8期4卷 55-61页

作者： Marisa rivas Dora Vignale roxana M.Ordonez Iris Catiana Zampini María rosa Alberto Jorge e.Sayago María I.Isla INQUINOA(CONICeT) TucumánArgentina Cátedra de Botánica Sistemática y Fitogeografía Facultad de Ciencias AgrariasUniversidad Nacional de JujuyAlberdiSan Salvador de JujuyArgentina Cátedra de elementos de Química Orgánica y Biológica Facultad de Ciencias Naturales e Instituto Miguel LilloTucumánArgentina Cátedra de Fitoquímica Facultad de BioquímicaQuímica y FarmaciaUniversidad Nacional de Tucumán(4000)S.M.de TucumánTucumánArgentina Fundación Miguel lillo TucumánArgentina

There is an increasing interest in food plant with health-giving effects. The aim of this research was to evaluate the phytochemical and nutraceutical profiles of Cyclanthera pedata fruits, a native fruit of the Andean region used by Incas communities called achojcha. Soluble protein (SP), total sugar (TS), free phenolic compounds (FPC), ascorbic acid (AA), total monomeric anthocyanin (TMA), condensed and hydrolizable tannin (CT, HT) were evaluated by sprectrophotometric methods in fresh fruits with and without heating and in flour obtained from fruits. Multielemental composition by ICP-MS was done. Antioxidant activity (AOA) was determined by ABTS and Linoleic acid-b-carotene methods. The inhibitory capacity of LOX, a pro-inflammatory enzyme was also analyzed. The achojcha fresh fruits and achojcha flour showed low amount calories. The flour was high in potassium (7400 mg·K/100 g) and low in sodium (77 mg Na/100 g). High levels of FPC (670 mg GAe/100 g) were found together with elevated levels of AA (123 mg AA/ 100 g). The TMA (0.6 mg C3-Ge/100 g) as well as HT (3.4 mg PB2e/100 g) were also detected in flour. All preparations obtained with fresh and dried fruits showed AOA with SC50 values between 1.8 to 14.5 μg GAe/mL. Inhibitory capacity on LOX was also demonstrated (IC50 values of 40 μg GAe/mL). The fresh fruits and flour showed nutraceutical characteristics that are demanded by functional food and could be used as dietary supplement.

关键词： achojcha Fruit achojcha Flour Cyclanthera pedata Nutritional Properties Functional Properties

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Nutraceutical Properties and Toxicity Studies of Flour Obtained from Capsicum pubescens Fruits and Its Comparison with“Locoto”Commercial Powder

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Food and Nutrition Sciences 2014年第8期5卷 715-724页

作者： Marisa rivas Dora Vignale roxana M.Ordonez I.Catiana Zampini M.rosa Alberto Jorge e.Sayago María I.Isla Instituto de Química del Noroeste Argentino(INQUINOA) CONICETSan Miguel de TucumánArgentina Cátedra de Biología Celular Facultad de Ciencias AgrariasUniversidad Nacional de JujuySan Salvador de JujuyArgentina Cátedra de Botánica Sistemática y Fitogeografía Facultad de Ciencias AgrariasUniversidad Nacional de JujuySan Salvador de JujuyArgentina Cátedra de Fitoquímica Facultad de BioquímicaQuímica y FarmaciaUniversidad Nacional de TucumánSan Miguel de TucumánArgentina Cátedra de elementos de Química Orgánica y Biológica Facultad de Ciencias Naturales e Instituto Miguel LilloUniversidad Nacional de TucumánSan Miguel de TucumánArgentina Fundación Miguel lillo San Miguel de TucumánArgentina

The aim of this research was to evaluate the phytochemical profiles of flour from red, yellow and green fruits of Capsicum pubescens (commun name: locoto) and compare with “locoto” commercial powder (Lcp). Soluble protein (SP), total sugar (TS), free phenolic compounds (FPC), ascorbic acid (AA), total monomeric anthocyanin (TMA), condensed and hydrolizable tannin (CT, HT) and carotenoids (C) were determined by spectrophotometric methods. Multielemental composition by ICP-MS was also done. The flour showed low amounts of calories and high potassium and low sodium levels. Flour from “locoto” fruits contained mainly carotenoids (0.82 to 20 g eβ-C/100g DW), polyphenolic compounds (681 - 822 mg GAe/100g DW) and ascorbic acid (100 - 199 mg AA/100g DW). The polyphenolic profile of Lcp was similar to flour obtained in our laboratory but the level of carotenoid was lower than that of flour. The fiber content of flour was around 3% in all cases. All preparations obtained from flour and Lcp showed antioxidant activity with SC50 values between 1.4 and 3 μg GAe/mL. Inhibitory capacity on Lipo-oxygenase enzyme was also demonstrated. Non mutagenic effect was detected. The “locoto” flour showed nutraceutical characteristics that are demanded by functional food and could be used as a dietary supplement.

关键词： Locoto Fruit Locoto Flour Capsicum pubescens Nutritional Properties Functional Properties

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腺苷受体是调节大脑内侧前额叶皮质星形胶质细胞大麻素1型(CB1)受体对突触可塑性作用的开关

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神经损伤与功能重建 2024年第4期19卷 250-250页

作者： Joana Gon?alves-ribeiro Oksana K Savchak Sara Costa-Pinto Joana I Gomes rafael rivas-Santisteban Alejandro lillo Javier Sánchez romero Ana M Sebasti?o Marta Navarrete Gemma Navarro rafael Franco Sandra H Vaz Instituto de Farmacologia e Neurociencias Faculdade de MedicinaUniversidade de Lisboa Instituto de Medicina Molecular Joao Lobo Antunes Faculdade de MedicinaUniversidade de Lisboa department of Biochemistry and Physiology School of Pharmacy and Food ScienceUniversitat de Barcelona CiberNed Network Center for Neurodegenerative DiseasesNational Spanish Health Institute Carlos Ⅲ 5. Instituto CajalCSIC PhD Program in Neuroscience Universidad Autonoma de Madrid-Instituto Cajal Institut de Neurociencies Universitat de Barcelona Molecular Neurobiology Laboratory Department of Biochemistry and Molecular BiomedicineFaculty of Biology School of Chemistry Universitat de Barcelona

内侧前额叶皮质(mPFC)参与诸如工作记忆等认知功能。星形胶质细胞大麻素1型受体(CB1r)诱导细胞质内钙离子(Ca2+)浓度变化,对神经元功能产生影响。mPFC的星形胶质细胞也表达腺苷A1和A2A受体(A1r,A2Ar),但目前尚不清楚这些细胞中的CB1r与... 详细信息

内侧前额叶皮质(mPFC)参与诸如工作记忆等认知功能。星形胶质细胞大麻素1型受体(CB1r)诱导细胞质内钙离子(Ca2+)浓度变化,对神经元功能产生影响。mPFC的星形胶质细胞也表达腺苷A1和A2A受体(A1r,A2Ar),但目前尚不清楚这些细胞中的CB1r与腺苷受体之间的交流。我们在这里展示,通过CB1r-A2Ar或CB1r-A1r异源二聚体,星形胶质细胞Ca2+信号传递发生了进一步的调节,最终影响mPFC突触可塑性。当A1r和A2Ar被激活时,CB1r介导的Ca2+瞬变出现增加或减少,揭示了腺苷受体可能是星形胶质细胞CB1r的调节器。CB1r的激活导致mPFC的长时程增强(LTP)增强,受A1r控制,但不受A2Ar控制。值得注意的是,在IP3r2KO小鼠中,由于没有显示出星形胶质细胞Ca2+水平升高,CB1r的激活减少了LTP,这种效果不受A1r或A2Ar的调节。本研究表明,CB1r在mPFC LTP上具有稳态作用,受到A1r的控制,可能是由于这些受体在星形胶质细胞中的交流,最终改变了CB1r Ca2+信号传递。

关键词： CB1受体腺苷受体星形胶质细胞内侧前额叶皮质突触可塑性

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阿根廷图库曼省引进虹鳟鱼产生的问题及其对策

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人类环境杂志 1998年第7期27卷 584-585页

作者： Hugo r. Fernandez unt.edu.ar or flobo unt.edu.ar Luis A. Fernandez 张甲珅 CONICeT Facultad de Ciencias Naturales Miguel lillo 205 (4000) Tucuman Argentina e-mail: hrf Fundacion Miguel lillo Miguel lillo 251 (4000) Tucuman Argentina e-mail: hrt

引言国际间正常和意外引进水生生物的原因很多,并且发生着历史性变化。一些广为推崇的外来鱼种有鲤鱼(Carassius auratus,鲤科),银汉鱼(Odonthestes bonar-

关键词：鲑科鱼虹鳟鱼引进产品生态影响对策

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