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Angle-tunable intersubband photoabsorption and enhanced photobleaching in twisted bilayer graphene

Nano Research 2021年第8期14卷 2797-2804页

作者： Eva A.A.Pogna Xianchong Miao Driele von Dreifus Thonimar v.Alencar marcus v.o.moutinho Pedro venezuela Cristian Manzoni Minbiao Ji Giulio Cerullo Ana Maria de Paula Istituto di Nanoscienze CNR-NANo Laboratory NESTPiazza San Silvestro 12Pisa 56127Italy State Key Laboratory of Surface Physics and Department of Physics Fudan UniversityShanghai 200433China Departamento de Fisica Institute de Ciencias ExatasUniversidade Federal de Minas GeraisBelo Horizonte-MG 31270-901Brazil Departamento de Fisica Institute de Ciencias Exatas e BiologicasUniversidade Federal de Ouro PretoOuro Preto-MG 35400-000Brazil Ndcleo Multidisciplinar de Pesquisas em Computagao-NUMPEX-CoMP Campus Duque de CaxiasUniversidade Federal do Rio de JaneiroDuque de Caxias-RJ25265-970Brazil Institute de Fisica Universidade Federal FluminenseUFFNiteroi-RJ24210-346Brazil IFN-CNR Dipartimento di FisicaPolitecnico di MilanoPiazza L.da Vinci 32Milano 20133Italy

van der Waals heterostructures obtained by artificially stacking two-dimensional crystals represent the frontier of material engineering,demonstrating properties superior to those of the starting *** control of the interlayer twist angle has opened new possibilities for tailoring the optoelectronic properties of these *** bilayer graphene with a strong interlayer coupling is a prototype of twisted heterostructure inheriting the intriguing electronic properties of *** the effects of the twist angle on its out-of-equilibrium optical properties is crucial for devising optoelectronic *** this aim,we here combine excitation-resolved hot photoluminescence with femtosecond transient absorption *** hot charge carrier distribution induced by photo-excitation results in peaked absorption bleaching and photo-induced absorption bands,both with pronounced twist angle *** simulations of the electronic band structure and of the joint density of states enable to assign these bands to the blocking of interband transitions at the van Hove singularities and to photo-activated intersubband *** tens of picoseconds relaxation dynamics of the observed bands is attributed to the angle-dependence of electron and phonon heat capacities of twisted bilayer graphene.

关键词： twisted bilayer graphene transient absorption microscopy hot-photoluminescence van der Waals heterostructures optoelectronic properties van Hove singularities

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Acetic acid additive in NaNo_(3)aqueous electrolyte for long-lifespan Mg-air batteries

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Journal of Magnesium and Alloys 2024年第2期12卷 825-839页

作者： Yaqing Zhou Fan Sun Gunahua Lin Sandrine Zanna Antoine Seyeux Philippe marcus Jolanta´Swiatowska Chimie ParisTech-CNRS PSL UniversityInstitut de Recherche de Chimie Paris11 rue Pierre et Marie CurieParis 75005France

Mg-air batteries have attracted tremendous attention as a potential next-generation power source for portable electronics and e-transportation due to their remarkable high theoretical volumetric energy density,environmental sustainability,and ***,the fast hydrogen evolution reaction(HER)in NaCl-based aqueous electrolytes impairs the performance of Mg-air batteries and leads to poor specific capacity,low energy density,and low ***,the conventionally used NaCl solute was proposed to be replaced by NaNo_(3)and acetic acid additive as a corrosion inhibitor,therefore an electrolyte engineering for long-life time Mg-air batteries is *** resulting Mg-air batteries based on this optimized electrolyte demonstrate an improved discharge voltage reaching~1.8 v for initial 5 h at a current density of 0.5 mA/cm^(2) and significantly prolonged cells'operational lifetime to over 360 h,in contrast to only~17 h observed in NaCl electrolyte.X-ray photoelectron spectroscopy and time-of-flight secondary ion mass spectrometry were employed to analyse the composition of surface film and scanning electron microscopy combined with transmission electron microscopy to clarify the morphology changes of the surface layer as a function of acetic acid *** thorough studies of chemical composition and morphology of corrosion products have allowed us to elucidate the working mechanism of Mg anode in this optimized electrolyte for Mg-air batteries.

关键词： Acetic acid additive in NaNo_(3)electrolyte Electrolyte engineering Corrosion surface film Surface characterization Hydrogen evolution

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Insights into the hydrogen evolution reaction in vanadium redox flow batteries:A synchrotron radiation based X-ray imaging study

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Journal of Energy Chemistry 2024年第4期91卷 132-144页

作者： Kerstin Köble Alexey Ershov Kangjun Duan Monja Schilling Alexander Rampf Angelica Cecilia TomášFaragó marcus Zuber Tilo Baumbach Roswitha Zeis Helmholtz Institute Ulm Karlsruhe Institute of Technology89081 UlmGermany Laboratory for Applications of Synchrotron Radiation Karlsruhe Institute of Technology76131 KarlsruheGermany Institute for Photon Science and Synchrotron Radiation Karlsruhe Institute of Technology76344 Eggenstein-LeopoldshafenGermany Department of Electrical Electronicsand Communication EngineeringFaculty of EngineeringFriedrich-Alexander-Universität Erlangen-Nürnberg(FAU)91058 ErlangenGermany Department of Mechanical and Industrial Engineering University of TorontoToronto M5S 3G8OntarioCanada

The parasitic hydrogen evolution reaction(HER)in the negative half-cell of vanadium redox flow batteries(vRFBs)causes severe efficiency ***,a deeper understanding of this process and the accompanying bubble formation is *** benchmarking study locally analyzes the bubble distribution in thick,porous electrodes for the first time using deep learning-based image segmentation of synchrotron X-ray *** large three-dimensional data set was processed precisely in less than one minute while minimizing human errors and pointing out areas of increased HER activity in *** study systematically varies the electrode potential and material,concluding that more negative electrode potentials of-200 m v *** hydrogen electrode(RHE)and lower cause more substantial bubble formation,resulting in bubble fractions of around 15%–20%in carbon felt ***,the bubble fractions stay only around 2%in an electrode combining carbon felt and carbon *** detected areas with high HER activity,such as the border subregion with more than 30%bubble fraction in carbon felt electrodes,the cutting edges,and preferential spots in the electrode bulk,are potential-independent and suggest that larger electrodes with a higher bulk-to-border ratio might reduce HER-related performance *** described combination of electrochemical measurements,local X-ray microtomography,AI-based segmentation,and 3D morphometric analysis is a powerful and novel approach for local bubble analysis in three-dimensional porous electrodes,providing an essential toolkit for a broad community working on bubble-generating electrochemical systems.

关键词： vanadium redox flow battery Synchrotron X-ray imaging Tomography Hydrogen evolution reaction Gas bubbles Deep learning

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Leveraging Robust Artificial Intelligence for Mechatronic Product Development—A Literature Review

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International Journal of Intelligence Science 2024年第1期14卷 1-21页

作者： Alexander Nüßgen René Degen marcus Irmer Fabian Richter Cecilia Boström Margot Ruschitzka CAD CAM Center Cologne Institute of Automotive Engineering Cologne (IFK) Faculty of Automotive Systems and Production Cologne University of Applied Science Cologne Germany Division of Electricity Department of Electrical Engineering Uppsala University Uppsala Sweden

Mechatronic product development is a complex and multidisciplinary field that encompasses various domains, including, among others, mechanical engineering, electrical engineering, control theory and software engineering. The integration of artificial intelligence technologies is revolutionizing this domain, offering opportunities to enhance design processes, optimize performance, and leverage vast amounts of knowledge. However, human expertise remains essential in contextualizing information, considering trade-offs, and ensuring ethical and societal implications are taken into account. This paper therefore explores the existing literature regarding the application of artificial intelligence as a comprehensive database, decision support system, and modeling tool in mechatronic product development. It analyzes the benefits of artificial intelligence in enabling domain linking, replacing human expert knowledge, improving prediction quality, and enhancing intelligent control systems. For this purpose, a consideration of the v-cycle takes place, a standard in mechatronic product development. Along this, an initial assessment of the AI potential is shown and important categories of AI support are formed. This is followed by an examination of the literature with regard to these aspects. As a result, the integration of artificial intelligence in mechatronic product development opens new possibilities and transforms the way innovative mechatronic systems are conceived, designed, and deployed. However, the approaches are only taking place selectively, and a holistic view of the development processes and the potential for robust and context-sensitive artificial intelligence along them is still needed.

关键词： Artificial Intelligence Mechatronic Product Development Knowledge Management Data Analysis optimization Human Experts Decision-Making Processes v-Cycle

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opportunities and Challenges of Plant Bioactive Compounds for Food and Agricultural-Related Areas

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Phyton-International Journal of Experimental Botany 2022年第6期91卷 1105-1127页

作者： Maicon S.N.dos Santos João H.C.Wancura Carolina E.D.oro Rogério M.Dallago marcus v.Tres Laboratory of Agroindustrial Processes Engineering Federal University of Santa MariaCachoeira do Sul96508-010Brazil Department of Teaching Research and DevelopmentSul Rio-Grandense Federal InstituteCharqueadas96745-000Brazil Department of Food Engineering Regional Integrated University of Upper Uruguay and MissionsErechim99709-910Brazil

The growing development of biological products highlights the social and environmental responsibility that several industrial companies are facing in recent *** this context,the advancement of bioprocessing as an alternative for exploring the potential of ecologically based products,especially in biofuels,food,and agro-industrial business,exposes the rational efficiency of the application of renewable sources in different industrial *** strongly associated with food production concentrate large amounts of wastes rich in bioactive compounds.A range of highly effective technologies has been highly explored to recover large concentrations of prominent compounds present in these *** advances in this scenario assurance value addition to these by-products,in addition to highlighting their various technological applications,considering the biorefinery and ecologically based production ***,this review article described a detailed and systematic approach to the importance of using bioactive compounds and exploring the main sources of these ***,some recent and innovative research that has achieved encouraging results was ***,the study included the main extraction technologies that have been investigated as a strategy of prospecting the application of bioactive compounds and optimizing the processes for obtaining natural compounds from plant ***,future outlooks were presented to contribute to the innovative opportunities and applicability of highly promising technologies and manipulations of bioactive compounds from a range of perspectives.

关键词： Biological security renewable biological resources sustainable production

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Frequency Extrapolation through Sparse Sums of Lorentzians

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Journal of Earth Science 2014年第1期25卷 117-125页

作者： Fredrik Andersson marcus Carlsson Maarten v de Hoop Centre for Mathematical Sciences Lund University Department of Mathematics Purdue University

Sparse sums of Lorentzians can give good approximations to functions consisting of linear combination of piecewise continuous functions. To each Lorentzian, two parameters are as- signed： translation and scale. These parameters can be found by using a method for complex fre- quency detection in the frequency domain. This method is based on an alternating projection scheme between Hankel matrices and finite rank operators, and have the advantage that it can be done in weighted spaces. The weighted spaces can be used to partially revoke the effect of finite band-width filters. Apart from frequency extrapolation the method provides a way of estimating discontinuity locations.

关键词： sparse sum Lorentzians Hankel matrices finite rank operator discontinuity location.

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Site-directed deuteration of dronedarone preserves cytochrome P4502J2 activity and mitigates its cardiac adverse effects in canine arrhythmic hearts

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Acta Pharmaceutica Sinica B 2022年第10期12卷 3905-3923页

作者： Aneesh v.Karkhanis Gopalakrishnan venkatesan Ryuichi Kambayashi Jacqueline Wen Hui Leow marcus Qingrui Han Hiroko Izumi-Nakaseko Ai Goto Jeremy Kah Sheng Pang Boon Seng Soh Pipin Kojodjojo Atsushi Sugiyama Eric Chun Yong Chan Department of Pharmacy Faculty of ScienceNational University of SingaporeSingapore 117543Singapore Department of Pharmacology Faculty of MedicineToho UniversityTokyo 143-8540Japan Institute of Molecular and Cell Biology Agency for ScienceTechnology and ResearchSingapore 138673Singapore Department of Biological Sciences Faculty of ScienceNational University of SingaporeSingapore 117558Singapore Department of Medicine Yong Loo Lin School of MedicineNational University of SingaporeSingapore 119228Singapore

Cytochrome P4502J2(CYP2J2)metabolizes arachidonic acid(AA)to cardioprotective epoxyeicosatrienoic acids(EETs).Dronedarone,an antiarrhythmic drug prescribed for treatment of atrial fibrillation(AF)induces cardiac adverse effects(AEs)with poorly understood *** previously demonstrated that dronedarone inactivates CYP2J2 potently and irreversibly,disrupts AA-EET pathway leading to cardiac mitochondrial toxicity rescuable via EET *** this study,we investigated if mitigation of CYP2J2 inhibition prevents dronedarone-induced cardiac *** first synthesized a deuterated analogue of dronedarone(termed poyendarone)and demonstrated that it neither inactivates CYP2J2,disrupts AA-EETs metabolism nor causes cardiac mitochondrial toxicity in *** patch-clamp experiments demonstrated that pharmacoelectrophysiology of dronedarone is unaffected by ***,we show that dronedarone treatment or CYP2J2 knockdown in spontaneously beating cardiomyocytes indicative of depleted CYP2J2 activity exacerbates beat-to-beat(BTB)variability reflective of proarrhythmic *** contrast,poyendarone treatment yields significantly lower BTB variability compared to dronedarone in cardiomyocytes indicative of preserved CYP2J2 ***,poyendarone and dronedarone display similar antiarrhythmic properties in the canine model of persistent AF,while poyendarone substantially reduces beat-to-beat variability of repolarization duration suggestive of diminished proarrhythmic *** findings prove that deuteration of dronedarone prevents CYP2J2 inactivation and mitigates dronedarone-induced cardiac AEs.

关键词： Arachidonic acid Atrial fibrillation CYP2J2 Drug-induced proarrhythmia Epoxyeicosatrienoic acids Mechanism-based inactivation Dronedarone

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Individual variation in dispersal associated behavioral traits of the invasive Chinese mitten crab （Eriocheir sinensis, H. Milne Edwards, 1854） during initial invasion of Lake v^inern, Sweden

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Current Zoology 2014年第3期60卷 410-416页

作者： Tomas BRoDIN marcus K. DRoTZ Department of Ecology and Environmental Science Umea University Sweden Lake vanem Museum of Natural and Cultural History Framnisvsgen 2 53154 Lidkoping Sweden

Understanding and predicting species range-expansions and biological invasions is an important challenge in modern ecology because of rapidly changing environments. Recent studies have revealed that consistent within-species variation in behavior (i.e. animal personality) can be imperative for dispersal success, a key stage in the invasion process. Here we investigate the composition and correlation of two important personality traits associated with invasion success, activity and boldness, and how they are connected to sex and individual size in a newly colonised population of the Chinese mitten crabEriocheir sinensisin Lake vänern, Sweden. We found no effect of sex or size on behavioral expressions ofE. sinensisbut a clear positive correlation between boldness and activity. In addition, this study generates important baseline data for monitoring behavioral development, and thereby changing ecological impact, of an invading population over time. This has implications for predicting ecological effects of invasive species as well as for managing ecological invasions.

关键词：中华绒螯蟹生物入侵行为特征个体差异中国瑞典米尔恩分散

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Update of cholangioscopy and biliary strictures

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World Journal of Gastroenterology 2011年第34期17卷 3864-3869页

作者： marcus W Chin Michael F Byrne Department of Gastroenterology and Hepatology Vancouver General Hospital Amy Athelstan Saw Fellow University of Western AustraliaPerth 6009 Australia Department of Gastroenterology and Hepatology Vancouver General Hospital University of British ColumbiaVancouver V5Z1M9 Canada

Cholangioscopy remains another modality in the investigation of biliary strictures. At cholangioscopy, the"tumour vessel" sign is considered a specific sign formalignancy. Through its ability to not only visualisemucosa, but to take targeted biopsies, it has a greater accuracy, sensitivity and specificity for malignant strictures than endoscopic retrograde cholangiopancreatography guided cytopathological acquisition. Cholangioscopy however, is time consuming and costly, requires greater technical expertise, and should be reserved for the investigation of undifferentiated strictures after standard investigations have failed.

关键词：胆道狭窄敏感性胆管

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Application of pan-sharpening algorithm for correlative multimodal imaging using AFM-IR

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npj Computational Materials 2019年第1期5卷 714-722页

作者： Nikolay Borodinov Natasha Bilkey marcus Foston Anton v.Ievlev Alex Belianinov Stephen Jesse Rama K.vasudevan Sergei v.Kalinin olga S.ovchinnikova Center for Nanophase Materials Science Oak Ridge National LaboratoryOak RidgeTN 37831USA Department of Energy Environmental&Chemical EngineeringWashington University in St.LouisOne Brookings DriveSt.LouisMO 63130USA

The coupling of atomic force microscopy with infrared spectroscopy(AFM-IR)offers the unique capability to characterize the local chemical and physical makeup of a broad variety of materials with nanoscale ***,in order to fully utilize the measurement capability of AFM-IR,a three-dimensional dataset(2D map with a spectroscopic dimension)needs to be acquired,which is prohibitively time-consuming at the same spatial resolution of a regular AFM *** this paper,we provide a new approach to process spectral AFM-IR data based on a multicomponent pan-sharpening *** approach requires only a low spatial resolution spectral and a limited number of high spatial resolution single wavenumber chemical maps to generate a high spatial resolution hyperspectral image,greatly reducing data acquisition *** a result,we are able to generate highresolution maps of component distribution,produce chemical maps at any wavenumber available in the spectral range,and perform correlative analysis of the physical and chemical properties of the *** highlight our approach via imaging of plant cell walls as a model system and showcase the interplay between mechanical stiffness of the sample and its chemical *** believe our pan-sharpening approach can be more generally applied to different material classes to enable deeper understanding of that structure-property relationship at the nanoscale.

关键词： utilize modal walls

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