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Pd nanocluster-decorated CoFe composite supported on nitrogen carbon nanotubes as a high-performance trifunctional electrocatalyst

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Green Energy & Environment 2022年第5期7卷 933-947页

作者： Revanasiddappa manjunatha Li Dong Zibo Zhai Jianyi Wang Qianru Fu Wei Yan Jiujun Zhang Institute for Sustainable Energy/College of Sciences Shanghai UniversityShanghai200444China Zhaoqing Leoch Battery Technology Co.Ltd. Zhaoqing518000China

Rational design and synthesis of low-cost trifunctional electrocatalysts with improved stability and superior electrocatalytic activity for oxygen reduction reaction(ORR),oxygen evolution reaction(OER),and hydrogen evolution reaction(HER) are highly desirable but remain as the bottlenecks at the current state of *** this paper,the cobalt-iron(Co-Fe) composite supported on nitrogen-doped carbon nanotubes(CoFe composite/NCNTs) is *** intrinsic OER and HER catalytic activities of this CoFe composite/NCNTs composite are significantly improved with palladium(Pd) nanocluster decoration [Pd-coated(CoFe composite/NCNTs)].The as-prepared Pd-coated(CoFe composite/NCNTs) catalyst exhibits excellent trifunctional electrocatalytic activity and stability due to the interfacial coupling between Pd and(CoFe composite/NCNTs).This catalyst is successfully employed in the water electrolysis cell as both OER and HER electrode catalysts,flexible rechargeable Zn-air battery as the bifunctional ORR and OER electrode *** cell voltage of this catalyst-coated electrodes requires only 1.60 V to achieve 10 mA cm^(-2) current density for water electrolysis cell,which is comparable to and even better than that of Pt/C and Ir/C based *** primary Zn-air battery using this catalyst shows a constant high open-circuit voltage(OCV) of 1.47 V and a maximum power density of 261 mW cm^(-2) in the flooded mode *** importantly,a flexible Zn-air battery with this catalyst runs very smoothly without a change in voltage gap during flat,bending,and twisting positions.

关键词： catalyst functional cluster

Efficient and recyclable palladium enriched magnetic nanocatalyst for reduction of toxic environmental pollutants

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Journal of Environmental Sciences 2021年第3期33卷 189-204页

作者： manjunatha Kempasiddaiah Vishal Kandathil Ramesh B.Dateer Mahiuddin Baidya Shivaputra A.Patil Siddappa A.Patil Centre for Nano and Material Sciences Jain UniversityJain Global CampusKanakapuraRamanagaramBangalore 562112India Department of Chemistry Indian Institute of Technology MadrasChennai 600036Tamil NaduIndia Pharmaceutical Sciences Department College of PharmacyRosalind Franklin University of Medicine and ScienceNorth ChicagoIL 60064USA

In this paper,highly stable,powerful,and recyclable magnetic nanoparticles tethered Nheterocyclic carbene-palladium(Ⅱ)((CH_(3))_(3)-NHC-Pd@Fe_(3)O_(4))as magnetic nanocatalyst was successfully synthesized from a simplistic multistep synthesis under aerobic conditions through easily available low-cost *** synthesized(CH_(3))_(3)-NHC-Pd@Fe_(3)O_(4) magnetic nanocatalyst was characterized from various analytical tools and catalytic potential of the(CH_(3))_(3)-NHC-Pd@Fe_3 O_4 magnetic nanocatalyst was studied for the catalytic reduction of toxic 4-nitrophenol(4-NP),hexavalent chromium(Cr(Ⅵ)),Methylene Blue(MB)and Methyl Orange(MO)at room temperature in aqueous ***-Visible spectroscopy was employed to monitor the reduction ***(CH_(3))_(3)-NHC-Pd@Fe_(3)O_(4) magnetic nanocatalyst exhibited excellent catalytic activity for the reduction of toxic environmental ***,(CH_(3))_(3)-NHC-Pd@Fe_(3)O_(4) magnetic nanocatalyst could be easily and rapidly separated from the reaction mixture with the help of an external magnet and recycled minimum five times in reduction of 4-NP,MB,MO and four times in Cr(Ⅵ)without significant loss of catalytic potential and remains stable even after reuse.

关键词： Magnetic nanocatalyst Wastewater treatment Chemical kinetics Catalyst recyclability

Modified distance regularized level set evolution for brain ventricles segmentation

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Visual Computing for Industry,Biomedicine,and Art 2020年第1期3卷 329-340页

作者： Thirumagal Jayaraman Sravan Reddy M manjunatha Mahadevappa Anup Sadhu Pranab Kumar Dutta School of Medical Science and Technology IIT KharagpurKharagpur 721302India Department of Electronics and Communications JNTUA-College of EngineeringPulivendula 516390India EKO CT&MRI Scan Centre Medical CollegeCalcutta 700073India Department of Electrical Engineering IIT KharagpurKharagpur 721302India

Neurodegenerative disorders are commonly characterized by atrophy of the brain which is caused by neuronal *** are one of the prominent structures in the brain;their shape changes,due to their content,the cerebrospinal *** the morphological changes of ventricles,aids in the diagnosis of atrophy,for which the region of interest needs to be separated from the *** study presents a modified distance regularized level set evolution segmentation method,incorporating regional intensity *** proposed method is implemented for segmenting ventricles from brain images for normal and atrophy subjects of magnetic resonance imaging and computed tomography *** of the proposed method were compared with ground truth images and produced sensitivity in the range of 65%–90%,specificity in the range of 98%–99%,and accuracy in the range of 95%–98%.Peak signal to noise ratio and structural similarity index were also used as performance measures for determining segmentation accuracy:95%and 0.95,*** parameters of level set formulation vary for different *** optimization procedure was followed to fine tune *** proposed method was found to be efficient and robust against noisy *** proposed method is adaptive and multimodal.

关键词： Ventricles Atrophy Segmentation Level set Diagnosis

MHD Flow and Nonlinear Thermal Radiative Heat Transfer of Dusty Prandtl Fluid over a Stretching Sheet

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Fluid Dynamics & Materials Processing 2020年第2期16卷 131-146页

作者： K.Ganesh Kumar S.manjunatha N.G.Rudraswamy Department of Mathematics SJM Institute of TechnologyChitradurga577502India Department of Engineering Mathematics Faculty of EngineeringChrist UniversityBengaluru560074India Department of Studies and Research in Mathematics Kuvempu UniversityShimoga577451India

Boundary layer flows and melting heat transfer of a Prandtl fluid over a stretching surface in the presence of fluid particle suspensions has been *** converted set of boundary layer equations are solved numerically by RKF-45 *** numerical results for flow and heat transfer characteristics are deliberated for various physical ***,the skin friction coefficient and Nusselt number are also presented in Tabs.2 and *** is found that the heat transfer rates are advanced in occurrence of nonlinear radiation compered to linear ***,it is noticed that velocity and temperature profile increases by increasing Prandtl parameter.

关键词： Prandtl fluid melting effect dusty fluid nonlinear radiation

Slip flow of MHD Casson fluid in an inclined channel with variable transport properties

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Communications in Theoretical Physics 2020年第9期72卷 21-38页

作者： K V Prasad Hanumesh Vaidya C Rajashekhar Sami Ullah Khan G manjunatha J U Viharika Department of Mathematics Vijayanagara Sri Krishnadevaraya UniversityVinayaka NagarBallari-583105KarnatakaIndia Bhaskaracharya Study Chair Karnataka State Akkamahadevi Women's UniversityVijayapuraKarnatakaIndia Department of Mathematics COMSTAS University IslamabadSahiwal Campus 54000Pakistan Department of Mathematics Manipal Institute of TechnologyManipal Academy of Higher EducationManipalKarnataka576104-India

Due to the instructive role of the peristaltic phenomenon in the human body, interests have been developed in recent years towards peristaltic transport with various thermo-physical *** current investigation reveals the effects of the magnetic field and variable transport properties on the peristaltic transport of a Casson fluid slip flow through an inclined *** coupled partial differential equations regulate the fluid flow. Through the perturbation method, the momentum and energy equations are solved for small values of variable viscosity and thermal conductivity, and the closed-form solution is obtained for mass transfer. The impact on physiological quantities of related parameters of interest is evaluated and discussed via graphs. The results obtained for the current flow represent some interesting behaviors which have applications in the biomedical field.

关键词： velocity slip thermal slip concentration slip variable viscosity yield stress

Gamma and X-ray radiation compatibility of Ti–Ta–Hf–Zr alloys used for coronary stent applications

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Nuclear Science and Techniques 2018年第1期29卷 16-22页

作者： L. Seenappa H. C. manjunatha K. N. Sridhar Chikka Hanumantharayappa Department of Physics Government College for WomenKolar Karnataka 563101 India Department of Physics Government First Grade CollegeKolar Karnataka 563101 India Vivekananda Degree College Bangalore Karnataka 560055India Research and Development Centre Bharathiar UniversityCoimbatore 641046 India

We have studied the gamma and X-ray radiation compatibility of Ti-based alloys such as Ti–37 Ta–26 Hf–13 Zr-24(wt%) [Alloy 1], Ti–40 Ta–22 Hf–11.7 Zr-26.3(wt%) [Alloy 2], Ti–45 Ta–18.4 Hf–10 Zr-26.6(wt%) [Alloy3], Ti–50 Ta–15 Hf–8 Zr-27(wt%) [Alloy 4], Ti–55 Ta–12 Hf–7 Zr-26(wt%) [Alloy 5], and Ti–60 Ta–10 Hf–5 Zr-25(wt%) [Alloy 6]. Gamma and X-ray radiation compatibility is studied by evaluating the mass attenuation coefficient,mean free path, HVL, TVL effective atomic number,effective electron density, exposure buildup factor, and relative dose. We have compared these parameters for studied alloys with that of arteries. The alloys Ti–55 Ta–12 Hf–7 Zr-26 and Ti–60 Ta–10 Hf–5 Zr-25 have added properties such as gamma/X-ray radiation compatibility,high elastic admissible strain, high mechanical strength,and excellent biocompatibility. Hence, we may suggest that, among Ti–Ta–Hf–Zr alloys, these alloys are best materials for coronary stent applications.

关键词： Stentalloys X-ray Gamma Mass attenuation coefficient

Plasticity of spermatogonial stem cells

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Asian Journal of Andrology 2015年第3期17卷 355-359页

作者： Paul S Cooke Liz Simon manjunatha K Nanjappa Theresa I Medrano Suzanne E Berry Department of Physiological Sciences College of Veterinary Medicine University of Florida Gainesville FL 32608 USA Department of Physiology Louisiana State University Health Sciences Center New Orleans LA 70112 USA Department of Comparative Biosciences College of Veterinary Medicine University of Illinois at Urbana-Champaign Urbana IL 61802 USA

There have been significant breakthroughs over the past decade in the development and use of pluripotent stem cells as a potential source of cells for applications in regenerative medicine. It is likely that this methodology will begin to play an important role in human clinical medicine in the years to come. This review describes the plasticity of one type of pluripotent cell, spermatogonial stem cells （SSCs）, and their potential therapeutic applications in regenerative medicine and male infertility. Normally, SSCs give rise to sperm when in the testis. However, both human and murine SSCs can give rise to cells with embryonic stem （ES） cell-like characteristics that can be directed to differentiate into tissues of all three embryonic germ layers when placed in an appropriate inductive microenvironment, which is in contrast to other postnatal stem cells. Previous studies have reported that SSCs expressed an intermediate pluripotent phenotype before differentiating into a specific cell type and that extended culture was necessary for this to occur. However, recent studies from our group using a tissue recombination model demonstrated that SSCs differentiated rapidly into another tissue, in this case, prostatic epithelium, without expression of pluripotent ES cell markers before differentiation. These results suggest that SSCs are capable of directly differentiating into other cell types without going through an intermediate ES cell-like stage. Because SSCs do not require reprogramming to achieve a pluripotent state, they are an attractive source of pluripotent cells for use in regenerative medicine.

关键词： pluripotency regenerative medicine spermatogenesis testis

Pd/Fe_(3)O_(4) supported on bio-waste derived cellulosic-carbon as a nanocatalyst for C-C coupling and electrocatalytic application

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Frontiers of Chemical Science and Engineering 2022年第10期16卷 1514-1525页

作者： Vishal Kandathil Akshay Moolakkil Pranav Kulkarni Alaap Kumizhi Veetil manjunatha Kempasiddaiah Sasidhar Balappa Somappa R.Geetha Balakrishna Siddappa A.Patil Centre for Nano and Material Sciences Jain UniversityJain Global CampusBangalore 562112India Organic Chemistry Section Chemical Sciences&Technology DivisionNational Institute for Interdisciplinary Science and Technology(CSIR)Thiruvananthapuram 695019India

The current work describes the synthesis of a new bio-waste derived cellulosic-carbon supportedpalladium nanoparticles enriched magnetic nanocatalyst(Pd/Fe_(3)O_(4)@C)using a simple multi-step process under aerobic *** mild reaction conditions,the Pd/Fe_(3)O_(4)@C magnetic nanocatalyst demonstrated excellent catalytic activity in the Hiyama cross-coupling reaction for a variety of ***,the Pd/Fe_(3)O_(4)@C magnetic nanocatalyst exhibited excellent catalytic activity up to five recycles without significant catalytic activity loss in the Hiyama cross-coupling ***,we explored the use of Pd/Fe_(3)O_(4)@C magnetic nanocatalyst as an electrocatalyst for hydrogen evolution ***,the Pd/Fe_(3)O_(4)@C magnetic nanocatalyst exhibited better electrochemical activity compared to bare carbon and magnetite(Fe_(3)O_(4)nanoparticles)with an overpotential of 293 mV at a current density of 10 mA·cm^(–2).

关键词： bio-waste cellulosic-carbon Pd/Fe_(3)O_(4) Hiyama cross-coupling hydrogen evolution reaction recyclability

Impact of heat shock on heat shock proteins expression, biological and commercial traits of Bombyx mori

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Insect Science 2006年第4期13卷 243-250页

作者： VASUDHA B. CHAVADI APARNA H. SOSALEGOWDA manjunatha H.B OREGOWDA Departments of Sericulture Dharwad 580003 Karnataka India Departments of Biochemisrty Karnatak University Dharwad 580 003 Karnataka India

We report the thermotolerance of new bivoltine silkworm, Bombyx mori strains NB4D2, KSO1, NP2, CSR2 and CSR4 and differential expression of heat shock proteins at different instars. Different instars of silkworm larva were subjected to heat shock at 35℃, 40℃ and 45℃ for 2 hours followed by 2 hours recovery. Heat shock proteins were analyzed by SDS-PAGE. The impact of heat shock on commercial traits of cocoons was analyzed by following different strategies in terms of acquired thermotolerance over control. Comparatively NP2 exhibited better survivability than other strains. Resistance to heat shock was increased as larval development proceeds in the order of first instar 〉 second instar 〉 third instar 〉 fourth instar 〉 fifth instar in all silkworm strains. Expression of heat shock proteins varies in different instars. 90 kDa in the first, second and third instars, 84 kDa in the fourth instar and 84, 62, 60, 47 and 33 kDa heat shock proteins in fifth instar was observed in response to heat shock. Relative influence of heat shock on commercial traits that correspond to different stages was significant in all strains. In NB4D2, cocoon and shell weight significantly increased to 17.52% and 19.44% over control respectively. Heat shock proteins as molecular markers for evaluation and evolution of thermotolerant silkworm strains for tropics was discussed.

关键词： biological and commercial traits Bombyx mori heat shock heat shockproteins molecular chaperones thermotolerance