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Petroleum Science 2022年第6期19卷 3171-3181页

作者： Xue-man Wang Cheng-Long Wen Yu fan State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology Advanced Catalysis and Green Manufacturing Collaborative Innovation Centerand School of Petrochemical EngineeringChangzhou UniversityChangzhouJiangsu213164China

Hierarchical SAPO-11 molecular sieve(ACS-11) was successfully synthesized employing the Al2O3/carbon(Al_(2)O_(3)/C) composite obtained through the pyrolysis of Al-based metal-organic framework(Al-MOF-96)as *** other carbon-based mesoporogens with strong hydrophobicity,the Al_(2)O_(3)/C interacts with phosphoric acid and generates the AlPO_(4)/C structure,which promotes the Al2O3/C dispersion in the synthesis gel of SAPO-11 and avoids the phase separation between *** Al_(2)O_(3)/C as mesoporogen decreases the crystallite size of SAPO-11 via preventing the aggregation of ***,the addition of Al_(2)O_(3)/C improves the Si distribution in the ACS-11 ***,ACS-11 has smaller crystallites,more mesopores,and a greater amount of medium Bronsted acid centers than the conventional microporous SAPO-11 and the SAPO-11 synthesized using activated carbon as *** corresponding Pt/ACS-11 catalyst exhibits the maximal selectivity to multi-branched C10isomers(23.28%) and the minimal cracking selectivity(15.83%) in n-decane hydroisomerization among these *** research provides a new approach for preparing hierarchical silicoaluminophosphate molecular sieve-based catalysts to produce high-quality fuels.

关键词： Hierarchical SAPO-11 Al_(2)O_(3)/C composite Hydroisomerization Branched isomers

Chemoprophylaxis, diagnosis, treatments, and discharge management of COVID-19: An evidence-based clinical practice guideline(updated version)

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Military Medical Research 2020年第3期7卷 249-282页

作者： Ying-Hui Jin Qing-Yuan Zhan Zhi-Yong Peng Xue-Qun Ren Xun-Tao Yin Lin Cai Yu-Feng Yuan Ji-Rong Yue Xiao-Chun Zhang Qi-Wen Yang Jianguang Ji Jian Xia Yi-Rong Li Fu-Xiang Zhou Ya-Dong Gao Zhui Yu Feng Xu Ming-Li Tu Li-Ming Tan Min Yang fang Chen Xiao-Ju Zhang Mei Zeng Yu Zhu Xin-Can Liu Jian Yang Dong-Chi Zhao Yu-Feng Ding Ning Hou Fu-Bing Wang Hao Chen Yong-Gang Zhang Wei Li Wen Chen Yue-Xian Shi Xiu-Zhi Yang Xue-Jun Wang Yan-Jun Zhong Ming-Juan Zhao Bing-Hui Li Lin-Lu Ma Hao Zi Na Wang Yun-Yun Wang Shao-Fu Yu Lu-Yao Li Qiao Huang Hong Weng Xiang-Ying Ren Li-Sha Luo man-ru fan Di Huang Hong-Yang Xue Lin-Xin Yu Jin-Ping Gao Tong Deng Xian-Tao Zeng Hong-Jun Li Zhen-Shun Cheng Xiao-Mei Yao Xing-Huan Wang Center for Evidence-Based and Translational Medicine Zhongnan Hospital of Wuhan UniversityWuhan 430071China National Clinical Research Center for Respiratory Diseases China-Japan Friendship HospitalBeijing 100029China Department of Pulmonary and Critical Care Medicine China-Japan Friendship HospitalBeijing 10029China Leishenshan Hospital in Wuhan Wuhan 430200China Department of Critical Care Medicine Zhongnan Hospital of Wuhan UniversityWuhan 430071China Institutes of Evidence-based Medicine and Knowledge Translation Henan UniversityKaifeng 475000HenanChina Department of Medical Imaging Guizhou Provincial People’s HospitalGuiyang 550002China Departments of Orthopedics Zhongnan Hospital of Wuhan UniversityWuhan 430071China Department of Hepatobiliary Surgery Zhongnan Hospital of Wuhan UniversityWuhan 430071China National Clinical Research Center for Geriatrics West China Hospital of Sichuan UniversityChengdu 610041China Department of Geriatrics West China Hospital of Sichuan UniversityChengdu 610041China Department of Radiology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Department of Clinical Laboratory Peking Union Medical College Hospital(PUMCH)Peking Union Medical CollegeChinese Academy of Medical Sciences(CAMS)Beijing 100730China Center for Primary Health Care Research Lund University and Region Skåne25002 MalmöSweden Emergency Center Zhongnan Hospital of Wuhan UniversityWuhan 403371China Department of Allergology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Department of Radiation and Medical Oncology Zhongnan Hospital of Wuhan UniversityWuhan 43071China Department of Critical Care Medicine Renmin Hospital of Wuhan UniversityWuhan 430060China Department of Emergency Medicine and Chest Pain Center Qilu Hospital of Shandong UniversityJinan 250002China Department of Respiratory and Critical Care Medicine Suizhou Central HospitalHubei University of MedicineSuizhou 441300HubeiChina Department of Clinic Pharmacy Second People’s Hospital of Huaihua Ci

The novel severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)is the cause of a rapidly spreading illness,coronavirus disease 2019(COVID-19),affecting more than seventeen million people around the *** and treatment guidelines for clinicians caring for patients are *** the early stage,we have issued"A rapid advice guideline for the diagnosis and treatment of 2019 novel coronavirus(2019-nCoV)infected pneumonia(standard version)";now there are many direct evidences emerged and may change some of previous recommendations and it is ripe for develop an evidence-based *** formed a working group of clinical experts and *** steering group members proposed 29 questions that are relevant to the management of COVID-19 covering the following areas:chemoprophylaxis,diagnosis,treatments,and discharge *** searched the literature for direct evidence on the management of COVID-19,and assessed its certainty generated recommendations using the Grading of Recommendations,Assessment,Development and Evaluation(GRADE)*** were either strong or weak,or in the form of ungraded consensus-based ***,we issued 34 *** them,6 were strong recommendations for,14 were weak recommendations for,3 were weak recommendations against and 11 were ungraded consensus-based *** covered topics of chemoprophylaxis(including agents and Traditional Chinese Medicine(TCM)agents),diagnosis(including clinical manifestations,reverse transcription-polymerase chain reaction(RT-PCR),respiratory tract specimens,IgM and IgG antibody tests,chest computed tomography,chest X-ray,and CT features of asymptomatic infections),treatments(including lopinavirritonavir,umifenovir,favipiravir,interferon,remdesivir,combination of antiviral drugs,hydroxychloroquine/chloroquine,interleukin-6 inhibitors,interleukin-1 inhibitors,glucocorticoid,qingfei paidu decoction,lianhua qingwen granules/capsules,convalescent plasma,lung

关键词： COVID-19 SARS-CoV-2 Recommendation Chemoprophylaxis Diagnosis Treatment Discharge management Traditional Chinese medicine guideline

Synthesis of ZSM-22/SAPO-11 composite molecular sieve-based catalysts with small crystallites and superior n-alkane hydroisomerization performance

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Petroleum Science 2023年第4期20卷 2585-2595页

作者： Xue-man Wang Cheng-Long Wen Yu fan State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing102249China Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology Advanced Catalysis and Green Manufacturing Collaborative Innovation CenterSchool of Petrochemical EngineeringChangzhou UniversityChangzhouJiangsu213164China

To improve oil quality,ZSM-22/SAPO-11 composite molecular sieves were synthesized by adding ZSM-22 into a synthetic gel of SAPO-11 for n-decane *** mass ratios of ZSM-22/(ZSM-22+SAPO-11)in the composite molecular sieves were optimized and the optimal ZSM-22/SAPO-11 composite(ZS-9)was *** electrostatic repulsions between the ZSM-22 precursors and the SAPO-11 crystalline nuclei produced small ZSM-22 and SAPO-11 crystallites in ZS-9,which increased the specific surface area and mesopore volume and thereby exposed more acid *** comparison with conventional SAPO-11,ZSM-22 and their mechanical mixture,ZS-9 with smaller crystallites and the optimal medium and strong Brønsted acid centers(MSBAC)content displayed a higher yield of branched C_(10) isomers(81.6%),lower cracking selectivity(11.9%)and excellent *** correlation between the i-C_(10) selectivity and the MSBAC density of molecular sieves indicated that the selectivity for branched C_(10) isomers first increased and then decreased with increasing MSBAC density on the molecular sieves,and the maximum selectivity(87.7%)occurred with a density of 9.6×10^(−2)μmol m^(−2).

关键词： ZSM-22/SAPO-11 composite molecular sieves Medium and strong brønsted acid centers Crystallite size Branched C_(10)isomers

Berry-Esseen Bounds for Self-Normalized Martingales

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Communications in Mathematics and Statistics 2018年第1期6卷 13-27页

作者： Xiequan fan Qi-man Shao Center for Applied Mathematics Tianjin UniversityTianjin 300072China Department of Statistics Chinese University of Hong KongShatinNTHong Kong

A Berry–Esseen bound is obtained for self-normalized martingales under the assumption of finite *** bound coincides with the classical Berry–*** of the *** to Student’s statistic and autoregressive process are also... 详细信息

关键词： Self-normalized process Berry-Esseen bounds Martingales Student’s statistic Autoregressive process

Reaction mechanism of methyl nitrite dissociation during co catalytic coupling to dimethyl oxalate:A density functional theory study

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Chinese Journal of Chemical Engineering 2016年第1期24卷 132-139页

作者： Chen fan man Luo Wende Xiao Key Laboratory of Advanced Control and Optimization for Chemical Processes Ministry of Education East China University of Science and Technology (ECUST) School of Chemistry and Chemical Engineering Shanghai Jiao Tong University (SJTU)

Dissociation of methyl nitrite is the first step during CO catalytic coupling to dimethyl oxalate followed by hydrogenation to ethyl glycol in a typical coal to liquid process. In this work, the first-principle calculations based on density functional theory were performed to explore the reaction mechanism for the non-catalytic dissociation of methyl nitrite in the gas phase and the catalytic dissociation of methyl nitrite on Pd(111) surface since palladium supported on alpha-alumina is the most effective catalyst for the coupling. For the non-catalytic case, the calculated results show that the CH_3O–NO bond will break with a bond energy of 1.91 eV, and the produced CH_3O radicals easily decompose to formaldehyde, while the further dissociation of formaldehyde in the gas phase is difficult due to the strong C–H bond. On the other hand, the catalytic dissociation of methyl nitrite on Pd(111) to the adsorbed CH_3O and NO takes place with a small energy barrier of 0.03 eV. The calculated activation energies along the proposed reaction pathways indicate that(i) at low coverage, a successive dehydrogenation of the adsorbed CH_3O to CO and H is favored while(ii) at high coverage, hydrogenation of CH_3O to methanol and carbonylation of CH_3O to methyl formate are more preferred. On the basis of the proposed reaction mechanism,two meaningful ways are proposed to suppress the dissociation of methyl nitrate during the CO catalytic coupling to dimethyl oxalate.

关键词： Methyl nitrite Catalytic Non-catalytic Dissociation Density functional theory

Diagnosis based on electromagnetic navigational bronchoscopyguided biopsied peripheral lung lesions in a 10-year-old girl:A case report

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World Journal of Clinical Cases 2023年第15期11卷 3651-3657页

作者： fan-Zheng Meng Qiong-Hua Chen man Gao Li'e Zeng Jie-ru Lin Jing-Yang Zheng Department of Pediatrics The First Hospital of Jilin UniversityChangchun 130021Jilin ProvinceChina Department of Respiratory Medicine The Third Clinical Medical CollegeFujian Medical UniversityQuanzhou Women's and Children's HospitalQuanzhou 362000Fujian ProvinceChina Department of Respiratory Medicine Quanzhou Women's and Children's HospitalQuanzhou 362000Fujian ProvinceChina Department of Respiratory Medicine Quanzhou Women's and Children's HospitalThe Third Clinical Medical CollegeFujian Medical UniversityQuanzhou 362000Fujian ProvinceChina

BACKGROUND Electromagnetic navigational bronchoscopy(ENB)is an emerging diagnostic tool that enables practitioners to biopsy peripheral lung tissues that were previously only accessible under computed tomography(CT)***,few studies have investigated ENB use in ***,we report a case of a 10-yearold girl with peripheral lung lesions who complained of a 7-d persistent *** was diagnosed with Streptococcus parasanguinis infection based on findings obtained using ENB-guided transbronchial lung biopsy(TBLB).CASE SUMMARY A 10-year-old girl presented with constitutional symptoms of cough and fever of 7 days’*** CT scans detected peripheral lung lesions and no endobronchial *** performed under the guidance of an ENB Lungpro navigation system was safe,well-tolerated,and effective for biopsying peripheral lung *** of biopsied samples indicated the patient had a pulmonary Streptococcus parasanguinis infection,which was treated with antibiotics instead of more invasive treatment *** patient’s symptoms resolved after she received a 3-wk course of oral *** of pretreatment and post-treatment CT scans revealed absorption of some lung lesions within 7 mo of hospital *** ENB-guided TBLB biopsying of peripheral lung lesions in this child is a safe,well-tolerated,and effective alternative to conventional interventions.

关键词： Electromagnetic navigational bronchoscopy Lungpro Transbronchial lung biopsy Child Diagnosis Case report

Thermal conductivity prediction of MgAl2O4:a non-equilibrium molecular dynamics calculation

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Journal of Iron and Steel Research International 2020年第5期27卷 500-505页

作者： Cheng-ming Ni Hua-wei fan Xu-dong Wang man Yao School of Materials Science and Engineering Dalian University of TechnologyDalian 116000LiaoningChina

Magnesium aluminate spinel(MgAl2O4)is widely used in steel metallurgy *** conductivity at high temperature signifcantly infuences the cooling process of blast furnace and the heat preservation of steel *** efect of external(temperature)and internal(antisite defect and grain boundary)factors on the thermal conductivity of MgAl2O4 was studied with non-equilibrium molecular *** main factors afecting the thermal conductivity of MgAl2O4 were *** the temperature range of 100-2000 K,the results showed that the thermal conductivity of MgAl2O4 changed from 11.54 to 4.95 W/(m K)with the increase in temperature and was relatively stable at the temperature above 1000 *** thermal conductivity of MgAl2O4 declined frst and then rose with the increase in the antisite defects,and the minimum value was 6.95 W/(m K)at the inversion parameter i=*** addition,grain boundaries reduced the thermal conductivity of MgAl2O4 by 20%-30%at temperature below 1000 K comparing with the non-grain boundary *** grain boundary rotation angle at temperature above 1000 K had less efect on the thermal conductivity than that below 1000 *** simulation scheme for thermal conductivity of MgAl2O4 can also be applied to the study of other nonmetallic ceramics.

关键词： Non-equilibrium molecular dynamics Thermal conductivity Magnesium aluminate spinel Antisite defect Grain boundary

Kernel Quantile Estimator with ICI Adaptive Bandwidth Selection Technique

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Acta Mathematica Sinica,English Series 2014年第4期30卷 710-722页

作者： Jie Yu fan man Lai TANG Mao Zai TIAN Department of Statistics University of Pittsburgh Department of Mathematics and Statistics Hang Seng Management College School of Statistics Lanzhou University of Finance and Economics Center for Applied Statistics School of StatisticsRenmin University of China

In this article, we consider a class of kernel quantile estimators which is the linear combi- nation of order statistics. This class of kernel quantile estimators can be regarded as an extension of some existing estimators. The exact mean square error expression for this class of estimators will be provided when data are uniformly distributed. The implementation of these estimators depends mostly on the bandwidth selection. We then develop an adaptive method for bandwidth selection based on the intersection confidence intervals （ICI） principle. Monte Carlo studies demonstrate that our proposed approach is comparatively remarkable. We illustrate our method with a real data set.

关键词： Adaptive bandwidth selection ICI principle kernel estimator quantiles

Thermal environment investigation of asymmetric radiation coupled with convection heating

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Building Simulation 2022年第7期15卷 1309-1321页

作者： man fan Jia Wang Lanlan Zhang Han Li Xiangfei Kong Chenxiao Zheng School of Energy and Environmental Engineering Hebei University of TechnologyTianjin 300401China State Key Laboratory of Building Safety and Built Environment Beijing 100013China National Engineering Research Center of Building Technology Beijing 100013China School of Mechanical Engineering Tianjin University of CommerceTianjin 300134China

The couple of radiation with convection heating owned advantages of less energy utilization,healthier and more comfortable indoor ***,local thermal discomfort was often induced by large vertical temperature difference and radiation asymmetry *** work studied indoor thermal environment characteristics under different coupling ways of radiation and convection heating terminals through experiments and CFD *** studied five scenarios were denoted as:(Ⅰ)lateral air supply+adjacent side wall radiation,(Ⅱ)lateral air supply+opposite side wall radiation,(Ⅲ)lateral air supply+floor radiation,(Ⅳ)lateral air supply+adjacent side wall radiation+floor radiation,and(Ⅴ)lateral air supply+opposite side wall radiation+floor *** overall thermal comfort indices(including air diffusion performance index(ADPI),predicted mean vote(PMV),and predicted percent of dissatisfaction(PPD))and local thermal comfort indices under different scenarios were *** Scenarios Ⅰ-Ⅲ,the local dissatisfaction rates caused by vertical air temperature difference were 0.4%,0.1%,and 0.2%,respectively,which belonged to"A”class according to the ISO-7730 *** the vertical asymmetric radiation temperature of Scenario Ⅰ-Ⅱ was about 6.5℃ lower than that of Scenario Ⅲ-Ⅳ-Ⅴ.The ADPI for Scenarios Ⅲ-Ⅴ were about respectively 5.7%,16.7%,and 21.0%higher than that of Scenarios Ⅰ-Ⅱ,indicating that a large radiation area and radiation angle coefficient could reduce the discomfort caused by radiant temperature *** coupling mode improved local discomfort by decreasing vertical temperature difference and radiation asymmetry temperature wherefore improving the PMV from-1.6 *** lateral air supply coupled with asymmetric radiation heating could potentially improve the thermal comfort of occupied area,while the comprehensive effect of thermal environmental improvement,energy-saving,and cost-effectiveness needes to be further investigated.

关键词： asymmetric radiation lateral air supply overall thermal comfort-local thermal comfort CFD simulation

Complementary doping of van der Waals materials through controlled intercalation for monolithically integrated electronics

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Nano Research 2020年第5期13卷 1369-1375页

作者： Ming Ke Huu Duy Nguyen Hang fan man Li Huan Wu Yongjie Hu School of Engineering and Applied Science University of CaliforniaLos AngelesCalifornia 90095USA

Doping control has been a key challenge for electronic applications of van der Waals ***,we demonstrate complementary doping of black phosphorus using controlled ionic intercalation to achieve monolithic building *** characterize the anisotropic electrical transport as a function of ion concentrations and report a widely tunable resistivity up to three orders of magnitude with characteristic concentration dependence corresponding to phase transitions during *** a further step,we develop both p-type and n-type field effect transistors as well as electrical diodes with high device stability and *** addition,enhanced charge mobility from 380 to 820 cm^2/(V·s)with the intercalation process is observed and explained as the suppressed neutral impurity scattering based on our ab initio *** study provides a unique approach to atomically control the electrical properties of van der Waals materials,and may open up new opportunities in developing advanced electronics and physics platforms.

关键词： nanoelectronics two-dimensional(2D)materials and heterostructures FET diode tunable properties black phosphorus