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Micelle-directed self-assembly of single-crystal-like mesoporous stoichiometric oxides for high-performance lithium storage

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National Science Review 2024年第4期11卷 195-205页

作者： Yanhua Wan Changyao Wang Xingmiao Zhang Yang Yin Mengmeng Liu Bing ma Linlin duan Yuzhu ma Wei Zhang Changlin Zheng dongliang Chao Fei Wang Yongyao Xia Wei Li department of Chemistry Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of Polymers College of Chemistry and Materials ScienceFudan University State Key Laboratory of Surface Physics and department of Physics Fudan University

due to their uncontrollable assembly and crystallization process,the synthesis of mesoporous metal oxide single crystals remains a formidable ***,we report the synthesis of single-crystal-like mesoporous Li2TiSiO5by using soft micelles as *** key lies in the atomic-scale self-assembly and step-crystallization processes,which ensure the formation of single-crystal-like mesoporous Li2TiSiO5microparticles via an oriented attachment growth mechanism under the confinement of an in-situ formed carbon *** mesoporous Li2TiSiO5anode achieves a superior rate capability(148 mah g-1at5.0 A g-1) and outstanding long-term cycling stability(138 mah g-1after 3000 cycles at 2.0 A g-1) for lithium storage as a result of the ultrafast Li+diffusion caused by penetrating mesochannels and nanosized crystal frameworks（5-10 nm）.In comparison,bulk Li2TiSiO5exhibits poor rate capability and cycle performance due to micron-scale diffusion *** method is very simple and reproducible,heralding a new way of designing and synthesizing mesoporous single crystals with controllable frameworks and chemical functionalities.

关键词： mesoporous materials micelles single-crystal-like Li2TiSiO5 lithium-ion batteries

dietary supplementation of benzoic acid and essential oils combination enhances intestinal resilience against LPS stimulation in weaned piglets

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Journal of Animal Science and Biotechnology 2024年第2期15卷 878-897页

作者： Chang Cui Yulong Wei Yibo Wang Wen ma Xiaoyu Zheng Jun Wang Ziwei ma Caichi Wu Licui Chu Shihai Zhang Wutai Guan Fang Chen Guangdong Provincial Key Laboratory of Animal Nutrition Control College of Animal ScienceSouth China Agricultural UniversityGuangzhou 510642China College of Animal Science and National Engineering Research Center for Breeding Swine Industry South China Agricultural UniversityGuangzhou 510642China Guangdong Laboratory for Lingnan Modern Agriculture South China Agricultural UniversityGuangzhou 510642China

Background The benefits of combining benzoic acid and essential oils(BAO)to mitigate intestinal impairment during the weaning process have been well established,while the detailed underlying mechanism has not been fully *** research has primarily focused on the reparative effects of BAO on intestinal injury,while neglecting its potential in enhancing intestinal stress *** In this study,we investigated the pre-protective effect of BAO against LPS-induced stress using a modified experimental *** were pre-supplemented with BAO for 14 d,followed by a challenge with LPS or saline to collect blood and intestinal *** Our findings demonstrated that BAO supplementation led to significant improvements in piglets’final weight,average daily gain,and feed intake/body gain ***,BAO supplementation positively influenced the composition of intestinal microbiota,increasing beneficial Actinobacteriota and Alloprevotella while reducing harmful desulfobacterota,Prevotella and ***,BAO supplementation effectively mitigated oxidative disturbances and inflammatory responses induced by acute LPS *** was evidenced by elevated levels of T-AOC,SOd,and GSH,as well as decreased levels of MdA,TNF-α,and IL-6 in the ***,piglets subjected to LPS challenge and pre-supplemented with BAO exhibited significant improvements in intestinal morphological structure and enhanced integrity,as indicated by restored expression levels of Occludin and Claudin-1 compared to the non-supplemented *** analysis revealed that BAO supplementation enhanced the jejunal antioxidative capacity by increasing GSH-Px levels and decreasing MdA levels under the LPS challenge and stimulated the activation of the Nrf2 signaling ***,the reduction of TLR4/NF-κB/maPK signaling pathways activation and proinflammatory factor were also observed in the jejunal of those piglets fed with ***

关键词： Anti-stress Benzoic acid Essential oils Intestine LPS Weaned piglets

Weather-driven Solar Power Forecasting Using d-Informer:Enhancing Predictions with Climate Variables

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Energy Engineering 2024年第5期121卷 1245-1261页

作者： Chenglian ma Rui Han Zhao An Tianyu Hu Meizhu Jin School of Electrical Engineering Northeast Electric Power UniversityJilin132013China Shenzhen Institute of Advanced Technology Chinese Academy of SciencesShenzhen518055China

Precise forecasting of solar power is crucial for the development of sustainable energy *** forecasting approaches often fail to adequately consider the crucial role of weather factors in photovoltaic(PV)power generation and encounter issues such as gradient explosion or disappearance when dealing with extensive time-series *** overcome these challenges,this research presents a cutting-edge,multi-stage forecasting method called *** method skillfully merges the differential transformation algorithm with the Informer model,leveraging a detailed array of meteorological variables and historical PV power generation *** d-Informer model exhibits remarkable superiority over competing models across multiple performance metrics,achieving on average a 67.64%reduction in mean squared error(MSE),a 49.58%decrease in mean absolute error(maE),and a 43.43%reduction in root mean square error(RMSE).Moreover,it attained an R2 value as high as 0.9917 during the winter season,highlighting its precision and *** significant advancement can be primarily attributed to the incorporation of a multi-head self-attention mechanism,which greatly enhances the model’s ability to identify complex interactions among diverse input variables,and the inclusion of weather variables,enriching the model’s input data and strengthening its predictive accuracy in time series ***,the experimental results confirm the effectiveness of the proposed approach.

关键词： Power forecasting deep learning weather-driven solar power

In^(3+)-doped Sr_(2)Fe_(1.5)Mo_(0.5)O_(6−δ)cathode with improved performance for an intermediate-temperature solid oxide fuel cell

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Nano Research 2024年第1期17卷 407-415页

作者： Yumei ma Lijie Zhang Kang Zhu Binze Zhang Ranran Peng Changrong Xia Ling Huang State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China department of materials Science and Engineering University of Science and Technology of ChinaHefei 230026China

Promoting the oxygen reduction reaction(ORR)is critical for commercialization of intermediate-temperature solid oxide fuel cells(IT-SOFCs),where Sr_(2)Fe_(1.5)Mo_(0.5)O_(6)−δ(SFM)is a promising cathode by working as a mixed ionic and electronic *** this work,doping of In^(3+)greatly increases the oxygen vacancy concentration and the content of adsorbed oxygen species in Sr_(2)Fe_(1.5)Mo_(0.5−x)InxO_(6−δ)(SFMInx),and thus effectively promotes the ORR *** a typical example,SFMIn_(0.1)reduces the polarization resistance(R_(p))from 0.089 to 0.046Ω∙cm^(2)at 800°C,which is superior to those doped with other metal *** addition,SFMIn0.1 increases the peak power density from 0.92 to 1.47 W∙cm^(−2)at 800°C with humidified H_(2)as the fuel,indicating that In3+doping at the Mo site can effectively improve the performance of SOFC cathode material.

关键词： solid oxide fuel cell cathode In3+doping oxygen reduction reaction(ORR) Sr_(2)Fe_(1.5)Mo_(0.5)O_(6-δ)

Bubble dynamics properties of B-particles in a quasi-2d gas-solid fluidized bed:Computational particle fluid dynamics numerical simulation and post-processed by digital image analysis technique

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Particuology 2024年第3期86卷 223-238页

作者： Zemin Yuan Zhong Huang Guotao Qin Guanjia Zhao Suxia ma Hairui Yang Guangxi Yue Key Laboratory of Clean and Efficient Combustion and Utilization in the Circulating Fluidized Bed Taiyuan University ofTechnologyTaiyuan030024China department of Energy and Power Engineering Tsinghua UniversityBeijing100084.China

Bubble dynamics properties play a crucial and significant role in the design and optimization of gas-solid fluidized *** this study,the bubble dynamics properties of four B-particles were investigated in a quasi-two-dimensional(quasi-2d)fluidized bed,including bubble equivalent diameter,bubble size distribution,average bubble density,bubble aspect ratio,bubble hold-up,bed expansion ratio,bubble radial position,and bubble *** studies were performed by computational particle fluid dynamics(CPFd)numerical simulation and post-processed with digital image analysis(dIA)technique,at superficial gas velocities ranging from 2u_(mf) to 7u_(mf).The simulated results shown that the CPFd simulation combining with dIA technique post-processing could be used as a reliable method for simulating bubble dynamics properties in quasi-2d gas-solid fluidized ***,it seemed not desirable for the simulation of bubble motion near the air distributor at higher superficial gas velocity from the simulated average bubble density *** superficial gas velocity significantly affected the bubble equivalent diameter and evolution,while it had little influence on bubble size distribution and bubble aspect ratio distribution for the same *** time-averaged bubble hold-up and bed expansion ratio increased with the increase of superficial gas *** core-annular flow structures could be found in the fluidized bed for all *** average bubble rising velocity increased with the increasing bubble equivalent *** bubble lateral movement,the smaller bubbles might be more susceptible,and superficial gas velocity had a little influence on the absolute lateral velocity of *** simulated results presented a valuable and novel approach for studying bubble dynamics *** comprehensive understanding of bubble dynamics behaviors in quasi-2d gas-solid fluidized beds would provide support in the design,operation,and optimization of gas-solid

关键词： Bubble dynamics properties CPFd simulation Quasi-2d gas-solid fluidized bed digital image analysis

Recent Advances in 0d Ni/Co-based Hollow Electrocatalysts for Electrochemical Water Splitting

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Chemical Research in Chinese Universities 2024年第3期40卷 437-450页

作者： GE Wenjing CHEN Xiaocui ma Ruizhao ZHENG Siyuan SHANG Ningzhao ZHAO Xiaoxian department of Chemistry College of ScienceHebei Agricultural UniversityBaoding 071001P.R.China

Electrochemical water splitting using renewable energy sources has been recognized as a sustainable way to produce hydrogen energy due to the characteristics of low-carbon and no ***,the slow hydrogen/oxygen evolution reactions(HER/OER)seriously hinder the practical application of large-scale water *** this paper,the 0d Ni/Co-based hollow material is discussed in detail because of adjustable morphology,low mass density and abundant active sites,which provides an effective solution for improving the HER/OER reaction *** synthesis methods of hollow materials,such as hard template,soft template and self-template are ***,catalysts with different structural designs of hollow structures are reviewed,including hollow single-shelled structure,hollow core-shelled structure,hollow double-shelled structure and hollow multi-shelled structure(HoMS)***,the research progress of the 0d Ni/Co-based HoMS electrocatalysts in recent years and their prominent performances in water splitting are ***,the challenges and development prospects of designing Ni/Co-based HoMS catalysts in water splitting in the future are discussed.

关键词： Electrochemical watersplitting Morphological regulation Hollow structure Hollow multi-shelled structure(HoMS)

Ammonia storage and slip under steady and transient state in close-coupled SCR

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Journal of Environmental Sciences 2024年第4期138卷 470-481页

作者： Shiyu Liu Zhaohuan Zhang Zexian Guo Boyuan Wang Buyu Wang Xiao ma Shijin Shuai State Key Laboratory of Automotive safety and Energy Tsinghua UniversityBeijing 100084China Institute for Aero Engine Tsinghua UniversityBeijing 100084China

The close-coupled selective catalytic reduction(cc-SCR)catalyst is an effective technology to reduce tailpipe NOx emission during cold *** paper investigated the optimal ammonia storage under steady and transient state in the *** study showed that a trade-off between NOx conversion efficiency and ammonia slip is observed on the pareto solutions under steady state,and the optimal ammonia storage is calculated with ammonia slip less than 10μL/L based on the ChinaⅥemission *** rapid temperature increase will lead to severe ammonia slip in the transient test cycle.A simplified 0-d calculation method on ammonia slip under transient state is proposed based on kinetic model of ammonia adsorption and *** addition,the effect of ammonia storage,catalyst temperature and temperature increasing rate on ammonia slip are *** optimal ammonia storage is calculated with maximum ammonia slip less than 100μL/L according to the oxidation efficiency of ammonia slip catalyst(ASC)downstream *** was found that the optimal ammonia storage under transient state is much lower than that under steady state in cc-SCR at lower temperature,and a phase diagram is established to analyze the influence of temperature and temperature increasing rate on optimal ammonia storage.

关键词： Close-coupled SCR Ammonia storage and slip Steady and transient state Generic algorithm

Analyst Coverage,Forecasting Bias,and Corporate Innovation:Evidence from China

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Journal of Systems Science and Information 2024年第1期12卷 1-24页

作者： Xinping ma Yiru WANG Jianping LI Biao SHI School of Economics and management University of Chinese Academy of SciencesBeijing 100049China School of Finance Nankai UniversityTianjin 300071China Institutes of Science and development Chinese Academy of SciencesBeijing 100190China

due to information asymmetry and strategic innovation,firms often encounter challenges related to insufficient driving forces and low-quality innovation *** always act as information intermediaries who help foster the advancement of corporate innovation activities and the conversion of innovation *** study examines the impact of analyst coverage and forecasting bias on corporate innovation,employing data from China A-shared listed firms spanning the period 2007 to *** measure corporate innovation from two perspectives:Input and ***,we use the ratio of research and development(R&d)expenditure to sales as a proxy for the innovation input and the number of patent citations excluding self-citations to measure innovation *** find that analyst coverage promotes corporate innovation,which is consistent with the“bright”side of analyst ***,the positive effect of analyst coverage hinges on effectively transmitting and disclosing accurate information to investors in the capital *** on this,analysts'forecasting bias includes forecasting dispersion and optimism *** find evidence that an increase in analysts'forecast dispersion leads to a decrease in corporate innovation ***,this paper presents a novel approach by employing the regression discontinuity method to examine the effect of analyst optimistic bias on firm *** empirical findings reveal that overly optimistic forecasts by analysts exacerbate innovation *** analyses enrich the research on analyst coverage and corporate innovation,providing an empirical basis for improving the capital market with the help of analysts.

关键词： analyst coverage forecasting bias corporate innovation innovation quality

A statistical analysis of the Kappa-type energy spectrum distribution of radiation belt electrons observed by Van Allen Probes

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Earth and Planetary Physics 2024年第2期8卷 368-374页

作者： LuHuai Jiao Xin ma YuanNong Zhang TaiFeng Jin Song Fu BinBin Ni department of Space Physics School of Electronic InformationWuhan UniversityWuhan 430072China

The energy spectrum of energetic electrons is a key factor representing the dynamic variations of Earth’s Van Allen radiation *** measurements have indicated that the commonly used maxwellian and Kappa distributions are inadequate for capturing the realistic spectral distributions of radiation belt *** we adopt the Kappa-type(KT)distribution as the fitting function and perform a statistical analysis to investigate the radiation belt electron flux spectra observed by the Van Allen *** calculating the optimal values of the key KT distribution parameters(i.e.,κandθ2)from the observed spectral shapes,we fit the radiation belt electron fluxes at different L-shells under different geomagnetic *** this manner,we obtain typical values of the KT distribution parameters,which are statistically feasible for modeling the radiation belt electron flux profiles during either geomagnetically quiet or active periods.A comparison of the KT distribution model results with those using the maxwellian or Kappa distribution reveals the advantage of the KT distribution for studying the overall properties of the radiation belt electron spectral distribution,which has important implications for deepening the current understanding of the radiation belt electron dynamics under evolving geomagnetic conditions.

关键词： radiation belt electron Kappa-type distribution fitting geomagnetic storm