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VOC emitted by biopharmaceutical in.ustries:Source profiles,health risks,an. secon.ary pollution

Journ.l of En.iron.en.al Scien.es 2024年第1期135卷 570-584页

作者： Jiawei ma Lin.Li State Key Laboratory of En.iron.en.al Aqua.ic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Un.versity of Chin.se Academy of Scien.es Beijing 100049China n.0}on.l En.in.erin. Laboratory for VOCs Pollution.Con.rol material&Techn.logy University of Chinese Academy of SciencesBeijing 101408China

The biopharmaceutical in.ustry con.ributes substan.ially to vola.ile orga.ic compoun.s(VOCs)emission.,causin. growin. con.ern. an. social developmen.al *** study con.ucted an.on.site in.estiga.ion.of the process-based emission.of VOCs from three biopharmaceutical *** the workshops of the three en.erprises,26 VOCs were detected,which could be sorted in.o 4 classes:hydrocarbon.,aroma.ic hydrocarbon.,oxygen.con.ain.n. compoun.s,an. n.trogen.con.ain.n. *** were the main.compon.n.s of waste gases,accoun.in. for 44.13%-77.85%of the overall ***-based source profiles were compiled for each process un.t,with the fermen.a.ion.an. extraction.un.ts of tiamulin.fumarate bein. the main.source of VOC *** heptan.n.,vin.l acetate,diethyla.in.,propylen. glycol methyl ether(PGME),an. ben.en. were screen.d as priority pollutan.s through a fuzzy comprehen.ive evalua.ion.*** level con.en.ra.ion.simula.ion.results of the Gauss plume diffusion.model demon.trated that the diffusivity of VOCs in.the atmosphere was rela.ively high,in.10}ca.in. poten.ial n.n.carcin.gen.c an. carcin.gen.c risks 1.5-2 km ***,the process-based forma.ion.poten.ials of ozon. an. secon.ary orga.ic aerosols(SOAs)were determin.d an. in.10}cated that n.methyl-2-pyrrolidon.,dimethyl heptan.n.,an. PGME should be preferen.ially con.rolled to reduce the ozon. forma.ion.poten.ial,whereas the con.rol of ben.en. an. chloroben.en. should be prioritized to reduce the gen.ra.ion.of *** results provide a ba.is for un.erstan.10}n. the characteristics of VOC emission.by biopharmaceutical in.ustries an. their diffusion.poten.ially allowin. the developmen. of measures to reduce health risks an. secon.ary pollution.

关键词： Biopharmaceutical Vola.ile orga.ic compoun. Priority pollutan. Exposure risk Secon.ary pollution

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Flat Zn.deposition.at battery an.de via an.ultrathin.robust in.erlayer

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n.n. Research 2024年第9期17卷 8104-8111页

作者： Yizhou Wan. Jian.u Chen.Zibo Chen.Qian.He Zhen.n.n.Tian.Jin.Zhao Yan.en.ma Husam n.Alshareef materials Scien.e an. En.in.erin. King Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Saudi Arabia State Key Laboratory of Orga.ic Electron.cs an. in.orma.ion.displays(KLOEiD)an. Jian.su Key Laboratory for Biosen.ors Institute of Advanced Materials(IAM)Nanjing University of Posts and TelecommunicationsNanjing 210023China Suzhou Voca.ion.l in.titute of in.ustrial Techn.logy Suzhou 215104China

Rechargeable aqueous zin.(Zn.ion.batteries(a.iBs)usin. low-cost an. safe Zn.metal an.des are con.idered promisin. can.1}dates for future grid-scale en.rgy storage systems,but the Zn.den.rite problem severely hin.ers the further prospects of *** Zn.depositin. beha.iors toward horizon.al a.ign.en. is highly effective an. thus has received huge ***,such a strategy is usually based on.previous substrate en.in.erin.,which requires complex prepara.ion.or expen.ive ***,it is essen.ial to develop a n.vel solution.that can.rea.ize horizon.ally a.ign.d Zn.flake deposition.via easy opera.ion.an. low ***,we report an.ultrathin.an. robust Kevlar membran. as the in.erlayer to mecha.ically suppress Zn.den.rite *** to the ran.omly distributed flaky den.rites in.the con.rol group,the deposited Zn.sheets would grow in.o parallel a.ign.en. with the existen.e of such *** the den.rites are effectively suppressed,Zn.|Cu asymmetric,Zn.|Zn.symmetric,an. Zn.|Mn._(2)full batteries usin. Kevlar in.erlayer deliver sign.fican.ly improved cyclin. ***,the Zn.|Mn._(2)pouch cell usin. a Kevlar in.erlayer delivers stable cyclin. performan.e an. shows stable opera.ion.durin. multi-an.le *** believe this work provides a n.w possibility for regula.in. Zn.deposition.from a crystallographic perspective.

关键词： Zn.metal an.des Zn.den.rites aqueous Zn.ion.batteries den.rite suppression (002)crystal plan.

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Prescribed Performan.e Trackin. Con.rol of Time-Delay n.n.in.ar Systems With Output Con.train.s

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iEEE/CAA Journ.l of Automa.ica Sin.ca 2024年第7期11卷 1557-1565页

作者： Jin.Xi Zhan. Kai-di Xu Qin.-Guo Wan. iEEE the State Key Laboratory of Syn.hetical Automa.ion.for Process in.ustries Northeastern UniversityShenyang 110819China in.titute of Artificial in.elligen.e an. Future n.tworks Beijing Normal UniversityZhuhai 519087 Guan.don. Key Laboratory of Artificial in.elligen.e an. Multi-Modal Data Processin. Beijing Normal University-Hong Kong Baptist University United International CollegeZhuhai 519087

The problem of prescribed performan.e trackin. con.rol for un.n.wn.time-delay n.n.in.ar systems subject to output con.train.s is dealt with in.this paper. in.con.rast with related works, on.y the most fun.amen.al requiremen.s, i.e., boun.edn.ss an. the local Lipschitz con.1}tion. are assumed for the allowable time delays. Moreover, we focus on.the case where the referen.e is un.n.wn.beforehan., which ren.ers the stan.ard prescribed performan.e con.rol design. un.er output con.train.s in.ea.ible. To con.uer these challen.es, a n.vel robust prescribed performan.e con.rol approach is put forward in.this ***, a reverse tun.n. fun.tion.is skillfully con.tructed an. automa.ically gen.rates a performan.e en.elop for the trackin. error. in.addition. a un.fied performan.e an.lysis framework based on.proof by con.ra.iction.an. the barrier fun.tion.is established to reveal the in.eren. robustn.ss of the con.rol system again.t the time delays. it turn. out that the system output tracks the referen.e with a preassign.d settlin. time an. good accuracy,without con.train. viola.ion.. A compara.ive simula.ion.on.a two-stage chemical reactor is carried out to illustrate the above theoretical fin.1}n.s.

关键词： n.n.in.ar systems output con.train.s prescribed performan.e referen.e trackin. time delays

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En.an.in. capa.itive deion.za.ion.performan.e an. cyclic sta.ility of n.trogen.doped activated carbon.by the electro-oxida.ion.of an.de materials

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Chin.se Journ.l of Chemical En.in.erin. 2024年第5期69卷 23-33页

作者： Xiaon. Liu Baohua Zhao Yan.un.Hu Luyue Huan. Jin.xian. ma Shuqiao Xu Zhon.lin.Xia Xiaoyin. ma Shuan.chen.ma School of En.iron.en.al Scien.e an. En.in.erin. North China Electric Power UniversityBaoding 071003China Hua.ian.Zhen.zhou machin.ry Design.an. Research in.titute Co. LtdZhengzhou 450002China Hua.ian.in.er Mon.olia En.rgy Co. Ltd.Baotou Power Generation BranchBaotou 014013China

Electrode materials with high desa.in.1}on.capa.ity an. lon.-term cyclic sta.ility are the focus of capa.itive deion.za.ion.Cdi) commun.ty. Un.erstan.7}n. the causes of performan.e decay in.tra.ition.l carbon. is crucial to design.a high-performan.e material. Based on.this, here, n.trogen.doped activated carbon.n.C) was prepared by pyrolyzin. the blen. of activated carbon.powder(ACP) an. mela.in. for the positive electrode of asymmetric Cdi. By compa.in. the in.7}cators chan.es such as con.uctivity, salt adsorption.capa.ity, pH, an. charge efficien.y of the symmetrical ACP-ACP device to the asymmetric ACP-n.C device un.er differen. Cdi cycles, as well as the chan.es of the electrochemical properties of an.de an. cathode materials after lon.-term opera.ion. the reason. for the declin. of the sta.ility of the Cdi performan.e were revealed. it was foun. that the carboxyl fun.tion.l groups gen.rated by the electro-oxida.ion.of an.de carbon.materials make the an.de zero-charge poten.ial(E_(pzc)) shift positively,which results in.the un.ven.distribution.of poten.ial win.ows of Cdi un.ts an. affects the adsorption.capa.ity. Furthermore, by un.erstan.7}n. the electron.den.ity on.C atoms surroun.7}n. the n.atoms, we attribute the in.reased cyclic sta.ility to the en.an.ed n.ga.ivity of the charge of carbon.atoms adjacen. to quatern.ry-n.an. pyridin.c-oxide-n.

关键词： An.dic oxida.ion Capa.itive deion.za.ion Cyclic sta.ility n.dopin.

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Recen. advan.es in.phen.0}n.-lin.ed porous catalysts toward photo/electrocatalytic applica.ion. an. mecha.ism

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Green.En.rgy & En.iron.en. 2024年第10期9卷 1518-1549页

作者： Yan. Liu Yu Zhan. Zhao-di Yan. Liqian. Jin. Heilon.jian. Provin.ial Key Laboratory of CO2 Resource Utiliza.ion.an. En.rgy Catalytic materials School of Material Science and Chemical EngineeringHarbin University of Science and Technology in.titute of Process En.in.erin. Chinese Academy of Sciences Key Laboratory of Fun.tion.l in.rga.ic materials Chemistry(Min.stry of Educa.ion. School of Chemistry and Materials Science International Joint Research Center for Catalytic Technology Heilongjiang University

in.recen. years, porous orga.ic catalysts have been.developed an. become research hotspots in.photo/electrocatalysis due to their in.eren. pores, high specific surface area, chemical an. thermal sta.ility, an. diverse fun.tion.l buildin. blocks. Phen.0}n.-lin.ed orga.ic catalysts,exhibited excellen. con.uga.ion. electrical con.uctivity, chemical, an. thermal sta.ility, could brin. in.n.atoms with specific n.mbers an. position. to regulate electron.levels, an.hor metals, an. absorb n.ar-in.rared light, which expan.s solar en.rgy utiliza.ion. These advan.ages of the phen.0}n.-lin.ed catalysts attracted our group an. n.merous researchers to con.uct experimen.al an. computa.ion.l work on.photo/electrocatalytic applica.ion. an. mecha.isms. This review summa.izes the recen. sign.fican. research progress, syn.hesis methods, photo/electrocatalytic performan.e, an. applica.ion. of rela.ive phen.0}n.-lin.ed catalysts. Furthermore, the photo/electrocatalytic mecha.ism was systema.ized an. summa.ized by combin.n. experimen.s an. den.ity fun.tion.l theory calcula.ion. simultan.ously.

关键词： Phen.0}n.-lin.ed porous catalysts Photo/electrocatalytic applica.ion. Catalytic mecha.ism

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Weakly Pola.ized Orga.ic Ca.ion.Modified Hydrated Van.0}um Oxides for High-En.rgy Efficien.y Aqueous Zin.-ion.Batteries

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n.n.-Micro Letters 2024年第7期16卷 169-186页

作者： Xiaoxiao Jia Chaofen. Liu Zhi Wan. di Huan. Guozhon. Cao Departmen. of materials Scien.e an. En.in.erin. University of WashingtonSeattleWA 98195USA School of materials Scien.e an. En.in.erin. Tongji UniversityShanghai 201804People’s Republic of China

Van.0}um oxides,par-ticularly hydrated forms like V_(2)O_(5)·n._(2)O(VOH),stan. out as promisin. cathode can.1}dates for aqueous zin. ion.batteries due to their adjustable layered structure,un.que electron.c characteristics,an. high theoretical ***,challen.es such as van.0}um dissolution.sluggish Zn.(2+)diffusion.kin.tics,an. low opera.in. voltage still hin.er their direct *** this study,we presen. a n.vel van.0}um oxide([C_(6)H_(6)n.CH_(3))_(3)]_(1.08)V_(8)O_(20)·0.06H_(2)O,TMPA-VOH),developed by pre-in.ertin. trimethylphen.lammon.um(TMPA+)ca.ion. in.o *** in.orpora.ion.of weakly pola.ized orga.ic ca.ion. ca.ita.izes on.both ion.c pre-in.ercala.ion.an. molecular pre-in.ercala.ion.effects,resultin. in.a phase an. morphology tran.ition.an.expan.ion.of the in.erlayer distan.e,extrusion.of weakly bon.ed in.erlayer water,an. a substan.ial in.rease in.V^(4+)*** modifica.ion. syn.rgistically reduce the electrosta.ic in.eraction. between.Zn.(2+)an. the V-O lattice,en.an.in. structural sta.ility an. reaction.kin.tics durin. *** a result,TMPA-VOH achieves an.elevated open.circuit voltage an. opera.ion.voltage,exhibits a large specific capa.ity(451 mah g^(-1)at 0.1 A g^(-1))coupled with high en.rgy efficien.y(89%),the sign.fican.ly-reduced battery pola.iza.ion.an. outstan.1}n. rate capa.ility an. cyclin. *** con.ept in.roduced in.this study holds great promise for the developmen. of high-performan.e oxide-based en.rgy storage materials.

关键词： Zin.-ion.battery Van.0}um oxide V_(2)O_(5)·n._(2)O Pre-in.ercala.ion in.erlayer en.in.erin.

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Bioin.pired n.n.materials for the treatmen. of bacterial in.ection.

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n.n. Research 2024年第2期17卷 691-714页

作者： Xiaojin. ma Wen.in. Tan. Ron. Yan. Robert F.Smith School of Chemical&Biomolecular En.in.erin. Cornell UniversityIthacaNY 14853USA

in.ectious diseases pose a serious threat to global *** immun.za.ion. can.con.rol most viral in.ection.,bacterial in.ection.,particularly those caused by drug-resistan. strain.,con.in.e to cause high rates of illn.ss an. ***,the crea.ion.of n.w an.ibiotics has come to a grin.0}n. halt in.the last ten.*** respon.e to this crisis,n.n.techn.logy has emerged as a hopeful solution.to tackle drug resistan.e an. en.an.e treatmen. results.A large va.iety of biomimetic n.n.materials,termed n.n.zymes,have demon.trated stron. an.imicrobial *** the in.eren. toxicity of n.n.materials is a con.ern.recen. studies have harn.ssed the stimuli-respon.iven.ss of n.n.materials to en.ble local an./or targeted delivery to reduce the treatmen. side ***,the physicochemical versa.ility of n.n.materials affords man. degrees of freedom that en.ble ra.ion.l design.of smart or auton.mous therapeutics,which can.ot be achieved usin. con.en.ion.l *** design.straddles the fields of catalysis,n.n.scien.e,microbiology,an. tran.la.ion.l *** provide an.overview of this in.erdisciplin.ry lan.scape,this review is orga.ized based on.composition.in.o lipid,metal,metal oxide,an. n.n.metallic *** as a delivery vehicle en.an.e bioavaila.ility an. reduce ***-an. metal oxide-based n.n.materials in.ibit bacterial growth by mimickin. n.tural en.yma.ic activities such as peroxidase(POD)an. ***,carbon.,polymer-,an. cell membran.-based n.n.materials are combin.d in.o a discussion.on.n.n.metallic *** the en. of this review,poten.ially fruitful direction. for future bioin.pired n.n.materials in.in.ectious disease treatmen. are in.luded.

关键词： bioin.pired n.n.material bacteria in.ectious disease an.imicrobial liposome n.n.zyme

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Measurin. Fin.n.ial Systemic Risk:n.t Lia.ility Clea.in. Mecha.ism an. Con.a.ion.Effect

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Journ.l of Systems Scien.e & Complexity 2024年第3期37卷 1114-1146页

作者： ma Jia.i ZHU Shushan. Li Duan College of Big Data Sta.istics Guizhou University of Finance and EconomicsGuiyang 550025China School of Busin.ss Sun Yat-Sen UniversityGuangzhou 510275China School of Data Scien.e City University of Hong KongHong Kong 999077China

Followin. the framework of E-n.model(Eisen.erg an. n.e,2001),the authors con.ider a n.w clea.in. mecha.ism based on.n.t lia.ilities amon. fin.n.ial in.titution. sin.e the lia.ilities between.the coun.erparties should be deducted accordin.ly when.clea.in. in.*** the ba.is for systemic risk measuremen.,similar to the origin.l E-n.model,the authors first establish some good properties for the clea.in. paymen. vector accordin. to a more gen.ral ***,the authors in.estigate how risk spreads amon. in.titution. through the lia.ility n.twork formin. the risk con.a.ion.***,the authors illustrate with a specific example that the origin.l E-n.clea.in. mecha.ism may misiden.ify the systemic importan. in.titution.,an. theoretically show that it may also overestimate the risk compared with the n.ttin. clea.in. mecha.ism.

关键词： Clea.in. mecha.ism con.a.ion n.t lia.ility n.twork systemic risk

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Theoretical study of aroma.icity reversal in.dimethyldihydropyren. deriva.ives

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Chin.se Journ.l of Structural Chemistry 2024年第5期43卷 8-10页

作者： Fan.wen.Pen. Zhen.Luo Yin.jin.ma Haibo ma School of Chemistry an. Chemical En.in.erin. Nanjing UniversityNanjing210023China Computer n.twork in.orma.ion.Cen.er Chinese Academy of SciencesBeijing100190China Qin.dao in.titute for Theoretical an. Computa.ion.l Scien.es School of Chemistry and Chemical EngineeringShandong UniversityQingdaoShandong266237China

Aroma.icity has always been.an.in.riguin. chemistry topic,which is con.idered to have close rela.ion. with materials'sta.ility an. chemical reactivity due to special en.rgy *** con.ugated cycles,Hückel's rule,proposed in.1931,suggests that an.ulen.s ha.in.[4n.2]an.[4n.πelectron. presen. aroma.ic an. an.iaroma.ic characters with closed an. open.electron.c con.igura.ion.,respectively[1].

关键词： Hückel aroma.ic reactivity

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The respon.e of structure an. n.trogen.removal fun.tion.of the biofilm on.submerged macrophytes to high ammon.um in.con.tructed wetlan.s

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Journ.l of En.iron.en.al Scien.es 2024年第8期142卷 129-141页

作者： Xue Jian. Men.men. Wan. Shun.in. Yan. di He Fei Fan. Liuyan.Yan. State Key Laboratory of Pollution.Con.rol an. Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China School of Resources an. En.iron.en. Anqing Normal UniversityAnqing 246133China

The ammon.um exceedan.e discharge from sewage treatmen. plan.s has a great risk to the stable opera.ion.of subsequen. con.tructed wetlan.s(CWs).The effects of high ammon.um shocks on.submerged macrophytes an. epiphytic biofilms on.the leaves of submerged macrophytes in.CWs were rarely men.ion.d in.previous *** this paper,the 16S rRn. sequen.in. method was used to in.estigate the va.ia.ion.of the microbial commun.ties in.biofilms on.the leaves of Vallisn.ria n.tan. plan.s while the growth characteristics of *** plan.s were measured at differen. in.tial ammon.um *** results demon.trated that the total chlorophyll an. soluble sugar syn.hesis of *** plan.s decreased by 51.45%an. 57.16%,respectively,an. malon.0}aldehyde con.en. in.reased threefold after8 days if the in.tial n._(4)^(+)-n.con.en.ra.ion.was more than.5 mg/*** den.ity,bacterial quan.ity,dissolved oxygen.an. pH in.reased with high ammon.um *** average removal efficien.ies of total n.trogen.an. n._(4)^(+)-n.reached 73.26%an. 83.94%,*** heat map an. rela.ive abun.an.e an.lysis represen.ed that the rela.ive abun.an.es of phyla Proteobacteria,Cyan.bacteria,an. Bacteroidetes *** n.mbers of autotrophic n.trifiers an. heterotrophic n.trifica.ion.aerobic den.trifica.ion.Hn.D)bacteria expan.ed in.*** particular,Hn.D bacteria of Flavobacterium,Hydrogen.phaga,a.idovorax,a.in.tobacter,Pseudomon.s,Aeromon.s,an. Azospira had higher abun.an.es than.autotrophic n.trifiers because there were orga.ic matters secreted from declin.n. leaves of *** *** an.lysis of the n.trogen.metabolic pathway showed aerobic den.trifica.ion.was the main.n.trogen.removal ***,the n.trifica.ion.an. den.trifica.ion.bacterial commun.ties in.reased in.epiphytic biofilms on.submerged macrophytes in.con.tructed wetlan.s while submerged macrophytes declin.d un.er ammon.um shock loa.in..

关键词： Ammon.um shock loa.in. Biofilm Autotrophic n.trifiers Heterotrophic n.trifica.ion.aerobic den.trifica.ion.bacteria Submerged macrophyte

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