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Frontiers in high entropy alloys and high entropy functional materials

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Rare Metals 2024年第10期43卷 4639-4776页

作者： Wen-Tao Zhang Wen huang Fu-Jie Yu Qi Zhao Xin-Dong Zhu Tao Feng yao Jiang Xiao-Ming Li Xue-Fei Miao He Zhu Si Lan Xue-Qian Wang Bao-Long Shen Zhe Jia Feng-Qi Zhang Wei Wang Qi Liu {2.g Ren Xun-Li Wang Xiao-Ya Cui Xiao-{2.g Wang Ya-Nan Chen Bing-Bing Fan Meng-Ru Li Qi-Long Gao Jia-Ming Guo Zeng-Bao Jiao Zhi-Min Guo Yu-Ping Zhao Qian Yu Rui huang ling-Kun Zhang Yi-Ping Lu Xu-Bo Li Huai-Jun lin {2. ma Wei-Ming {2.g Zhi-Hua Shen Hai-{2. He Yong-Gang Sun Yong-Jiang huang De-Zhuang Wang Qing-Feng Liu Fei-{2.g Wang Hui Liu Hong-Hui Wu Li-Qiang Wang {2.g Lu Nan Wang Tian-Li Wang Wei-Bing Liao Yi-Han Wang Yuan Wu Yu-Zhen Yin Jie Pan Yi Zhang Qing Wang Jian-{2.g Zhang Tao {2.g Yasir Sohail Jin-Yu Zhang Hua Ji Qiang Li Wei-Di Liu Zhi-Gang Chen Xiong-Jun Liu Wen ma Liang mao Zhen-Duo Wu School of materials Science and Engineering Nanjing University of Science and Technology Jiangsu key laboratory for Advanced Metallic {2.terials School of Materials Science and Engineering Southeast University Department of Physics City University of Hong Kong School of materials Science and Engineering Tianjin University School of Physics and Microelectronics Zhengzhou University Department of Mechanical Engineering Research Institute for Advanced Manufacturing The Hong Kong Polytechnic University Center of Electron Microscopy and state key {2. of Silicon materials School of Materials Science and Engineering Zhejiang University key laboratory of Solidification Control and Digital Preparation Technology (Liaoning Province) School of Materials Science and Engineering Dalian University of Technology Institute of Advanced Wear & Corrosion Resistance and Functional materials Jinan University School of Mechanics and Civil Engineering China University of Mining and Technology School of Physical Sciences Great Bay University School of materials Science andEngineering Harbin Institute of Technology state key {2. of materials-Oriented chemical Engineering College of Chemical Engineering Nanjing Tech University Beijing Advanced Innovation Center for materials Genome Engineering Research Institute for Carbon Neutrality University of Science and Technology Beijing Department of Mechanical Engineering The University of Hong Kong School of Computing Macquarie University key laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University state key {2. for Advanced Metals and materials University of Science and Technology Beijing state key {2. of materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Institute of materials Shanghai University Department of materials Science and Engineering C

Owing to their exceptional properties, high-entropy alloys(HEAs) and high-entropy materials have emerged as promising research areas and shown diverse applications. Here,the recent advances in the field are comprehensively reviewed,organized into five sections. The first section introduces the background of HEAs, covering their definition, significance,application prospects, basic properties, design principles, and microstructure. The subsequent section focuses on cutting-edge high-entropy structural materials, highlighting developments such as nanostructured alloys, grain boundary engineering,eutectic systems, cryogenic alloys, thin films, micro-nano-lattice structures, additive manufacturing, high entropy metallic glasses, nano-precipitate strengthened alloys, composition modulation, alloy fibers, and refractory systems. In the following section, the emphasis shifts to functional materials, exploring HEAs as catalysts, magneto-caloric materials, corrosion-resistant alloys, radiation-resistant alloys, hydrogen storage systems, and materials for biomedicine. Additionally, the review encompasses functional high-entropy materials outside the realm of alloys, including thermoelectric, quantum dots, nanooxide catalysts, energy storage materials, negative thermal expansion ceramics,and high-entropy wave absorption materials. The paper concludes with an outlook, discussing future directions and potential growth areas in the field. Through this comprehensive review,researchers, engineers, and scientists may gain valuable insights into the recent progress and opportunities for further exploration in the exciting domains of high-entropy alloys and functional materials.

关键词： Cutting-edge structural materials Cutting-edgefunctional materials High entropy alloys

Revealing alkali metal ions transport mechanism in the atomic channels of Au@a-MnO_(2.

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Journal of Energy chemistry 2023年第7期82卷 350-358,I0008页

作者： Jingzhao Chen Yong Su Hongjun Ye Yushu Tang Jitong yan Zhiying Gao Dingding Zhu Jingming yao Xuedong Zhang Tingting yang Baiyu Guo Hui Li Qiushi Dai Yali Liang Jun ma Bo Wang Haiming Sun Qiunan Liu Jing Wang Congcong Du Liqiang Zhang Yongfu Tang Jianyu huang Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066004HebeiChina School of materials Science and Engineering Xiangtan UniversityXiangtan 411105HunanChina Hebei key laboratory of Applied {2. College of Environmental and Chemical EngineeringYanshan UniversityQinhuangdao 066004HebeiChina

Understanding alkali metal ions’(e.g.,Li^(+)/Na^(+)/K^(+))transport mechanism is challenging but critical to improving the performance of alkali metal *** using a-MnO_(2.nanowires as cathodes,the transport kinetics of Li^(+)/Na^(+)/K^(+)in the 2.2.channels of a-MnO_(2.with a growth direction of[001]is *** show that ion radius plays a decisive role in determining the ion transport and *** of the ion radii,Li^(+)/Na^(+)/K^(+)can all go through the 2.2.channels of a-MnO_(2.,generating large stress and causing channel merging or ***,smaller ions such as Li^(+)and Na^(+)cannot only transport along the[001]direction but also migrate along thedirection to the nanowire surface;for large ion such as K^(+),diffusion along thedirection is *** different ion transport behavior has grand consequences in the electro{2. of metal oxygen batteries(MOBs).For Li-O_(2.battery,Li^(+)transports uniformly to the nanowire surface,forming a uniform layer of oxide;Na^(+)also transports to the nanowire surface but may be clogged locally due to its larger radius,therefore sporadic pearl-like oxides form on the nanowire surface;K^(+)cannot transport to the nanowire surface due to its large radius,instead,it breaks the nanowire locally,causing local deposition of potassium *** study provides atomic scale understanding of the alkali metal ion transport mechanism which may be harnessed to improve the performance of MOBs.

关键词： Ion transport In-situ TEM STEM Metal oxygen batteries Metal ion batteries

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银川都市圈大气挥发性有机物的污染特征及臭氧生成潜势初步分析

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环境化学 2022年第3期41卷 801-812页

作者：马陈熀王章玮刘建军黄海梅刘垚严晓瑜陆耀辉王纯杰张晓山中国科学院生态环境研究中心城市与区域生态国家重点实验室北京100085 宁夏回族自治区气象服务中心银川750002 中国科学院大学北京100049

2.19年6月和8月在宁夏回族自治区银川市及周边6个点位进行了环境空气挥发性有机物(VOCs)的观测研究。利用苏码罐采样-三级冷阱预浓缩-GC-MS/FID技术测定环境空气样品中56种挥发性有机物组分;分析该地区环境空气中挥发性有机物的污染特... 详细信息

2.19年6月和8月在宁夏回族自治区银川市及周边6个点位进行了环境空气挥发性有机物(VOCs)的观测研究。利用苏码罐采样-三级冷阱预浓缩-GC-MS/FID技术测定环境空气样品中56种挥发性有机物组分;分析该地区环境空气中挥发性有机物的污染特征和来源,计算各组分臭氧和二次有机气溶胶的生成潜势。结果表明,工业区、商业/交通/居民混合区以及工业/交通混合区采样点环境空气中挥发性有机物的浓度和组成有共性也有其特殊性,各采样点均受到机动车尾气排放的影响;短链烷烃和长链烷烃占比较高,分别为TVOCs的30.85%—45.2.%和15.17%—48.79%,烯烃在宁东煤化工区采样点占比(43.77%)最高,而炔烃、芳香烃在平罗采样点占比最高,分别为2..98%和14.00%。烯烃对各采样点臭氧生成潜势(OFP)贡献率为2..2.%—85.2.%,芳香烃对各采样点二次有机气溶胶生成潜势(SOAP)贡献最大(61.49%—89.52.)。

关键词：挥发性有机物环境空气臭氧二次有机气溶胶生成潜势

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二次电池研究进展

物理化学学报 2022年第12期38卷 22-167页

作者：黄俊达朱宇辉冯煜韩叶虎谷振一刘日鑫杨冬月陈凯张相禹孙威辛森余彦尉海军张旭于乐王华刘新华付永柱李国杰吴兴隆马灿良王飞陈龙周光敏吴思思卢周广李秀婷刘继磊高鹏梁宵常智叶华林李彦光周亮尤雅王鹏飞杨超刘金平孙美玲毛明磊陈浩张山青黄岗余丁山徐建铁熊胜林张进涛王莹任玉荣杨春鹏徐韵涵陈亚楠许运华陈子峰杲祥文浦圣达郭少华李强曹晓雨明军皮欣朋梁超凡伽龙王俊雄焦淑红姚雨晏成林周栋李宝华彭新文陈冲唐永炳张桥保刘奇任金粲贺艳兵郝晓鸽郗凯陈立宝马建民电子科技大学材料与能源学院成都611731 中国科学院化学研究所北京100190 厦门大学材料学院福建厦门361005 中国科学技术大学材料科学与工程系合肥230026 东北师范大学物理学院长春130024 南京大学现代工程与应用科学学院南京210046 中国科学院长春应用化学研究所长春130022 北京化工大学有机无机复合材料国家重点实验室北京100029 北京工业大学材料与制造学部北京100124 北京航空航天大学化学学院北京100191 北京航空航天大学交通科学与工程学院北京100191 郑州大学化学学院郑州450001 郑州大学橡塑模具国家工程研究中心郑州450002 东北师范大学化学学院长春130024 山西大学分子科学研究所太原030006 复旦大学材料科学系上海200433 华东理工大学化工学院上海200237 清华大学深圳国际研究生院广东深圳518055 南方科技大学材料科学与工程系广东深圳518055 深圳大学高等研究院广东深圳518060 湖南大学材料科学与工程学院长沙410082 湖南大学化学化工学院长沙410082 中南大学材料科学与工程学院长沙410083 苏州大学功能纳米与软物质研究院江苏苏州215123 武汉理工大学材料复合新技术国家重点实验室武汉430070 西安交通大学电气工程学院西安710049 武汉理工大学化学化工与生命科学学院武汉430070 华中科技大学光学与电子信息学院武汉430074 Centre for Catalysis and Clean Energy School of Environment and ScienceGriffith UniversityGold CoastQLD4214Australia 中山大学化学学院广州510275 华南理工大学环境与能源学院广州510006 山东大学化学与化工学院济南250100 香港中文大学化学系中国香港999077 常州大学材料科学与工程学院江苏常州213164 天津大学化工学院天津300350 天津大学材料科学与工程学院天津300350 Department of materials University of OxfordOxfordOX13PH 青岛大学新能源科学与工程系山东青岛266071 河南工业大学化学化工学院郑州450001 华中科技大学材料科学与工程学院武汉430074 苏州大学能源学院江苏苏州215006 华南理工大学轻工科学与工程学院广州510641 中国科学院深圳先进技术研究院广东深圳518055 湖南大学物理与微电子科学学院长沙410082 香港城市大学物理系中国香港999077 Department of Mechanical and materials Engineering University of Western OntarioLondonOntario N6A 5B9Canada 西安交通大学化学学院西安710049 中南大学粉末冶金国家重点实验室长沙410083

能源的存储和利用是当今科学和技术发展中的重大课题之一,尤其是作为高效的电能/化学能转化装置的二次电池相关技术一直是科学家研究的热点领域。在此背景下,本文较为系统地介绍目前二次电池的重要研究进展,将从二次电池的发展历史引入... 详细信息

能源的存储和利用是当今科学和技术发展中的重大课题之一,尤其是作为高效的电能/化学能转化装置的二次电池相关技术一直是科学家研究的热点领域。在此背景下,本文较为系统地介绍目前二次电池的重要研究进展,将从二次电池的发展历史引入,再到其相关的基础理论知识的介绍。随后较为详细地讨论当前不同体系的二次电池及相关应的关键材料的研究进展,涉及到锂离子电池、钠离子电池、钾离子电池、镁离子电池、锌离子电池、钙离子电池、铝离子电池、氟离子电池、氯离子电池、双离子电池、锂-硫(硒)电池、钠-硫(硒)电池、钾-硫(硒)电池、多价金属-硫基电池、锂-氧电池、钠-氧电池、钾-氧电池、多价金属-氧气电池、锂-溴(碘)电池、水系金属离子电池、光辅助电池、柔性电池、有机电池、金属-二氧化碳电池等。此外,也介绍了电池研究中常见的电极反应过程表征技术,包括冷冻电镜、透射电镜、同步辐射、原位谱学表征、磁性表征等。本文将有助于研究人员对二次电池进行全面系统的了解与把握,并为之后二次电池的研究提供很好的指导作用。

关键词：二次电池电池体系电池材料电化学知识表征技术

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