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Preparation of PVA/gO/h-BN Janus Film with High Thermal Conductivity and Excellent Flexibility via a Density Deposition Self-assembly method

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Chinese Journal of Polymer Science 2024年第8期42卷 1217-1226页

作者： Fang-hua Luo Zhi-Tao Dong guo-hua Chen Chen ma huai-Yuan Wang College of Chemistry and Chemical Engineering Northeast Petroleum UniversityDaqing 163318China College of materials Science and Engineering Huaqiao UniversityXiamen 361000China School of Chemical Engineering and Technology and State Key Laboratory for Chemical Engineering Tianjin UniversityTianjin 300350China

Janus films with asymmetric physical/chemical properties have attracted con siderable attention due to their promising applications in personal thermal management,electronic skin s,sensors,actuators,***,traditional methods for fabricating Janus films conventionally need the assistance of an interface or auxiliary equipment,which are usually complex and ***,flexible poly(vinyl alcohol)(PVA)/graphene oxide(gO)/h-BN(recorded as PVA/gO/h-BN)Janus films with thermally,optically,and electrically anisotropic properties are fabricated by a simple density deposition self-assem bly method,which just utilizes the density difference between gO and h-BN during water *** results show that the two sides of the acquired Janus films have obvious asymmetric *** the original state of the PVA/gO/h-BN Janus films,the thermal conductivity of the gO side(10.06 W·m^(-1)·K^(-1))is generally lower than that of the h-BN side(10.48W·m^(-1)·K^(-1)).But after gO is reduced,the thermal conductivity of the rgO side reaches 12.17 W·m^(-1)·K^(-1),surpassing that of the h-BN *** addition,the relative reflectance of the h-BN side of Janus film is also significantly higher than that of the rgO side,and the su rface resistance difference between the two sides is about 4 orders of *** prepared PVA/gO/h-BN Janus films show great application potential in human thermal management,light conversion switches,and electronic *** study provides a simple and versatile strategy for fabricating Janus films with multifunctional(such as thermal,optical,and electrical)anisotropies.

关键词： Janus films PVA/gO/h-BN Density deposition self-assembly method

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Subgrain-assisted spontaneous grain refinement in rapid solidification of undercooled melts

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Journal of materials Science & Technology 2024年第7期174卷 234-248页

作者： Jianbao Zhang Dongpeng hua Dexu Cui Xin Li Ke hua Yixuan He Haifeng Wang Yuhong Zhao State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsNorthwestern Polytechnical UniversityXi’an 710072China School of materials Science and Engineering North University of ChinaTaiyuan 030051China

The grain refinement mechanism for rapid solidification of undercooled melts is still an open problem even after 60 years of on-going *** this work,rapid solidification of undercooled Ni and equi-atomic FeCoNiPd melts was studied and spontaneous grain refinement was found at both low and high *** a detailed electron backscattered diffraction analysis,subgrain-induced grain orien-tation scattering and splitting were found to occur along with the transition from coarse dendrites to fine equiaxed grains at low and high undercooling,respectively,indicating that subgrains play an im-portant role during the formation of fine equiaxed *** this basis,a compromise mechanism of subgrain-assisted spontaneous grain refinement was *** the dendrite re-melting induced thermo-mechanical process and fluid flow induced dendrite deformation occur simultaneously during the post-recalescence stage,stress accumulation would be maximum at both low and high undercooling,thus inducing dynamic recrystallization,during which the formation and rotation of subgrains make the grain orientations scattering and even ***,the grain/subgrain size of undercooled FeCoNiPd ascribing to its unique co-segregation behavior keeps almost invariable from low to high undercooling,indicating that the co-segregation strategy would be effective to inhibit grain growth after rapid solidifi-cation and would be useful in practice.

关键词： Rapid solidification Undercooling Spontaneous grain refinement grain growth High entropy alloy

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Proteome profiling to advance management of metabolic dysfunction-associated fatty liver disease

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Hepatobiliary Surgery and Nutrition 2024年第1期13卷 147-149页

作者： mohammed Eslam Nahum méndez-Sánchez ming-hua Zheng Storr Liver Centre Westmead Institute for Medical ResearchWestmead Hospital and University of SydneySydneyNSWAustralia Liver Research Unit Medica Sur Clinic FoundationMexico CityMexico mAFLD Research Center Department of HepatologyThe First Affiliated Hospital of Wenzhou Medical UniversityWenzhouChina Institute of Hepatology Wenzhou Medical UniversityWenzhouChina Key Laboratory of Diagnosis and Treatment for The Development of Chronic Liver Disease in Zhejiang Province WenzhouChina

metabolic dysfunction-associated fatty liver disease(mAFLD)is a complex,heterogenous and progressive disease that is characterised by substantial phenotypic variability,which results in disparate clinical presentations and outcomes(1-4).Notably,only a proportion of patients with mAFLD progress to the more advanced stages of the ***,the identification of the subgroups that have a high risk of disease progression is of paramount importance for clinical care,as well as drug development and clinical trials(5).

关键词： metabolic dysfunction-associated fatty liver disease(mAFLD) fatty liver disease(FLD) fibrosis proteome biomarkers

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Room temperature self-healing liquid metals:capabilities,applications and challenges

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International Journal of Smart and Nano materials 2024年第3期15卷 469-501页

作者： Chen hua Jianye gao Jing Liu Key Lab of Cryogenic Science and Technology Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijingChina School of Future Technology University of Chinese Academy of SciencesBeijingChina School of Biomedical Engineering Tsinghua UniversityBeijingChina

Self-healing materials span diverse application fields,including flexible electronics,soft robotics,and energy ***,conventional self-healing materials pose a challenge in achiev-ing the delicate balance between flexibility and electrical ***,they also suffer from prolonged healing times,incomplete healing,and high manufacturing *** metals possess excellent self-healing capabilities owing to their unique combination of fluidic and metallic properties,high surface tension,and reversible solid-liquid phase change at room temperature,offering an intriguing material option for addressing the challenges associated with flexibility and elec-trical *** this review article,we comprehensively examine the domain of self-healing liquid metals from the standpoint of typical mechanisms underlying self-healing pro-cesses,as well as practical strategies employed for achieving such ***,we explore representative applications that showcase the potential of these materials while aiming to provide a valuable reference for advancing and enhancing the field of self-healing *** pro-spect along this direction is made.

关键词： Self-healing Liquid metal Smart materials

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Donor-acceptor covalent organic frameworks-confined ultrafine bimetallic Pt-based nanoclusters for enhanced photocatalytic H_(2)generation

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Nano Research 2024年第7期17卷 5835-5844页

作者： Yu Liu Yawen Shi hua Wang Shengbo Zhang Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Key Laboratory for Green Chemical Technology of the Ministry of EducationSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300350China School of Environmental Science and Engineering Tianjin Key Laboratory of Biomass/Wastes UtilizationTianjin UniversityTianjin 300350China

Photocatalytic hydrogen generation from hydrogen storage media is an effective and promising approach for the green hydrogen industry as well as for achieving carbon neutrality ***,the lower photocatalytic efficiency due to the limited light trapping capacity,low electron transfer rate,and severe aggregation of nanoparticles caused by high surface energy seriously restricts their practical ***,we constructed a series of donor–acceptor(D–A)type covalent organic frameworks to confine ultrafine bimetallic Pt-based nanoclusters for photocatalytic hydrogen generation from ammonia borane(AB)*** visible light irradiation at 20℃,PtCo_(2)@covalent organic framework(COF)showed the highest photocatalytic activity with a turnover frequency(TOF)of 486 min−*** and density functional theory(DFT)calculations reveal that the high catalytic activity is mainly attributed to the strong electronic interactions between D–A type COF and ultrafine PtCo_(2)***,the D–A type COF can significantly enhance the light-trapping ability by fine-tuning the electron-acceptor type in the framework,and accelerate the photogenerated electron transfer from D–A type COF to PtCo_(2)nanocluster,which promotes the adsorption and activation of H_(2)O and AB molecules and accelerates hydrogen ***,PtCo_(2)@COF also exhibited ultra-high durability due to the significantly enhanced resistance to nanocluster aggregation caused by the nanopore confinement effect of D–A type *** believe that this work will provide a theoretical guide for the rational design of efficient D–A COFbased catalysts for photocatalysis.

关键词： light trapping electron transfer donor-acceptor covalent organic frameworks(D-A COFs) bimetallic nanoclusters photocatalysis

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The crosstalk between enteric nervous system and immune system in intestinal development,homeostasis and diseases

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Science China(Life Sciences) 2024年第1期67卷 41-50页

作者： Xindi Wang Chenbo Ding hua-Bing Li Shanghai Institute of Immunology State Key Laboratory of Oncogenes and Related GenesShanghai Jiao Tong University School of MedicineShanghai 200025China Shanghai Jiao Tong University School of medicine-Yale Institute for Immune metabolism Shanghai Jiao Tong University School of MedicineShanghai 200025China

The gut is the largest digestive and absorptive organ,which is essential for induction of mucosal and systemic immune responses,and maintenance of metabolic-immune *** intestinal components contain the epithelium,stromal cells,immune cells,and enteric nervous system(ENS),as well as the outers,such as gut microbiota,metabolites,and *** dyshomeostasis of intestinal microenvironment induces abnormal intestinal development and functions,even colon diseases including dysplasia,inflammation and *** recent studies have identified that ENS plays a crucial role in maintaining the immune homeostasis of gastrointestinal(gI)*** crosstalk between ENS and immune cells,mainly macrophages,T cells,and innate lymphoid cells(ILCs),has been found to exert important regulatory roles in intestinal tissue programming,homeostasis,function,and *** this review,we mainly summarize the critical roles of the interactions between ENS and immune cells in intestinal homeostasis during intestinal development and diseases progression,to provide theoretical bases and ideas for the exploration of immunotherapy for gastrointestinal diseases with the ENS as potential novel targets.

关键词： enteric nervous system macrophages T cells innate lymphoid cells neuro-immune interactions

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Arsenic and fluoride co-enrichment of groundwater in the loess areas and associated human health risks:A case study of Dali County in the guanzhong Basin

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China geology 2024年第3期7卷 445-459页

作者： Rui-ping Liu Fei Liu hua-qing Chen Yu-ting Yang hua Zhu You-ning Xu Jian-gang Jiao Refaey m El-Wardany Xi'an Center China Geological SurveyMinistry of Natural ResourcesXi'an 710054China Observation and Research Station of Environmental geology of Typical mines in Shaanxi Province MNRXi'an 710054China Key Laboratory for geo-hazards in Loess Area MNRXi'an 710054China Dalian Ocean and Fishery Comprehensive Administration Supervision Lochus Dalian 116000China Pingliang City Development and Reform Commission Pingliang 744000China School of Earth Science and Resources Chang’an UniversityXi'an 710054China Faculty of Science Al-Azhar UniversityAssiut 71524Egypt

This study aims to reveal the occurrence and origin of typical groundwater with high arsenic and fluoride concentrations in the loess area of the guanzhong Basin—a Neogene faulted *** findings are as follows:(1)groundwater samples with high arsenic and fluoride concentrations collected from the loess area and the terraces of the Weihe River accounted for 26%and 30%,respectively,of the total samples,with primary hydrochemical type identified as HCO_(3)-*** karst and sand areas exhibit relatively high groundwater quality,serving as preferred sources for water *** is recommended that local governments fully harness groundwater in these areas;(2)groundwater with high arsenic and fluoride concentrations in the loess area and the alluvial plain of rivers in Dali County is primarily distributed within the guanzhong Basin,which represents the drainage zone of groundwater;(3)arsenic and fluoride in groundwater originate principally from natural and anthropogenic sources;(4)the human health risk assessments reveal that long-term intake of groundwater with high arsenic and fluoride concentrations pose cancer or non-cancer risks,which are more serious to kids compared to *** study provides a theoretical basis for the prevention and treatment of groundwater with high arsenic and fluoride concentrations in loess areas.

关键词： Arsenic Fluoride groundwater Cancer risk Kid and adult Human health risk assessment Hydrogeological survey engineering Environmental geological survey engineering Loess areas

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Strain gradient Finite Element Formulation of Flexoelectricity in Ferroelectric material Based on Phase-Field method

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Acta mechanica Solida Sinica 2024年第4期37卷 570-579页

作者： Shuai Wang Hengchang Su min Yi Li-hua Shao National Key Laboratory of Strength and Structural Integrity Institute of Solid MechanicsSchool of Aeronautic Science and EngineeringBeihang UniversityBeijing100191People’s Republic of China State Key Laboratory of mechanics and Control for Aerospace Structures and Institute for Frontier Science and Key Laboratory for Intelligent Nano materials and Devices of ministry of Education and College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsNanjing210016People’s Republic of China

Flexoelectricity is a two-way coupling effect between the strain gradient and electric field that exists in all dielectrics,regardless of point group ***,the high-order derivatives of displacements involved in the strain gradient pose challenges in solving electromechanical coupling problems incorporating the flexoelectric *** this study,we formulate a phase-field model for ferroelectric materials considering the flexoelectric effect.A four-node quadrilateral element with 20 degrees of freedom is constructed without introducing high-order shape *** microstructure evolution of domains is described by an independent order parameter,namely the spontaneous polarization governed by the time-dependent ginzburg–Landau *** model is developed based on a thermodynamic framework,in which a set of microforces is introduced to construct the constitutive relation and evolution *** the flexoelectric part of electric enthalpy,the strain gradient is determined by interpolating the mechanical strain at the node via the values of gaussian integration points in the isoparametric *** model is shown to be capable of reproducing the classic analytical solution of dielectric materials incorporating the flexoelectric *** model is verified by duplicating some typical phenomena in flexoelectricity in cylindrical tubes and truncated pyramids.A comparison is made between the polarization distribution in dielectrics and *** model can reproduce the solution to the boundary value problem of the cylindrical flexoelectric tube,and demonstrate domain twisting at domain walls in ferroelectrics considering the flexoelectric effect.

关键词： Flexoelectricity Phase-field method Ferroelectrics Domain configuration

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Optical system for extremely large spectroscopic survey telescope

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Science China(Physics,mechanics & Astronomy) 2024年第7期67卷 158-174页

作者： Ding-qiang Su hua Bai Xiangyan Yuan Xiangqun Cui Key Laboratory of the ministry of Education School of Astronomy and Space ScienceNanjing UniversityNanjing 210023China Nanjing Institute of Astronomical Optics and Technology(NIAOT) Chinese Academy of SciencesNanjing 210042China University of Chinese Academy of Sciences Nanjing 211135China School of Astronomy and Space Science University of Chinese Academy of SciencesBeijing 101408China

This article presents research work on a spectroscopic survey *** idea is as follows:for such a telescope,a pure reflecting optical system is designed,which should have an aperture and a field of view(FOV)both as large as possible and excellent image quality,and then a strip lensm(lens-prism)atmospheric dispersion corrector(S-ADC)is added,only for correcting the atmospheric *** the fund limitation and the simplicity of scaling up,some 12-m telescopes are designed as ***,Korsch,and meinel put forward the four-mirror Nasmyth systems I and II,which are used in this *** of 1.5°,2°,and 2.5°are *** all systems,the image qualities are *** the S-ADC relaxes the optical glass size restriction,this 12-m telescope with a FOV of 2.5°can be magnified in proportion to a 16-m *** etendue(from Frenchétendue)and focal surface will now be the largest in the *** such a telescope,a pure reflecting optical system can also be obtained.A subsequent coudésystem is designed with excellent image quality.

关键词： telescopes spectroscopic survey

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The dynamics beamline at SSRF

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Nuclear Science and Techniques 2024年第9期35卷 56-67页

作者： Zhen Liu Li-hua Wang Yong Jiang Ya-Jun Tong hua-Chun Zhu Te Ji min Chen Zheng Jiang Xiang-Jun Wei Shanghai Advanced Research Institute Chinese Academy of SciencesShanghai 201204China ShanghaiTech University Shanghai 201210China

The dynamics beamline(D-Line),which combines synchrotron radiation infrared spectroscopy(SR-IR)and energy-disper-sive X-ray absorption spectroscopy(ED-XAS),is the first beamline in the world to realize concurrent ED-XAS and SR-IR measurements at the same sample position on a millisecond time-resolved *** combined technique is effective for investigating rapid structural changes in atoms,electrons,and molecules in complicated disorder systems,such as those used in physics,chemistry,materials science,and extreme ***,ED-XAS and SR-IR can be used independently in the two branches of the *** ED-XAS branch is the first ED-XAS beamline in China,which uses a tapered undulator light source and can achieve approximately 2.5×10^(12)photons/s·300 eV BW@7.2 keV at the sample *** exchange-able polychromator operating in the Bragg-reflection or Laue-transmission configuration is used in different energy ranges to satisfy the requirements for beam size and energy *** focused beam size is approximately 3.5μm(H)×21.5μm(V),and the X-ray energy range is 5–25 *** one-and two-dimensional position-sensitive detectors with frame rates of up to 400 kHz enables time resolutions of tens of microseconds to be *** distinctive techniques,such as the concurrent measurement of in situ ED-XAS and infrared spectroscopy,time-resolved ED-XAS,high-pressure ED-XAS,XmCD,and pump-probe ED-XAS,can be applied to achieve different scientific goals.

关键词： ED-XAS SR-IR Time-resolved D-line SSRF

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