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Paleozoic tectonic evolution of the proto-Korean Peninsula along the East Asian continental margin from detrital zircon U-Pb geochronology and Hf isotope geochemistry

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Geoscience Frontiers 2024年第1期15卷 97-117页

作者： Yirang Jang Sung Won Kim Vinod O.Samuel Sanghoon Kwon Seung-Ik Park m.santosh Keewook Yi Department of Earth and Environmental Sciences Chonnam National UniversityGwangju 61186Republic of Korea Geology Division Korea Institute of Geoscience and Mineral ResourcesDaejeon 34132Republic of Korea Department of Earth System Sciences Yonsei UniversitySeoul 03722Republic of Korea Department of Geology Kyungpook National UniversityDaegu 41566Republic of Korea School of Earth Sciences and Resources China University of Geosciences BeijingBeijing 100083China Department of Earth Science University of AdelaideAdelaide SA 5005Australia Yonsei Frontiers Lab Yonsei UniversitySeoul 03722Republic of Korea Division of Earth and Environmental Sciences Korea Basic Science InstituteChungbuk 28119Republic of Korea

Detrital zircon geochronology and Hf isotope analysis can be used for inferring provenance characteristics,and to evaluate the tectonic evolution of sedimentary basins and their link with regional orogenesis.The Paleozoic sequences of the Okcheon Belt consist of the Lower Paleozoic Joseon and the Upper Paleozoic Pyeongan supergroups with middle Paleozoic hiatus locally on top of the Neoproterozoic bimodal volcanic rocks,reflecting an intracontinental rift setting between the two basements(viz.Gyeonggi and Yeongnam massifs)at southern part of the Korean Peninsula.Our detrital zircon U-Pb ages and Lu-Hf isotope results show that all these Paleozoic strata commonly have Paleoproterozoic and Paleozoic zircon ages with rare meso-to Neoproterozoic ages.The individual zircon populations display following features,allowing estimation of their sedimentary provenances:(i)The Paleoproterozoic zircons(ca.1.85 Ga and 2.50 Ga)with similar ranges ofεHf(t)values are most common in the basement rocks of the Korean Peninsula,and were sourced from both the Gyeonggi and Yeongnam massifs.(ii)The meso-to Neoproterozoic zircons,preserved only in the middle to Late Cambrian clastic sedimentary rocks within the carbonate sequences probably reflect proximal provenance.(iii)The youngest Paleozoic zircons of each formation,almost coincident with their deposition ages,suggest presence of syndepositional magmatism,indicating proximal magmatic sources during their deposition.(iv)The Cambrian-Ordovician zircons,from the Lower Paleozoic sequences,but rare in the successive Upper Paleozoic sequences,suggest a provenance change after the hiatus between the two sedimentary successions.(v)The Permian zircons showing differentεHf(t)values indicate that detrital sources were varied at that time.The integrated results in our study suggest provenance variability linked to diverse tectonic environments,reflecting prolonged subduction-related crustal evolution of the proto-Korean Peninsula during the Paleozoic.

关键词： Detrital zircon U-Pb and Hf isotopes Paleozoic metasedimentary rocks Okcheon Belt Taebaeksan zone Korean Peninsula

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mantle contributions to granitoids associated with Sn mineralization:Geochemical and isotopic evidence from the giant Dachang deposit,South China

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Geoscience Frontiers 2024年第1期15卷 187-208页

作者： Tingyi Wang Qihai Shu Xiaoping Xia Chao Li Yanning Wang Jiahao Chen Xiang Sun m.santosh Qingfei Wang State Key Laboratory of Geological Processes and mineral Resources China University of GeosciencesBeijing 100083China Frontiers Science Center for Deep-time Digital Earth China University of Geosciences(Beijing)Beijing 100083China State Key Laboratory of Isotope Geochemistry Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China National Research Center for Geoanalysis Chinese Academy of Geological SciencesBeijing 100037China Department of Earth Science University of AdelaideAdelaideSouth Australia 5005Australia State Key Laboratory of Nuclear Resources and Environment East China University of TechnologyNanchang 330013China

major Sn deposits are commonly linked to crust-derived and highly evolved granites,with magma generation aided by mantle heating.However,whether and how the mantle components contribute to Sn polymetallic mineralization remains unclear.In this study,in combination with a compilation of equivalent data in the region,we provide new constraints on this issue based on detailed investigations on the petrogenesis and metallogenic significance of granitoids including the causative batholith and later granodiorite porphyry dike in the giant Dachang Sn deposit from South China.The former has zircon U-Pb ages of 93-91 ma and belongs to highly evolved S-type biotite granite,which experienced fractionation of massive feldspar.The latter shows zircon U-Pb ages of 90 ma and displays I-type granite features.The batholith was mainly derived from the dehydration melting of biotite in the metasedimentary sources,as revealed by the relatively low whole-rock Pb contents(m)and high Ba/Pb ratios(2.71-17.1)and initial T(ti-zr)of 790℃.Compared with the adjacent crust-derived S-type granites(-24.8--5.1)and I-type granites(-11.0 to-5.2),the Dachang S-type biotite granites present higher zirconεHf(t)values(-9.1 to-2.1).Furthermore,the low magmatic zirconδ18O values(6.2‰)and higher apatite LREE(3277-4114 ppm)and Sr(1137-1357 ppm)contents than of arc-type basic rocks were discerned.These characteristics jointly hint the contributions of mantle components.The higher initial T(ti-zr)(>850℃),whole-rock mg#(52 to 58),apatiteεNd(t)(-9.2 to-6.5)and zirconεHf(t)(-7.6 to 2.5)values but lower zirconδ18O values(6.33 to 8.30‰)of the later granodiorite porphyry dike than those of the batholith also suggest that mantle material was involved in the generation of the dikes,which is evident by the variational features of zircon and apatite trace elements.In addition,at the zircon Hfm and Eu/Eu*>0.05,the higher zirconΔFmQ values(mostly from-1.8 to 2.0)and H2O contents(100-1100 ppm)of the Dachang granitoids than the pure crust-derived S-type gr

关键词： Highly evolved S-type biotite granite I-type granodiorite porphyry dike Crust-mantle mixing mantle contributions Dachang Sn mineralization

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Fluoride contamination in groundwater:A global review of the status,processes,challenges,and remedial measures

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Geoscience Frontiers 2024年第2期15卷 1-29页

作者： E.Shaji K.V.Sarath m.santosh P.K.Krishnaprasad B.K.Arya manisha S.Babu Department of Geology University of KeralaKariavattom CampusThiruvananthapuramKerala 695581India School of Earth Sciences and Resources China University of Geosciences(Beijing)29 Xueyuan RoadBeijing 100083China Department of Earth Science University of AdelaideAdelaideSA 5005Australia Department of Geology Central University of KeralaTejaswini HillsPeriyeKasaragodKerala 671316India

Groundwater pollution by fluoride is one of the prime concerns of the world population due to its toxicity,which results in adverse health impacts.In this paper,we review the current scenario of the fluoride contamination of groundwater in various countries across the globe and its impact on human health.During the last decade,several newly affected regions have been reported all over the world,with more than 100 countries affected by fluoride contamination in groundwater(concentration exceeding the acceptable limit of 1.5 mg/L defined by the World Health Organization).Fluoride poisoning is mainly due to the unsupervised ingestion of products for dental and oral hygiene and over-fluoridated drinking water.It is estimated that more than 200 million people from different countries are affected by fluoriderelated groundwater issues and health problems.The highest among these are from the countries in Africa(38),Asia(28),and Europe(24),followed by countries like South America(5),North America(3),and Australia(2).The source of fluoride in drinking water is primarily geogenic,together with forage,grasses and grains,tea,and anthropogenic sources.These countries affected were correlated with climatic zones and geological factors to gain insights into geospatial relations.Our analyses show that most of the fluoride pollution-prone zones are located in high-grade metamorphic terranes with granitoid or alkaline intrusions,geothermal hot springs,and volcanic regions with arid or semi-arid climatic conditions.This study also finds that children across the globe are more vulnerable than adults to fluoride contamination.The review finds that,although there are efficient fluoride removal techniques,including filters with next-generation nanomaterials,to date,there has not been a single technique developed that can claim to be a practically robust solution for fluoride removal from drinking water.Therefore,we suggest developing next-generation filters that can retain essential minerals in water and remove only harmful ones and se

关键词： Fluoride Groundwater Water contamination WHO standards Climate zones Remediation Sustainable Development Goals

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Paleo-mesoarchean sedimentary record in the Dharwar Craton,India:Implications for Archean ocean oxygenation

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Geoscience Frontiers 2024年第1期15卷 126-154页

作者： G.Harshitha C.manikyamba m.santosh Cheng-Xue Yang A.Keshav Krishna V.V.Sesha Sai I.Panduranga Reddy CSIR-National Geophysical Research Institute(NGRI) Uppal RoadHyderabad 500007India Department of Geology Osmania UniversityHyderabad 500007India School of Earth Science and Resources China University of GeosciencesBeijing 100083China Department of Earth Science University of AdelaideAdelaide SA5005Australia Yonsei Frontier Lab Yonsei UniversitySeoul 03722Republic of Korea Geological Survey of India State UnitNagpurIndia

The early Archean oceans were marked by significant redox changes which have subsequently shaped the Earth’s biosphere.Archean chemical sediments of banded Iron and manganese formations provide important geochemical proxies for these historical shifts in the redox conditions and to trace the ancient sedimentation patterns and protoliths.In this study,we investigate the proto-ore of the Archean mn-formations of the Sandur,Chitradurga and Shimoga greenstone belts of Dharwar Craton of southern Peninsular India,which is geochemically characterised as quartz arenites,mn-arenites,Fe-arenites,mn-argillites and Fe-argillites.The geochemical systematics suggest their deposition in shallow to deeper shelf in the Archean proto-ocean.The detrital zircon U-Pb systematics of mn arenites and argillites indicate their maximum depositional age of 3230±52 ma representing the oldest onset of sedimentation during the Paleo-mesoarchean timeframe in the Chitradurga Group of Dharwar Supergroup.The detrital influx proxies suggest variations in sedimentation rates associated with the Archean transgressive-regressive cycles and fluctuating hydrodynamic conditions,together reflecting an increasing trend in the contributions of recycled sediment from Sandur to Chitradurga and Shimoga greenstone belts.The available detrital zircon ages of the mn arenites and argillites from these greenstone belts indicate a~600 ma prolonged period of mn deposition for which high-T hydrothermal fluids from Archean mid-oceanic ridges supplied the manganese.The trace element compositions of the concordant detrital zircons suggest 3.3-3.1 Ga Dharwar basement TTG/granitoid source which is corroborated by the zircon crystallization temperatures of 690-820℃.The source-normalisedα-dose rates of the detrital zircons signify greater degrees of sediment transport and multi-cycle nature which correspond to the earliest episode of crustal growth in the Indian sub-continent associated with the mesoarchean Ur supercontinent.The clastic-chemogenic sedimentation attained thr

关键词： mn-arenites-argillites Dharwar Craton Zircon U-Pb geochronology Passive margin sediments Ocean oxygenation

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Geochronology and Geochemistry of Ore-related Granitoids in the Giant Gariatong Rb Deposit,Tibet and Implications for Rb metallogeny in China

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Acta Geologica Sinica(English Edition) 2024年第1期98卷 83-103页

作者： LIN Bin TANG Juxing TANG Pan SUN Yan QI Jing msantosh XIE Jinling DENG Shilin LI Faqiao XIE Fuwei ZHOU Aorigele mNR Key Laboratory of metallogeny and mineral Assessment Institute of Mineral ResourcesChinese Academy of Geological SciencesBeijing 100037China SinoProbe Laboratory Chinese Academy of Geological SciencesBeijing 100094China The Key Laboratory of the ministry of Education on Solid Waste Treatment and Recycling School of Environment and ResourceSouthwest University of Science and TechnologyMianyangSichuan 621010China School of Earth Sciences and Resources China University of Geosciences(Beijing)Beijing 100083China Department of Earth Sciences University of AdelaideAdelaide SA-5005Australia Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 610031China Regional Geological Survey Team of the Tibetan Bureau of Geology and mineral Exploration and Development Lhasa 851400China College of Earth Science and Key Laboratory of Tectonic Controlled mineralization and Oil Reservoirs Chengdu University of TechnologyChengdu 610059China

Rubidium(Rb)deposits mostly occur in the South China and Central Asia orogenic belts and are often closely associated with highly differentiated granites.This study investigates a newly-discovered giant Rb deposit at Gariatong in the Central Lhasa terrane in Tibet.Detailed field studies and logging data revealed that the Rb mineralization mainly occurs in monzogranite and is related to greisenization.LA-ICP-mS U-Pb dating of zircon yielded ages of 19.1±0.2 ma and 19.0±0.2 ma for greisenized monzogranite and fresh monzogranite,respectively.The monzogranites are characterized as strongly peraluminous,with high contents of SiO2,Al2O3,K2O and Na2O as well as a high differentiation index.They are enriched in light rare earth and large ion lithophile elements with significant negative Eu anomalies and depleted high fieldstrength elements.Petrological and geochemical features of these ore-related monzogranites suggest that they are highly fractionated S-type granites,derived from remelting of crustal materials in a post-collisional setting.The geochemistry of zircon and apatite points to a low oxygen fugacity of the ore-related monzogranite during the magma’s evolution.The discovery of the Gariatong Rb deposit suggests that the Central Lhasa terrane may be an important region for rare metal mineralization.

关键词： LA-ICP-mS U-Pb dating geochemistry Rb metallogeny Gariatong Tibet

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The Early-middle Triassic Supervolcano in the Yangtze Block,South China and associated obstacles to biotic recovery

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Geoscience Frontiers 2024年第1期15卷 69-83页

作者： Haifeng Chen Hao Zou msantosh Huawen Cao Franco Pirajno Changcheng Huang mingcai Hou State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Chengdu University of TechnologyChengduSichuan 610059China College of Earth Science Chengdu University of TechnologyChengduSichuan 610059China School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China Department of Earth Science University of AdelaideAdelaideSA 5005Australia Yonsei Frontier Lab Yonsei UniversitySeoulSouth Korea Centre of Exploration Targeting The University of Western Australia35 Stirling HighwayCrawleyWA 6009Australia

The end-Permian mass extinction was one of the major global crises spanning the entire Early Triassic or longer.Eruptions of volcanos were one of the factors that delayed the biotic recovery after this event.Supervolcano eruptions can cause catastrophic effects on global environment,climate,and life.Here we investigate the tuff layers from Early-middle Triassic boundary in the Yangtze Block and identify a supervolcano eruption event.The zircon U-Pb ages of the section-Langdai,section-Daijiagou and section-Longmendong tuff samples are 247.1±1.9 ma,247.6±2.0 ma and 247.7±1.7 ma,respectively.These ages mark the Olenekian-Anisian boundary.The zircon grains from the tuff layers have negativeεHf(t)(-15.3 to-0.8),two-stage Hf model(TDm2)ages(1.7 to 2.2 Ga)and display high-δ18O values(mostly>10‰).Clay minerals and quartz dominate the rock composition.The whole rock compositions show that the tuff layers were derived from magma of intermediate to felsic composition,which formed by the remelting of Paleoproterozoic materials of continental crust.The volcanic eruption site is located in the Jinshajiang-Ailaoshan-Song ma suture zone in the southwestern margin of the Yangtze Block.A combination of the closure of the Paleo-Tethys Ocean Basin and the collision of the Indochina Block and South China contributed to the eruption,which was a supervolcano eruption under the active continental margin arc settings.We speculate that this supervolcano eruption might have contributed to the delayed biotic recovery after the end-Permian mass extinction.

关键词： Early-middle Triassic Tuff layer Supervolcano Yangtze Block Biotic recovery

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Composition and evolution of the continental crust:Retrospect and prospect

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Geoscience Frontiers 2022年第5期13卷 1-15页

作者： J.L.R.Touret m.santosh J.m.Huizenga Institut de minéralogie Physique des MatériauxCosmochimieSorbonne Universités4 Place JussieuF-75005 ParisFrance 121 Rue de la Réunion 75020 ParisFrance School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China Department of Earth Science University of AdelaideAdelaideSA 5005Australia Faculty of Environmental Sciences and Natural Resource management Norwegian University of Life SciencesP.O.Box 5003NO-1432ÅsNorway EGRU(Economic Geology Research Centre) James Cook UniversityTownsvilleQueensland 4811Australia Department of Geology University of JohannesburgPO Box 524Auckland Park 2006South Africa

Until the middle of the 20th century,the continental crust was considered to be dominantly granitic.This hypothesis was revised after the Second World War when several new studies led to the realization that the continental crust is dominantly made of metamorphic rocks.magmatic rocks were emplaced at peak metamorphic conditions in domains,which can be defined by geophysical discontinuities.Low to medium-grade metamorphic rocks constitute the upper crust,granitic migmatites and intrusive granites occur in the middle crust,and the lower crust,situated between the Conrad and moho discontinuities,comprises charnockites and granulites.The continental crust acquired its final structure during metamorphic episodes associated with mantle upwelling,which mostly occurred in supercontinents prior to their disruption,during which the base of the crust experienced ultrahigh temperatures(>1000℃,ultrahigh temperature granulite-facies metamorphism).Heat is provided by underplating of mantle-derived mafic magmas,as well as by a massive influx of low H_(2)O activity mantle fluids,i.***.high-density CO_(2) and highsalinity brines.These fluids are initially stored in ultrahigh temperature domains,and subsequently infiltrate the lower crust,where they generate anhydrous granulite mineral assemblages.The brines can reach upper crustal levels,possibly even the surface,along major shear zones,where granitoids are generated through brine streaming in addition to those formed by dehydration melting in upper crustal levels.

关键词： Brines CO_(2) Continental crust Granulite Lower crust

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Contrasting sources and enrichment mechanisms in lithium-rich salt lakes:A Li-H-O isotopic and geochemical study from northern Tibetan Plateau

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Geoscience Frontiers 2024年第2期15卷 315-333页

作者： Fei Xue Hongbing Tan Xiying Zhang msantosh Peixin Cong Lu Ge Chao Li Guohui Chen Yu Zhang School of Earth Sciences and Engineering Hohai UniversityNanjing 210098PR China Key Laboratory of Comprehensive and Highly Efficient Utilization of Salt Lake Resources Qinghai Provincial Key Laboratory of Geology and Environment of Salt LakesQinghai Institute of Salt LakesChinese Academy of SciencesQinghai 810008PR China School of Earth Sciences and Resources China University of Geosciences BeijingBeijing 100083PR China Department of Earth Sciences University of AdelaideSA 5005Australia Yonsei Frontier Lab Yonsei UniversitySeoul 0372Korea

Lithium(Li),a crucial mineral resource for modern high-tech industries,is notably abundant in the northern Tibetan Plateau,primarily within lithium-rich salt lakes.However,the exploration and development of these resources are hindered due to an incomplete understanding of their nature and origin.Here we present results from a comprehensive study on the hydrochemical parameters,whole-rock geochemistry,H-O isotopes,and Li concentrations in surface brine,river water,geothermal springs,and associated rocks from two representative lithium-enriched salt lakes,the Laguo Co(LGC)and Cangmu Co(CmC)in Tibet to understand the genetic mechanisms.Our water-salt balance calculations and H-O isotopic analysis reveal that Li in LGC and CmC primarily originates from the Suomei Zangbo(SmZB,~91%)and Donglong Zangbo(DLZB,~75%)rivers,respectively.It is estimated that the LGC and CmC took a minimum of 6.0 ka and 3.0 ka to accumulate their current lithium resources,respectively.The distinct geological characteristics reflect evolutionary differences between the two lakes,suggesting diverse lithium sources and enrichment processes.The high lithium ion concentration and light lithium isotope composition in the SmZB river waters indicate the genetic relationship with lithium-enriched geothermal springs in the Tibetan Plateau.Our results suggest that lithium in the LGC originates from lithium-enriched geothermal springs and is primarily supplied through the small-scale SmZB river.In contrast,the formation and evolution of CmC are influenced by the northern Lunggar rifts,receiving a prolonged and stable input from the DLZB,resulting in high lithium concentrations and isotopic values.The absence of lithium-enriched geothermal springs and the prevalence of silicate rocks in the CmC catchment suggest that lithium may be sourced from the weathering of silicate rocks,such as granitic pegmatite veins containing lithium-rich beryl,widely distributed in the upstream area of DLZB.The forward modeling approach,quantifying the contribution fractions o

关键词： Lithium isotopes Hydrochemistry Salt lakes Enrichment mechanism Tibetan Plateau

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Thermoelectric characteristics of semiconductor minerals in earth's deep crust and their seismogenic significance

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Geoscience Frontiers 2022年第2期13卷 159-164页

作者： Shuhao Wang Junfeng Shen m.santosh Yuanyuan Li Cheng-Xue Yang Liangkun ma School of Earth Sciences and Resources China University of GeosciencesBeijing 100083China Department of Earth Science University of AdelaideAdelaideSA 5005Australia

Geo-electric anomalies are generated during the process of stress accumulation and release associated with earthquakes.However,the mechanism of these anomalies remains equivocal.Based on the analysis of thermoelectric characteristics of semiconductor minerals of the earth’s deep crust such as graphite,ferrosilicon alloy,magnetite etc.,we perform finite element analysis to evaluate the principles governing the thermoelectric power generated by minerals and rocks.The results show that graphite,ferrosilicon alloy and magnetite all exhibit Seebeck effect and can be superimposed.And the thermo-electric field can be enhanced with the activation temperature increases,the content of thermoelectric minerals increases,the size of aggregates increases,and the spacing of thermoelectric minerals grains decreases.Seismogenic processes would generate a similar thermal gradient.The natural semiconductor minerals in this thermal field show a thermoelectric effect,forming a thermoelectric field that interferes with the background electric field.This study indicates that thermoelectric effect may have an important influence on the formation of geoelectric field.

关键词： Natural semiconductor minerals Seebeck effects Geoelectric anomalies Earthquakes Deep crust

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Effect of chemical composition on zircon radiation damage dating:Implications for low-temperature thermochronology

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Geoscience Frontiers 2023年第6期14卷 368-379页

作者： mingpu Fan Xiaoming Liu Shengsi Sun Yunpeng Dong John C.Ayers m.santosh State Key Laboratory of Continental Dynamics Department of GeologyNorthwest UniversityXi’an 710069China Vanderbilt University Department of Earth&Environmental SciencesPMB 3518052301 Vanderbilt PlaceNashvilleTN 37235-1805USA School of Earth Science and Resources China University of GeosciencesBeijing 100083China Department of Earth Science University of AdelaideAdelaideSA 5005Australia Yonsei Frontier Lab Yonsei UniversitySeoul 03722Republic of Korea

Zircon radiation damage dating is a low-temperature thermochronological method that can reveal the cooling histories of magmatic intrusions and discriminate sedimentary provenance in combination with other dating methods.This method has broad application prospects because of its advantages of nondestructive,high efficiency,and capable of double(or multiple)dating,involving only multiple measurements by Raman spectrometer and laser ablation-inductively coupled plasma-mass spectrometry.However,several factors,such as zircon chemical composition and the non-uniformity of radiation damage annealing kinetics,can cause poor precision when using this method and thus restricts its wide application.This study examined the effect of chemical composition(P,Ti,Dy,Th,U,and Hf)on Raman spectra using synthetic zircon crystals grown in a lithium-molybdate flux.The results show that the full width at half-maximum(FWHm)of the v_(3)(SiO_(4))band has positive linear correlations with the concentrations of P,Ti,Dy,Th,and U in decreasing order of influence,while the FWHm is unaffected by Hf at concentrations10 wt.%.Furthermore,the Raman shift is negatively correlated with Th,U,and Dy concentrations,positively correlated with Hf,and shows no obvious correlation with Ti and P.Thus,our study shows that chemical composition is a non-ignorable factor for calculating zircon radiation damage age using Raman spectroscopy,especially for zircon with relatively high concentrations of P,rare earth elements(REEs),Th,U,and Hf.The obtained multiple linear regression equation provides a potential means for estimating the FWHm at zero dose and implication for improving the dating precision of this method.In addition,the observed effects of REEs,Th,U,and Hf on the Raman shift of the v_(3)(SiO_(4))band indicate that chemical composition in zircon might affect the estimation of the P-T conditions of geological processes when using entrapped zircon inclusions in host minerals or the field of zircon as an in situ pres

关键词： Synthetic zircon Raman spectroscopy Chemical composition Radiation damage dating Cooling age

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