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Photoelectrochemical activity of ZnO:Ag/rGO photo-anodes synthesized by two-steps sol-gel method

Chinese Physics B 2022年第5期31卷 691-702页

作者： D Ben Jemia m Karyaoui m A Wederni A Bardaoui m V martinez-Huerta m Amlouk R Chtourou Laboratory of Nanomaterials and Renewable Energy Systems LANSER Research and Technology Center of EnergyBorj-Cedria Science and Technology ParkBP 952050 Hammam-LifTunisia Faculty of Science of Tunis University of Tunis El ManarTunisia Laboratory of Physics of materials and Nanomaterials Applied to the Environment(LaPhymNE) Faculty of Sciences of GabesCite ErriadhUniversity of Gabes6079 GabesTunisia lnstitute of Catalysis and Petrochemistry CSICin MadridSpain Laboratory of Nanomaterials Nanotechnology and Energy(L2NE)University of Tunis El ManarTunisia

This work investigated the influence of silver plasmon and reduced graphene oxide(r GO)on the photoelectrochemical performance(PEC)of Zn O thin films synthesized by the sol-gel *** physicochemical properties of the obtained photo-anodes were systematically studied by using several characterization *** x-ray diffraction analysis showed that all samples presented hexagonal wurtzite structure with a polycrystalline *** and energy dispersive x-ray(EDX)studies confirmed the existence of both Ag and r GO in Zn O:Ag/r GO thin *** estimated grain size obtained from scanning electron microscopy(SEm)analysis decreased with Ag doping,then increased to a maximum value after r GO *** UV-vis transmission spectra of the as-prepared Zn O:Ag and Zn O:Ag/r GO thin films have shown a reduction in the visible range with a redshift at the absorption *** bandgaps were estimated to be around 3.17 e V,2.7 e V,and 2.52 e V for Zn O,Zn O:Ag,and Zn O:Ag/r GO,***,the electrical measurements revealed that the charge exchange processes were enhanced at the Zn O:Ag/r GO/electrolyte interface,accompanied by an increase in the(PEC)performance compared to Zn O and Zn O:Ag ***,the photocurrent density of Zn O:Ag/r GO(0.2 m A·cm^(-2)) was around 4 and 2.22 times higher than photo-anodes based on undoped Zn O(0.05 m A·cm^(-2)) and Zn O:Ag(0.09 m A·cm^(-2)),***,from the flat band potential and donor density,deduced from the mott-Schottky,it was clear that all the samples were n-type semiconductors with the highest carrier density for the Zn O:Ag/r GO photo-anode.

关键词： zinc oxide reduced graphene oxide silver doping sol-gel photoelectrochemical performance

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SEmI-ANALYTICAL SOLUTION FOR FREE VIBRATION OF THICK FUNCTIONALLY GRADED PLATES RESTED ON ELASTIC FOUNDATION WITH ELASTICALLY RESTRAINED EDGE

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Acta mechanica Solida Sinica 2011年第4期24卷 340-354页

作者： m.Shaban m.m.Alipour Faculty of mechanical Engineering Islamic azad University Parand Branch

This paper deals with free vibration analysis of functionally graded thick circular plates resting on the Pasternak elastic foundation with edges elastically restrained against translation and *** equations are obtained based on the first order shear deformation theory（FSDT） with the assumption that the mechanical properties of plate materials vary continuously in the thickness direction.A semi-analytical approach named differential transform method is adopted to transform the differential governing equations into algebraic recurrence *** eigenvalue equation for free vibration analysis is solved for arbitrary boundary *** between the obtained results and the results from analytical method confirms an excellent accuracy of the present ***,comprehensive studies on the FG plates rested on elastic foundation are *** effects of parameters,such as thickness-to-radius,material distribution,foundation stiffness parameters,different combinations of constraints at edges on the frequency,mode shape and modal stress are also investigated.

关键词： free vibration thick circular plates two-parameter elastic foundation elasticallyrestrained edges

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mHD stagnation point flow of a micropolar fluid towards a heated surface

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Applied mathematics and mechanics(English Edition) 2011年第1期32卷 45-54页

作者： m.ASHRAF m.m.ASHRAF Centre for Advanced Studies in Pure and Applied mathematics Bahauddin Zakariya University

The problem of two dimensional stagnation point flow of an electrically conducting micropolar fluid impinging normally on a heated surface in the presence of a uniform transverse magnetic field is analyzed. The governing continuity, momentum, angular momentum, and heat equations together with the associated boundary conditions are reduced to dimensionless form using suitable similarity transformations. The reduced self similar non-linear equations are then solved numerically by an algorithm based on the finite difference discretization. The results are further refined by Richardson＇s extrapolation. The effects of the magnetic parameter, the micropolar parameters, and the Prandtl number on the flow and temperature fields are predicted in tabular and graphical forms to show the important features of the solution. The study shows that the velocity and thermal boundary layers become thinner as the magnetic parameter is increased. The micropolar fluids display more reduction in shear stress as well as heat transfer rate than that exhibited by Newtonian fluids, which is beneficial in the flow and thermal control of polymeric processing.

关键词： magnetohydrodynamics (mHD) stagnation flow micropolar fluids finitedifferences similarity transformations boundary layer

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modeling and analysis of piezoelectric beam with periodically variable cross-sections for vibration energy harvesting

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Applied mathematics and mechanics(English Edition) 2016年第8期37卷 1053-1066页

作者： m.HAJHOSSEINI m.RAFEEYAN Department of mechanical Engineering Yazd University

A bimorph piezoelectric beam with periodically variable cross-sections is used for the vibration energy harvesting. The effects of two geometrical parameters on the first band gap of this periodic beam are investigated by the generalized differential quadrature rule （GDQR） method. The GDQR method is also used to calculate the forced vibration response of the beam and voltage of each piezoelectric layer when the beam is subject to a sinusoidal base excitation. Results obtained from the analytical method are compared with those obtained from the finite element simulation with ANSYS, and good agreement is found. The voltage output of this periodic beam over its first band gap is calculated and compared with the voltage output of the uniform piezoelectric beam. It is concluded that this periodic beam has three advantages over the uniform piezoelectric beam, i.e., generating more voltage outputs over a wide frequency range, absorbing vibration, and being less weight.

关键词： vibration energy harvesting piezoelectric cantilever beam periodically variable cross-section vibration band gap forced vibration analysis generalized differential quadrature rule (GDQR)

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Compton profiles of NiO and TiO_2 obtained from first principles GWA spectral function

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Chinese Physics B 2016年第6期25卷 407-415页

作者： S m Khidzir m F m Halid W A T Wan Abdullah Department of Physics Universiti of Malaya

In this work,we first use momentum density studies to understand strongly correlated electron behavior,which is typically seen in transition metal *** observe that correlated electron behavior as seen in bulk NiO is due to the Fermi break located in the middle of overlapping spectral functions obtained from a GW（G is Green’s function and W is the screened Coulomb interaction） approximation（GWA） calculation while in the case of TiO2 we can see that the origin of the constant momentum distribution in lower momenta is due to a pile up of spectra before the Fermi *** observations are then used to compare our calculated Compton profiles with previous experimental studies of Fukamachi and *** calculations for NiO are observed to follow the same trend as the experimental profile but it is seen to have a wide difference in the case of TiO2 before the Fermi *** ground state momentum densities differ significantly from the quasiparticle momentum density,thus stressing the importance of the quasiparticle wave function as the input for the study of charge density and the electron localization *** we perform a calculation of the quasiparticle renormalization function,giving a quantitative description of the discontinuity of the GWA momentum density.

关键词： elastic and Compton scattering density functional theory local density approximation gradient and other corrections elements oxides nitrides borides carbides chalcogenides

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Catalytic effect of SrTiO_3 on the hydrogen storage behaviour of mgH_2

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Journal of Energy Chemistry 2019年第1期28卷 46-53页

作者： m.S.Yahya m.Ismail School of Ocean Engineering University Malaysia Terengganu

The effects of Sr TiO_3 on the hydrogen storage properties of mgH_2 have been studied for the first *** onset dehydrogenation temperature of the mgH_2-10 wt% SrTiO_3 is found to be 275 ℃, which is 55 ℃ lower as compared to the as-milled mgH_2. The composite is able to absorb 4.3 wt% of hydrogen in 60 min instead of 1.1 wt% for the as-milled mg H_2. meanwhile, the composite is able to release 5.3 wt% of hydrogen in 17 min compared to 1.9 wt% by the as-milled mg H_2 at 320 ℃. The calculated Eaof the mg H_2-10 wt% SrTiO_3 is 109 k J/mol, which is 26.3 kJ/mol lower than the calculated Eaof the as-milled mgH_2. The Sr TiO_3 is not decomposed during the ball milling and the re/dehydrogenation processes. The catalytic effect shown by the SrTiO_3 is owing to its ability to change the physical structure of the mgH_2 particles during the ball milling process.

关键词： Hydrogen storage magnesium hydride Catalytic effect Sorption properties

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EFFECT OF GAmmA RAYS IN THE PREPARATION OF POLYmER AND HYDROGEL FROm ACRYLAmIDE mONOmER

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Chinese Journal of Polymer Science 2003年第4期21卷 437-442页

作者： m.m.Alam m.F.mina F.Akhtar NRCD INST AERE GPO Box-3787 Dhaka BangladeshNRCD INST AERE GPO Box-3787 Dhaka BangladeshNRCD INST AERE GPO Box-3787 Dhaka Bangladesh

The formation of polymer and hydrogel from aqueous solutions having 20, 30 and 40% concentrations ofacrylamide monomer by γ-ray irradiation processing in the dose range 0.06-30 kGy using a Co-60 source and theircharacterization have been observed. Polymer conversion and gel fraction are found to depend on radiation doses. Polymerconversion increases with the increase of dose, depending on the solution concentration, where maximum conversion isachieved at 0.18, 0.16 and 0.10 kGy for 20%, 30% and 40% concentrations, respectively. On the other hand, gel fractionincreases with dose from the gel point (0.12 kGy) for all concentrations, where 100% conversion of gel occurs at doses≥5 kGy. Tensile strength, viscosity and molecular weight (m_w) of polymer samples increase with both the dose and theconcentration, showing a high value of m_w up to≈10~8. Swelling of hydrogels under water with respect to time varies due tothe variation of cross-linking density formed in the gels and the maximum swelling mainly occurs within 24 h. A remarkable change of surface morphology reveals characteristic features of monomer, polymer and hydrogel films.

关键词： Polymer Hydrogel γ-Radiation Cross-linking Swelling

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New Exact Solutions of Two Nonlinear Physical models

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Communications in Theoretical Physics 2010年第4期53卷 596-604页

作者： m.m.Hassan mathematics Department Faculty of Science Minia University

Abundant new exact solutions of the Schamel-Korteweg-de Vries （S-KdV） equation and modified Zakharov- Kuznetsov equation arising in plasma and dust plasma are presented by using the extended mapping method and the availability of symbolic computation. These solutions include the Jacobi elliptic function solutions, hyperbolic function solutions, rational solutions, and periodic wave solutions. In the limiting cases, the solitary wave solutions are obtained and some known solutions are also recovered.

关键词： modified Zakharov-Kuznetsov equation Schamel-Korteweg-de Vries equation traveling and periodic wave solutions extended mapping method

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Alternating current characterization of nano-Pt(Ⅱ)octaethylporphyrin(PtOEP) thin film as a new organic semiconductor

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Chinese Physics B 2016年第6期25卷 426-432页

作者： m Dongol m m El-Nahass A El-Denglawey A A Abuelwafa T Soga Nano and Thin Film Laboratory Physics DepartmentFaculty of ScienceSouth Valley University Physics Department Faculty of EducationAin Shams University Physics Department Faculty of Applied Medical ScienceTaif University Department of Frontier materials Nagoya Institute of Technology

Alternating current（AC） conductivity and dielectric properties of thermally evaporated Au/Pt OEP/Au thin films are investigated each as a function of temperature（303 K–473 K） and frequency（50 Hz–5 mHz）.The frequency dependence of AC conductivity follows the Jonscher universal dynamic *** AC-activation energies are determined at different *** is found that the correlated barrier hopping（CBH） model is the dominant conduction *** variation of the frequency exponent s with temperature is analyzed in terms of the CBH *** barrier height Wm,hopping distance Rω,and the density of localized states N（EF） are valued at different *** constant ε1（ω,T） and dielectric loss ε2（ω,T） are discussed in terms of the dielectric polarization *** dielectric modulus shows the non-Debye relaxation in the *** extracted relaxation time by using the imaginary part of modulus（m’’）is found to follow the Arrhenius law.

关键词： PtOEP thin films AC conductivity dielectric constants organic semiconductors solar cell nano materials

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New ternary superconducting compound LaRu2As2： Physical properties from density functional theory calculations

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Chinese Physics B 2017年第3期26卷 453-460页

作者： m A Hadi m S Ali S H Naqib A K m A Islam Department of Physics University of Rajshahi Rajshahi 6205 Bangladesh Department of Physics Pabna University of Science and Technology Pabna 6600 Bangladesh International Islamic University Chittagong Chittagong 4203 Bangladesh

In this paper, we perform the density functional theory （DFT） -based calculations by the first-principles pseudopo- tential method to investigate the physical properties of the newly discovered superconductor LaRu2As2 for the first time. The optimized structural parameters are in good agreement with the experimental results. The calculated independent elas- tic constants ensure the mechanical stability of the compound. The calculated Cauchy pressure, Pugh＇s ratio as well as Poisson＇s ratio indicate that LaRu2As2 should behave as a ductile material. Due to low Debye temperature, LaRu2As2 may be used as a thermal barrier coating （TBC） material. The new compound should exhibit metallic nature as its valence bands overlap considerably with the conduction bands. LaRu2As2 is expected to be a soft material and easily machinable because of its low hardness value of 6.8 GPa. The multi-band nature is observed in the calculated Fermi surface. A highly anisotropic combination of ionic, covalent and metallic interactions is expected to be in accordance with charge density calculation.

关键词： new superconductor LaRu2As2 density functional theory (DFT) calculations mechanical proper-ties electronic features

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