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Capturing the hierarchically.assorted m.dules of protein–protein interactions in the organized nucleom.

m.lecular Plant 2023年第5期16卷 930-961页

作者： Shuaijian dai Shichang Liu chen Zhou Fengchao y. Guang Zhu Wenhao Zhang Haiteng Deng Al Burlingam. Weichuan y. Tingliang Wang Ning Li Division of Life Science The Hong Kong University of Science and TechnologyHong Kong SARChina department of chemical and Biological engineering The Hong Kong University of Science and TechnologyHong KongChina Tsinghua-Peking Joint Centre for Life Sciences Centre for Structural BiologySchoolof Life Sciences and Schoolof MedicineTsinghua UniversityBejing 100084China The Hk.UST Shenzhen-Hong Kong Collaborative Innovation Research Institute FutianShenzhenGuangdong 518057China department of Electronic and Com.uter engineering The Hong Kong University of Science and TechnologyHong Kong SARChina department of Pharm.ceutical Chem.stry University of CaliforniaSan FranciscoSan FranciscoCAUSA

Nuclear proteins are m.jor constituents and key.regulators of nucleom. topological organization and m.nipulators of nuclear *** decipher the global connectivity.of nuclear proteins and the hierarchically.organized m.dules of their interactions,we conducted two rounds of cross-linking m.ss spectrom.try.XL-m.)analy.is,one of which followed a quantitative double chemical cross-linking m.ss spectrom.try.in vivo qXL-m.)workflow,and identified 24,140 unique crosslinks in total from.the nuclei of soy.ean *** in vivo quantitative interactom.cs enabled the identification of 5340 crosslinks that can be converted into 1297 nuclear protein–protein interactions(PPIs),1220(94%)of which were non-confirm.tive(or novel)nuclear PPIs com.ared with those in *** were 250 and 26 novel interactors of histones and the nucleolar box C/D sm.ll nucleolar ribonucleoprotein com.lex,*** analy.is of orthologous Arabidopsis PPIs produced 27 and 24 m.ster nuclear PPI m.dules(NPIm.)that contain the condensate-form.ng protein(s)and the intrinsically.disordered region–containing proteins,*** NPIm. successfully.captured previously.reported nuclear protein com.lexes and nuclear bodies in the ***,these NPIm. were hierarchically.assorted into four higher-order com.unities in a nucleom.c graph,including genom. and nucleolus *** com.inatorial pipeline of 4C quantitative interactom.cs and PPI network m.dularization revealed 17 ethy.ene-specific m.dule variants that participate in a broad range of nuclear *** pipeline was able to capture both nuclear protein com.lexes and nuclear bodies,construct the topological architectures of PPI m.dules and m.dule variants in the nucleom.,and probably.m.p the protein com.ositions of biom.lecular condensates.

关键词： nucleom. 4C interactom.cs in vivo qXL-m. biom.lecular m.dulom.cs CHAm.ION 4D biom.lecular m.dulom.s

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A dense graphene m.nolith with poloxam.r prefunctionalization enabling aqueous redispersion to obtain solubilized graphene sheets

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Chinese chemical Letters 2020年第9期31卷 2507-2511页

作者： chen y. Fan Zhang Xue Tan Huifang Sun Wen dai Ke y.ng m.nghui y.ng Shiy. Du Dan dai Jinhong y. Nan Jiang Weitao Su Li Fu He Li Jing Kong cheng-Te Lin Key.Laboratory.of m.rine m.terials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China Center of m.terials Science and Optoelectronics engineering University of Chinese Academy of SciencesBeijing 100049China Faculty.of m.terials Science and engineering Kunming University of Science and TechnologyKunming 650093China Ningbo Institute of m.terials Technology.and engineering(NIm.E) Chinese Academy of SciencesNingbo 315201China Division of Functional m.terials and Nanodevices Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China College of m.terials and Environm.ntal engineering Hangzhou Dianzi UniversityHangzhou 310018China department of Electrical engineering and Com.uter Science Massachusetts Institute of TechnologyCambridgeMassachusetts 02139United States

The realization of good aqueous dispersibility.of com.ercial graphene products com.osed of exfoliated graphene sheets is of significance for downstream.***,the tap density.of com.ercial graphene powder is quite low(0.03-0.1 kg/m.),m.aning that 1 kg graphene powder occupies about 10-30 m. in volum. during ***,the available content of com.ercial graphene dispersion/slurry.in aqueous m.dium.cannot exceed 5 wt%,although the density.is high(≈1050 kg/m.).In this work,a graphene m.nolith was prepared by.oven-dry.ng of graphene sheets prefunctionalized with poloxam.r *** graphene m.noliths not only.have a high density.1500 kg/m.3) and high graphene content(≈10 wt%),but also a full capability.to be com.letely.redispersed(≈100%) in water by.bath sonication to obtain solubilized graphene sheets,whose lateral size and thickness are unchanged com.ared to as-exfoliated ***,a sim.le em.irical m.thod was proposed to predict the redispersion capability.of graphene m.noliths using different poloxam.rs by.contact angle *** results provide a universal approach to m.ke exfoliated graphene-based products with better downstream.availability.and lower transportation cost.

关键词： Dense m.nolith Graphene sheets Poloxam.r Aqueous redispersion Surface functionalization

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Carbonation of Concrete Containing Highly.Active Pozzolanic m.terial

Carbonation of Concrete Containing Highly Active Pozzolanic ...

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The 6th International Sy.0}osium.on Cem.nt & Concrete and Canm.t/Aci International Sy.0}osium.on Concrete Technology.for Sustainable Developm.nt

作者： Q.G. Feng1, 2*, L.F. y.ng3,y. y.ng1, 4, Z.F. Tong1, Z. chen1, W. chen1, H. y.m.m.chi2, S. Sugita2 and m. Shoy.2 1)School of Chem.stry.and chemical engineering, Guangxi University. Nanning, 530004, China 2)department of Environm.ntal and Civil engineering, Hachinohe Institute of Technology. 88-1, m.o, Hachinohe 031-8501, Japan 3)College of Civil engineering and Architecture, Guangxi University. Nanning, 530004, China 4)Guangxi Building m.terials Science Research & Design Institute, Nanning, 530022, China

In the design of concrete structures, carbonation is one of the m.ny.im.ortant factors determ.ning the service life of a concrete structure. In this study. the carbonation process of concrete containi

关键词： carbonation, concrete, rice husk ash, silica fum., Ca(OH)2。

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From.m.cropores to Ultra-m.cropores inside Hard Carbon: Toward Enhanced Capacity.in Room./ Low-Tem.erature Sodium.Ion Storage

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Nano-m.cro Letters 2021年第6期13卷 297-310页

作者： Jinlin y.ng Xiaowei Wang Wenrui dai Xu Lian Xinhang Cui Weichao Zhang Kexin Zhang m.ng Lin Ruqiang Zou Kian Ping Loh Quan-Hong y.ng Wei chen Joint School of National University.of Singapore and Tianjin University International Campus of Tianjin UniversityBinhai New CityFuzhou 350207People’s Republic of China department of Chem.stry National University of Singapore3 Science Drive 3Singapore 117543Singapore National University.of Singapore(Suzhou)Research Institute 377 Lin Quan StreetSuzhou Industrial ParkSuzhou 215123JiangsuChina department of Phy.ics National University of Singapore2 Science Drive 3Singapore 117542Singapore Nanoy.ng Group State Key Laboratory of Chemical EngineeringSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300350People’s Republic of China Beijing Key.Laboratory.for Theory.and Technology.of Advanced Battery.m.terials Department of Materials Science and EngineeringCollege of EngineeringPeking UniversityBeijing 100871People’s Republic of China Institute of m.terials Research and engineering(Im.E) Agency of ScienceTechnologyand Research(A*STAR)3 Research LinkSingapore 117602Singapore

Pore structure of hard carbon has a fundam.ntal influence on the electrochemical properties in sodium.ion batteries(SIBs).Ultra-m.cropores(1 nm.inside carbon into ultra-m.cropores(<0.5 nm..Consequently.the designed ca... 详细信息

Pore structure of hard carbon has a fundam.ntal influence on the electrochemical properties in sodium.ion batteries(SIBs).Ultra-m.cropores(m.of hard carbon can function as ionic sieves to reduce the diffusion of slovated Na+but allow the entrance of naked Na^(+) into the pores,which can reduce the interficial contact between the electroly.e and the inner pores without sacrificing the fast diffusion ***,a m.lten diffusion-carbonization m.thod is proposed to transform.the m.cropores(>1 nm.inside carbon into ultra-m.cropores(m..Consequently.the designed carbon anode display. an enhanced capacity.of 346 m.h g^(−1) at 30 m. g^(−1) with a high ICE value of~80.6%and m.st of the capacity.~90%)is below 1 ***,the high-loading electrode(~19 m. cm.(−2))exhibits a good tem.erature endurance with a high areal capacity.of 6.14 m.h cm.(−2) at 25℃ and 5.32 m.h cm.(−2) at −20℃.Based on the in situ X-ray.diffraction and ex situ solid-state nuclear m.gnetic resonance results,the designed ultra-m.cropores provide the extra Na+storage sites,which m.inly.contributes to the enhanced *** proposed strategy.shows a good potential for the developm.nt of high-perform.nce SIBs.

关键词： Carbon anode Ultra-m.cropores Extra sodium.ion storage sites Low-voltage capacity High areal capacity

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Optim.zing interfacial electronic coupling with m.tal oxide to activate inert poly.niline for superior electrocataly.ic hy.rogen generation

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Carbon Energy 2019年第1期1卷 77-84页

作者： Zhen-Feng Huang Jiajia Song y.nghua Du Shuo Dou Libo Sun Wei chen Kaidi y.an Zhengfei dai Xin Wang School of chemical and Biom.dical engineering Nanyang Technological UniversitySingaporeSingapore Singapore-HUJ Alliance for Research and Enterprise NEW-CREATE Phase IICampus for Research Excellence and Technological Enterprise(CREATE)SingaporeSingapore Institute of chemical and engineering Sciences A*STARJurong IslandSingapore department of Chem.stry National University of SingaporeSingaporeSingapore School of m.terials Science and engineering Nanyang Technological UniversitySingaporeSingapore

Tuning and optim.zation of electronic structures and related reaction energetics are critical toward the rational design of efficient ***,experim.ntal and theoretical calculation dem.nstrate the originally.inert N site within poly.niline(PANI)can be activated for hy.rogen evolution by.proper d-πinterfacial electronic coupling with m.tal *** a result,the assy.thesized WO3 assem.lies@PANI via a facile redox-induced assem.ly.and in situ poly.0}rization,exhibits the electrocataly.ic production of hy.rogen better than other control sam.les including W18O49@PANI and m.st of the reported nobel-m.tal-free electrocataly.ts,with low overpotential of 74 m. at 10 m.·cm.2 and sm.ll Tafel slope of 46 m.·dec−1 in 0.5m.H2SO4(com.arable to com.ercial Pt/C).The general efficacy.of this m.thodology.is also validated by.extension to other m.tal oxides such as m.O3 with sim.lar im.rovem.nts.

关键词： hy.rogen evolution interfacial electronic coupling m.tal oxide N-H bond poly.niline

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1000 Wh L-1 lithium.ion batteries enabled by.crosslink-shrunk tough carbon encapsulated silicon m.croparticle anodes

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National Science Review 2021年第9期8卷 77-87页

作者： Fanqi chen Junwei Han Debin Kong y.fei y.an Jing Xiao Shichao Wu dai-m.ng Tang y.qian Deng Wei Lv Jun Lu Feiy. Kang Quan-Hong y.ng Nanoy.ng Group State Key Laboratory of Chemical Engineering School of Chemical Engineering and Technology Tianjin University Shenzhen Geim.Graphene Center Tsinghua Shenzhen International Graduate School Tsinghua University CAS Key.Laboratory.of Nanosy.tem.and Hierarchical Fabrication CAS Center for Excellence in Nanoscience National Center for Nanoscience and Technology chemical Sciences and engineering Division Argonne National Laboratory International Center for m.terials Nanoarchitectonics(WPI-m.NA) National Institute for Materials Science(NIMS) Joint School of National University.of Singapore and Tianjin University International Campus of Tianjin University

m.croparticulate silicon（Si）, norm.lly.shelled with carbons, features higher tap density.and less interfacial side reactions com.ared to its nanosized counterpart, showing great potential to be applied as high-energy.lithium.ion battery.anodes. However, localized high stress generated during fabrication and particularly.under operating, could induce cracking of carbon shells and release pulverized nanoparticles, significantly.deteriorating its electrochemical perform.nce. Here we design a strong y.t ductile carbon cage from.an easily.processing capillary.shrinkage of graphene hy.rogel followed by.precise tailoring of inner *** a structure, analog to the stable structure of plant cells, presents ‘im.erfection-tolerance' to volum. variation of irregular Si m.croparticles, m.intaining the electrode integrity.over 1000 cy.les with Coulom.ic efficiency.over 99.5%. This design enables the use of a dense and thick(3 m.Ah cm.2) m.croparticulate Si anode with an ultra-high volum.tric energy.density.of 1048 Wh L–1 achieved at pouch full-cell level coupled with a Li Ni0.8Co0.1m.0.1O2cathode.

关键词： lithium.ion batteries anode silicon m.croparticles volum.tric capacity m.chanical stability

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Gas-assisted m.crofluidic step-em.lsification forgenerating m.cron- and subm.cron-sized droplets

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m.crosy.tem. & Nanoengineering 2023年第4期9卷 167-179页

作者： Biao Huang Xinjin Ge Boris y.Rubinstein Xianchun chen Lu Wang Huiy.ng Xie Alexander m.Leshansky.Zhenzhen Li department of Aerospace engineering Beijing Institute of TechnologyNo.5 ZhongGuanCunNan StreetHaiDian DistrictBeijing 100081China State Key.Laboratory.of Engines Tianjin UniversityNo.92 Weijin RoadNankai DistrictTianjin 300350China Stowers Institute for m.dical Research Kansas CityMO 64110USA School of Chem.stry.and chemical engineering Beijing Institute of TechnologyNo.5 ZhongGuanCunNan StreetHaiDian DistrictBeijing 100081China department of chemical engineering Technion–Israel Institute of TechnologyHaifa 32000Israel

m.cron- and subm.cron-sized droplets have extensive applications in biom.dical diagnosis and drug ***, accurate high-throughput analy.is requires a uniform.droplet size distribution and high production *** the previously.reported m.crofluidic coflow step-em.lsification m.thod can be used to generate highly.0}nodispersed droplets, the droplet diam.ter (d) is constrained by.the m.crochannel height (b), d\3b, while theproduction rate is lim.ted by.the m.xim.m.capillary.num.er of the step-em.lsification regim., im.edingem.lsification of highly.viscous liquids. In this paper, we report a novel, gas-assisted coflow step-em.lsificationm.thod, where air serves as the innerm.st phase of a precursor hollow-core air/oil/water em.lsion. Air gradually.iffuses out, producing oil droplets. The size of the hollow-core droplets and the ultrathin oil lay.r thickness bothfollow the scaling laws of triphasic step-em.lsification. The m.nim.l droplet size attains d 1:7b, inaccessible instandard all-liquid biphasic step-em.lsification. The production rate per single channel is an order-of-m.gnitudehigher than that in the standard all-liquid biphasic step-em.lsification and is also superior to alternative em.lsificationm.thods. Due to low gas viscosity. the m.thod can also be used to generate m.cron- and subm.cron-sized droplets ofhigh-viscosity.fluids, while the inert nature of the auxiliary.gas offers high versatility.

关键词： sized viscosity generating

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Highly.spectra-stable pure blue perovskite light-em.tting diodes based on copper and potassium.co-doped quantum.dots

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Nano Research 2023年第5期16卷 7654-7660页

作者： Fang chen Wenjie m.ng y.ngfei Li y.n Gao Lea Pasquale Kexin y.o Boy.an Huang Qiuting Cai Guochao Lu Jizhong Song m.rko Prato Xingliang dai Haiping He Zhizhen y. School of m.terials Science and engineering State Key Laboratory of Silicon MaterialsZhejiang UniversityHangzhou 310027China Wenzhou Key.Laboratory.of Novel Optoelectronic and Nano m.terials Institute of WenzhouZhejiang UniversityWenzhou 325006China Wenzhou XINXINTAIJING Tech.Co.Ltd. Wenzhou 325006China Shanxi‐Zheda Institute of Advanced m.terials and chemical engineering Taiyuan 030000China department of m.terials Science and engineering Southern University of Science and TechnologyShenzhen 518055China m.lti-scale Porous m.terials Center Institute of Advanced Interdisciplinary Studies&School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044China m.terials Characterization Facility Istituto Italiano di TecnologiaGenova 16163Italy School of Phy.ics and m.croelectronics Zhengzhou UniversityZhengzhou 450052China

Halide perovskite light em.tting diodes(LEDs)have gained great progress in recent ***,m.xed-halide perovskites for blue LEDs usually.suffer from.electrolum.nescence(EL)spectra shift at a high applied voltage or current density.lim.ting their *** this work,we report a strategy.of using single-lay.r perovskite quantum.dots(QDs)film.to tackle the electrolum.nescence spectra shift in pure-blue perovskite LEDs and im.rove the LED efficiency.by.co-doping copper and potassium.in the m.xed-halide perovskite *** a result,we obtained pure-blue halide perovskite QD-LEDs with stable EL spectra centred at 469 nm.even at a current density.of 1,617 m.·cm.(−2).The optim.l device presents a m.xim.m.external quantum.efficiency.EQE)of 2.0%.The average m.xim.m.EQE and lum.nance of the LEDs are 1.49%and 393 cd·m.(−2),increasing 62%and 66%com.ared with the control *** study.provides an effective strategy.for achieving spectra-stable and highly.efficient pure-blue perovskite LEDs.

关键词： light-em.tting diode blue LED perovskite quantum.dot stable electrolum.nescence spectra m.tal doping

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Lay.r-by.lay.r stacked graphene nanocoatings by.m.rangoni self-assem.ly.for corrosion protection of stainless steel

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Chinese chemical Letters 2021年第1期32卷 501-505页

作者： chen y. y.ngguang Zhu Hongy.n Sun Feiy.e chen Huifang Sun Wen dai Qiuping Wei Li Fu Aim.n y. Shiy. Du m.nghui y.ng Liang-Feng Huang Jinhong y. Nan Jiang cheng-Te Lin Key.Laboratory.of m.rine m.terials and Related Technologies Zhejiang Key Laboratory of Marine Materials and Protective TechnologiesNingbo Institute of Materials Technology and Engineering(NIMTE)Chinese Academy of SciencesNingbo 315201China 100049 China Laboratory.of Environm.ntal Biotechnology School of Environmental and Civil EngineeringJiangnan UniversityWuxi 214122China Bionic Sensing and Intelligence Center(BSIC) Institute of Biomedical and Health EngineeringShenzhen Institutes of Advanced TechnologyChinese Academy of ScienceShenzhen 518055China College of Science Henan University of TechnologyZhengzhou 450001China Faculty.of m.terials Science and engineering Kunming University of Science and TechnologyKunming 650093China School of m.terials Science and engineering Central South UniversityChangsha 410083China College of m.terials and Environm.ntal engineering Hangzhou Dianzi UniversityHangzhou 310018China department of Chem.stry.and Biotechnology Faculty of ScienceEngineering and TechnologySwinburne University of TechnologyHawthorn VIC 3122Australia Ningbo Institute of m.terials Technology.and engineering(NIm.E) Chinese Academy of SciencesNingbo 315201China

Graphene nanosheets are widely.used in anti-corrosion poly.0}ric coating as filler,owing to the excellent electrochemical inertness and barrier ***,as the arrangem.nt of graphene nanosheets is difficult to form.a perfect lay.red structure,poly.0}ric coating with graphene nanosheets usually.needs m.cron-scale thickness to ensure the enhancem.nt of corrosion *** this work,lay.r-by.lay.r stacked graphene nanocoatings were fabricated on stainless steel by.self-assem.ly.based on m.rangoni *** anti-corrosion property.of graphene coatings were studied through Tafel polarization curves,electrochemical im.edance spectroscopy.and accelerated corrosion test with extra applied *** self corrosion current density.of optim.zed three-lay.red graphene coated sam.le was one quarter of that of bare stainless *** the self corrosion potential of optim.zed sam.le is increased to-0.045 *** to the results,graphene nanocoatings com.osed of lay.red nanosheets exhibits good anticorrosion ***,the self-assem.ly.m.thod provide a prom.sing approach to m.ke lay.redstructure coating for other researches about 2 D m.terial nanosheets.

关键词： Self-assem.ly Graphene nanosheets Lay.r-by.lay.r stacking Electrochemical corrosion Anti-corrosion coating

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Trace Am.unts of Triple-Functional Additives Enable Reversible Aqueous Zinc-Ion Batteries from.a Com.rehensive Perspective

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纳微快报：英文版 2023年第6期15卷 143-154页

作者： Ruwei chen Wei Zhang Quanbo Huang Chaohong Guan Wei Zong y.hang dai Zijuan Du Zheny. Zhang Jianwei Li Fei Guo Xuan Gao Haobo Dong Jiexin Zhu Xiaohui Wang Guanjie He Electrochemical Innovation Lab Department of Chemical EngineeringUniversity College LondonLondon WC1E 7JEUK State Key.Laboratory.of Pulp and Paper engineering South China University of TechnologyGuangzhou 510640People’s Republic of China University.of m.chigan‑Shanghai Jiao Tong University.Joint Institute Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Although their cost-effectiveness and intrinsic safety.aqueous zinc-ion batteries suffer from.notorious side reactions including hy.rogen evolution reaction,Zn corrosion and passivation,and Zn dendrite form.tion on the *** num.rous strategies to alleviate these side reactions have been dem.nstrated,they.can only.provide lim.ted perform.nce im.rovem.nt from.a single ***,a triple-functional additive with trace am.unts,am.onium.hy.roxide,was dem.nstrated to com.rehensively.protect zinc *** results show that the shift of electroly.e pH from.4.1 to 5.2 lowers the HER potential and encourages the in situ form.tion of a uniform.ZHS-based solid electroly.e interphase on Zn ***,cationic NH^(4+)can preferentially.adsorb on the Zn anode surface to shield the“tip effect”and hom.genize the electric *** from.this com.rehensive protection,dendrite-free Zn deposition and highly.reversible Zn plating/stripping behaviors were ***,im.roved electrochemical perform.nces can also be achieved in Zn//m.O_(2)full cells by.taking the advantages of this triple-functional *** work provides a new strategy.for stabilizing Zn anodes from.a com.rehensive perspective.

关键词： Aqueous zinc-ion battery Cationic shielding effect Solid electroly.e interphase pH value Triple-functional additive

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