检索结果-南通市图书馆

Interfacial Zn2+-solvation regulator towards reversible and stable Zn anode

Journal of Energy Chemistry 2025年第1期100卷 684-692页

作者： Miao Zhou Xiongbin luo Hang Li Shan Guo Zhuang Tong Xiaotao Zhou Xu Li Zhaohui Hou Shuquan Liang Guozhao Fang College of Mechanical Engineering Key Laboratory of Hunan Province for Advanced Carbon-based Functional Materials Hunan Institute of Science and Technology School of Materials Science and Engineering Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province Central South University College of Materials and Metallurgy Guizhou University National Energy Metal Resources and New Materials Key Laboratory Central South University

Aqueous zinc-ion batteries （AZIBs） are fundamentally challenged by the instability of the electrode/electrolyte interface,predominantly due to irreversible zinc （Zn） deposition and hydrogen ***,the intricate mechanisms behind the electrochemical discrepancies induced by interfacial Zn2+-solvation and deposition behavior demand comprehensive *** molecules endowed with special functional groups （such as hydroxyl,carboxyl,etc.） have the potential to significantly optimize the solvation structure of Zn2+and regulate the interfacial electric double layer （EDL）.By increasing nucleation overpotential and decreasing interfacial free energy,these functional groups facilitate a lower critical nucleation radius,thereby forming an asymptotic nucleation model to promote uniform Zn ***,this study presents a pioneering approach by introducing trace amounts of n-butanol as solvation regulators to engineer the homogenized Zn （H-Zn） anode with a uniform and dense *** interfacial reaction and structure evolution are explored by in/ex-situ experimental techniques,indicating that the H-Zn anode exhibits dendrite-free growth,no by-products,and weak hydrogen evolution,in sharp contrast to the bare ***,the H-Zn anode achieves a remarkable Zn utilization rate of approximately 20% and simultaneously sustains a prolonged cycle life exceeding 500 ***,the H-Zn//NH4V4O10（NVO） full battery showcases exceptional cycle stability,retaining 95.04%capacity retention after 400 cycles at a large current density of 5 A *** study enlightens solvation-regulated additives to develop Zn anode with superior utilization efficiency and extended operational lifespan.

关键词： Solvation

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Cortico-striatal gamma oscillations are modulated by dopamine D3 receptors in dyskinetic rats

引用

Neural Regeneration Research 2025年第4期20卷 1164-1177页

作者： Pengfei Wang yuewei Bi Min Li Jiazhi Chen Zhuyong Wang Huantao Wen Ming Zhou Minjie luo Wangming Zhang Neurosurgery Center Department of Pediatric NeurosurgeryGuangdong Provincial Key Laboratory on Brain Function Repair and RegenerationZhujiang HospitalSouthern Medical UniversityGuangzhouGuangdong ProvinceChina

Long-term levodopa administration can lead to the development of levodopa-induced *** oscillations are a widely recognized hallmark of abnormal neural electrical activity in levodopa-induced ***,studies have reported increased oscillation power in cases of levodopa-induced ***,little is known about how the other electrophysiological parameters of gamma oscillations are altered in levodopa-induced ***,the role of the dopamine D3 receptor,which is implicated in levodopa-induced dyskinesia,in movement disorder-related changes in neural oscillations is *** found that the cortico-striatal functional connectivity of beta oscillations was enhanced in a model of Parkinson’s ***,levodopa application enhanced cortical gamma oscillations in cortico-striatal projections and cortical gamma aperiodic components,as well as bidirectional primary motor cortex(M1)↔dorsolateral striatum gamma *** of PD128907(a selective dopamine D3 receptor agonist)induced dyskinesia and excessive gamma oscillations with a bidirectional M1↔dorsolateral striatum ***,administration of PG01037(a selective dopamine D3 receptor antagonist)attenuated dyskinesia,suppressed gamma oscillations and cortical gamma aperiodic components,and decreased gamma causality in the M1→dorsolateral striatum *** findings suggest that the dopamine D3 receptor plays a role in dyskinesia-related oscillatory activity,and that it has potential as a therapeutic target for levodopa-induced dyskinesia.

关键词： aperiodic components dopamine D3 receptor dorsolateral striatum functional connectivity gamma oscillations levodopa-induced-dyskinesia local field potentials neuromodulation Parkinson’s disease primary motor cortex

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Resolving the developmental mechanisms of cardiac microthrombosis of SARS-CoV-2 based on single-cell transcriptome analysis

引用

Science China Life Sciences 2025年第1期68卷 103-115页

作者： Xizi luo Nan Zhang yuntao Liu Beibei Du Xuan Wang Tianxu Zhao Bingqiang Liu Shishun Zhao Jiazhang Qiu Guoqing Wang State Key Laboratory for Diagnosis and Treatment of Severe Zoonotic Infectious Diseases Key Laboratory for Zoonosis Research of the Ministry of EducationCollege of Basic MedicineJilin University State Key Laboratory for Diagnosis and Treatment of Severe Zoonotic Infectious Diseases Key Laboratory for Zoonosis Research of the Ministry of EducationCollege of Veterinary MedicineJilin University College of Mathematics Jilin University Bioinformatic Lab School of MathematicsShandong University Department of Cardiology China-Japan Union HospitalJilin University

The coronavirus disease 2019（COVID-19） outbreak caused by the severe acute respiratory syndrome coronavirus-2（SARS-CoV-2） developed into a global health emergency. Systemic microthrombus caused by SARS-CoV-2 infection is a common complication in patients with COVID-19. Cardiac microthrombosis as a complication of SARS-CoV-2 infection is the primary cause of cardiac injury and death in patietns with severe COVID-19. In this study, we performed single-cell sequencing analysis of the right ventricular free wall tissue from healthy donors,patients who died during the hypercoagulable period of characteristic coagulation abnormality（CAC）, and patients who died during the fibrinolytic period of CAC. We collected 61,187 cells enriched in 24 immune cell subsets and 13 cardiac-resident cell subsets. We found that in the course of SARS-CoV-2 infected heart microthrombus, MyO1EhighRASGEF1Bhighmonocyte-derived macrophages promoted hyperactivation of the immune system and initiated the extrinsic coagulation pathway by activating chemokines CCL3, CCL5. This series of events is the main cause of cardiac microthrombi following SARS-CoV-2 infection. In a SARS-CoV-2 infected heart microthrombus, excessive immune activation is accompanied by an increase in cellular iron content, which in turn promotes oxidative stress and intensifies intercellular competition. This induces cells to alter their metabolic environment, resulting in increased sugar uptake via the glycosaminoglycan synthesis pathway. In addition, high levels of reactive oxygen species generated by elevated iron levels promote increased endogenous malondialdehyde synthesis in a subpopulation of cardiac endothelial cells. This exacerbates endothelial cell dysfunction and exacerbates the coagulopathy process.

关键词： SARS-CoV-2 cardiac microthrombosis immune hyperactivation cell competition

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Cortical hem signaling center: functions, development, and potential implications for evolution and brain disorders

引用

Neural Regeneration Research 2025年第4期20卷 1079-1080页

作者： Victor V.Chizhikov Igor y.Iskusnykh Department of Anatomy and Neurobiology University of Tennessee Health Science CenterMemphisTNUSA

Development of the telencephalon relies upon several signaling centers-localized cellular populations that supply secreted factors to pattern the cortical *** such signaling center is the cortical hem,which arises during embryonic development at the telencephalic dorsal midline,adjacent to the choroid plexus and hippocampal primordium(Figure 1A).While the cortical hem has also been described in reptiles and birds,most of our knowledge about the developmental roles of the cortical hem is derived from the analysis in *** cortical hem produces several types of secreted molecules,including wingless-related integration site(Wnt)and bone morphogenetic(Bmp)*** cortical hem is particularly important for the development of the hippocampus,which is involved in learning and memory,and the neocortex,which is the most complex brain region that mediates multiple types of behavior and higher cognitive functions(Mangale et al.,2008;Dal-Valle-Anton and Borrell,2022).

关键词： epithelium Figure center

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

南秦岭刘岭群砂岩碎屑锆石LA-ICP-MS U-Pb年龄及其构造意义

引用

地质通报 2014年第9期33卷 1363-1378页

作者：陈龙耀罗玉凌刘晓春曲玮胡娟中国地质科学院地质力学研究所北京100081 中国海洋石油总公司规划计划部北京100010

秦岭造山带的构造演化是理解华北与扬子陆块缝合过程的关键,位于商丹断裂带以南的刘岭群是揭示秦岭造山带晚古生代构造演化历史的重要窗口。采用LA-ICP-MS对刘岭群3个变质砂岩样品中的碎屑锆石进行了U-Th-Pb同位素测定,获得最年轻的一... 详细信息

秦岭造山带的构造演化是理解华北与扬子陆块缝合过程的关键,位于商丹断裂带以南的刘岭群是揭示秦岭造山带晚古生代构造演化历史的重要窗口。采用LA-ICP-MS对刘岭群3个变质砂岩样品中的碎屑锆石进行了U-Th-Pb同位素测定,获得最年轻的一组年龄区间为377～395Ma,主要年龄峰值约为442Ma、780～850Ma和900～970Ma,表明刘岭群沉积时代可以持续到晚泥盆世,物质来源于北秦岭构造带。结合刘岭群北侧武关杂岩的最新研究成果可以确定,刘岭群和武关杂岩共同构成了华北陆块南缘中—晚泥盆世弧前盆地的沉积序列,暗示古秦岭洋的最终闭合发生在泥盆纪之后,而华北与扬子陆块碰撞的主缝合线应位于刘岭群的南侧。

关键词：碎屑锆石 LA-ICP-MS U-Pb年龄物质来源晚古生代古秦岭洋刘岭群秦岭造山带

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

海岸带蓝碳研究及其展望

引用

中国科学：地球科学 2015年第11期45卷 1641-1648页

作者：章海波骆永明刘兴华付传城中国科学院海岸带环境过程与生态修复重点实验室中国科学院烟台海岸带研究所烟台264003 中国科学院大学资源与环境学院北京100049

海岸带蓝碳是海洋碳汇的重要组成部分,在应对全球气候变化中具有十分重要的作用.通过系统调研,综述了海岸带蓝碳的组成、碳通量及其影响因素.针对海岸带蓝碳组成,重点阐述了红树林、盐沼和海草床这三种海岸带地区最具固碳效率生态系统... 详细信息

海岸带蓝碳是海洋碳汇的重要组成部分,在应对全球气候变化中具有十分重要的作用.通过系统调研,综述了海岸带蓝碳的组成、碳通量及其影响因素.针对海岸带蓝碳组成,重点阐述了红树林、盐沼和海草床这三种海岸带地区最具固碳效率生态系统的有机碳捕获与埋藏特征.在此基础上,从海岸带地区的水-气、土-气、地下水(孔隙水)向上交换的垂直界面,以及河口-(潮滩)湿地-近海的陆海水平界面两个维度分析了海岸带系统中不同形态碳的交换、输送过程及其通量,探讨了海岸带碳库收支对全球碳循环的影响.同时,结合海岸带人类活动特点以及对气候变化的响应规律,提出当前中国海岸带地区的蓝碳和碳汇功能正在经受着新一轮沿海土地开发、流域筑坝建库、近海富营养化及海平面上升等系列复杂因素的剧烈作用.因此,要充分结合中国海岸带地区的自然与社会属性特点,以陆海统筹为指导,进一步深化海岸带蓝碳研究,提高对不同区域及海岸带类型的固碳效率、碳库总量和生物地球化学循环过程的认识,建立和完善固碳增汇技术体系,构建海岸带蓝碳系统的综合观测网络与管理平台,服务于中国海岸带地区的蓝碳保护和生态文明建设.

关键词：海岸带蓝碳生物地球化学循环碳埋藏碳通量

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Effect of Bi/Si Ratio of BiBSi Glass on Its Structure, Properties and Laser Sealing Shear Strength for Vacuum Glazing

引用

Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 13-24页

作者： LIU Wei JIAO Jinxu luo Dusha ZHOU Junjie SHI Lifen WANG Weiwei LI Changqing WANG Peng XIONG Dehua LI Hong State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhan 430070China Silica-Based Materials Laboratory of Anhui Province CNBM Research Institute for Advanced Glass Materials Group Co.LtdBengbu 233018China State Key Laboratory of Advanced Technology for Float Glass CNBM Research Institute for Advanced Glass Materials Group Co.LtdBengbu 233018China

The low-melting glass of Bi2O_(3)-B2O_(3)-SiO_(2)(BiBSi)system was used for the first time for laser sealing of vacuum *** the condition of constant boron content,how the structure and properties vary with Bi/Si ratio in low-melting glass was *** addition,the relationships between laser power,low-melting glass solder with different Bi/Si ratios and laser sealing shear strength were *** results show that a decrease in the Bi/Si ratio can cause a contraction of the glass network of the low-melting glass,leading to an increase of its characteristic temperature and a decrease of its coefficient of thermal *** laser sealing,the copper ions in the low-melting glass play an endothermic role.A change in the Bi/Si ratio will affect the valence state transition of the copper ions in the low-melting *** absorbance of the low-melting glass does not follow the expected correlation with the Bi/Si ratio,but shows a linear correlation with the content of divalent copper *** greater the concentration of divalent copper ions,the greater the absorbance of the low-melting glass,and the lower the laser power required for laser *** shear strength of the low melting glass solder after laser sealing was tested,and it was found that the maximum shear strength of Z1 glass sample was the highest up to 2.67 MPa.

关键词： Bi2O_(3)-B2O_(3)-SiO_(2)(BiBSi) Bi/Si ratio low-melting glass laser sealing vacuum glazing

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Dissolution properties of imidazolium dipicrylamine in N-methl pyrrolidone at different temperatures

Dissolution properties of imidazolium dipicrylamine in N-met...

引用

第十七届全国化学热力学和热分析学术会议

作者： L.B.Xiao F.Q.Zhao y.luo H.X.Gao N.Li X.L.Xing H.F.Huang R.Z.Hu School of chemical Engineering and Enviroment Beijing Institute of Technology

Imidazolium dipicrylamine is a new nitroaromatic compound. The solubility of imidazolium dipicrylamine is 0.027 g. The oxygen balance of imidazolium dipicrylamine is-71.0%, which has better oxygen balance than 2,4,6-trinitroluene（-74.0%）. The density of imidazolium dipicrylamine is 1.72 g·cm-3, which is much higher than the density of 2,4,6- trinitroluene（1.65 g·cm-3）. The dissolution behaviors of imidazolium dipicrylamine in N-methl pyrrolidone（NMP） were studied by a RD496-2000 Calvet microcalorimeter at different temperatures. The values of heat effect at different temperatures and the relationships between the heat effect and the amount of substance were determined. The measured molar enthalpies（ΔdissH） for imidazolium dipicrylamine in NMP are-27.14 k J·mol-1,-22.31 k J·mol-1,-20.59 k J·mol-1, and-20.38 k J·mol-1, and the differential enthalpies（ΔdifH） are-27.86 k J·mol-1,-23.25 k J·mol-1,-21.31 k J·mol-1, and-21.16 k J·mol-1 at 298.15 K, 303.15 K, 308.15 K and 313.15 K, respectively. The kinetic equations of dissolution processes of imidazolium dipicrylamine in NMP at different temperatures are dα/dt =10-2.64（1-α）0.79（T=298.15K）, dα/dt =10-2.43（1-α）0.82（T=303.15K）, dα/dt =10-2.40（1-α）1.00（T=308.15K）, dα/dt =10-2.37（1-α）0.78（T=313.15K）, respectively. The values of activation energy E and pre-exponential factor A are obtained as 10.24 k J·mol-1 and 10-0.68 s-1.

关键词： imidazolium dipicrylamine dissolution N-methyl pyrrolidone kinetics

来源： cnki会议评论

在线全文

cnki会议

学校读者我要写书评

暂无评论

中全新世以来中国中部高山植被生产力和土壤侵蚀演变的古生态学证据

引用

中国科学：地球科学 2021年第12期51卷 2140-2149页

作者：程颖刘鸿雁王红亚陈德亮 Philippe CIAIS 罗耀吴秀臣印轶陕西师范大学地理科学与旅游学院西安710119 北京大学城市与环境学院北京100871 Regional Climate Group Department of Earth SciencesUniversity of GothenburgGothenburg S-40530Sweden Laboratoire des Sciences du Climat et de l’Environnement(LSCE) CEA CNRS UVSQGif Sur Yvette 91191France 北京师范大学地表过程与资源生态国家重点实验室北京100875 北京师范大学地理科学学部北京100875 California Institute of Technology PasadenaCA91125USA

尽管普遍认为高山生态系统对气候变化的响应非常敏感,但很少有研究探究气候变化对高山植被生产力和土壤侵蚀的影响.基于古生态学记录,探究了全新世中期以来处于东亚季风影响区的太白山高海拔区植被生产力和土壤侵蚀的演变.高分辨率高山... 详细信息

尽管普遍认为高山生态系统对气候变化的响应非常敏感,但很少有研究探究气候变化对高山植被生产力和土壤侵蚀的影响.基于古生态学记录,探究了全新世中期以来处于东亚季风影响区的太白山高海拔区植被生产力和土壤侵蚀的演变.高分辨率高山湖沼记录显示,植被生产力与年平均温度密切相关,而土壤侵蚀主要受到东亚夏季风所带来的降水的影响.即在5800~4000cal. a BP期间,年平均温度较低而夏季降水充沛,高山生态系统表现为低的植被生产力且土壤侵蚀严重.但是,从4000cal. a BP开始,年平均温度升高而夏季降水减少,植被生产力显著提高且土壤侵蚀减缓.这些结果表明,古生态学记录可为研究较长时间尺度上的生态系统服务提供有力证据,可帮助制定气候变化下的生态系统可持续发展政策.

关键词：花粉植被动态高山湖沼沉积物侵蚀强度古生态指标

来源：

维普期刊数据库

同方期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Potassium ions and cyano group modified g-C3N4 for effective generation of H2O2 through two-electron oxygen reduction

引用

Science China Chemistry 2025年第1期68卷 192-200页

作者： Dongying Wang Shulan Pu yongmin Chen Ke Lei yujie Duan Linjiao Mao Xuhui Zeng Xi luo yuntao Zhang yuqin Dong Jin Zhong Zhang yan Sun School of Mechanical Engineering Chengdu University Department of Chemistry and Biochemistry University of California

Potassium ions （K+） doped graphitic carbon nitride （g-C3N4） was prepared by a thermal etching method using potassium hydroxide （KOH） as an ion *** transform infrared spectroscopy （FTIR） and X-ray photoelectron spectroscopy （XPS）results showed that the generation of the cyano group was detected while introducing K+.Under simulated sunlight irradiation,the sample with a K+doping amount of 10%showed the highest hydrogen peroxide （H2O2） generation rate of2,140.2μmol *** apparent quantum yield （AQy） at 400 nm and the solar-to-chemical conversion （SCC） are 4.35%and1.23%,respectively.K+acted as a bridge between g-C3N4layers,which enhanced charge transfer ***,the cyano group enhanced the adsorption capacity of protons （H+） and promoted the yield of *** catalyst exhibited excellent photocatalytic stability based on four-cycle *** addition,a mechanism study showed that superoxide radicals （·O2-）were the most important active species in the reaction *** production of H2O2was achieved through consecutive single-electron *** study deepens the understanding of the oxygen reduction reaction process and opens up a new venue for improving H2O2generation.

关键词： photocatalysis hydrogen peroxide oxygen reduction reaction potassium doping cyano group

来源：

同方期刊数据库评论

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：