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Highly Active Interfacial Sites in SFT-SnO_(2) Heterojunction Electrolyte for Enhanced Fuel Cell Performance via Engineered Energy Bands:Envisioned Theoretically and Experimentally

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Energy & Environmental Materials 2024年第3期7卷 384-397页

作者： Sajid Rauf Muhammad Bilal Hanif Faiz Wali Zuhra Tayyab Bin Zhu Naveed Mushtaq Yatao Yang Kashif Khan peter D.lund Martin Motola Wei Xu College of Electronic and Information Engineering and State Key Laboratory of Radio frequency Heterogeneous Integration Shenzhen UniversityShenzhen 518000China Department of Inorganic Chemistry Faculty of Natural SciencesComenius University in BratislavaIlkovicova 684215BratislavaSlovakia College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China School of Energy and Environment Southeast UniversityNo.2 Si Pai LouNanjing 210096China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China New Energy Technologies Group Department of Applied PhysicsAalto University School of ScienceP.O.Box 15100Fl-00076AaltoEspoo Finland

Extending the ionic conductivity is the pre-requisite of electrolytes in fuel cell technology for high-electrochemical *** this regard,the introduction of semiconductor-oxide materials and the approach of heterostructure formation by modulating energy bands to enhance ionic conduction acting as an electrolyte in fuel ***(n-type;SnO_(2))plays a key role by introducing into p-type SrFe_(0.2)Ti_(0.8)O_(3-δ)(SFT)semiconductor perovskite materials to construct p-n heterojunction for high ionic ***,two different composites of SFT and SnO_(2)are constructed by gluing p-and n-type SFT-SnO_(2),where the optimal composition of SFT-SnO_(2)(6∶4)heterostructure electrolyte-based fuel cell achieved excellent ionic conductivity 0.24 S cm^(-1)with power-output of 1004 mW cm^(-2)and high OCV 1.12 V at a low operational temperature of 500℃.The high power-output and significant ionic conductivity with durable operation of 54 h are accredited to SFT-SnO_(2)heterojunction formation including interfacial conduction assisted by a built-in electric field in fuel cell ***,the fuel conversion efficiency and considerable Faradaic efficiency reveal the compatibility of SFT-SnO_(2)heterostructure electrolyte and ruled-out short-circuiting ***,the first principle calculation provides sufficient information on structure optimization and energy-band structure modulation of SFT-SnO_(2).This strategy will provide new insight into semiconductor-based fuel cell technology to design novel electrolytes.

关键词： high ionic conductivity interfacial conduction modulated energy band structure p-n heterojunction semiconductors

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新型固定床可回热式光热制氢系统结构设计研究

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太阳能学报 2021年第7期42卷 269-277页

作者：蒋川韩一峰吴炎琳杨嵩王军路德·彼得江苏省太阳能技术重点实验室南京210096 中国电建集团华东勘测设计研究院有限公司杭州311122 芬兰阿尔托大学科学学院艾斯堡FI-00076

针对热化学制氢过程,提出一种基于氧化铈固定床结构的新型光热氧化还原制氢反应器。采用集总参数法,建立瞬态还原、回热、氧化过程的数学模型。通过优化腔体数量、氮气输送速率、还原温度等参数,获取现有技术条件下固相回热率、制氢效... 详细信息

针对热化学制氢过程,提出一种基于氧化铈固定床结构的新型光热氧化还原制氢反应器。采用集总参数法,建立瞬态还原、回热、氧化过程的数学模型。通过优化腔体数量、氮气输送速率、还原温度等参数,获取现有技术条件下固相回热率、制氢效率的理论最大值分别为81%和27%,并开展关于气相回热率和聚光比的敏感度分析。

关键词：太阳能聚光光热腔体接收/反应器热化学制氢数值模拟固定床

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旅行医学必备手册

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国外科技新书评介 2016年第7期 12-12页

作者： peter lund 马雪征不详中国检验检疫科学研究院卫生检疫研究所

近几十年来，随着旅游业的发展，全球化航空运输变得更加便捷快速，极大地方便了旅行者，同时也成为传染病传播的桥梁。美国一项关于旅行者的队列研究表明：64％的旅行者在旅途中出现健康问题，其中8％的人因此就医；26％的旅行者回国... 详细信息

近几十年来，随着旅游业的发展，全球化航空运输变得更加便捷快速，极大地方便了旅行者，同时也成为传染病传播的桥梁。美国一项关于旅行者的队列研究表明：64％的旅行者在旅途中出现健康问题，其中8％的人因此就医；26％的旅行者回国后患病，其中12％的人去医院接受诊治。

关键词：旅行者手册医学航空运输健康问题队列研究旅游业全球化

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Comparative analysis of ceramic-carbonate nanocomposite fuel cells using composite GDC/NLC electrolyte with different perovskite structured cathode materials

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Frontiers of Chemical Science and Engineering 2018年第1期12卷 162-173页

作者： Muhammad I. Asghar Sakari Lepikko Janne Patakangas Janne Halme peter D. lund New Energy Technologies Group Department of Applied Physics Aalto University P.O. BOX 15100 FI-00076 Aalto Finland

A comparative analysis of perovskite structured cathode materials, La0.65Sr0.35Mn03 （LSM）, La0.8Sr0.2CoO3 （LSC）, La0.6Sr0.4FeO3 （LSF） and La0.6Sr0.4Co0.2Fe0.803 （LSCF）, was performed for a ceramic-carbonate nanocomposite fuel cell using composite electrolyte consisting of Gd0.1Ce0.9O1.95 （GDC） and a eutectic mixture of Na2CO3 and Li2CO3. The compatibility of these nanocomposite electrode powder materials was investigated under air, CO2 and air/CO2 atmospheres at 550 ℃. Microscopy measurements together with energy dispersive X-ray spectroscopy （EDS） elementary analysis revealed few spots with higher counts of manganese relative to lanthanum and strontium under pure CO2 atmosphere. Furthermore, electrochemical impedance （EIS） analysis showed that LSC had the lowest resistance to oxygen reduction reaction （ORR）（14.12 Ω·cm^2） followed by LSF （15.23 Ω·cm^2）, LSCF （19.38Ω·cm^2） and LSM （〉 300 Ω·cm^2）. In addition, low frequency EIS measurements （down to 50 gHz） revealed two additional semi-circles at frequencies around 1 Hz. These semicircles can yield additional information about electrochemical reactions in the device. Finally, a fuel cell was fabricated using GDC/NLC nanocomposite electrolyte and its composite with NiO and LSCF as anode and cathode, respectively. The cell produced an excellent power density of 1.06 W/cm^2 at 550 ℃ under fuel cell conditions.

关键词： electrode fuel cell low-temperature nano- composite perovskite

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Parameter identification and generality analysis of photovoltaic module dual-diode model based on artificial hummingbird algorithm

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Clean Energy 2023年第6期7卷 1219-1232页

作者： Zhen Li Jianke Hu Yifeng Han Hefeng Li Jun Wang peter D.lund Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology School of Energy&EnvironmentSoutheast UniversityNanjing 210096China PowerChina Huadong Engineering Corporation Limited No.201 Gaojiao RoadHangzhou 311122China School of Science Aalto UniversityFI-00076Aalto(Espoo)Finland

The aim of this study is to propose a photovoltaic(PV)module simulation model with high accuracy under practical working conditions and strong applicability in the engineering field to meet various PV system simulation *** previous model-building methods,this study combines the advantages of analytical and metaheuristic ***,the applicability of various metaheuristic algorithms is comprehensively compared and the seven parameters of the PV cell under standard test conditions are extracted using the double diode model,which verifies that the artificial hummingbird algorithm has higher accuracy than other ***,the seven parameters under different conditions are corrected using the analytical *** terms of the correc-tion method,the ideal factor correction is added on the basis of previous methods to solve the deviation between simulated data and measured data in the non-linear ***,the root mean squared error between the simulated current data and the measured current data of the proposed model under three different temperatures and irradiance is 0.0697,0.0570 and 0.0289 A,respectively.

关键词： photovoltaic modules dual-diode model parameter identification metaheuristic algorithms parameter correction

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Fulminant isolated cardiac sarcoidosis with pericardial effusion and acute heart failure: Challenging aspects of diagnosis and treatment

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World Journal of Clinical Cases 2016年第3期4卷 76-80页

作者： Nina Fluschnik Gunnar lund peter Moritz Becher Stefan Blankenberg Kai Muellerleile Department of General and Interventional Cardiology University Heart Center Department of Diagnostic and Interventional Radiology University Medical Center Hamburg Eppendorf

This case report illustrates challenging aspects of diagnosis and treatment of isolated sarcoid heart disease(SHD) and the role of cardiovascular magnetic resonance(CMR) imaging. Here, we present a previously healthy 45-year-old man, who was admitted with pericardial effusion and symptoms of acute heart failure. CMR followed by targeted left ventricular endomyocardial biopsy(EMB) revealed the diagnosis of isolated SHD. The combined use of CMR and EMB was crucial in diagnosing SHD. Furthermore, this case report demonstrates the value of CMR for monitoring response to therapy and lesion healing.

关键词： Heart failure Cardiac sarcoidosis Cardiovascular magnetic resonance imaging Endomyocardial biopsy Internal cardiac defibrillator

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Novel LaFe_(2)O_(4)spinel structure with a large oxygen reduction response towards protonic ceramic fuel cell cathode

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Journal of Rare Earths 2023年第3期41卷 413-421,I0004页

作者： Jinping Wang Yuzheng Lu Naveed Mushtaq M.A.K Yousaf Shah Sajid Rauf peter D.lund Muhammad Imran Asghar School of Energy and Power Engineering Nanjing Institute of TechnologyNanjing 211167China School of Electronic Engineering Nanjing Xiao Zhuang UniversityNanjing 211171China Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096China College of Electronics and Information Engineering Shenzhen UniversityShenzhen 518000China New Energy Technologies Group Department of Applied PhysicsAalto University School of ScienceP.O.Box.15100FI00076AaltoEspooFinland Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials Faculty of Physics and Electronic ScienceHubei UniversityWuhan 430062China

Highly active and stable electrocatalysts are mandatory for developing high-performance and longlasting fuel *** current study demonstrates a high oxygen reduction reaction(ORR)electrocatalytic activity of a novel spinel-structured LaFe_(2)O_(4)via a self-doping *** LaFe_(2)O_(4)demonstrates excellent ORR activity in a protonic ceramic fuel cell(PCFC)at temperature range of 350-500℃.The high ORR activity of LaFe_(2)O_(4)is mainly attributed to the facile release of oxide and proton ions,and improved synergistic incorporation abilities associated with interplay of multivalent Fe^(3+)/Fe^(2+)and La^(3+)*** LaFe_(2)O_(4)as cathode over proton conducting BaZr_(0.4)Ce_(0.4)Y_(0.2)O_(3)(BZCY)electrolyte,the fuel cell has delivered a high-power density of 806 mW/cm^(2)operating at 500℃.Different spectroscopic and calculations methods such as UV-visible,Raman,X-ray photoelectron spectroscopy and density functional theory(DFT)calculations were performed to screen the potential application of LaFe_(2)O_(4)as *** study would help in developing functional cobalt-free ORR electrocatalysts for low temperature-PCFCs(LT-PCFCs)and solid oxide fuel cells(SOFCs)applications.

关键词： LaFe_(2)O_(4)cathode Facile Fe^(3+/2+)ions resale Oxygen reductionreaction(ORR) Excellent electrocatalyst Protonic ceramicfuel cell(PCFC) Rare earths

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Continuous cardiac output measured with a Swan-Ganz catheter reacts too slowly in animal experiments with sudden circulatory failure

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Animal Models and Experimental Medicine 2022年第3期5卷 258-265页

作者： Sigríður Olga Magnúsdóttir Carsten Simonsen Bodil Steen Rasmussen peter Enemark lund Benedict Kjærgaard Biomedical Research Laboratory Aalborg University HospitalAalborgDenmark Department of Clinical Medicine Aalborg UniversityAalborgDenmark Department of Cardiothoracic Surgery Aalborg University HospitalAalborgDenmark Department of Anesthesia and Intensive Care Aalborg University HospitalAalborgDenmark Unit of Clinical Biostatistics Aalborg University HospitalAalborgDenmark

Background : In many animal experiments, it is vital to detect sudden changes in cardiac output(CO). This porcine study compared CO that was measured with a SwanGanz pulmonary catheter with the gold standard(which was a transit-time flow probe around the pulmonary artery) during interventions that caused hemodynamic *** : In one series, 7 pigs were exposed to sudden changes in CO. In another series, 9 pigs experienced more prolonged changes in CO. All the pigs had a Swan-Ganz catheter placed into the pulmonary artery and a flow probe around the pulmonary artery. Adrenaline infusion and controlled hemorrhage were used to increase and decrease CO, respectively. The measurements of CO before and after each intervention were compared for correlation, agreement, and the time delay that it took each method to detect at least a 30% change in CO. A Bland– Altman test was used to identify correlations and agreements between the *** : In the first series, there was a delay of 5– 7 min for the Swan Ganz catheter to register a 30% change in cardiac output, compared with the flow probe. However,during prolonged changes in CO in the second series, there was a good correlation between the 2 methods. Mixed venous oxygen saturation reacted faster to changes than did CO;both were measured via the Swan-Ganz *** : In many animal studies, the use of Swan-Ganz catheters is suitable;however, in experiments with sudden hemodynamic instability, the flow probe is the most advantageous method for measuring CO.

关键词： cardiac output flow probe hemodynamics pigs Swan-Ganz catheter

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Semiconductor Electrochemistry for Clean Energy Conversion and Storage

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Electrochemical Energy Reviews 2021年第4期4卷 757-792页

作者： Bin Zhu Liangdong Fan Naveed Mushtaq Rizwan Raza Muhammad Sajid Yan Wu Wenfeng Lin Jung‑Sik Kim peter D.lund Sining Yun Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and EnvironmentSoutheast UniversityNanjing 210096JiangsuChina Shenzhen Key Laboratory of New Lithium‑Ion Batteries and Mesoporous Materials College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060GuangdongChina Clean Energy Research Lab(CERL) Department of PhysicsCOMSATS University IslamabadLahore CampusLahore 54000Pakistan Engineering Research Center of Nano‑Geo Materials of Ministry of Education Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074HubeiChina Department of Chemical Engineering School of AeronauticalAutomotiveChemical and Materials EngineeringLoughborough UniversityLoughborough LE113TUUK Department of Aeronautical&Automotive Engineering School of AeronauticalAutomotiveChemical and Materials EngineeringLoughborough UniversityLoughborough LE113TUUK Department of Engineering Physics/Advanced Energy Systems School of ScienceAalto University00076 AaltoEspooFinland Functional Materials Laboratory(FML) School of Materials Science and EngineeringXi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina

Semiconductors and the associated methodologies applied to electrochemistry have recently grown as an emerging field in energy materials and *** example,semiconductor membranes and heterostructure fuel cells are new technological trend,which differ from the traditional fuel cell electrochemistry principle employing three basic functional components:anode,electrolyte,and *** electrolyte is key to the device performance by providing an ionic charge flow pathway between the anode and cathode while preventing electron *** contrast,semiconductors and derived heterostructures with electron(hole)conducting materials have demonstrated to be much better ionic conductors than the conventional ionic *** energy band structure and alignment,band bending and built-in electric field are all important elements in this context to realize the necessary fuel cell *** review further extends to semiconductor-based electrochemical energy conversion and storage,describing their fundamentals and working principles,with the intention of advancing the understanding of the roles of semiconductors and energy bands in electrochemical devices for energy conversion and storage,as well as applications to meet emerging demands widely involved in energy applications,such as photocatalysis/water splitting devices,batteries and solar *** review provides new ideas and new solutions to problems beyond the conventional electrochemistry and presents new interdisciplinary approaches to develop clean energy conversion and storage technologies.

关键词： Semiconductor electrochemistry Fuel cells Lithium-ion batteries Solar cells Built-in electric field Energy system integration

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Bone and Soft Tissue Blood Flow during Normobaric and Hyperbaric Oxygen Breathing in Healthy Divers

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Journal of Biomedical Science and Engineering 2014年第12期7卷 973-981页

作者： Agneta C.Larsson Johan Uusijarvi Jan E.Naslund Iréne lund peter Lindholm Department of Physiology and Pharmacology Karolinska InstituteStockholmSweden Department of Anaesthesia&Intensive Care Division of Hyperbaric MedicineKarolinska HospitalStockholmSweden Department of Radiology Karolinska HospitalStockholmSweden

Purpose: The study aimed to investigate, using a photoplethysmographic (PPG) technique, how pulsatile blood flow within the patellar bone and skin over the patella reacts to normobaric (NBO) and hyperbaric oxygen breathing (HBO). Methods: Eleven healthy volunteers, breathed air or oxygen. Subjects were blinded to breathing gas. A range of partial pressures of oxygen were administered in 10 minute intervals: 21 kPa, 101 kPa (NBO), 21 kPa, (compression to 280 kPa), 59 kPa, 280 kPa (HBO), 59 kPa, (decompression), and 21 kPa. Changes were measured continuously for each individual. Results: Hyperoxia decreased pulsatile patellar blood flow ~32 resp. 38% and skin blood flow ~36 resp. 42% during the first 2 - 3 minutes of NBO resp. HBO. This decrease was normalized within 5 minutes after exposure. The results were similar when switching from air to NBO (101 kPa) and from air at pressure (59 kPa) to HBO (280 kPa). Conclusions: The study shows that pulsatile patellar skin and bone blood flow, decreases significantly as a reaction to oxygen breathing in healthy subjects. The results suggest that a non-invasive PPG technique could be used to monitor blood flow changes in bone during oxygen treatment.

关键词： Photopletysmography Hyperbaric Oxygen Bone Osteomyelitis Blood Flow

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