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Enhanced thermoelectric and mechanical properties of Bi_(0.5)Sb_(1.5)Te_(3. alloy with dispersed yttrium oxide ceramic nanoparticles

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Rare Metals 2024年第4期43卷 1758-1768页

作者： Cun-Cheng li Ming-Wei zhang Ji-Wu xin Lei Wei Wen-Yu Zhao school of Materials Science and Engineering Shandong University of TechnologyZibo255000China school of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore639798Singapore State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Reducing thermal conductivity while avoiding adverse interfacial reactions during sintering is crucial for improving the thermoelectric performance of Bi_(2)Te_(3.based *** ceramic nanoparticles are good candidates for achieving this *** this study,we designed and prepared a series of p-type Bi_(0.5)Sb_(1.5)Te_(3.nanocomposites decorated with Y_(2)O_(3.ceramic nanoparticles via ball-milling dispersion and spark-plasma *** to the chemical stability of the ceramics,no traces of atomic doping or interfacial reactions were *** measurements revealed that the Y_(2)O_(3.nanoparticles distributed along the grain boundaries acted as energy-dependent carrier-filtering centers to improve the scattering parameter and Seebeck coefficient,contributing to the elevated power factor even with a decreased electrical ***,the incorporated Y_(2)O_(3.nanoparticles and various defect structures they induced effectively strengthened the phonon scattering and suppressed the lattice thermal ***,a peak figure of merit(ZT)of 1.23.at 3.3.K was achieved for 0.4%Y_(2)O_(3./Bi_(0.5)Sb_(1.5)Te_(3.,which is 13.higher than that of the *** addition,the Vickers hardness of the composite material was 3.%higher than that of the *** study demonstrates the effectiveness of ceramic nanoparticles in synergistic ally improving the thermoelectric and mechanical properties,which may be further extended to other thermoelectric systems.

关键词： Bi_(0.5)Sb_(1.5)Te_3.alloy Y_(2)O_(3. ceramic nanoparticles Microstructures Thermoelectric performance Mechanical properties

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Tipping Point Detection Using Reservoir Computing

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Research 2024年第1期2023卷 779-790页

作者： xin li Qunxi Zhu Chengli Zhao Xuzhe Qian Xue {3. Xiaojun Duan Wei lin College of Science National University of Defense TechnologyChangshaHunan 410073China Research Institute of Intelligent Complex Systems and MOE Frontiers Center for Brain Science Fudan UniversityShanghai 200433China Shanghai Artificial Intelligence Laboratory Shanghai 200232China school of Mathematical Sciences SCMSSCAMand CCSBFudan UniversityShanghai 200433China

Detection in high fidelity of tipping points,the emergence of which is often induced by invisible changes in internal structures or/and external interferences,is paramountly beneficial to understanding and predicting complex dynamical systems(CDSs).Detection approaches,which have been fruitfully developed from several perspectives(e.g.,statistics,dynamics,and machine learning),have their own advantages but still encounter difficulties in the face of high-dimensional,fluctuating ***,using the reservoir computing(RC),a recently notable,resource-conserving machine learning method for reconstructing and predicting CDSs,we articulate a model-free framework to accomplish the detection only using the time series observationally recorded from the underlying unknown CDSs.

关键词： computing record ping

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Predominant types of regional cold waves in North china and their historical changes

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Atmospheric and Oceanic Science Letters 2024年第4期17卷 46-51页

作者： xinyi Cheng Yiyi zhang Jiandong li xin Hao Center for Climate System Prediction Research/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters/Key Laboratory of Meteorological Disaster Ministry of EducationNanjing University of Information Science&TechnologyNanjingChina Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjingChina

寒潮事件对东亚地区的社会经济,生态系统和人体健康影响巨大.根据1980-2019年间10月至次年3.的每日寒潮记录和K-means聚类,本文识别出了中国两种不同类型的区域性寒潮(T1和T2). T1区域性寒潮主要影响东北地区,T2区域性寒潮则主要影响... 详细信息

寒潮事件对东亚地区的社会经济,生态系统和人体健康影响巨大.根据1980-2019年间10月至次年3.的每日寒潮记录和K-means聚类,本文识别出了中国两种不同类型的区域性寒潮(T1和T2). T1区域性寒潮主要影响东北地区,T2区域性寒潮则主要影响华北和东部地区.与T1区域性寒潮相比, T2区域性寒潮强度更强,持续时间更长,影响范围更广. 1980–2019年期间, T1区域性寒潮的频率显著增加,而T2区域性寒潮的频率则没有趋势变化. T1和T2区域性寒潮事件均与西伯利亚高压增强有关,然而与它们相关的对流层中层波列明显不同.在T1区域性寒潮事件发生期间,西伯利亚-蒙古上空出现负-正模态的500-hPa位势高度异常波列,削弱了东亚大槽,导致西伯利亚冷空气东移.T1区域寒潮频次增加趋势可能与全球变暖引起的500-hPa位势高度的线性趋势变化有关.与T2区域寒潮事件相关的波列则在乌拉尔山脉,蒙古和华北地区形成了脊-槽-脊环流异常,导致冷空气向东南方向入侵.本文得出结论,由于两类区域寒潮影响不同,西伯利亚高压增强和对流层中层波列模态在我国区域性寒潮事件的预报中应综合考虑.

关键词：寒潮 K-means聚类西伯利亚高压波列

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Salinity Acclimation Induces Reduced Energy Metabolism,Osmotic Pressure Regulation and Transcriptional Reprogramming in Hypotrichida Ciliate Gastrostyla setifera

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Journal of Ocean university of china 2024年第2期23卷 539-549页

作者： JI xin BI Luping ZOU Songbao li Wenlu JI Daode zhang Qianqian school of Ocean Yantai UniversityYantai 264005China Key Laboratory of Coastal Environmental Processes and Ecological Remediation Yantai Institute of Coastal Zone ResearchChinese Academy of SciencesYantai 264003China Zhejiang Institute of Freshwater Fisheries Huzhou 313001China Muping Coastal Environment Research Station Yantai Institute of Coastal Zone ResearchChinese Academy of SciencesYantai 264117China

Coastal and estuarine protists are frequently exposed to salinity *** the tolerance and stress responses of microalgae to salinity have been extensively studied,there have been scarce studies on the physiological response of heterotrophic protists to salinity *** this study,we investigated the physiological response of the heterotrophic ciliate Gastrostyla setifera to a salinity of 3.via a transcriptomic *** first transcriptome of genus Gastrostyla was obtained utilizing a group of manually isolated ciliate individuals(cells)and RNA-seq *** completeness of the transcriptome was *** expressed gene(DEG)analysis was performed among the transcriptomes of *** acclimated in saline water(salinity 3.and those cultured in fresh *** results demonstrated a significant alternation in gene transcription,in which the ciliate exhibits a transcripttomic acclimation in responding salinity *** up-regulated DEGs were enriched in the pathways of cytoskeleton proteins,membrane trafficking,protein kinases and protein *** may represent enhanced functions of ion transport,stress response and cell *** involved in energy metabolism and biosynthesis were markedly down-regulated,reflecting decreased cell ***,we detected significantly down-regulated genes involved in several pathways of amino acid catabolism,which may lead to accumulation of amino acids in the ciliate *** acid could act as compatible solutes in the cytoplasm to maintain the osmotic balance in saline ***,this work is an initial exploration to the molecular basis of the heterotrophic protist responding to salinity *** result sheds light on the mechanisms of enhancement of cell protection,reduction of cell activity,and osmotic pressure regulation in ciliates acclimated to salinity.

关键词： salinity stress heterotrophic protist ciliate Gastrostyla setifera transcriptome differentially expressed gene

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Bimagnetic metal constructed core-shell structure of Fe@Co nanowires for multi-band microwave absorption

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Progress in Natural Science:Materials International 2024年第02期34卷 354-361页

作者： Ping-an Yang Rui Cai Haibo Ruan Nanqing zhang xin Huang Rui li Yuxin zhang Yi Lu Zhihao Zhou school of Automation Chongqing University of Posts and Telecommunications Chongqing Key Laboratory of Materials Surface & Interface Science Chongqing University of Arts and Sciences College of Engineering and Technology Zunyi Normal College College of Material Science and Engineering Chongqing University

Controlled fabrication of materials by surface modification techniques has been a hot research topic. In this paper,one-dimensional(1D) core-shell structure Fe@Co nanowires(NWs) were successfully prepared by anchoring 0-dimensional(0D) Co nanoparticles on 1D Fe NWs based on the in situ reduction method. The electromagnetic parameters of the specimens at a filler mass fraction of 25 wt% were tested and the microwave loss mechanism was deeply analyzed. Binary magnetic metals in a core-shell structure have excellent multi-band microwave absorption capability(S-band, X-band and Ku-band). This is due to the heterogeneous interface and magnetic coupling effects tuning the dielectric and magnetic loss. This study offers a workable plan for creating effective multi-band magnetic metal-based microwave absorbers.

关键词： Core-shell structure Interface Magnetic coupling Microwave absorption One-dimensional nanowires

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Rapid Phase Ambiguity Elimination Methods for DOA Estimator via Hybrid Massive MIMO Receive Array

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Chinese Journal of Electronics 2024年第1期33卷 175-184页

作者： Xichao ZHAN Zhongwen SUN Feng SHU Yiwen CHEN xin CHENG Yuanyuan WU Qi zhang Yifan li Peng zhang school of Information and Communication Engineering Hainan University school of Electronic and Optical Engineering Nanjing University of Science and Technology

For a sub-connected hybrid multiple-input multiple-output(MIMO) receiver with K subarrays and N antennas, there exists a challenging problem of how to rapidly remove phase ambiguity in only single time-slot. A direction of arrival(DOA) estimator of maximizing received power(Max-RP) is proposed to find the maximum value of K-subarray output powers, where each subarray is in charge of one sector, and the center angle of the sector corresponding to the maximum output is the estimated true DOA. To make an enhancement on precision, Max-RP plus quadratic interpolation(Max-RP-QI) method is designed. In the proposed Max-RP-QI, a quadratic interpolation scheme is adopted to interpolate the three DOA values corresponding to the largest three receive powers of *** achieve the Cramer Rao lower bound, a Root-MUSIC plus Max-RP-QI scheme is developed. Simulation results show that the proposed three methods eliminate the phase ambiguity during one time-slot and also show low computational complexities. The proposed Root-MUSIC plus Max-RP-QI scheme can reach the Cramer Rao lower bound,and the proposed Max-RP and Max-RP-QI are still some performance losses 2–4 d B compared to the Cramer Rao lower bound.

关键词： Phased arrays Interpolation Wireless sensor networks Direction-of-arrival estimation Simulation Receiving antennas Massive MIMO

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Heteroepitaxial growth of Au@Pd core–shell nanocrystals with intrinsic chiral surfaces for enantiomeric recognition

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Rare Metals 2024年第1期43卷 225-235页

作者： Feng-Xia Wu Feng-Hua li Xia-li Lv Qi-Xian zhang Guo-Bao Xu Wen-{3. Niu State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Shaoxing Institute of Technology Shanghai UniversityShaoxing 312000China university of Science and Technology of china Hefei 230026China school of Materials Science and Engineering Shanghai UniversityShanghai 200436China Zhejiang Institute of Advanced Materials Shanghai UniversityJiashan 314113China university of Chinese Academy of Sciences Beijing 100039China

Noble metal surfaces with intrinsic chirality serve as an ideal candidate for investigating enantioselective chemistry due to their superior chemical durability and high catalytic ***,significant advance has been made in synthesizing metal nanocrystals with intrinsic ***,the majority reports are limited to ***,through a heteroepitaxial growth strategy,the synthesis of metal nanocrystals with intrinsic chirality to palladium was extended for the first time and their application in enantioselective recognition was *** heteroepitaxial growth strategy allows for transferring the chirality of homochiral Au nanocrystals to Au@Pd core–shell *** employing the chiral Au@Pd nanocrystals as enantiomeric recognizing elements,a series of electrochemical sensors for chiral discrimination were *** optimal conditions,the peak potential between D-dihydroxyphenylalanine(D-DOPA)and L-dihydroxyphenylalanine(L-DOPA)is about 80 m V,and the peak current of D-DOPA is 2 times as much as that of L-DOPA,which enables the determination of the enantiomeric excess(EE,%)of ***,this report not only introduces a heteroepitaxial growth strategy to synthesize metal nanocrystals with intrinsic chirality,but also demonstrates the superior capability of integrating intrinsic chirality and catalytic properties into metal nanocrystals for chiral recognition.

关键词： Core–shell nanostructures Chirality transfer Electrochemical sensors Chiral recognition Chiroplasmonics

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Towards wafer-scale growth of two-dimensional cerium dioxide single crystal with high dielectric performance

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Nano Research 2024年第9期17卷 8592-8599页

作者： Zhuofeng Shi Muhammad Imran Xiaohui Chen xin liu Yaqi Zhu Zhaoning Hu Saiyu Bu Jialin {3. Chunhu li Xiaodong {3. li lin College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266000China school of Materials Science and Engineering Peking UniversityBeijing 100871China Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular ScienceCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China Key Laboratory of Marine Chemistry Theory and Technology Ministry of EducationCollege of Chemistry and Chemical EngineeringOcean University of ChinaQingdao 266100China

Owing to the atomically thin nature,two-dimensional(2D)oxide materials have been widely reported to exhibit exciting transport and dielectric properties,such as fine gate controllability and ultrahigh carrier mobility,that outperform their bulk ***,unlike the successful synthesis of bulk oxide single crystals,reliable methods for synthesizing large-area single crystal of 2D oxide,that would suppress the negative influence from defective grain boundaries,remain unavailable,especially for nonlayered ***,we report that the lattice symmetry between the substrate and cerium dioxide(CeO_(2))would allow for the aligned nucleation and epitaxial growth of CeO_(2)on sapphire substrates,enabling the wafer-sized growth of CeO_(2)single *** careful tuning of the growth temperature and oxygen flow rate contributed to the harvesting of CeO_(2)wafer with reduced thickness and enhanced growth *** removal of grain boundaries improved the dielectric performance in terms of high dielectric strength(E_(bd)≈8.8 MV·cm^(-1)),suppressed leakage current,along with high dielectric constants(ε_(r)≈24).Our work demonstrates that with fine dielectric performance and ease of synthesizing wafer-sized single crystals,CeO_(2)can function as potential candidate as gate insulator for 2D-materials based nanoelectronics,and we believe the reported protocol of aligned nucleation can be extended to other 2D oxides.

关键词： dielectric materials two-dimensional materials chemical vapor deposition cerium dioxide

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Ir single atoms on NiFeZn-LDH matrix for exceptional oxygen evolution reaction

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Nano Research 2024年第8期17卷 7039-7044页

作者： Muhammad Israr Muhammad Humayun Jiaqi zhang Khadim Shah xin Tan Chen Chen Yadong li Department of Chemistry Tsinghua UniversityBeijing 100084China Energy Water and Environment LabCollege of Humanities and SciencePrince Sultan UniversityRiyadh11586Saudi Arabia

To address the sluggish kinetics of the oxygen evolution reaction(OER),a potential approach is to rationally design and fabricate extremely effective single atom catalysts(SACs).Using an appropriate matrix to stabilize single-atom active centers with optimal geometric and electronic structures is crucial for enhancing catalytic ***,we report the design and fabrication of Ir single atoms on NiFeZn layered double hydroxide(Ir-SAC/NiFeZn-LDH)electrocatalyst for highly efficient and stable *** is investigated that the NiFeZn support exhibits abundant defect sites and unsaturated coordination *** sites function to anchor and stabilize single Ir single atoms on the *** strong synergetic electronic interaction between the Ir single atoms and the NiFeZn matrix resulted in remarkable OER performance of the as-fabricated Ir-SAC/NiFeZn *** a loading Ir content of 1.09 wt.%,this catalyst demonstrates a highly stable OER activity,with an overpotential of 196 mV at 10 mA·cm^(−2) and a small Tafel slope of 3. mV·dec^(−1) for the OER in a 1 M KOH *** results significantly surpass the performance of the commercially available IrO_(2) catalyst.

关键词： Ir single atoms layered double hydroxides rational design geometric optimization oxygen evolution reaction

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Near infrared emissions from both high efficient quantum cutting (173.) and nearly-pure-color upconversion in NaY(WO_(4))_(2):Er^(3.)/Yb^(3.) with thermal management capability for silicon-based solar cells

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light(Science & Applications) 2024年第1期13卷 113-126页

作者： Duan Gao Baojiu Chen Xuezhu Sha Yuhang zhang xin Chen li Wang Xizhen zhang Jinsu zhang Yongze Cao Yichao Wang Lei li Xiangping li Sai Xu Hongquan Yu lihong Cheng school of Science Dalian Maritime UniversityDalian 116026 LiaoningChina

Raising photoelectric conversion efficiency and enhancing heat management are two critical concerns for siliconbased solar *** this work,efficient Yb^(3.) infrared emissions from both quantum cutting and upconversion were demonstrated by adjusting Er^(3.) and Yb^(3.) concentrations,and thermo-manage-applicable temperature sensing based on the luminescence intensity ratio of two super-low thermal quenching levels was discovered in an Er^(3.)/Yb^(3.) codoped tungstate *** quantum cutting mechanism was clearly decrypted as a two-step energy transfer process from Er^(3.) to Yb^(3.).The two-step energy transfer efficiencies,the radiative and nonradiative transition rates of all interested 4 f levels of Er^(3.) in NaY(WO_(4))_(2) were confirmed in the framework of Föster-Dexter theory,Judd-Ofelt theory,and energy gap law,and based on these obtained efficiencies and rates the quantum cutting efficiency was furthermore determined to be as high as 173.in NaY(WO_(4))_(2):5 mol%Er^(3.)/50 mol%Yb^(3.) *** and nearly pure infrared upconversion emission of Yb3.under 1550 nm excitation was achieved in Er^(3.)/Yb^(3.)co-doped NaY(WO_(4))_(2) by adjusting Yb^(3.) doping *** Yb^(3.) induced infrared upconversion emission enhancement was attributed to the efficient energy transfer ^(4)I_(11/2)(Er^(3.))+^(2)F_(7/2)(Yb^(3.))→^(4)I_(15/2)(Er^(3.))+^(2)F_(5/2)(Yb^(3.))and large nonradiative relaxation rate of ^(4)I_(9/2).Analysis on the temperature sensing indicated that the NaY(WO_(4))_(2):Er^(3.)/Yb^(3.)serves well the solar cells as thermos-managing ***,it was confirmed that the fluorescence thermal quenching of ^(2)H_(11/2)/^(4)S_(3.2) was caused by the nonradiative relaxation of ^(4)S_(3.2).All the obtained results suggest that NaY(WO_(4))_(2):Er^(3.)/Yb^(3.) is an excellent material for silicon-based solar cells to improve photoelectric conversion efficiency and thermal management.

关键词： quantum thermal relaxation

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