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Recent advances of versatile reagents as controllable building blocks in organic synthesis

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Chinese Chemical Letters 2024年第2期35卷 24-43页

作者： Shaomin Chen luigi Vaccaro Yanlong Gu Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of EducationHubei Key Laboratory of Material Chemistry and Service FailureSchool of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhan 430074China Laboratory of Green S.O.C. Dipartimento di ChimicaBiologia e BiotecnologieUniversità degli Studi di PerugiaVia Elce di Sotto 8Perugia 06123Italy School of Chemistry and Chemical Engineering The Key Laboratory for Green Processing of Chemical Engineering of Xinjiang BingtuanShihezi UniversityShihezi 832004China

Diversity-oriented synthesis is a powerful and interesting synthetic tool for the rapid construction of structurally complex and privileged scaffolds from readily accessible starting *** date,diversity-oriented synthesis mostly relies on the employment of versatile *** reagents can be regulated as controllable and flexible building blocks for multipurpose *** the past decade,a variety of multifunctional reagents have been ***,most versatile reagents usually need multi-step synthesis,thus restricting their wide application to a large *** terms of the practicalities and universalities,we prefer to pay more attention to the utilization of simple and practical versatile reagents with multiple reactivities,mainly including atropaldehyde acetals,aryl methyl ketones,vinylene carbonate,vinyl azides,aryldiazonium salts,rongalite,halodifluoromethyl *** importantly,these versatile reagents can also play different roles simultaneously in the same reaction,in which their different reactivities are converged into the final target *** strategy can not only offer more possibilities for the synthesis of several active pharmaceutical ingredients,but also minimize the occurrence of some side reactions by lessening the varieties of ***,a perspective is given at the end of this review.

关键词： Versatile reagents Divergent synthesis Dual synthons Bond cleavage Tandem reactions

ARBITRARILY HIGH-ORDER ENERGY-CONSERVING METHODS FOR HAMILTONIAN PROBLEMS WITH QUADRATIC HOLONOMIC CONSTRAINTS

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Journal of Computational Mathematics 2024年第4期42卷 1145-1171页

作者： Pierluigi Amodio luigi Brugnano Gianluca Frasca-Caccia Felice Iavernaro Dipartimento di Matematica Università di BariItaly Dipartimento di Matematica e Informatica"U.Dini" Università di FirenzeItaly Dipartimento di Matematica Università di SalernoItaly

In this paper,we define arbitrarily high-order energy-conserving methods for Hamilto-nian systems with quadratic holonomic *** derivation of the methods is made within the so-called line integral *** tests to illustra... 详细信息

关键词： Constrained Hamiltonian systems Quadratic holonomic constraints Energy-conserving methods Line integral methods Hamiltonian Boundary Value Methods HB-VMs

Edge-Enabled Metaverse:The Convergence of Metaverseand Mobile Edge Computing

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Tsinghua Science and Technology 2024年第3期29卷 795-805页

作者： Nyothiri Aung Sahraoui Dhelim Liming Chen Huansheng Ning luigi Atzori Tahar Kechadi Information Engineering College Xinjiang Institute of EngineeringUrumqi 830023Chinaand also with School of Computer ScienceUniversity College DublinDublinD04 V1W8Ireland School of Computing Ulster UniversityBelfastBT151EDUK School of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China Department of Electrical and Electronic Engineering University of CagliariSardinia 09124Italy School of Computer Science University College DublinDublinD04 V1W8Ireland

Metaverse is a virtual environment where users are represented by their avatars to navigate a virtual world having strong links with its physical *** state-of-the-art Metaverse architectures rely on a cloud-based approach for avatar physics emulation and graphics rendering *** current centralized architecture of such systems is unfavorable as it suffers from several drawbacks caused by the long latency of cloud access,such as low-quality *** this end,we propose a Fog-Edge hybrid computing architecture for Metaverse applications that leverage an edge-enabled distributed computing *** applications leverage edge devices’computing power to perform the required computations for heavy tasks,such as collision detection in the virtual universe and high-computational 3D physics in virtual *** computational costs of a Metaverse entity,such as collision detection or physics emulation,are performed at the device of the associated physical *** validate the effectiveness of the proposed architecture,we simulate a distributed social Metaverse *** simulation results show that the proposed architecture can reduce the latency by 50%when compared with cloud-based Metaverse applications.

关键词： industrial Metaverse edge computing Blockchain virtual environment task offloading fog computing

Autonomous Vehicle Platoons In Urban Road Networks:A Joint Distributed Reinforcement Learning and Model Predictive Control Approach

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IEEE/CAA Journal of Automatica Sinica 2024年第1期11卷 141-156页

作者： luigi D’Alfonso Francesco Giannini Giuseppe Franzè Giuseppe Fedele Francesco Pupo Giancarlo Fortino IEEE the Department of Computer Engineering ModelingElectronics and SystemsUniversitàdella CalabriaVia Pietro BucciCubo 42-CRende(CS)87036Italy the Department of Mechanical Engineering Energy Engineering and ManagementUniversitàdella CalabriaVia Pietro BucciCubo 42-CRende(CS)87036Italy

In this paper, platoons of autonomous vehicles operating in urban road networks are considered. From a methodological point of view, the problem of interest consists of formally characterizing vehicle state trajectory tubes by means of routing decisions complying with traffic congestion criteria. To this end, a novel distributed control architecture is conceived by taking advantage of two methodologies: deep reinforcement learning and model predictive control. On one hand, the routing decisions are obtained by using a distributed reinforcement learning algorithm that exploits available traffic data at each road junction. On the other hand, a bank of model predictive controllers is in charge of computing the more adequate control action for each involved vehicle. Such tasks are here combined into a single framework:the deep reinforcement learning output(action) is translated into a set-point to be tracked by the model predictive controller;conversely, the current vehicle position, resulting from the application of the control move, is exploited by the deep reinforcement learning unit for improving its reliability. The main novelty of the proposed solution lies in its hybrid nature: on one hand it fully exploits deep reinforcement learning capabilities for decisionmaking purposes;on the other hand, time-varying hard constraints are always satisfied during the dynamical platoon evolution imposed by the computed routing decisions. To efficiently evaluate the performance of the proposed control architecture, a co-design procedure, involving the SUMO and MATLAB platforms, is implemented so that complex operating environments can be used, and the information coming from road maps(links,junctions, obstacles, semaphores, etc.) and vehicle state trajectories can be shared and exchanged. Finally by considering as operating scenario a real entire city block and a platoon of eleven vehicles described by double-integrator models, several simulations have been performed with the a

关键词： Distributed model predictive control distributed reinforcement learning routing decisions urban road networks

A giant scrotal pendulous fibroma mimicking a supernumerary testis

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Asian Journal of Andrology 2024年第2期26卷 227-228页

作者： luigi Quaresima Rocco Francesco Delle Fave Giordano Polisini Daniela Fasanella Willy Giannubilo Urology Division Civitanova Marche HospitalCivitanova Marche 62012Italy Department of Clinical and Specialist Sciences Division of UrologyPolytechnic University of the Marche Region Medical SchoolAncona 60126Italy Department of Life Health and Environmental SciencesUniversity of L'AquilaL'Aquila 67100Italy

DearEditor,Pendulous fibroma,also called acrochordon,is a benign skin neoplasm,originating from the ***,small in size,it can arise from any point of the dermis(frequently from the axillary area,inguinal region,eyelid,or neck),and in some cases,it can be *** fibromas are more frequent in obese subjects,and most of the time,they are sporadic,although sometimes,they can be observed in Birt-Hogg-Dube *** some rare cases,they can reach considerable ***,they are associated with diabetes mellitus,obesity,and intestinal ***,the pedicle undergoes torsion,causing pain and ischemic necrosis of the fibroma,which requires rapid removal of the *** present a case of giant pendulous fibroma of the *** patient has given his consent to the publication of his clinical information and photographic images in an anonymous form.

关键词： frequent obesity clinical

Experimental and Finite Element Analysis of Corroded High-Pressure Pipeline Repaired by Laminated Composite

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Computer Modeling in Engineering & Sciences 2024年第8期140卷 1783-1806页

作者： Seyed Mohammad Reza Abtahi Saeid Ansari Sadrabadi Gholam Hosein Rahimi Gaurav Singh Hamid Abyar Daniele Amato luigi Federico Faculty of Mechanical Engineering Tarbiat Modares UniversityTehran***Iran A.Leon Linton Department of Mechanical Robotics and Industrial EngineeringLawrence Technological UniversitySouthfieldMI48075USA Department of Mechanical Engineering Faculty of EngineeringMeybod UniversityYazd***Iran Department of Industrial Engineering University of SalernoVia Giovanni PaoloⅡFiscianoItaly Italian Aerospace Research Center(C.I.R.A.) Via MaioriseCapuaCE81043Italy

Repairs of corroded high-pressure pipelines are essential for fluids transportation under high *** of the methods used in their repairs is the use of layered *** composite used must have the necessary ***,the experiments and analytical solutions presented in this paper are performed according to the relevant standards and codes,including ASME PCC-2,ASME B31.8S,ASME B31.4,ISO 24817 and ASME *** addition,the experimental tests are replicated numerically using the finite element *** the strain gauges at different distances from the defect location,can reduce the nonlinear effects,deformation,and fluctuations due to the high *** direct relationship between the depth of an axial defect and the stress concentration is observed at the inner side edges of the *** reparation reduces the non-linearities related to the sharp variation of the geometry and a more reliable numerical simulation could be performed.

关键词： High-pressure pipeline composite repair ASME PCC-2 ISO 24817

Deep-learning-empowered synthetic dimension dynamics: morphing of light into topological modes

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Advanced Photonics 2024年第2期6卷 61-68页

作者： Shiqi Xia Sihong Lei Daohong Song luigi Di Lauro Imtiaz Alamgir Liqin Tang Jingjun Xu Roberto Morandotti Hrvoje Buljan Zhigang Chen Nankai University TEDA Institute of Applied Physics School of Physics The MOE Key Laboratory of Weak-Light Nonlinear Photonics Shanxi University Collaborative Innovation Center of Extreme Optics INRS-EMT University of Zagreb Department of PhysicsFaculty of Science

Synthetic dimensions(SDs) opened the door for exploring previously inaccessible phenomena in high-dimensional space. However, construction of synthetic lattices with desired coupling properties is a challenging and unintuitive task. Here, we use deep learning artificial neural networks(ANNs) to construct lattices in real space with a predesigned spectrum of mode eigenvalues, and thus to validly design the dynamics in synthetic mode dimensions. By employing judiciously chosen perturbations(wiggling of waveguides at desired frequencies), we show resonant mode coupling and tailored dynamics in SDs. Two distinct examples are illustrated: one features uniform synthetic mode coupling, and the other showcases the edge defects that allow for tailored light transport and confinement. Furthermore, we demonstrate morphing of light into a topologically protected edge mode with modified Su–Schrieffer–Heeger photonic lattices. Such an ANN-assisted construction of SDs may advance toward “utopian networks,” opening new avenues for fundamental research beyond geometric limitations as well as for applications in mode lasing,optical switching, and communication technologies.

关键词： synthetic dimensions deep learning mode manipulation topological mode morphing photonic lattices

Unlocking the versatile potential:Adipose-derived mesenchymal stem cells in ocular surface reconstruction and oculoplastics

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World Journal of Stem Cells 2024年第2期16卷 89-101页

作者： Pier luigi Surico Anna Scarabosio Giovanni Miotti Martina Grando Carlo Salati Pier Camillo Parodi Leopoldo Spadea Marco Zeppieri Schepens Eye Research Institute of Mass Eye and Ear Harvard Medical SchoolBostonMA 02114United States Department of Ophthalmology Campus Bio-Medico UniversityRome 00128Italy Department of Plastic Surgery University Hospital of UdineUdine 33100Italy Department of Internal Medicine Azienda Sanitaria Friuli OccidentaleSan Vito al Tagliamento 33078Italy Department of Ophthalmology University Hospital of UdineUdine 33100Italy Eye Clinic Policlinico Umberto I“Sapienza”University of RomeRome 00142Italy

This review comprehensively explores the versatile potential of mesenchymal stem cells(MSCs)with a specific focus on adipose-derived *** and oculoplastic surgery,encompassing diverse procedures for ocular and periocular enhancement,demands advanced solutions for tissue restoration,functional and aesthetic refinement,and *** immunomodulatory,regenerative,and healing capacities of MSCs,this review underscores the potential use of adipose-derived MSCs as a cost-effective alternative from bench to bedside,addressing common unmet needs in the field of reconstructive and regenerative surgery.

关键词： Stem cells Adipose stem cell Ocular therapy Oculoplastics Regenerative

Successful treatment of acute liver failure due to Wilson’s disease: Serendipity or fortuity?

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World Journal of Hepatology 2024年第8期16卷 1111-1119页

作者： Valeria Delle Cave Fabiola Di Dato Pier luigi Calvo Maria Immacolata Spagnuolo Raffaele Iorio Department of Translational Medical Science Section of PediatricsUniversity of Naples Federico IINaples 80131Italy Pediatric Gastroenterology Unit Regina Margherita Children's HospitalAzienda Ospedaliera-Universitaria Cittàdella Salute e della ScienzaTurin 10126Italy

BACKGROUND Acute liver failure(ALF)may be the first and most dramatic presentation of Wilson’s disease(WD).ALF due to WD(WD-ALF)is difficult to distinguish from other causes of liver disease and is a clear indication for liver *** is no firm recommendation on specific and supportive medical treatment for this *** To critically evaluate the diagnostic and therapeutic management of WD-ALF patients in order to improve their survival with native *** A retrospective analysis of patients with WD-ALF was conducted in two pediatric liver units from 2018 to *** During the study period,16 children(9 males)received a diagnosis of WD and 2 of them presented with *** first was successfully treated with an unconventional combination of low doses of D-penicillamine and zinc plus steroids,and survived without liver *** second,exclusively treated with supportive therapy,needed a hepatotransplant to overcome *** Successful treatment of 1 WD-ALF patient with low-dose D-penicillamine and zinc plus steroids may provide new perspectives for management of this condition,which is currently only treated with liver transplantation.

关键词： Fulminant liver failure Copper Chelator Zinc Steroids Liver transplantation Autoimmune hepatitis Prognostic score 24 hour-urinary copper excretion Native liver