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In-situ diagnostic of femtosecond laser probe pulses for high resolution ultrafast imaging

Light(Science & Applications) 2021年第7期10卷 1326-1338页

作者： Chen Xie Remi Meyer luc froehly Remo Giust Francois Courvoisier Ultrafast Laser Laboratory Key Laboratory of Opto-electronic Information Technology of Ministry of EducationSchool of Precision Instruments and Opto-electronics EngineeringTianjin University300072 TianjinChina FEMTO-ST Institute Univ.Bourgogne Franche-ComtéCNRS15B avenue des Montboucons25030 Besançon CedexFrance

Ultrafast imaging is essential in physics and chemistry to investigate the femtosecond dynamics of nonuniform samples or of phenomena with strong spatial *** relies on observing the phenomena induced by an ultrashort laser pump pulse using an ultrashort probe pulse at a later *** years have seen the emergence of very successful ultrafast imaging techniques of single non-reproducible events with extremely high frame rate,based on wavelength or spatial frequency ***,further progress in ultrafast imaging towards high spatial resolution is hampered by the lack of characterization of weak probe *** pump–probe experiments realized within solids or liquids,because of the difference in group velocities between pump and probe,the determination of the absolute pump–probe delay depends on the sample *** addition,pulse-front tilt is a widespread issue,unacceptable for ultrafast imaging,but which is conventionally very difficult to evaluate for the low-intensity probe *** we show that a pump-induced micro-grating generated from the electronic Kerr effect provides a detailed in-situ characterization of a weak probe *** allows solving the two issues of absolute pump–probe delay determination and pulse-front tilt *** approach is valid whatever the transparent medium with nonnegligible Kerr index,whatever the probe pulse polarization and *** it is nondestructive and fast to perform,this in-situ probe diagnostic can be repeated to calibrate experimental conditions,particularly in the case where complex wavelength,spatial frequency or polarization encoding is *** anticipate that this technique will enable previously inaccessible spatiotemporal imaging in a number of fields of ultrafast science at the micro-and nanoscale.

关键词： pump polarization laser

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