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Science China Chemistry 2024年第7期67卷 2199-2205页

作者： Hongyan Long sha Zhao Chunyan Jian Xiuli Wu Fengfei lu Minghong Liao Fengrui Che Xingxing Wu Yonggui Robin Chi State Key Laboratory of Green Pesticide Key Laboratory of Green Pesticide and Agricultural BioengineeringMinistry of EducationGuizhou UniversityGuiyang 550025China School of Chemistry Chemical Engineeringand BiotechnologyNanyang Technological UniversitySingapore 637371Singapore

Organoseleniums exhibit a diverse set of biological activities that are pivotal for drug discovery and are widely explored in synthetic chemistry and material *** many transformations have been developed for non-enantioselective C–Se bond formations,the catalyst-controlled stereoselective preparation of chiral organoseleniums continues to be of considerable *** particular,there are limited studies on the enantioselective seleno-Michael addition reactions to access chiral selenium functional ***,we disclose a carbene-catalyzed highly enantioselective nucleophilic C–Se bond construction through formal[3+3]annulations between selenocarboxamides and bromoenals,affording seleno-thiazinone products with good yields and excellent *** choice of a weak inorganic base was pivotal to suppressing the unproductive racemization and decomposition of the selenium ***,the catalytically generated chiral selenium-containing heterocyclic products feature remarkable antimicrobial activities that could serve as promising lead scaffolds for further agrochemical development.

关键词： seleno-Michael addition organocatalysis N-heterocyclic carbene seleno-heterocycles antimicrobial activity

Spin-orbit torque effect in silicon-based sputtered Mn_(3)Sn film

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Chinese Physics B 2024年第10期33卷 394-399页

作者： sha lu Dequan Meng Adnan Khan Ziao Wang Shiwei Chen Shiheng Liang School of Physics Hubei UniversityWuhan 430062China Key Laboratory for Intelligent Sensing System and Security of Ministry of Education Wuhan 430062China

Noncollinear antiferromagnet Mn_(3)Sn has shown remarkable efficiency in charge-spin conversion,a novel magnetic spin Hall effect,and a stable topological antiferromagnetic state,which has resulted in great interest from researchers in the field of spin-orbit *** research has primarily focused on the spin-orbit torque effect of epitaxially grown noncollinear antiferromagnet Mn_(3)Sn ***,this method is not suitable for large-scale industrial *** this study,amorphous Mn_(3)Sn films and Mn_(3)Sn/Py heterostructures were prepared using magnetron sputtering on silicon *** spin-torque ferromagnetic resonance measurement demonstrated that only the conventional spin-orbit torque effect generated by in-plane polarized spin currents existed in the Mn_(3)Sn/Py heterostructure,with a spin-orbit torque efficiency of ***,we prepared the perpendicular magnetized Mn_(3)Sn/CoTb heterostructure based on amorphous Mn_(3)Sn film,where the spin-orbit torque driven perpendicular magnetization switching was achieved with a lower critical switching current density(3.9×10^(7)A/cm^(2))compared to Ta/CoTb *** research reveals the spin-orbit torque effect of amorphous Mn_(3)Sn films and establishes a foundation for further advancement in the practical application of Mn_(3)Sn materials in spintronic devices.

关键词： spintronics noncollinear antiferromagnetism spin-orbit torque

Molecular features of gastroenteropancreatic neuroendocrine carcinoma: A comparative analysis with lung neuroendocrine carcinoma and digestive adenocarcinomas

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Chinese Journal of Cancer Research 2024年第1期36卷 90-102页

作者： Jianwei Zhang Hanxiao Chen Junli Zhang sha Wang Yanfang Guan Wenguang Gu Jie Li Xiaotian Zhang Jian Li Xicheng Wang Zhihao lu Jun Zhou Zhi Peng Yu Sun Yang shao lin Shen Minglei Zhuo Ming lu Key Laboratory of Carcinogenesis and Translational Research(Ministry of Education/Beijing) Department of Gastrointestinal OncologyPeking University Cancer Hospital&InstituteBeijing 100142China Department of Radiation Therapy National Cancer Center/National Clinical Research Center for Cancer/Cancer Hospital&Shenzhen HospitalChinese Academy of Medical Sciences and Peking Union Medical CollegeShenzhen 518172China Key Laboratory of Carcinogenesis and Translational Research(Ministry of Education/Beijing) Department I of Thoracic OncologyPeking University Cancer Hospital&InstituteBeijing 100142China Medical Department Nanjing Geneseeq Technology Inc.Nanjing 210061China Geneplus-Beijing Beijing 102200China State Key Laboratory of Holistic Integrative Management of Gastrointestinal Cancers Beijing Key Laboratory of Carcinogenesis and Translational ResearchDepartment of Gastrointestinal OncologyPeking University Cancer Hospital&InstituteBeijing 100142China Key Laboratory of Carcinogenesis and Translational Research(Ministry of Education/Beijing) Department of PathologyPeking University Cancer Hospital&InstituteBeijing 100142China

Objective: There is an ongoing debate about whether the management of gastroenteropancreatic(GEP)neuroendocrine carcinoma(NEC) should follow the guidelines of small-cell lung cancer(SCLC). We aim to identify the genetic differences of GEPNEC and its ***: We recruited GEPNEC patients as the main cohort, with lung NEC and digestive adenocarcinomas as comparative cohorts. All patients undergone next-generation sequencing(NGS). Different gene alterations were compared and analyzed between GEPNEC and lung NEC(LNEC), GEPNEC and adenocarcinoma to yield the remarkable ***: We recruited 257 patients, including 99 GEPNEC, 57 LNEC, and 101 digestive *** the mutations, KRAS, RB1, TERT, IL7R, and CTNNB1 were found to have different gene alterations between GEPNEC and LNEC samples. Specific genes for each site were revealed: gastric NEC(TERT amplification),colorectal NEC(KRAS mutation), and bile tract NEC(ARID1A mutation). The gene disparities between small-cell NEC(SCNEC) and large-cell NEC(LCNEC) were KEAP1 and CDH1. Digestive adenocarcinoma was also compared with GEPNEC and suggested RB1, APC, and KRAS as significant genes. The TP53/RB1 mutation pattern was associated with first-line effectiveness. Putative targetable genes and biomarkers in GEPNEC were identified in22.2% of the patients, and they had longer progression-free survival(PFS) upon targetable treatment [12.5 months vs. 3.0 months, HR=0.40(0.21-0.75), P=0.006].Conclusions: This work demonstrated striking gene distinctions in GEPNEC compared with LNEC and adenocarcinoma and their clinical utility.

关键词： Neuroendocrine carcinoma gastroenteropancreatic lung genetic alterations molecular markers

Jamming Assisted Covert Wireless Communication in Multi-Channel Systems

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China Communications 2024年第9期21卷 211-224页

作者： Che Bohan sha Nan Yang Weiwei lu Xingbo Gao Chang Army Engineering University of PLA Nanjing 210007China Beijing University of Posts and Telecommunications Beijing 100876China

This paper investigates the jammerassisted multi-channel covert wireless communication(CWC)by exploiting the randomness of sub-channel selection to confuse the *** particular,we propose two sub-channel selection transmission schemes,named random sub-channel selection(RSS)scheme and maximum sub-channel selection(MSS)scheme,to enhance communication *** each proposed scheme,we first derive closed-form expressions of the transmission outage probability(TOP),the average effective rate,and the minimum average detection error probability(DEP).Then,the average effective covert rate(ECR)is maximized by jointly optimizing the transmit power at the transmitter and the number of *** results show that there is an optimal value of the number of sub-channels that maximizes the average *** also find that to achieve the maximum average ECR,a larger number of subchannels are needed facing a stricter covertness constraint.

关键词： covert wireless communication jamming multi-channel system

Insight into the development of electrolytes for aqueous zinc metal batteries from alkaline to neutral

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Chinese Chemical Letters 2024年第2期35卷 232-241页

作者： An Duan sha luo Wei Sun School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China

Aqueous zinc metal batteries are considered as promising candidates for next-generation electrochemical energy storage devices,especially for large-scale energy storage,due to the advantages of high-safety,high energy density and low *** the bridge connecting cathode and anode,electrolyte provides a realistic operating *** alkaline and neutral aqueous zinc metal batteries,issues associated with electrolyte and anode are still *** this review,we reveal the development and evolution of electrolytes for aqueous zinc metal batteries from alkaline to neutral via the description of fundamentals and challenges in terms of comparison and *** also elaborate the strategies in electrolytes regulation and highlight the basic roles and progresses in additives engineering.

关键词： Aqueous electrolytes Zinc metal batteries pH-dependent chemistry Electrolyte regulation Additives engineering

Percutaneous ultrasound-guided coaxial core needle biopsy for the diagnosis of multiple splenic lesions: A case report

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World Journal of Gastrointestinal Surgery 2024年第2期16卷 616-621页

作者： sha-Hong Pu Wu-Yong-Ga Bao Zhen-Peng Jiang Rui Yang Qiang lu Department of Medical Ultrasound West China Hospital of Sichuan UniversityChengdu 610041Sichuan ProvinceChina

BACKGROUND The overlap of imaging manifestations among distinct splenic lesions gives rise to a diagnostic ***,a definitive diagnosis primarily relies on his-tological *** ultrasound(US)-guided coaxial core needle biopsy(CNB)not only procures sufficient tissue to help clarify the diagnosis,but reduces the incidence of puncture-related *** SUMMARY A 41-year-old female,with a history of pulmonary tuberculosis,was admitted to our hospital with multiple indeterminate splenic ***-scale ultrasono-graphy demonstrated splenomegaly with numerous well-defined hypoechoic *** contrast-enhanced computed tomography(CT)showed an en-larged spleen with multiple irregular-shaped,peripherally enhancing,hypodense *** emission CT revealed numerous abnormal hyperglycemia *** imaging findings strongly indicated the possibility of infectious disease as the primary concern,with neoplastic lesions requiring *** obtain the precise pathological diagnosis,the US-guided coaxial CNB of the spleen was ca-rried *** patient did not express any discomfort during the *** Percutaneous US-guided coaxial CNB is an excellent and safe option for obtaining precise splenic tissue samples,as it significantly enhances sample yield for exact pathological analysis with minimum trauma to the spleen parenchyma and sur-rounding tissue.

关键词： Spleen Splenic disease Ultrasound Biopsy Ultrasound-guided coaxial core needle biopsy Case report

Synergistic PM_(2.5)and O_(3)control to address the emerging global PM_(2.5)-O_(3)compound pollution challenges

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Eco-Environment & Health 2024年第3期3卷 325-337页

作者： Chao He Jianhua Liu Yiqi Zhou Jingwei Zhou lu Zhang Yifei Wang lu Liu sha Peng College of Resources and Environment Yangtze UniversityWuhan 430100China Hubei Key Laboratory of Petroleum Geochemistry and Environment Yangtze UniversityWuhan 430100China School of Geography and Ocean Science Nanjing UniversityNanjing 210023China Hydrology and Environmental Hydraulics Group Wageningen University and ResearchWageningen 6700 HBthe Netherlands State Key Laboratory of Freshwater Ecology and Biotechnology Institute of HydrobiologyChinese Academy of SciencesWuhan 430072China State Key Joint Laboratory for Environmental Simulation and Pollution Control School of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentNanjing UniversityNanjing 210023China Collaborative Innovation Center for Emissions Trading System Co-constructed by the Province and Ministry Hubei University of EconomicsWuhan 430205China

In recent years,the issue of PM_(2.5)-O_(3)compound pollution has become a significant global environmental *** study examines the spatial and temporal patterns of global PM_(2.5)-O_(3)compound pollution and exposure risks,firstly at the global and urban scale,using spatial statistical regression,exposure risk assessment,and trend analyses based on the datasets of daily PM_(2.5)and surface O_(3)concentrations monitored in 120 cities around the world from 2019 to ***,on the basis of the common emission sources,spatial heterogeneity,interacting chemical mechanisms,and synergistic exposure risk levels between PM_(2.5)and O_(3)pollution,we proposed a synergistic PM_(2.5)-O_(3)control framework for the joint control of PM_(2.5)and *** results indicated that:(1)Nearly 50%of cities worldwide were affected by PM_(2.5)-O_(3)compound pollution,with China,South Korea,Japan,and India being the global hotspots for PM2.5-O3 compound pollution;(2)Cities with PM_(2.5)-O_(3)compound pollution have exposure risk levels dominated by ST t ST(Stabilization)and ST t HR(High Risk).Exposure risk levels of compound pollution in developing countries are significantly higher than those in developed countries,with unequal exposure characteristics;(3)The selected cities showed significant positive spatial correlations between PM_(2.5)and O_(3)concentrations,which were consistent with the spatial distribution of the precursors NOx and VOCs;(4)During the study period,52.5%of cities worldwide achieved synergistic reductions in annual average PM_(2.5)and O_(3)*** average PM_(2.5)concentration in these cities decreased by 13.97%,while the average O_(3)concentration decreased by 19.18%.This new solution offers the opportunity to construct intelligent and healthy cities in the upcoming low–carbon transition.

关键词： PM_(2.5)-O_(3)compound pollution Population exposure risk Spatial correlation Synergistic treatment potential

Mechanical behavior of sliding zone soil under compression considering periodic saturation-drying: example from a giant reservoir landslide

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Journal of Earth Science 2024年

作者： sha lu Huiming Tang Liangqing Wang Xuexue Su Bing Lü Badong National Observation and Research Station of Geohazards， China University of Geosciences Faculty of Engineering， China University of Geosciences Wuhan， China

The reservoir landslide undergoes periodic saturation-drying cycles affected by reservoir fluctuation in hydropower project area， leading to the irreversible impact on the landslide materials. Sliding zone is the shearing part in formation of landslide and controls the further development of landslide. The mechanical behavior of sliding zone soil under compression is a crucial factor in the stability analysis in landslide. In this paper， the sliding zone soil from a giant landslide in the biggest hydropower project area， Three Gorges area， is taken as the research case. The particle-size distribution of the sliding zone soil from this landslide is studied and fractal dimension is adopted as representation. Periodic saturation-drying is introduced as the affecting factor on sliding zone soil properties. The triaxial compression test is conducted to reveal the mechanical behavior of the soil， including stress-strain behavior， elastic modulus， failure stress and strength parameters. These behavior of sliding zone soils with different fractal dimensions are studied under the effects of periodic saturation-drying cycles. The normalized stress-strain curves are displayed for further calculation. The data considering saturation-drying cycles are obtained and compared with the experimental results.

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The Extended Hybrid Carrier-Based Multiple Access Technology for High Mobility Scenarios

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China Communications 2024年第1期21卷 53-68页

作者： Ge Song Xiaojie Fang Xuejun sha School of Electronics and Information Engineering Harbin Institute of TechnologyHarbin 150001China

The hybrid carrier(HC)system rooted in the carrier fusion concept is gradually garnering *** this paper,we study the extended hybrid carrier(EHC)multiple access scheme to ensure reliable wireless *** employing the EHC modulation,a power layered multiplexing framework is realized,which exhibits enhanced interference suppression capability owing to the more uniform energy distribution *** implementation method and advantage mechanism are explicated respectively for the uplink and downlink,and the performance analysis under varying channel conditions is *** addition,considering the connectivity demand,we explore the non-orthogonal multiple access(NOMA)method of the EHC system and develop the EHC sparse code multiple access *** proposed scheme melds the energy spread superiority of EHC with the access capacity of NOMA,facilitating superior support for massive connectivity in high mobility *** results have verified the feasibility and advantages of the proposed *** with existing HC multiple access schemes,the proposed scheme exhibits robust bit error rate performance and can better guarantee multiple access performance in complex scenarios of nextgeneration communications.

关键词： extended hybrid carrier system high mo-Received:Jun.09,2023 Revised:Nov.20,2023 Editor:Yuanwei Liu bility communications multiple access

Establishment of a three-dimensional particle library for graded crushed stone based on a new aggregate morphology characterization method

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Journal of Traffic and Transportation Engineering(English Edition) 2024年第1期11卷 117-130页

作者： Haitao Ge Aimin sha Zhenqiang Han School of Future Transportation Chang'an UniversityXi'an 710064China University of Strasbourg INSA StrasbourgCNRSICubeUMR 7357Strasbourg F-67000France School of Highway Chang'an UniversityXi'an 710064China Key Laboratory for Special Area Highway Engineering of Ministry of Education Chang'an UniversityXi'an 710064China

The morphology of graded crushed stone(GCS)particles has an essential influence on the performance of aggregate *** impact of particle shape is a comprehensive effect that cannot be considered separately,leading to difficulties in establishing the relationship between the mixture properties and the aggregate morphology by using laboratory *** discrete element method(DEM)is an effective way widely adopted to reconstruct the morphology of particles and simulate performance tests of granular ***,selecting limited particles characterizing a real particle-assembly for simulation is still a challenge in current research due to the inherent rich variability of particle *** this study,based on the acquisition of three-dimensional(3D)aggregate shapes by using laser scanning,ellipsoid index(EDI)translating the particle shape as a function of surface area,volume,and contour length is proposed to comprehensively evaluate aggregate ***,a particle library capable of characterizing aggregate morphology distribution is established based on the statistics of the corresponding morphological characteristics of particle *** model reliability is validated by carrying out a series of experimental and numerical penetration tests with nine different *** established particle library can be used to model aggregate mixtures and the proposed simulation framework is promising for optimizing the mixture gradation design numerically.

关键词： Particle library Discrete element method 3D laser scanning Coarse aggregate Morphology characterization Gradation design