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An in-situ polymerized interphase engineering for high-voltage allsolid- state lithium-metal batteries

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Nano Research 2024年第4期17卷 2687-2692页

作者： lu nie Shaojie Chen Mengtian Zhang Tianyi Gao Yuyao Zhang Ran Wei Yining Zhang Wei Liu School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Tsinghua-Berkeley Shenzhen Institute&Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China

All-solid-state lithium batteries(ASSLBs)have attracted great interest due to their promising energy density and strong safety.However,the interface issues,including large interfacial resistance between electrode and electrolyte and low electrochemical stability of solid-state electrolytes against high-voltage cathodes,have restricted the development of high-voltage ASSLBs.Herein,we report an ASSLB with stable cycling by adopting a conformal polymer interlayer in-situ formed at the Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZTO)–cathode interfaces.The polymer can perfectlyﬁll the voids and create a stable interface contact between LLZTO and cathodes.In addition,the electric field across the polymer interlayer is reduced compared with pure solid polymer electrolyte(SPE),which facilitates the electrochemical stability with high-voltage cathode.The all-solid-state Li|LLZTO-SPE|LiFe_(0.4)Mn_(0.6)PO_(4)(LMFP)cells achieve a low interface impedance,high specific capacity,and excellent cycling performance.This work presents an effective and practical strategy to rationally design the electrode–electrolyte interface for the application of high-voltage ASSLBs.

关键词： all-solid-state lithium batteries interface contact electric field electrochemical stability

Challenges and strategies of lithium-rich layered oxides for Li-ion batteries

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Nano Research 2023年第1期16卷 391-402页

作者： lu nie Shaojie Chen Wei Liu School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China

Lithium-ion batteries are considered a promising energy storage technology in portable electronics and electric vehicles due to their high energy density,competitive cost,and environmental friendliness.Improving cathode materials is an effective way to meet the demand for better batteries,of which the utilization of high-voltage cathode materials is an important development trend.In recent years,lithium-rich layered oxides have gained great attention due to their desirable energy density.This review presents the relationships between lattice structure and electrochemical properties,the underlying degradation mechanisms,and corresponding modification strategies.The recent progress and strategies are then highlighted,including element doping,surface coating,morphology design,size control,etc.Finally,a concise perspective for future developments and practical applications of lithium-rich layered oxides has been provided.

关键词： lithium-ion batteries lithium-rich layered oxides lattice structure degradation mechanism element doping

Ultrafast Carbonized Wood of Electrode-Scaled Aligned-Porous Structure for High-Performance Lithium Batteries

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Transactions of Tianjin University 2023年第5期29卷 387-394页

作者： Shaojie Chen lu nie Hongsheng Shi Xiangchen Hu Zeyu Wang Xinshui Zhang Yuyao Zhang Qilin Hu Tianyi Gao Yi Yu Wei Liu School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China Shanghai Key Laboratory of High-Resolution Electron Microscopy Shanghai Tech UniversityShanghai 201210China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Nankai UniversityTianjin 300071China

The use of carbonized wood in various functional devices is attracting considerable attention due to its low cost,vertical channels,and high electrical conduction.However,the conventional carbonization method requires a long processing time and an inert atmosphere.Here,a microwave-assisted ultrafast carbonization technique was developed that carbonizes natural wood in seconds without the need for an inert atmosphere,and the obtained aligned-porous carbonized wood provided an excellent electrochemical performance as an anode material for lithium-ion batteries.This ultrafast carbonization technique simultaneously produced ZnO nanoparticles during the carbonization process that were uniformly distributed on the alignedporous carbon.The hierarchical structure of carbonized wood functionalized with ZnO nanoparticles was used as a host for achieving high-performance lithium-sulfur batteries:the highly conductive carbonized wood framework with vertical channels provided good electron transport pathways,and the homogeneously dispersed ZnO nanoparticles effectively adsorbed lithium polysulfide and catalyzed its conversion reactions.In summary,a new method was developed to realize the ultrafast carbonization of biomass materials with decorated metal oxide nanoparticles.

关键词： Lithium–Sulfur battery Shuttle effect Lithium-ion battery Biomass carbonization

All-sky Guide Star Catalog for CSST

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Research in Astronomy and Astrophysics 2024年第4期24卷 35-59页

作者： Hui-Mei Feng Zi-Huang Cao Man I Lam Ran Li Hao Tian Da-Yi Yin Yuan-Yu Yang Xin Zhang Dong-Wei Fan Yi-Qiao Dong Xin-Feng Li Wei Wang Long Li Hugh RAJones Yi-Han Tao Jia-lu nie Pei-Pei Wang Mao-Yuan Liu He-jun Yang Chao Liu Key Laboratory of Cosmic Rays(Tibet University) Ministry of EducationLhasa 850000China Institute for Frontiers in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China University of ChineseAcademy of Sciences Beijing 100049China Shanghai Institute of Technical Physics Chinese Academy of SciencesShanghai200083China Technology and Engineering Center for Space Utilization.Chinese Academy of Sciences Beijing 100094China Changchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Centre for Astrophysics University of HertfordshireHatfieldUK Beijing University of Technology Beijing 100124China

The China Space Station Telescope(CSST)is a two-meter space telescope with multiple back-end instruments.The Fine Guidance Sensor(FGS)is an essential subsystem of the CSST Precision Image Stability System to ensure the required absolute pointing accuracy and line-of-sight stabilization.In this study,we construct the Main Guide Star Catalog for FGS.To accomplish this,we utilize the information about the FGS and object information from the Gaia Data Release 3.We provide an FGS instrument magnitude and exclude variables,binaries,and high proper motion stars from the catalog to ensure uniform FGS guidance capabilities.Subsequently,we generate a HEALPix index,which provides a hierarchical tessellation of the celestial sphere,and employ the Voronoi algorithm to achieve a homogeneous distribution of stars across the catalog.This distribution ensures adequate coverage and sampling of the sky.The performance of the CSST guide star catalog was assessed by simulating the field of view of the FGS according to the CSST mock survey strategy catalog.The analysis of the results indicates that this catalog provides adequate coverage and accuracy.The catalog's performance meets the FGS requirements,ensuring the functioning of the FGS and its guidance capabilities.

关键词： catalogs astrometry instrumentation:detectors

新时代中国共产党人自我革命的唯物史观意蕴探析

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武汉商学院学报 2024年第1期38卷 92-96页

作者：聂鲁倩东南大学江苏南京210096

马克思主义唯物史观是揭示人类社会历史客观规律的科学理论,是新时代中国共产党人开展自我革命实践的哲学基础。中国共产党科学把握社会存在与社会意识的关系原理,在开展自我革命过程中坚持实事求是、重视思想建设。中国共产党深度运用... 详细信息

马克思主义唯物史观是揭示人类社会历史客观规律的科学理论,是新时代中国共产党人开展自我革命实践的哲学基础。中国共产党科学把握社会存在与社会意识的关系原理,在开展自我革命过程中坚持实事求是、重视思想建设。中国共产党深度运用社会基本矛盾理论,党的自我革命始终服务于解放和发展生产力,不断解决突出矛盾和时代问题。中国共产党深入践行群众史观,坚持自我革命以人民利益为先、重视人民监督。中国共产党勇于自我革命、坚持自我革命的成功实践深化了对历史辩证法的认识,为世界上其他政党治国理政提供了中国智慧与经验。

关键词：中国共产党自我革命唯物史观

Genetic basis of high level aminoglycoside resistance in Acinetobacter baumannii from Beijing,China

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Acta Pharmaceutica Sinica B 2014年第4期4卷 295-300页

作者： lu nie Yuemeng Lv Min Yuan Xinxin Hu Tongying nie Xinyi Yang Guoqing Li Jing Pang Jingpu Zhang Congran Li Xiukun Wang Xuefu You Institute of Medicinal Biotechnology Chinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100050China The First People's Hospital of Foshan Foshan 528000China State Key Laboratory for Infectious Diseases Prevention and Control National Institute for Communicable Disease Control and PreventionChinese Center for Disease Control and PreventionBeijing 102206China

The objective of this study was to investigate the genetic basis of high level aminoglycoside resistance in Acinetobacter baumannii clinical isolates from Beijing,China.173 A.baumannii clinical isolates from hospitals in Beijing from 2006 to 2009 were first subjected to high level aminoglycoside resistance(HLAR,MIC to gentamicin and amikacin>512 mg/mL)phenotype selection by broth microdilution method.The strains were then subjected to genetic basis analysis by PCR detection of the aminoglycoside modifying enzyme genes(aac(3)-Ⅰ,aac(3)-Ⅱc,aac(60)-Ⅰb,aac(60)-Ⅱ,aph(4)-Ⅰa,aph(30)-Ⅰ,aph(30)-Ⅱb,aph(30)-Ⅲa,aph(30)-Ⅵa,aph(2″)-Ⅰb,aph(2″)-Ⅰc,aph(2″)-Ⅰd,ant(2″)-Ⅰa,ant(3″)-Ⅰand ant(40)-Ⅰa)and the 16S rRNA methylase genes(armA,rmtB and rmtC).Correlation analysis between the presence of aminoglycoside resistance gene and HLAR phenotype were performed by SPSS.Totally 102(58.96%)HLAR isolates were selected.The HLAR rates for year 2006,2007,2008 and 2009 were 52.63%,65.22%,51.11%and 70.83%,respectively.Five modifying enzyme genes(aac(3)-Ⅰ,detection rate of 65.69%;aac(60)-Ⅰb,detection rate of 45.10%;aph(30)-Ⅰ,detection rate of 47.06%;aph(30)-Ⅱb,detection rate of 0.98%;ant(3″)-Ⅰ,detection rate of 95.10%)and one methylase gene(armA,detection rate of 98.04%)were detected in the 102 A.baumannii with aac(3)-Ⅰ+aac(60)-Ⅰ+þant(3″)-Ⅰ+armA(detection rate of 25.49%),aac(3)-Ⅰ+aph(30)-Ⅰ+ant(3″)-Ⅰ+armA(detection rate of 21.57%)and ant(3″)-Ⅰ+armA(detection rate of 12.75%)being the most prevalent gene profiles.The values of chi-square tests showed correlation of armA,ant(3″)-Ⅰ,aac(3)-Ⅰ,aph(30)-Ⅰand aac(60)-Ⅰb with HLAR.armA had significant correlation(contingency coefficient 0.685)and good contingency with HLAR(kappa 0.940).The high rates of HLAR may cause a serious problem for combination therapy of aminoglycoside with β-lactams against A.baumannii infections.As armA was reported to be able to cause high level aminoglycoside resistance to most of the clinical important aminoglycosides(gentamicin,amikacin,tobramycin,etc),the function of aminoglyco

关键词： Acinetobacter baumannii HLAR Aminoglycoside modifying enzyme 16S rRNA methylase Correlation analysis

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双层圆柱壳在均匀轴压下的屈曲行为

舰船科学技术 2024年第2期46卷 15-22页

作者：聂露清王黎辉唐文献江苏科技大学机械工程学院江苏镇江2120001

对双层不锈钢圆柱壳在均匀轴压下的屈曲性能进行研究,分别设计、制作和测量了3个名义相同的双层圆柱薄壳,其长径比均为1.7。通过对试样进行轴向压缩试验获得其载荷位移曲线和极限强度,采用弧长法对试样进行非线性屈曲分析,得到平衡曲线... 详细信息

对双层不锈钢圆柱壳在均匀轴压下的屈曲性能进行研究,分别设计、制作和测量了3个名义相同的双层圆柱薄壳,其长径比均为1.7。通过对试样进行轴向压缩试验获得其载荷位移曲线和极限强度,采用弧长法对试样进行非线性屈曲分析,得到平衡曲线和临界载荷并与试验结果进行对比。另外采用数值分析法研究双层圆柱壳的缺陷敏感性,进而推测出一种用于评估双层圆柱壳承载能力的理论公式。结果表明,双层圆柱壳的平均极限强度约为单层的1.85倍,双层圆柱壳是缺陷敏感结构,其缺陷敏感性与内层壳体缺陷敏感性趋于一致,且双层圆柱壳的缺陷敏感性随长径比的增加而降低,试验结果、数值计算和理论预测具有较高一致性。

关键词：轴向压缩双层圆柱壳屈曲分析缺陷敏感性

系统性炎症指标对下肢动脉硬化闭塞症患者发生肌少症的预测价值

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江苏大学学报（医学版） 2024年第1期34卷 74-78,92页

作者：聂璐杨启帆郑维淼徐强江苏大学附属武进医院介入血管科江苏常州213017 徐州医科大学武进临床学院江苏常州213017 江苏大学附属人民医院消化科江苏镇江212002

目的:评估全身免疫炎症指数(SII)、血小板/淋巴细胞比值(PLR)、中性粒细胞/淋巴细胞比值(NLR)、淋巴细胞/单核细胞比值(LMR)和C反应蛋白(CRP)等系统性炎症指标对下肢动脉硬化闭塞症(ASO)患者发生肌少症的预测价值。方法:本研究纳入江苏... 详细信息

目的:评估全身免疫炎症指数(SII)、血小板/淋巴细胞比值(PLR)、中性粒细胞/淋巴细胞比值(NLR)、淋巴细胞/单核细胞比值(LMR)和C反应蛋白(CRP)等系统性炎症指标对下肢动脉硬化闭塞症(ASO)患者发生肌少症的预测价值。方法:本研究纳入江苏大学附属武进医院和南京医科大学附属常州第二人民医院的251例ASO患者。依据第三腰椎腰大肌指数(PMI)将患者分为肌少症组和非肌少症组。收集患者的一般资料和相关血液指标,并计算SII、PLR、NLR和LMR。通过二分类Logistic回归分析确定ASO患者发生肌少症的危险因素,并采用受试者工作特征(ROC)曲线评估相关指标的预测效果。结果:251例ASO患者中,肌少症组和非肌少症组患者数分别为98例(39.0%)和153例(61.0%)。与非肌少症组相比,肌少症组患者年龄明显增加(P<0.001),SII、PLR、NLR和CRP水平明显增高(P<0.01),而BMI和LMR水平明显降低(P<0.01)。多因素Logistic回归分析结果表明,高龄、BMI偏低、SII上升均为ASO患者发生肌少症的独立危险因素。ROC曲线结果显示,年龄、BMI、SII和3项指标联合预测肌少症发生的曲线下面积分别为0.674、0.678、0.644和0.746(P均<0.001)。结论:年龄、BMI及系统性炎症指标中的SII对ASO患者肌少症的发生有一定的预测价值。

关键词：系统性炎症指标下肢动脉硬化闭塞症肌少症

Advancements in S-scheme heterojunction materials for photocatalytic environmental remediation

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Journal of Materials Science & Technology 2024年第2期169卷 182-198页

作者： Changliang nie Xiaohan Wang Ping lu Yukun Zhu Xin Li Hua Tang School of Environmental Science and Engineering State Key Laboratory of Bio-fibers and Eco-textilesQingdao UniversityQingdao266071China Institute of Biomass Engineering Key Laboratory of Energy Plants Resource and UtilizationMinistry of Agriculture and Rural AffairsSouth China Agricultural UniversityGuangzhou510642China School of Environmental Science and Engineering Shandong UniversityQingdao266237China

Recently,S-scheme heterojunctions have gained considerable attention in the field of photocatalytic environmental remediation as their potential to achieve efficient spatial charge separation coupled with strong redox capacities.Herein,this review provides an overview of the current state-of-the-art in the development of S-scheme-based photocatalysts for the purification of environmental contaminants.The review first covers the fundamentals of heterogeneous photocatalysis for environmental purification.Subsequently,an introduction to the background,mechanism,design principles,and characterization techniques of S-scheme heterojunctions is presented.Then,the review presents a comparison and summary of using various S-scheme photocatalysts for the removal of several target pollutants,such as bacteria,heavy metals,nitrogen oxides,antibiotics,and phenols.Additionally,the modification strategies of S-scheme heterojunction photocatalysts are also provided.Finally,a brief discussion of the challenges and prospects associated with S-scheme photocatalytic systems is demonstrated.

关键词： S-scheme heterojunctions Photocatalyst Pollutant Environmental remediation