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Crystals based on solid solution of Ag_(1-x) Tl_xBr_(1-x) I_x for the manufacturing of IR fibers

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Chinese Optics Letters 2015年第9期13卷 6-8页

作者： Alexandr Korsakov liya zhukova Dmitrii Salimgareev vladislav Zhukov Ural Federal University named after the first President of Russia

For the development of fiber optics for the range from 0.2 to 50.0 μm, one needs light-stable, nonhygroscopic, ductile crystals that would be transparent within this spectral range and have a lack of cleavage, and from which the flexible infrared （IR） fibers are extruded. The crystals based on solid solutions of silver and monadic thallium haides meet the conditions listed above. Consequently, by differential thermal and x ray analyses, we study the TIBr-TII phase diagram using the crystals with optimal compositions, which we grow ourselves. We also manu- facture light-stable nanocrystalline IR fibers that are transparent at longer wavelengths compared with AgC1-AgBr fibers.

关键词： I_x for the manufacturing of IR fibers Crystals based on solid solution of Ag IR

^(14)N_(2)和^(15)N_(2)在解离通道N(^(2)D_(5/2,3/2))+N(^(2)D_(5/2,3/2))阈值以上光解离产物精细结构分支比N(^(2)D_(5/2))/N(^(2)D_(3/2))的测量

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Chinese Journal of Chemical Physics 2024年第2期37卷 264-270,I0102,I0103页

作者：芦丽亚蒋攀程敏高蕻中国科学院化学研究所北京分子科学国家研究中心北京100190 中国科学院大学北京100049

精确测量解离产物的自旋-轨道耦合精细结构分支比对于进一步了解小分子的光解动力学具有十分重要的意义。本文利用真空紫外泵浦-真空紫外探测时间切片离子速度成像装置,测量了^(14)N_(2)的c4′1∑_(u)^(+)(v′=6)态和b′1∑_(u)^(+)(v′... 详细信息

精确测量解离产物的自旋-轨道耦合精细结构分支比对于进一步了解小分子的光解动力学具有十分重要的意义。本文利用真空紫外泵浦-真空紫外探测时间切片离子速度成像装置,测量了^(14)N_(2)的c4′1∑_(u)^(+)(v′=6)态和b′1∑_(u)^(+)(v′=21)态以及^(15)N_(2)的b′∑_(u)^(0)(=20)态和b′1∑_(u)^(+)(v′=20)态和b′1∑_(u)^(+)(v′=21)解离至通道N(2D_(5/2,3/2))+N(2D_(5/2.3/2))产物精细结构分支比N(2D_(5/2))/N(2D_(3/2)).实验结果表明,产物精细结构分支比N(2D_(5/2))/N(2D_(3/2))与^(14)N_(2)或^(15)N_(2)所在的转动能级无关而与其电子态和振动能级的性质有关。^(14)N_(2)的c4′1∑_(u)^(+)(v′=6)态和^(15)N_(2)的b′1∑_(u)^(+)(v′=20)态均接近解离通道N(2D_(5/2,3/2))+N(2D_(5/2,3/2))的阈值,产物精细结构分支比N(2D_(5/2))/N(2D_(3/2))数值均为-1.35;而^(14)N_(2)和^(15)N_(2)的b′∑_(u)^(+)(v′=21)态均远高于解离通道N(2D_(5/2,3/2))+N(2D_(5/2,3/2))的阈值,产物精细结构分支比N(2D_(5/2))/N(2D_(3/2))数值均为-1.00.本文猜测氮气在接近解离通道值时是一个遵循统计规律的解离过程,而在远高于解离通道阈值时是一个非绝热过程,这可能是本实验中观测到的产物精细结构分支比振动依赖现象的原因.要定量解释本实验的测量结果,需要在该解离通道阈值附近的氮气高精度势能曲线及其相互作用信息。

关键词：精细结构分支比真空紫外光氮气分子光解离动力学科里奥利作用

AC-current-induced magnetization switching in amorphous microwires

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Frontiers of physics 2018年第2期13卷 213-223页

作者： v. zhukova J. M. Blanco A. Chizhik M. Ipatov A. Zhukov Dpto. Fisica Aplicada I EUPDS UPV/EHU Plaza Europa 1 San Sebastidn 20018 Spain Dpto. Fisica de Materiales Facultad de Qulmica UPV/EHU 1072 20080 San Sebastidn Spain IKERBASQUE Basque Foundation for Science 58011 Bilbao Spain

We studied the influence of AC current flowing through microwires, on magnetization dynamics. We used a previously developed Sixtus-Tonks modified setup to evaluate the domain wall （DW） velocity within the microwire. However, instead of a magnetizing solenoid, we used a current flowing through the microwire. We observed that the AC current flowing through the annealed Co-rich microwire leads to remagnetization by fast domain wall propagation. The estimated DW velocity was approximately 4.5 km/s, which is similar to and even higher than that reported for the magnetic-field-driven domain wall propagation in Fe- and Co-rich microwires. We measured the DW velocity under tensile stress, and found that the DW velocity decreases under applied stress. An observed DW propagation induced by the current flowing through the microwire is explained considering the influence of an Oersted magnetic field on the outer domain shell. This field has a circular easy magnetization direction and magnetostatic interaction between the outer circumferentially magnetized shell and the inner axially magnetized core.

关键词： domain wall propagation magnetic microwire amorphous material magnetoelasticanisotropy

Quantitative tracking of trans-synaptic nose-to-brain transport of nanoparticles and its modulation by odor,aging,and Parkinson’s disease

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Nano Research 2023年第5期16卷 7119-7133页

作者： Alexander v.Romashchenko Dmitrii v.Petrovskii Sergey Yu.Trotsky Ksenia N.Morozova Nina B.Illarionova Maria v.zhukova Elena v.Kiseleva Marina B.Sharapova Daniil S.Zuev Konstantin E.Kuper Sergey Yu.Taskaev Anna I.Kasatova Dmitrii A.Kasatov Olga I.Solovieva Ivan A.Razumov Ludmila A.Gerlinskaya Mikhail P.Moshkin Yuri M.Moshkin The Federal Research Center Institute of Cytology and Genetics SB RASAcademician Lavrentiev Avenue10Novosibirsk 630090Russia International tomography center Institutskaya st.3ANovosibirsk 630090Russia G.K.Boreskov Institute of Catalysis SB RASAcademician Lavrentiev Avenue5Novosibirsk 630090Russia The Federal Research Center Budker Institute of Nuclear Physics SB RASAcademician Lavrentiev Avenue11Novosibirsk 630090Russia Institute of Computational Technologies Academician M.A.Lavrentiev avenue6Novosibirsk 630090Russia Institute of Gene Biology Russian Academy of SciencesMoscow 117334Russia Institute of Molecular and Cellular Biology SB RASAcad.Lavrentiev Ave8/2Novosibirsk 630090Russia Federal Research Centre of Biological Systems and Agrotechnologies RASst.January 929Orenburg 460000Russia

Nanoparticles(NPs)can be transported via the nose-to-brain(N_(2)B)***,quantitative data on their spatiotemporal dynamics and regulation of the N_(2)B transport are largely *** surveyed metal oxide/hydroxide NPs as magnetic resonance imaging(MRI)contrasts for quantitative N_(2)B *** containing divalent transition metals were the only ones capable of N_(2)B *** T1-weighted(T1W)MRI,we showed that Mn_(3)O_(4)-NPs were readily engulfed by olfactory receptor neurons(ORNs)without disrupting olfactory sensing,we mapped their N_(2)B *** neurons,the Mn_(3)O_(4)-NPs were localized to the cytosol,mitochondria,vesicles,moved at mixed fast and slow axonal transport velocities intraand extra-vesicularly through *** NPs’axonal transport is dependent on neuronal activity and microtubule *** Mn_(3)O_(4)-NPs were trans-synaptically transmitted through at least four synapses across the olfactory ***-synaptic transmission of the NPs was dependent on N-type Ca^(2+)channels and NMDA receptors but blocked by GABAB receptor activation.A five-parameter Weibull signal increase/decrease model fitted to the T1W MRI data allowed for estimating kinetic parameters of Mn_(3)O_(4)-NP accumulation/*** and relative accumulation rates,but not elimination,correlated negatively with the number of synapses from ORNs,indicating a coupling of the NPs’N_(2)B transport with spontaneous neuronal ***,olfactory stimuli(2,5-dimethylpyrazine and acetophenone)significantly modulated and rerouted the Mn_(3)O_(4)-NP N_(2)B transport odor ***,the NPs’trans-synaptic transmission was impaired by aging and the onset of Parkinson’s *** data suggest new approaches to diagnostics,functional neuroimaging,controlling N_(2)B drug delivery.

关键词： Mn_(3)O_(4)nanoparticles magnetic resonance imaging(MRI) nose-to-brain transport trans-synaptic transmission olfactory stimulation

Highly transparent ceramics for the spectral range from 1.0 to 60.0μm based on solid solutions of the system AgBr-AgI-TlI-TlBr

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Chinese Optics Letters 2021年第2期19卷 51-56页

作者： L.v.zhukova D.D.Salimgareev A.E.Lvov A.A.Yuzhakova A.S.Korsakov D.A.Belousov K.v.Lipustin v.M.Kondrashin Ural Federal University named after the first President of Russia B.N.Yeltsin Ekaterinburg 620002Russia

The article is devoted to the technology for obtaining optical ceramics of Ag Br-Tl I and Ag Br-Tl Br_(0.46)I_(0.54) systems and manufacturing samples with different *** new heterophase crystal ceramics are transparent without absorption windows in the spectral range from 1.0 to 60.0μ*** the ceramics’transparency spectra based on the Ag Br-Tl I and Ag Br-Tl Br_(0.46)I_(0.54) systems fusibility diagrams,with an increase in the thallium halides mass fraction,as well as the replacement of the bromine ion with iodine,the maximum transparency shifts to a long infrared region.

关键词： solid solution silver halides monovalent thallium

Real time monitoring for analysis of dam stability:Potential of nonlinear elasticity and nonlinear dynamics approaches

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Frontiers of Structural and Civil Engineering 2013年第2期7卷 188-205页

作者： T.CHELIDZE T.MATCHARASHvILI v.ABASHIDZE M.KALABEGISHvILI N.zhukova M.Nodia Institute of Geophysics Ivane Javakhishvili Tbilisi State UniversityTbilisi 0218Georgia European Centre on Geodynamical Hazards of High Dams 1 Alexidze str.Tbilisi 0171Georgia Georgian Technical University Tbilisi 0171Georgia

Large dams are complex structures with nonlinear dynamic *** often are forced to assess dam safety based on the available incomplete data,which is extremely *** important problem can be solved with the modern theory of complex *** is possible to derive characteristics of the whole unknown dynamics of a structure using few data sets of certain carefully selected representative parameter(s).By means of high quality continuous records of some geotechnical characteristic(s)of a dam and modern methods of time series linear/nonlinear analysis the main dynamical features of the entire,unknown process(here—dam deformation)can be *** created the cost-effective Monitoring Telemetric System for Dam Diagnostics(DAMWATCH),which consists of sensors(tiltmeters),terminal and central controllers connected by the GSM/GPRS Modem to the diagnostic *** tilt data recorded for varying reservoir level are compared with static design model of dam deformations computed by a finite element method(FEM)for the dam-reservoir-foundation ***,recently developed linear/nonlinear data analysis and prediction schemes may help to quantify fine dynamical features of the dam *** software package DAMTOOL has been developed for this *** differences between measured and theoretically predicted response parameters of the dam may signal abnormal behavior of the *** data obtained already by testing of the DAMWATCH/DAMTOOL system during operation of the high Enguri arc dam and reservoir(Georgia)show interesting long-term and short-term patterns of tilts in the dam body,which can be used for dam *** proposed real-time telemetric monitoring(DAMWATCH)complex and linear/nonlinear dynamical analysis system(DAMTOOL)are unique.

关键词： real time monitoring telemetry dam tilts diagnostic tools hysteresis nonlinear dynamics

The effect of high fat food on erythrocyte phospholipids, fatty acids composition and glutathione redox-system of rats with alimentary dyslipidemia

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Health 2010年第1期2卷 45-50页

作者： Natalia v. zhukova Yulia K. Karaman Natalia v. zhukova 不详

To evaluate the effects of high fat food consisted of tallow (19% of total diets) and cholesterol (2%) on modification of erythrocyte phospholipids, fatty acids composition and glutathione redox- system of male Wistar rats with alimentary dysli- pidemia. The results demonstrated that after 30 and 180 days of high-fat feed erythrocyte phos- phatidylinositol and phosphatidylcholine levels were reduced, phosphatidylserine were in-creased. Only on the 90 days of the experiment phosphatidylinositol level increased. In all grow- ups the erythrocyte 18:0 saturated fatty acids and 20:4n6, 22:4n6 polyunsaturated fatty acids (PUFA) were increased. Deficit of n3 PUFA- 20:5n3 and 22:6n3 after 90 and 180 days high fat feed promoted compensatory synthesis from 18:1n9 on 20:3n9. Erythrocyte maleic dialde-hyde increased, glutathione level decreased in all groups of rats after fed with high-fat feed. Glutathione reductase and glutathione peroxi-dase activity decreased in erythrocytes after 30 and 180 days of high-fat feed. In conclusion: high-fat diet during 30-90 days started adaptive answer in lipids of membrane and glutathione redox-system. Important mechanism of adapta-tion of a cellular membrane to high-fat diet is increase major, structuring a membrane phos-phatidylethanolamine and minor, most meta-bolic significant fractions phospholipids (phos- phatidylinositol), keeps homeostasis of 18:2n6 and 22:6n3, 20:3n9 compensatory synthesis, decrease in activity of processes lipid peroxi-dation, activation of enzymes of redox-system glutathione. But prolonging the high-fat feeding (180 days and more) formed failure compensa-tory processes (dysadaptation). It is a risk factor of developmening atherosclerosis, diabetes, steatogepatitis and other diseases.

关键词： Fatty Acids Phospholipids Adaptation Dyslipidemia GSH Glutathione Reductase Glutathione Peroxidase

Spiro-based triphenylamine molecule with steric structure as a cathode material for high-stable all organic lithium dual-ion batteries

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能源化学:英文版 2023年第8期83卷 24-31,I0003页

作者： liya Huang Zehao Yu Liubin Wang Bin Qin Fengshi Cai Zhihao Yuan Zhiqiang Luo Tianjin Key Lab for Photoelectric Materials&Devices Tianjin Key Laboratory of Organic Solar Cells and Photochemical ConversionSchoolof Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China College of Chemistry&Materials Science Hebei UniversityBaoding 071002HebeiChina Department of Chemistry The University of Hong KongPokfulam RoadHong Kong 999077China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Redox p-type organic compounds are promising cathode materials for dual-ion ***,the triphenylamine-based polymers usually with agglomerate and intertwined molecular chain nature limit the maximum reaction of their active sites with large-sized ***,we demonstrate the application of a small molecule with rigid spirofluorene structu re,namely 2,2’,7,7’-tetrakis(diphenylamine)-9,9’-spirobifluorene(Spiro-TAD),as a cathode material for lithium dual-ion *** inherent sterical structure endows the Spiro-TAD with good chemical stability and large internal space for fast diffusion kinetics of anions in the organic *** a result,the Spiro-TAD electrode shows significant insolubility and less steric hindrance,and gives a high actual capacity of 109 mA h g^(-1)(active groups utilization ratio approximately 100%) at 50 mA g^(-1)with a high discharge voltage of 3.6 v(***+/Li),excellent rate capability(60 mA h g^(-1)at 2000 mA g^(-1)) and extremely stable cycling life(98.4% capacity retention after 1400 cycles at 500 mA g^(-1)) in half *** good electrochemical performance is attributed to the robust and rapid adsorption/desorption of ClO4-anions,which can be proved by the in-situ FTIR and ***,an all-organic lithium dual-ion battery(a-OLDIBs) is constructed using the Spiro-TAD as cathode and 3,4,9,10-Perylenetetracarboxylic diimide(PTCDI) as anode and displays long-term cycling performance of 87.5 mA h g^(-1)after 800 *** study will stimulate further developments in designing all organic battery systems.

关键词： Spiro-basedmolecule Cathodematerial P-typeorganiccompounds Longcycling life All organic lithiumdual-ionbatteries

Evidence of Electronic Phase Separation in the Strongly Correlated Semiconductor YbB_(12)

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Chinese Physics Letters 2022年第12期39卷 65-70页

作者： A.Azarevich N.Bolotina O.Khrykina A.Bogach E.zhukova B.Gorshunov A.Melentev Z.Bedran A.Alyabyeva M.Belyanchikov v.voronov N.Yu.Shitsevalova v.B.Filipov N.Sluchanko Prokhorov General Physics Institute of the Russian Academy of Sciences Vavilov Str.38Moscow 119991Russia Shubnikov Institute of Crystallography Federal Scientific Research Centre‘Crystallography and Photonics’of Russian Academy of Sciences59 Leninskiy ProspectMoscow 119333Russia Center for Photonics and 2D Materials Moscow Institute of Physics and Technology(National Research University)141700 DolgoprudnyMoscow RegionRussia Institute for Problems of Materials Science NASUKrzhizhanovsky Str.303142 KyivUkraine

We investigate high-quality single-domain crystals of YbB_(12)using the precise x-ray diffraction technique in combination with the low-temperature polarized THz–infrared spectroscopy and accurate magnetotransport *** is shown for the first time that this archetypal strongly correlated system with a metal-insulator transition to a mysterious dielectric ground state with a metal Fermi surface[Science 362,65(2018)and ibid 362,32(2018)]is actually a heterogeneous compound in the regime of electronic phase *** in the configuration of the discovered dynamic charge stripes are proposed upon *** a result,a conclusion is drawn in favor of a crossover between different patterns of the filamentary electronic structure penetrating the semiconducting matrix of YbB_(12).We argue that the discovery of stripes in YbB_(12)is fundamental,elucidating the nature of exotic dielectric state in Kondo insulators.

关键词： insulator Kondo dielectric