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In situ meso-tetra(4-carboxyphenyl)porphyrin ligand substitution in Hf-MOF for enhanced catalytic activity and stability in photoredox reactions

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Rare Metals 2024年第6期43卷 2682-2694页

作者： Jie hu Hong-Xin Lao Xiu-Wu Xu Wei-Kang Wang Le-Le Wang Qin-Qin liu School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China College of Chemistry and Materials Engineering Research Center of Carbon NeutralityAnhui Normal UniversityWuhu 241002China Fujian Provincial Key Laboratory of Ecology-Toxicological Effects and Control for Emerging Contaminants Putian UniversityPutian 351100China

Though there are numerous intrinsic merits of metal-organic frameworks(MOFs),low charge separation efficiency has imposed heavy restrictions on their photocatalytic ***,in situ porphyrin ligand substitution,as a strategy for improving the charge separation efficiency and increasing the amounts of active sites,has been designed and realized in a Hf-biphenyl dicarboxylic acid(BPDC)***,a size and geometry matched meso-tetra(4-carboxyphenyl)porphyrin(TCPP)ligand was selected and doped into Hf-BPDC MOF by forming coordinating bonds with Hf centers,forming dualligand Hf-BPDC-TCPP *** resultant Hf-BPDC-TCPP MOF showed significantly improved activity and chemical stability in the photocatalytic H_(2)generation(261μmol·g^(-1)·h^(-1))and tetracycline(TC)degradation reactions(95.8%),which was 48 and 1.47 folds higher than that of the Hf-BPDC *** and electrochemical studies revealed that the introduction of porphyrin ligand could generate a stronger internal electric field for boosting the charge separation and transfer,increase the specific surface area for providing more active sites,and narrow the band gap to enhance the visible light *** in situ ligand substitution method provides a promising approach to build a tunable platform for constructing high-performance MOF photocatalysts.

关键词： Ligand substitution Metal organic frameworks Meso-tetra(4-carboxyphenyl)porphyrin Hydrogen evolution reaction Tetracycline degradation

Multipliers on Dirichlet Type Spaces

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Acta Mathematica Sinica,English Series 2001年第2期17卷 263-272页

作者： Peng Yan hu Department of Mathematics. normal College of Shenzhen university. Shenzhen. Guangdong 518060. P. R. china Ji huai SHI Department of Mathematics. university of Science and Technology of china. Hefei. anhui 230026, P. R. china Department of Mathematics Normal College of Shenzhen University Shenzhen Guangdong 518060 P. R. China Department of Mathematics University of Science and Technology of China Hefei Anhui 230026 P. R. China

In this paper, we characterize the pointwise multiplier space M(D_τ, D_μ) of Dirichlet type spaces in the unit ball of C^n for the values of τ, μ in three cases: (i)τn. and construct two functions to show that M... 详细信息

关键词： Dirichlet space Pointwise multiplier Holomorphic function

Coexistence of multiuser entanglement distribution and classical light in optical fiber network with a semiconductor chip

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Chip 2024年第2期3卷 1-10页

作者： Xu Jing Cheng Qian Xiaodong Zheng hu Nian Chenquan Wang Jie Tang Xiaowen Gu Yuechan Kong Tangsheng Chen Yichen liu Chong Sheng Dong Jiang Bin Niu Liangliang Lu National Key Laboratory of Solid-State Microwave Devices and Circuits Nanjing Electronic Devices InstituteNanjing 210016China Key Laboratory of Optoelectronic Technology of Jiangsu Province School of Physical Science and TechnologyNanjing Normal UniversityNanjing 210023China National Laboratory of Solid-State Microstructures Nanjing UniversityNanjing 210093China Research Center for Quantum Optics and Quantum Communication School of ScienceQingdao University of TechnologyQingdao 266520China School of Internet Anhui UniversityHefei 230039China Hefei National Laboratory Hefei 230088China

Building communication links among multiple users in a scalable and robust way is a key objective in achieving large-scale quantum *** a realistic scenario,noise from the coexisting classical light is inevitable and can ultimately disrupt the *** previous significant fully connected multiuser entanglement distribution experiments are conducted using dark fiber links,and there is no explicit relation between the entanglement degradations induced by classical noise and its error ***,a semiconductor chip with a high figure-of-merit modal overlap is fabricated to directly generate broadband polarization *** monolithic source maintains the polarization entanglement fidelity of above 96%for 42 nm bandwidth,with a brightness of 1.2×10^(7)Hz mW^(−1).A continuously working quantum entanglement distribution are performed among three users coexisting with classical *** finite-key analysis,secure keys are established and images encryption are enabled as well as quantum secret sharing between *** work paves the way for practical multiparty quantum communication with integrated photonic architecture compatible with real-world fiber optical communication network.

关键词： Quantum key distribution Semiconductor chip Raman noise Image encryption

Predicting stability of integrated circuit test equipment using upper side boundary values of normal distribution

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The Journal of china Universities of Posts and Telecommunications 2024年第2期31卷 85-93页

作者： Zhan Wenfa hu Xinyi Zheng Jiangyun Yu Chuxian Cai Xueyuan Zhang Lihua School of Electronic Engineering and Intelligent Manufacturing Anqing Normal UniversityAnqing 246133China School of Computer and Information Technology Anqing Normal UniversityAnqing 246133China

In response to the growing complexity and performance of integrated circuit(IC),there is an urgent need to enhance the testing and stability of IC test equipment.A method was proposed to predict equipment stability using the upper side boundary value of normal ***,the K-means clustering algorithm classifies and analyzes sample *** accuracy of this boundary value is compared under two common confidence levels to select the optimal threshold.A range is then defined to categorize unqualified test *** experimental verification,the method achieves the purpose of measuring the stability of qualitative IC equipment through a deterministic threshold value and judging the stability of the equipment by comparing the number of unqualified data with the threshold value,which realizes the goal of long-term operation monitoring and stability analysis of IC test equipment.

关键词： K-means clustering algorithm the upper side boundary of normal distribution threshold integrated circuit(IC)test equipment stability analysis

Heavy metals potentially drive co-selection of antibiotic resistance genes by shifting soil bacterial communities in paddy soils along the middle and lower Yangtze River

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Pedosphere 2024年第3期34卷 606-619页

作者： Ya ZHANG Hao WANG Minghui hu Rui CAI Yuqing MIAO Xiancan Zhu anhui Provincial Key Laboratory of Molecular Enzymology and Mechanism of Major Metabolic Diseases Anhui Provincial Key Laboratory of the Conservation and Exploitation of Biological ResourcesCollege of Life SciencesAnhui Normal UniversityWuhu 241000(China) School of Geography and Tourism Anhui Normal UniversityWuhu 241003(China)

Heavy metals(HMs)and antibiotic resistance have become serious environmental problems affecting soil and human *** microorganisms play key roles in pollutant degradation and biogeochemical cycling processes;however,the interactions among HMs,soil microbial communities,and antibiotic resistance genes(ARGs)in agricultural soils remain *** quantitative real-time polymerase chain reaction and NovaSeq sequencing,we evaluated heavy metal contents,abundances of ARGs,soil bacterial community structure and functions,and their correlations in paddy soils at 43 sampling sites along the middle and lower reaches of the Yangtze River,central and eastern *** results showed the co-occurrence of HMs,ARGs,and HM resistance genes across all paddy ***,significant positive associations were detected between HMs and resistance ***,czcA,and int1 were positively correlated with bacterial community *** Mantel test showed that bacterial community composition and functions were significantly associated with HMs and resistance genes,such as Cd,Cr,Zn,copA,czcA,int1,and ***,HMs and ARGs were the major factors shaping soil bacterial communities;thus,HMs triggered proliferation of HM and antibiotic resistances by influencing the mobile genetic element(int1)and soil microbial *** study revealed that HMs potentially drive the co-selection of ARGs by shifting soil bacterial community structure and functions,thereby increasing the potential risks to human health as well as ecological environment in the paddy soils along the middle and lower reaches of the Yangtze River.

关键词： agricultural ecosystem ecological risk heavy metal resistance microbial community soil contamination soil pollution

Magnetically responsive manipulation of droplets and bubbles

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Droplet 2024年第2期3卷 73-94页

作者： Shaojun Jiang Dong Wu Jiawen Li Jiaru Chu Yanlei hu CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Precision Machinery and Precision InstrumentationUniversity of Science and Technology of ChinaHefeiChina

Droplets and bubbles have a wide range of applications in industry,agriculture,and daily life,and their controllable manipulation is of significant scientific and technological *** magnetically responsive manipulation strategies have been developed to achieve precise control over droplets and *** manipulate nonmagnetic droplets or bubbles with magnetic fields,the presence of magnetic medium is *** additives can be added to the surface or interior of droplets and bubbles,allowing for on-demand manipulation by direct magnetic ***,magnetically responsive elastomer substrates can be used to actuate droplets and bubbles by controlling the deformation of microstructures on the substrates through magnetic *** strategy is based on untethered magnetic devices,which enables free mobility,facilitating versatile manipulation of droplets and bubbles in a flexible *** paper reviews the advances in magnetically responsive manipulation strategies from the perspective of droplets and *** overview of the different classes of magnetic medium,along with their respective corresponding droplet/bubble manipulation methods and principles,is first ***,the applications of droplet/bubble manipulation in biomedicine,microchemistry,and other fields are ***,the remaining challenges and future opportunities related to regulating droplet/bubble behavior using magnetic fields are discussed.

关键词： deformation bubble versatile

Rim^(18)F-fluorodeoxyglucose uptake of hepatic cavernous hemangioma on positron emission tomography/computed tomography:A case report

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World Journal of Clinical Cases 2024年第13期12卷 2243-2247页

作者： Yong-An hu Ya-Xin Guo Qi-Feng huang Department of Nuclear Medicine Jinhua Hospital of Zhejiang UniversityJinhua Municipal Central HospitalJinhua 321000Zhejiang ProvinceChina

BACKGROUND Peripheral FDG accumulation in a hepatic hemangioma presenting in a patient with prolonged fever is ***,clinicians should pay close attention to patients with hepatic *** SUMMARY A 54-year-old woman with a 4-wk history of daily fevers was admitted to our hospital.A whole body^(18)-Fluordesoxyglucose(PET-FDG)positron emission tomography/computed tomography(PET/CT)was performed to elucidate the source of the ***,whole body^(18)-FDG PET/CT raised the suspicion of a malignant lesion because of peripheral FDG accumulation(SUVmax 3.5 g/mL)higher than that of the normal liver parenchyma(SUVmax 1.6 g/mL)surrounding a hypoactive area,and no other abnormalities were ***,the patient underwent liver mass *** showed a hepatic cavernous hemangioma with fatty infiltration around the *** fever disappeared four days after surgery and the patient did not present any complications during *** Fatty infiltration in the peripheral parts of hepatic cavernous hemangioma may lead to subacute inflammation which further activate the Kupffer *** may cause prolonged fever and peripheral rim FDG accumulation on PET/CT.

关键词： ^(18)-Fluordesoxyglucose positron emission tomography/computed tomography Hepatocellular carcinoma Fever Fatty infiltration Case report

Patterns and drivers of avian taxonomic and phylogenetic beta diversity in china vary across geographical backgrounds and dispersal abilities

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Zoological Research 2024年第1期45卷 125-135页

作者： Jian-Chao Liang Zhi-Feng Ding Chun-Lin Li Yi-Ming hu Zhi-Xin Zhou Gan-Wen Lie Xiao-Nan Niu Wen-Bin huang hui-Jian hu Xing-Feng Si Guangdong Key Laboratory of Animal Conservation and Resource Utilization Guangdong Public Laboratory of Wild Animal Conservation and UtilizationInstitute of ZoologyGuangdong Academy of SciencesGuangzhouGuangdong 510260China School of Resources and Environmental Engineering Anhui UniversityHefeiAnhui 230601China Guangdong Eco-Engineering Polytechnic GuangzhouGuangdong 510520China huizhou Institute of Forestry(huizhou Botanical Garden Management Service Center) HuizhouGuangdong 516001China Administration of National Nature Reserve for Marine Ecology of Guangdong Nanpeng Islands ShantouGuangdong 515900China Zhejiang Zhoushan Archipelago Observation and Research Station Institute of Eco-ChongmingZhejiang Tiantong Forest Ecosystem National Observation and Research StationSchool of Ecological and Environmental SciencesEast China Normal UniversityShanghai 200241China

Geographical background and dispersal ability may strongly influence assemblage dissimilarity;however,these aspects have generally been overlooked in previous large-scale beta diversity ***,we examined whether the patterns and drivers of taxonomic beta diversity(TBD)and phylogenetic beta diversity(PBD)of breeding birds in china vary across(1)regions on both sides of the hu Line,which demarcates china’s topographical,climatic,economic,and social patterns,and(2)species with different dispersal *** and PBD were calculated and partitioned into turnover and nestedness components using a moving window *** representing climate,habitat heterogeneity,and habitat quality were employed to evaluate the effects of environmental *** distance was considered to assess the impact of dispersal *** partitioning analysis was applied to assess the relative roles of these *** general,the values of TBD and PBD were high in mountainous areas and were largely determined by environmental ***,different dominant environmental filters on either side of the hu Line led to divergent beta diversity ***,climate-driven species turnover and habitat heterogeneity-related species nestedness dominated the regions east and west of the line,***,bird species with stronger dispersal ability were more susceptible to environmental filtering,resulting in more homogeneous *** results indicated that regions with distinctive geographical backgrounds may present different ecological factors that lead to divergent assemblage dissimilarity patterns,and dispersal ability determines the response of assemblages to these ecological *** a single universal explanation for the observed pattern without considering these aspects may lead to simplistic or incomplete ***,a comprehensive understanding of large-scale beta diversity patterns and effective pla

关键词： Beta diversity Environmental filtering Dispersal limitation hu Line Species dispersal ability Breeding birds

Influence of self-similar stresses on scenario earthquake construction:An example along the Tanlu Fault

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Science china Earth Sciences 2024年第5期67卷 1687-1697页

作者： Feng hu huajian YAO Houyun YU Zeyu LU Jieyi HOU Song LUO Zhigang SHAO Xiaofei CHEN School of Earth and Space Sciences University of Science and Technology of ChinaHefei 230026China Mengcheng Geophysical National Field Scientific Observatory Hefei 230026China Department of Earth and Space Science Southern University of Science and TechnologyShenzhen 518055China Institute of Earthquake Prediction China Earthquake AdministrationBeijing 100036China

As a famous deep and large fault in eastern china,the Tanlu Fault passes through anhui,Jiangsu,and Shandong and into northeastern *** is important to improve the understanding of seismic hazard assessments in areas near *** start a scenario earthquake simulation in the M7.5 earthquake potential area of the Xinyi-Sihong segment of the Tanlu *** fault rupture length and width are constrained according to the scaling law of large intraplate earthquakes,the background normal stress is depth dependent,and the initial shear stresses are determined using trial and error by matching the earthquake *** the 120 km rupture length of the M7.5 earthquake,we compare the horizontal uniform stress model and self-similar stress perturbation *** findings reveal that the seismic source time function of the horizontal uniform stress model is similar to that of the Haskell model and that of the self-similar stress perturbation model is more similar to that of a real earthquake *** compare the dynamic rupture simulation and ground motion results under four different stress conditions and find that the shorter the characteristic length of the self-similar function is,the rougher the initial *** the M7.5earthquake with an epicenter in the vicinity of Suqian,the Xinyi-Tancheng segment,which is located in the IX-intensity zone north of the epicenter,vibrates more strongly on the northern side than on the southern side due to the influence of the lowvelocity zone and the peak slip *** response spectra analysis at stations in the study area is useful for improving the earthquake resistance capability.

关键词： Scenario earthquakes Self-similar stress Tanlu Fault Dynamic rupture Ground motion