检索结果-南通市图书馆

Investigating the effect of volatility on the hygroscopicities of acetate nanoparticle aerosols by surface plasmon resonance microscopy

在线全文

学校读者我要写书评

暂无评论

Journal of Environmental Sciences 2024年第4期138卷 167-178页

作者： Bo Yang Zhibo Xie jianguo liu Huaqiao Gui Jiaoshi Zhang Xiuli Wei Zetao Fan Douguo Zhang Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China University of Science and Technology of China Hefei 230026China CAS Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Advanced Laser Technology Laboratory of Anhui Province Department of Optics and Optical EngineeringUniversity of Science and Technology of ChinaHefei 230026China

Under high relative humidity(RH)conditions,the release of volatile components(such as acetate)has a significant impact on the aerosol *** this work,one surface plasmon resonance microscopy(SPRM)measurement system was introduced to determine the hygroscopic growth factors(GFs)of three acetate aerosols separately or mixed with glucose at different *** Ca(CH_(3)COO)_(2) or Mg(CH_(3)COO)_(2) aerosols,the hygroscopic growth trend of each time was lower than that of the previous time in three cyclic humidification from 70% RH to 90% RH,which may be due to the volatility of acetic acid leading to the formation of insoluble hydroxide(Ca(OH)_(2) or Mg(OH)_(2))under high RH *** the third calculated GF(using the Zdanovskii-Stokes-Robinson method)for Ca(CH_(3)COO)_(2) or Mg(CH_(3)COO)_(2) in bicomponent aerosols with 1:1 mass ratio were 3.20% or 5.33% lower than that of the first calculated GF at 90% *** calculated results also showed that the hygroscopicity change of bicomponent aerosol was negatively correlated with glucose content,especially when the mass ratio of Mg(CH_(3)COO)_(2) to glucose was 1:2,the GF at 90% RH only decreased by4.67% after three cyclic *** coupled plasma atomic emission spectrum(ICP-AES)based measurements also indicated that the changes of Mg^(2+)concentration in bicomponent was lower than that of the *** results of this study reveal thatduring the efflorescence transitions of atmospheric nanoparticles,the organic acids diffusion rate may be inhibited by the coating effect of neutral organic components,and the particles aging cycle will be prolonged.

关键词： Hygroscopic growth Volatility Acetate aerosols Nanoparticle aerosol Surface plasmon resonance

Beyond skyline and borders: Unraveling the evolution and drivers of tourism green development efficiency in the Beijing-Tianjin-Hebei urban agglomeration, China

在线全文

学校读者我要写书评

暂无评论

Journal of Geographical Sciences 2024年第9期34卷 1761-1796页

作者： HUANG Xingling liu jianguo College of Tourism and Service Management Nankai UniversityTianjin 300071China Tourism College of Beijing Union University Beijing 100101China Department of City and Regional Planning The University of North Carolina at Chapel HillNC 27599USA

Green development is a critical component of sustainable tourism, which prioritizes a comprehensive, ecologically-friendly, and people-oriented approach to development. This study presents a case study of the Beijing–Tianjin–Hebei(BTH) urban agglomeration from 2001 to 2021 to analyze the spatio-temporal evolution characteristics and influencing factors of tourism green development efficiency(TGDE). The study defines the concept of tourism green development and constructs an evaluation system, which is used to explore the internal differences and spatial patterns of TGDE within the urban agglomeration. The methodological approach includes the SBM–Undesirable model, kernel density estimation, Markov chain, and spatial gravity model. The findings indicate that the TGDE in the BTH urban agglomeration is generally favorable, displaying a temporal phase of “rising–declining–rising.” However, the study observes lower TGDE in tourism node cities compared to tourism regional center cities and tourism core hub cities. The non-equilibrium degree of each region indicates significant spatio-temporal evolution patterns and internal differences among the three regions, with a spatially decreasing distribution of “core hub-regional center-node city.” The TGDE in the urban agglomeration experienced an evolutionary trend of “first decreasing and then increasing” with apparent endogenous evolution characteristics. The linkage pattern of green development efficiency in the tourism industry between cities is relatively stable. Furthermore,neighboring cities generally exhibit a higher spatial connectivity strength of green development efficiency in the tourism industry compared to non-neighboring cities. Economic development level, industrial structure, and science and education level are identified as key factors that affect TGDE. However, the study finds that the factors influencing TGDE in tourism core hub cities, tourism regional center cities, and tourism node cities differ somewhat

关键词： BTH urban agglomeration tourism green development efficiency(TGDE) spatio-temporal evolution

Characteristics of rural domestic sewage discharge and their driving mechanisms: evidence from the Northern Region, China

在线全文

学校读者我要写书评

暂无评论

Frontiers of Environmental Science & Engineering 2024年第7期18卷 47-58页

作者： jianguo liu Ziyu Zhou Pengyu Li Zixuan Wang Ying Yan Xuezheng Yu Wenkai Li Tianlong Zheng Yingnan Cao Wenjun Wu Wenqian Cai Zhining Shi Junxin liu Key Laboratory of Environmental Pollution Control and Remediation at Universities of Inner Mongolia Autonomous Region College of Resources and Environmental EngineeringInner Mongolia University of TechnologyHohhot 010051China State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China SCEGC No.12 Construction Engineering Group Co. Ltd.Ankang 725000China State Environmental Protection Key Laboratory of Environmental Planning and Policy Simulation Chinese Academy of Environmental PlanningBeijing 100041China Technical Centre for Soil Agriculture and Rural Ecology and EnvironmentMinistry of Ecology and EnvironmentBeijing 100012China Sustainable Infrastructure and Resource Management(SIRM) UniSA STEMUniversity of South AustraliaSouth AustraliaMawson LakesSA 5095Australia

The traits of rural domestic sewage emission are unclear,negatively affecting rural domestic sewage treatment and sewage *** study used data from the Second National Pollution Source Census Bulletin to establish a data *** spatial distribution characteristics and main factors influencing rural sewage discharge in the Northern Region were studied using spatial autocorrelation analysis and structural *** findings demonstrated that(l)a significant Spearman correlation between drainage water volume(DwV),chemical oxygen demand(COD),ammonia nitrogen(NH_(3)-N),total nitrogen(TN),and total phosphorus(TP)and that the correlation coefficients between DWV and COD,NH,-N,TNand TP were 0.87**,1.0**,0.99**,0.99**,respectively;(2)rural sewage discharge showed spatial autocorrelation,and rural domestic sewage discharge in the districts and counties with an administration was significantly higher than in the surrounding areas;and(3)social development was the main driver rural domestic sewage changes(path coefficient was 0.407**),and the main factors influencing rural domestic sewage discharge were the urbanization rate,years of education,and population age *** study obtained the spatial variation law and clarified the main influencing factors of rural domestic sewage to provide data support and a theoretical basis for subsequent rural sewage collection and *** of the Inner Mongolia Autonomous Region in northern China as a typical case,provides a theoretical foundation for scientific decision-making on rural domestic sewage treatment at the national and regional levels and offers new perspectives for managing pollutants.

关键词： Rural domestic sewage Emission characteristics Spatial autocorrelation analysis Influencing factors

Local tetragonal distortion of Pt alloy catalysts for enhanced oxygen reduction reaction efficiency

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Carbon Energy 2024年第7期6卷 41-52页

作者： Xiaoke Li Xiao Duan Kang Hua Yongkang Wu Zhiyan Rui Rui Ding Aidong Li Chen Ouyang Jia Li Ting Li jianguo liu National Laboratory of Solid-State Microstructures College of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjingChina Long-Life Fuel Cell Key Laboratory in Sichuan Province Dongfang Electric(Chengdu)Hydrogen Fuel Cell Technology Co.Ltd.ChengduChina Institute of Energy Power Innovation North China Electric Power UniversityBeijingChina

Platinum-based alloy nanoparticles are the most attractive catalysts for the oxygen reduction reaction at present,but an in-depth understanding of the relationship between their short-range structural information and catalytic performance is still ***,we present a synthetic strategy that uses transition-metal oxide-assisted thermal ***/C catalysts with localized tetragonal distortion were obtained by controlling the thermal diffusion process of transition-metal *** localized structural distortion induced a significant strain effect on the nanoparticle surface,which further shortened the length of the Pt-Pt bond,improved the electronic state of the Pt surface,and enhanced the performance of the ***/C catalysts with special short-range structures achieved excellent mass activity(2.27 Amg_(Pt)^(-1))and specific activity(3.34 A cm^(-2)).In addition,the localized tetragonal distortion-induced surface compression of the Pt skin improved the stability of the *** mass activity decreased by only 13%after 30,000 *** catalyst activity and excellent durability have also been demonstrated in the proton exchange membrane fuel cell *** study provides valuable insights into the development of advanced Pt-based nanocatalysts and paves the way for reducing noble-metal loading and increasing the catalytic activity and catalyst stability.

关键词： electrocatalysts fuel cells local tetragonal distortion oxygen reduction

Quantifying the impacts of COVID-19 on Sustainable Development Goals using machine learning models

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Fundamental Research 2024年第4期4卷 890-897页

作者： Chenyang Shuai Bu Zhao Xi Chen jianguo liu Chunmiao Zheng Shen Qu Jian-Ping Zou Ming Xu School of Management Science and Real Estate Chongqing UniversityChongqing 400044China bSchool for Environment and Sustainability University of MichiganAnn ArborMI 489United Stats Michigan Institute for Computational Discovery&Engineering University of MichiganAnn ArborMI 48109United States College of Economics and Management Southwest UniversityChongqing 400044China Center for Systems Integration and Sustainability Department of Fisheries and WildlifeMichigan State UniversityEast LansingMI 48824United States Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China School of Management and Economics Beijing Institute of TechnologyBeijing 100081China Center for Energy&Environmental Policy Research Beijing Institute of TechnologyBejing 100081China Key Laboratory of Jiangxi Province for Persistent Plutants Control and Resources Recycle Nanchang Hangkong UniversityNanchang 330063China Department of Civil and Environmental Engineering University of MichiganAnn ArborMI 48109United States

The COvID-19 pandemic has posed severe threats to global sustainable ***,a comprehensive quantitative assessment of the impacts of COVID-19 on Sustainable Development Goals(SDGs)is still *** research quantified the post-COVID-19 SDG progress from 2020 to 2024 using projected GDP growth and population and machine learning models including support vector machine,random forest,and extreme gradient *** results show that the overall SDG performance declined by 7.7%in 2020 at the global scale,with 12 socioeconomic SDG performance decreasing by 3.0%-22.3%and 4 environmental SDG performance increasing by 1.6%-9.2%.By 2024,the progress of 12 SDGs will lag behind for one to eight years compared to their pre-COVID-19 trajectories,while extra time will be gained for 4 environment-related ***,the pandemic will cause more impacts on countries in emerging markets and developing economies than those on advanced economies,and the latter will recover more quickly to be closer to their pre-covID-19 trajectories by ***-COVID-19 economic recovery should emphasize in areas that can help decouple economic growth from negative environmental *** results can help government and non-state stakeholders identify critical areas for targeted policy to resume and speed up the progress to achieve SDGs by 2030.

关键词： Sustainable development goals COVID-19 Machine learning Global development Sustainable development assessment

Real-Time 4-Mode MDM Transmission Using Commercial 400G OTN Transceivers and All-Fiber Mode Multiplexers

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

ZTE Communications 2024年第1期22卷 106-110页

作者： REN Fang LI Yidan YE Bing liu jianguo CHEN Weizhang School of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China Department of WDM System Design ZTE CorporationBeijing 100029China

Weakly-coupled mode division multiplexing(MDM)technique is considered a promising candidate to enhance the capacity of an optical transmission system,in which mode multiplexers/demultiplexers(MMUX/MDEMUX)with low insertion loss and modal crosstalk are the key *** this paper,a low-modal-crosstalk 4-mode MMUX/MDEMUX for the weakly-coupled triple-ring-core few-mode fiber(TRC-FMF)is designed and fabricated with side-polishing *** measurement results show that a pair of MMUX/MDEMUX and 25 km weakly-coupled TRC-FMF MDM link achieve low modal crosstalk of lower than−17.5 dB and insertion loss of lower than 11.56 dB for all the four *** on the TRC-FMF and all-fiber MMUX/MDEMUX,an experiment for 25 km real-time 4-mode 3-λwavelength division multiplexing(WDM)-MDM transmission is conducted using commercial 400G optical transport network(OTN)*** experimental results prove weakly-coupled MDM techniques facilitate a smooth upgrade of the optical transmission system.

关键词： optical fiber couplers mode(de)multiplexers mode division multiplexing transmission

人口高质量发展水平测度、空间分布与动态演进

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

统计与决策 2024年第17期40卷 64-69页

作者：刘建国李悦兰州财经大学经济学院兰州730020

为更好地对人口高质量发展水平开展定量分析,文章从4个维度选取13个指标,对我国30个省份2011—2021年的人口高质量发展水平进行测度。在此基础上,采用空间相关性分析、核密度估计以及Markov链对我国人口高质量发展水平的空间分布特征与... 详细信息

为更好地对人口高质量发展水平开展定量分析,文章从4个维度选取13个指标,对我国30个省份2011—2021年的人口高质量发展水平进行测度。在此基础上,采用空间相关性分析、核密度估计以及Markov链对我国人口高质量发展水平的空间分布特征与动态演进趋势进行分析。结果显示:(1)全国层面,我国人口高质量发展水平呈上升趋势,空间集聚特征明显。(2)区域层面,地区发展不均衡现象突出,东部地区的人口高质量发展水平始终高于全国水平,地区整体水平提升速度快、差距小;中部地区稳步提升,极化现象明显缓和;西部地区水平较低,区域差距扩大。(3)不同发展水平均具有一定的稳定性,但也存在变化的可能性;同时,邻近省份人口高质量发展水平的变化也会影响本省人口高质量发展水平的跃迁。

关键词：人口高质量发展空间相关性动态演进核密度估计 Markov链

同方期刊数据库

同方期刊数据库博看期刊评论

在线全文

学校读者我要写书评

暂无评论

连续流选择性加氢技术研究进展

有机化学 2024年第5期44卷 1445-1457页

作者：密思怡马隆龙刘建国东南大学-蒙纳士大学苏州联合研究生院江苏苏州215000 东南大学能源与环境学院南京210096

流动氢化技术是合成制备精细化学品的重要手段,在制备药物中间体及生产高值化学品方面占比极大.非均相催化氢化法具有优良的经济环保性,通过使用负载型催化剂能有效减少污染物排放,提高底物转化率以及选择性.详细介绍了按催化剂负载方... 详细信息

流动氢化技术是合成制备精细化学品的重要手段,在制备药物中间体及生产高值化学品方面占比极大.非均相催化氢化法具有优良的经济环保性,通过使用负载型催化剂能有效减少污染物排放,提高底物转化率以及选择性.详细介绍了按催化剂负载方式分类的微反应器类型以及常用的固体催化剂,阐述了连续流技术在不同官能团催化氢化领域中取得的进展.在此基础上概述了作为十大新兴化学技术之一的流动化学,在催化加氢应用上具有极大远景,连续、自动化和智能化技术是制药和化学工业的未来.

关键词：氢化多相催化流动化学微反应器

基于PR—Henry改进模型的酸性天然气——地层水体系及其相平衡特征分析

在线全文

学校读者我要写书评

暂无评论

天然气工业 2024年第6期44卷 64-73页

作者：杨宇王建猛张骞刘建国刘荣和江良伟成都理工大学能源学院中海石油(中国)有限公司海南分公司中海石油(中国)有限公司天津分公司中国石油集团川庆钻探工程有限公司地质勘探开发研究院

准确表征酸性天然气—地层水体系的相平衡规律,对于天然气开发过程中的水溶气量和凝析水量分析具有重要意义,但目前常用的PR状态方程与Henry定律等理论对酸性天然气—地层水体系的相平衡研究还存在不适用的问题。为进一步考虑酸性气体... 详细信息

准确表征酸性天然气—地层水体系的相平衡规律,对于天然气开发过程中的水溶气量和凝析水量分析具有重要意义,但目前常用的PR状态方程与Henry定律等理论对酸性天然气—地层水体系的相平衡研究还存在不适用的问题。为进一步考虑酸性气体和地层水矿化度对体系相平衡的影响,改进并提高对天然气溶解度和饱和含水量的计算精度,在PR状态方程与Henry定律相结合建立的PR—Henry模型基础上,考虑了溶解盐对体系相平衡的影响,采用定标粒子理论(SPT)修正了Henry常数,建立了改进的PR—Henry模型,最后分析了天然气组成、压力、温度和盐水含盐量对天然气溶解量和饱和含水量的影响。研究结果表明:(1)模型计算结果与实测资料对比,平均相对偏差分别为5.3%和4.55%,表明该模型能够应用于不同温度、压力和组成的酸性天然气-地层水体系的相平衡计算;(2)天然气在地层水中的溶解量受天然气组成、温度、压力和地层水含盐量的影响;(3)天然气饱和含水量受温度和压力影响十分明显。结论认为,改进的PR—Henry模型为天然气开采过程评价和CO_(2)埋存溶解量计算提供了一种有效的方法,对于评估天然气可采储量及开发特征具有重要的参考意义。

关键词：酸性天然气相平衡计算 PR—Henry模型定标粒子理论影响因素