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Progress in Natural Science:Materials International 2023年第5期33卷 569-574页

作者： Jing liu airong liu Yi Wei Jiahui Fu Wei-xian Zhang College of Environmental Science and Engineering Tongji University State Key Laboratory for Pollution Control and Resource Reuse

Antimony(Sb) and recalcitrant organic dyes often coexist in dyeing wastewater, and the simultaneous removal of Sb and dyes has been a challenge for traditional biological method in the treatment of Sb-dyeing *** zero-valent iron(n ZVI) is particularly suitable for separating heavy metals and enhancing the biodegradability of recalcitrant organic compounds. Herein, n ZVI is integrated with bioreactors(n ZVI-bio system) to achieve enhanced removal of Sb and degradation of Congo red(CR) in wastewater. The n ZVI-bio system achieves a reduction in Sb levels from 2.5 g L-1to 0.064 mg L-1, with a color removal efficiency of up to 98.60 % and a reduction in COD from 167 mg L-1to 55 mg L-1. The excellent performance is mainly attributed to n ZVI pretreatment, which removes Sb and degrades CR into smaller and more biodegradable organic compounds,providing favorable environmental conditions for the subsequent biotreatment system. This suggests that integrated n ZVI-bio system has potential for the treatment of complex wastewater containing heavy metals and recalcitrant organic dyes.

关键词： Nanoscale zero-valent iron Biotreatment Antimony Congo red nZVI-bio system

Nanoencapsulation of arsenate with nanoscale zero-valent iron(nZVI):A 3D perspective

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Science Bulletin 2018年第24期63卷 1641-1648页

作者： airong liu Wei Wang Jing liu Rongbing Fu Wei-xian Zhang State Key Laboratory for Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongii UniversityShanghai 200092China School of Chemical Sdence and Engineering Tongji UniversztyShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

The principal forces driving the efficient enrichment and encapsulation of arsenic(As) into nanoscale zero-valent iron(nZVI) are the disordered arrangement of the atoms and the gradient chemical potentials within the core-shell interface. The chemical compositions and the fine structure of nZVI are characterized with a combination of spherical aberration corrected scanning transmission electron microscopy(Cs-STEM), X-ray energy-dispersive spectroscopy(XEDS), electron energy loss spectroscopy(EELS), and high-resolution X-ray photoelectron spectroscopy(HR-XPS). Atomically resolved EELS at the oxygen K-edge unfolds that the Fe species in nZVI are well stratified from Fe(Ⅲ) oxides in the outermost periphery to a mixed Fe(Ⅲ)/Fe(Ⅱ) interlayer, then Fe(Ⅱ) oxide and the pure Fe(0) phase. Reactions between As(Ⅴ)and nZVI suggest that a well-structured local redox gradient exists within the shell layer, which serves as a thermodynamically favorable conduit for electron transfer from the iron core to the surface-bound As(Ⅴ). HR-XPS with ion sputtering shows that arsenic species shift from As(Ⅴ), As(Ⅲ)/As(Ⅴ) to As(Ⅴ)/As(Ⅲ)/As(0) from the iron oxide shell–water interface to the Fe(0) core. Results reinforce previous work on the efficacy of nZVI for removing and remediating arsenic while the analytical TEM methods are also applicable to the study of environmental interfaces and surface chemistry.

关键词： Arsenate Nanoscale zero-valent iron Spherical aberration corrected scanning transmission electron microscopy X-ray energy-dispersive spectroscopy Electron energy-loss spectroscopy X-ray photoelectron spectroscopy

A glucose biosensor based on direct electrochemistry of glucose oxidase immobilized onto platinum nanoparticles modified graphene electrode

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Science China(Physics,Mechanics & Astronomy) 2012年第7期55卷 1163-1167页

作者： liu airong HUANG ShiMing State Key Laboratory of Pollutton Control and Resources Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Department of Physics Tongji UniversityShanghai 200092China

The platinum nanoparticles were adsorbed on graphene oxide sheets and played an important role in catalytic reduction of graphene oxide with hydrazine, leading to the formation of graphene-Pt nanoparticles. Because of their good electronic properties, biocompatibility and high surface area, graphene-Pt based composites achieved the direct electron transfer of redox enzyme and maintained their bioactivity well. The graphene-Pt nanocomposites were characterized using X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), high-resolution transmission electron microscopy (HR-TEM) and selected area electron diffraction (SAED). The amperometric biosensor fabricated by depositing glucose oxidase over Nafion-solubilized graphene-Pt electrode retained its biocatalytic activity and has offered fast and sensitive glucose quantification.

关键词： platinum nanoparticle glucose oxidase graphene biosensor

General formulas for drag coefficient and settling velocity of sphere based on theoretical law

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International Journal of Mining Science and Technology 2015年第2期25卷 219-223页

作者： Yang Hongli Fan Minqiang liu airong Dong Lianping Department of Mineral Processing College of Mining EngineeringTaiyuan University of Technology

The settlement of particles is of great importance in many areas. The accurate determination of drag coefficient and settling velocity in wide Reynolds number （Re） range remains a problem. In this paper, a series of new formulas for drag coefficient of spherical particles based on theoretical laws, such as the Stokes law, the Oseen law, and the Goldstein law, were developed and fitted using 480 groups of experimental data （Re 〈 2 × 10^5）. The results show that the 2nd approximation of a rational function containing only one parameter can describe Co-Re relationship accurately over the whole Re range of 0-2× 10^5. The new developed formulas containing five parameters show higher goodness over wide Re range than presently existing equations. The introduction of the Oseen law is helpful for improving the fitting goodness of the empirical formulas. On the basis of one of the Oseen-based Co-Re formulas giving the lowest sum of squared relative errors Qover the whole Re range （Re 〈 2 × 10^5）, a general formula for settling velocity ut based on dimensionless parameters was proposed showing high goodness.

关键词： Sphere Drag coefficient Settling velocity Reynolds number Theoretical equation

Multifaceted Aquatic Environmental Differences between Nanoplastics and Microplastics:Behavior and Fate

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Environment & Health 2024年第10期2卷 688-701页

作者： Sheng Wang Noor Sulaiman AL-Hasni Zhaoli liu airong liu State Key Laboratory for Pollution Control School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

Microplastics and nanoplastics are emerging pollutants of concern in the aquatic environment that are causing increasing global environmental and human health *** there has been extensive research on microplastics and nanoplastics,little has been said about the differences in their behavior in the aquatic environment,and many studies have considered them as the same class of hazardous materials;but in fact,microplastics and nanoplastics should be considered as two different types of environmentally hazardous *** this review,we propose that microplastics and nanoplastics behave in the aquatic environment in a size-dependent manner and should be *** we systematically analyzed the differences in the behavior of microplastics and nanoplastics in the aquatic environment in terms of five aspects:1)distribution behavior;2)adsorption behavior;3)reaction with natural colloids;4)aging and leaching behavior;5)interaction with *** paper has been written to draw academic attention to the different behaviors of microplastics and nanoplastics in the aquatic environment in order to distinguish between their effects on humans and the environment.

关键词： Microplastics Nanoplastics Aquatic environmental behavior Differences

Novel SNPs in IL-17F and IL-17A genes associated with somatic cell count in Chinese Holstein and Inner-Mongolia Sanhe cattle

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Journal of Animal Science and Biotechnology 2017年第2期8卷 361-369页

作者： Tahir Usman Yachun Wang Chao liu Yanghua He Xiao Wang Yichun Dong Hongjun Wu airong liu Ying Yu Key Laboratory of Animal Genetics Breeding and Reproduction Ministry of Agriculture of China National Engineering Laboratory for Animal BreedingCollege of Animal Science and Technology China Agricultural UniversityBeijing 100193 People's Republic of China College of Veterinary Sciences and Animal Husbandry Abdul Wali Khan University MardanMardan 23200Pakistan. Xieerltala Breeding Farm Hailaer 021012 Inner Mongolia China. Agricultural and Animal Husbandry Administration Bureau Hailaer 021000Inner Mongolia China.

Background： Bovine mastitis is the most common and costly disease of lactating cattle worldwide. Apart from milk somatic cell count（SCC） and somatic cell score（SCS）, serum cytokines such as interleukin-17（IL-17） and interleukin-4（IL-4） may also be potential indicators for bovine mastitis. The present study was designed to investigate the effects of single nucleotide polymorphisms（SNPs） in bovine IL-17 F and IL-17 A genes on SCC, SCS and serum cytokines in Chinese Holstein and Inner-Mongolia Sanhe cattle, and to compare the m RNA expression variations of the cows with different ***： A total of 464 lactating cows（337 Holstein and 127 Inner-Mongolia Sanhe cattle） were screened for SNPs identification and the data were analyzed using fixed effects of herd, parity, season and year of calving by general linear model procedure. The results revealed that SNP g.24392436 C ＆gt; T in IL-17 F and SNP g.24345410 A ＆gt; G in IL-17 A showed significant effects on SCC and IL-4 in Holstein（n = 337） and on IL-17 and IL-4 in Sanhe cattle（n = 127）. The homozygous GG genotype of SNP g.24345410 A ＆gt; G had significantly higher m RNA expression compared with the heterozygous AG ***： The results indicate that IL-17 F and IL-17 A could be powerful candidate genes of mastitis resistance and the significant SNPs might be useful genetic markers against mastitis in both dairy and dual purpose cattle.

关键词： Chinese Holstein Inner Mongolia Sanhe cattle Interleukin 17A Interleukin 17F Mastitis susceptibility

Effects of Hypoxia Stress and Different Level of Mn2+ on Antioxidant Enzyme of Tomato Seedlings

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American Journal of Plant Sciences 2010年第1期1卷 24-31页

作者： airong liu Shuangchen Chen Yinfa Mi Zhou Zhou Golam Jalal Ahammed 不详

The changes of antioxidant enzyme activities and related genes expression of tomato seedlings were evaluated under hypoxia stress with different levels of Mn2+. Activities of superoxide dismutase (SOD), peroxidase (POD), ascorbate peroxide (APX), glutathione reductase (GR), catalase (CAT), the contents of H2O2, ascorbic (AsA) and malondialdehyde (MDA) were studied to investigate how active oxygen damaged the membrane lipid under hypoxia stress. With 10-200 μmol?L-1 Mn2+, the activities of SOD, POD, APX, GR and the contents of H2O2, AsA, MDA of leaves and roots increased significantly, which indicated that low Mn2+ could eliminate the active oxygen and protect the membrane lipid from hurt. But the activities of catalase (CAT) decreased evidently in the root. When the concentration of Mn2+ reached 400-600 μmol?L-1 under hypoxia stress, the activities of SOD, POD, APX, GR and ASA content decreased remarkably. However, the contents of H2O2 and MDA increased contrarily. A series of resistance genes level achieved peak value with 10 μmol?L-1 Mn2+. The expression level of SOD, CAT, APX, POD, GR were 6.28, 2.19, 5.66, 5.21 and 6.79 times compared to control respectively. These results illustrated appropriate amount of Mn2+ could reduce the damage of active oxygen under hypoxia stress, but reversely, high level of Mn2+ just aggravated the already serious damage to the tomato seedlings.

关键词： Tomato Hypoxia Stress Mn2+ Antioxidant Enzyme

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煤用微乳液助滤剂的研制

煤炭转化 2007年第2期30卷 45-47页

作者：刘爱荣太原理工大学矿业工程学院太原助教030024

以表面活性剂SLL(自制乳化剂)及SLL和Span85复配物为乳化剂,醇为助乳化剂,煤油为分散介质,研究了制备丙烯酰胺反相微乳液的条件,并在水溶性引发剂的引发下进行了微乳液聚合.用聚合后的体系对6种不同变质程度的煤进行了煤泥真空过滤脱水... 详细信息

以表面活性剂SLL(自制乳化剂)及SLL和Span85复配物为乳化剂,醇为助乳化剂,煤油为分散介质,研究了制备丙烯酰胺反相微乳液的条件,并在水溶性引发剂的引发下进行了微乳液聚合.用聚合后的体系对6种不同变质程度的煤进行了煤泥真空过滤脱水实验,实验结果表明,经聚合得到的复合体对六种煤泥都具有很好的助滤脱水效果.

关键词：微乳液乳化剂微乳液聚合助滤剂过滤

石墨烯基金属氧化物纳米复合结构材料的制备及应用于水体中污染物的吸附研究进展

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科学通报 2014年第21期59卷 2039-2054页

作者：刘爱荣周文同济大学环境科学与工程学院污染控制与资源化研究国家重点实验室上海200092

石墨烯及氧化石墨烯材料具有良好的物理化学性质、巨大的比表面积,使其适合成为水处理中的吸附剂用于污染物的去除.石墨烯基金属氧化物纳米材料,兼具石墨烯和金属氧化物纳米粒子的固有特性,金属氧化物纳米粒子的存在不但阻止石墨烯的团... 详细信息

石墨烯及氧化石墨烯材料具有良好的物理化学性质、巨大的比表面积,使其适合成为水处理中的吸附剂用于污染物的去除.石墨烯基金属氧化物纳米材料,兼具石墨烯和金属氧化物纳米粒子的固有特性,金属氧化物纳米粒子的存在不但阻止石墨烯的团聚,石墨烯基材料也进一步防止了纳米粒子的凝聚,两者共存产生协同效应,使复合材料具有更大的比表面积和吸附效能用于污染物的去除.本文综述了用于环境中污染物去除的石墨烯基金属氧化物的种类、不同复合材料的性能以及复合材料对水体中重金属离子、有机污染物的吸附性能等,探讨污染物去除机理,并进一步展望适合于不同种类污染物去除的石墨烯基金属氧化物的结构性能特点.

关键词：金属氧化物石墨烯石墨烯氧化物纳米复合结构吸附剂

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一种放大位移型SMA阻尼器的减震控制分析

地震工程与工程振动 2008年第5期28卷 151-156页

作者：禹奇才刘春晖刘爱荣广州大学土木工程学院广东广州510006

利用形状记忆合金(SMA)材料的超弹性,本文提出了一种放大位移型SMA阻尼器,建立了装有该阻尼器的框架有限元模型并对该框架的地震反应实施了模拟减震控制。分不安装阻尼器、安装不放大位移阻尼器和安装放大2倍层间位移阻尼器三种工况,输... 详细信息

利用形状记忆合金(SMA)材料的超弹性,本文提出了一种放大位移型SMA阻尼器,建立了装有该阻尼器的框架有限元模型并对该框架的地震反应实施了模拟减震控制。分不安装阻尼器、安装不放大位移阻尼器和安装放大2倍层间位移阻尼器三种工况,输入El Centro和Taft地震动,对比研究了阻尼器的减震控制效果。分析结果表明:(1)放大位移型SMA阻尼器的控制效果优于不放大位移型SMA阻尼器;(2)该放大位移型SMA阻尼器对位移的控制效果优于对加速度的控制效果。

关键词：形状记忆合金阻尼器结构减震控制