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Achieving Negatively Charged Pt Single Atoms on Amorphous Ni(OH)_(2)Nanosheets with Promoted Hydrogen Absorption in Hydrogen Evolution

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Nano-Micro Letters 2024年第10期16卷 213-224页

作者： Yue liu Gui liu Xiangyu Chen Chuang Xue Mingke Sun Yifei liu Jianxin Kang Xiujuan Sun Lin Guo School of Chemistry Beijing Advanced Innovation Center for Biomedical EngineeringKey Laboratory of Bio-inspired Smart Interfacial Science and TechnologyBeihang UniversityBeijing 100191People's Republic of China School of Chemistry Key Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of EducationXiangtan UniversityXiangtan 411105HunanPeople'Republic of China

Single-atom(SA)catalysts with nearly 100%atom utilization have been widely employed in electrolysis for decades,due to the outperforming catalytic activity and ***,most of the reported SA catalysts are fixed through the strong bonding between the dispersed single metallic atoms with nonmetallic atoms of the substrates,which greatly limits the controllable regulation of electrocatalytic activity of SA *** this work,Pt-Ni bonded Pt SA catalyst with adjustable electronic states was successfully constructed through a controllable electrochemical reduction on the coordination unsaturated amorphous Ni(OH)_(2)nanosheet *** on the X-ray absorption fine structure analysis and first-principles calculations,Pt SA was bonded with Ni sites of amorphous Ni(OH)_(2),rather than conventional O sites,resulting in negatively charged Pt^(δ-).In situ Raman spectroscopy revealed that the changed configuration and electronic states greatly enhanced absorbability for activated hydrogen atoms,which were the essential intermediate for alkaline hydrogen evolution *** hydrogen spillover process was revealed from amorphous Ni(OH)_(2)that effectively cleave the H-O-H bond of H_(2)O and produce H atom to the Pt SA sites,leading to a low overpotential of 48 mV in alkaline electrolyte at-1000 mA cm^(-2)mg^(-1)_(Pt),evidently better than commercial Pt/C *** work provided new strategy for the control-lable modulation of the local structure of SA catalysts and the systematic regulation of the electronic states.

关键词： Hydrogen evolution reaction Amorphous Pt single atoms Hydrogen spillover

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Single image super-resolution:a comprehensive review and recent insight

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Frontiers of Computer Science 2024年第1期18卷 139-156页

作者： Hanadi AL-MEKHLAFI Shiguang liu College of Intelligence and Computing Tianjin UniversityTianjin 300350China

Super-resolution(SR)is a long-standing problem in image processing and computer vision and has attracted great attention from researchers over the *** main concept of SR is to reconstruct images from low-resolution(LR)to high-resolution(HR).It is an ongoing process in image technology,through up-sampling,de-blurring,and *** neural network(CNN)has been widely used to enhance the resolution of images in recent *** alternative methods use deep learning to improve the progress of image super-resolution based on ***,we review the recent findings of single image super-resolution using deep learning with an emphasis on distillation knowledge used to enhance image super-resolution.,it is also to highlight the potential applications of image super-resolution in security monitoring,medical diagnosis,microscopy image processing,satellite remote sensing,communication transmission,the digital multimedia industry and video ***,we present the challenges and assess future trends in super-resolution based on deep learning.

关键词： super-resolution deep learning single-image interpolation-based learning-based reconstruction-based

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A short review of antibacterial Cu-bearing stainless steel:antibacterial mechanisms,corrosion resistance,and novel preparation techniques

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Journal of Iron and Steel Research(International) 2024年第1期31卷 24-45页

作者： Shuai liu Han-jie Guo School of Artificial Intelligence Beijing Technology and Business UniversityBeijing100048China Beijing Key Laboratory of Special Melting and Preparation of High-End Metal Materials University of Science and Technology BeijingBeijing100083China

Cu-bearing stainless steel is widely used in the fields of food,medical and household sanitary equipment because of its surface finish and corrosion ***,the growth of bacteria on stainless steel leads to the formation of biofilms,which causes ***,the antibacterial property of stainless steel is a worthy research *** of breakthroughs in the field of corrosion resistance and antimicrobial properties are still ***,due to the scarcity of publications on the antibacterial mechanisms and processing methods of antibacterial Cu-bearing stainless steel,we review the current state of relevant research and *** toxicity of Cu,corrosion resistance mechanism of stainless steel,and antibacterial mechanism and preparation method of antibacterial stainless steel are *** addition,alloying,surface modification and other methods are found to have limitations in balancing the toxicity and antibacterial properties of copper and the relationship between the antibacterial properties and corrosion resistance of Cu-bearing stainless steel.A new preparation method of antibacterial stainless steel associated with selective laser melting(SLM)is *** is becoming a powerful additive manufacturing technology that can be used to manufacture customized and complex *** research status of SLM applied in antibacterial stainless steel preparation is ***,the future research direction of Cu-bearing antibacterial stainless steel is discussed.

关键词： Cu-bearing stainless steel Antibacterial Processing Additive manufacturing Corrosion resistance

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Graphene reinforced nanoarchitectonics of 3D interconnected magnetic-dielectric frameworks for high-efficient and anti-corrosive microwave absorbers

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Journal of Materials Science & Technology 2024年第1期168卷 194-207页

作者： Chenchen liu Xiaofang Feng Shuning liu Guo Lin Zhongxiang Bai Lingling Wang Ke Zhu Xiulan Li Xiaobo liu School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu611731China Sichuan Province Engineering Technology Research Center of Novel CN Polymeric Materials Chengdu611731China School of Chemical Engineering Northwest UniversityXi’an710069China Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-sen UniversityGuangzhou510275China

The combination of high efficiency and environmental stability is vital to promote the commercial appli-cations of microwave absorption(MA)materials,yet remains challenging in the absence of facile ***,we put forward a graphene-reinforced construct approach for one-pot synthesis of 3D intercon-nected magnetic-dielectric frameworks via pre-functionalization and subsequent *** in-teractions among discrete precursors are capable of manipulating the confined growth and interfacial *** enhancements in MA properties are triggered in a straightforward manner us-ing ultralow feeding fractions of graphene oxide *** minimum reflection loss is up to-60.1 dB(99.9999%wave absorption)and the effective absorption bandwidth reaches 5.9 GHz(almost covering the Ku band).Remarkably,based on the optimization by ultralow concentrations of graphene,the as-prepared nanoarchitecture simultaneously integrates strong absorption,broad bandwidth,and low matching *** embedded graphene nanosheets serve as high-speed electron transmission channels and hollow resonance cavities,facilitating multimode attenuations and impedance-matching ***-while,the graphene-reinforced framework suppresses the corrosion of magnetic components,whose cor-rosion rate reduces by an order of *** study provides a simple procedure to boost magnetic-dielectric absorbers for comprehensive MA performances and enhanced corrosion resistance.

关键词： 3D Magnetic-dielectric framework Graphene nanosheet Microwave absorption Anti-corrosion

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A novel silver-doped nickel oxide hole-selective contact for crystalline silicon heterojunction solar cells

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 93-101页

作者： Junfeng Zhao Xudong Yang Zhongqing Zhang Shengpeng Xie Fangfang liu Anjun Han Zhengxin liu Yun Sun Wei liu Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin Engineering Research Center of Thin Film Photoelectronic TechnologyInstitute of Photoelectronic Thin Film Devices and Technology of Nankai University(Ministry of Education)Tianjin 300350China Shanghai Institute of Microsystem and Information Technology Chinese Academy of SciencesShanghai 201800China

Based on its band alignment,p-type nickel oxide(NiO_(x))is an excellent candidate material for hole transport layers in crystalline silicon heterojunction solar cells,as it has a smallΔEV and largeΔEC with crystalline ***,to overcome the poor hole selectivity of stoichiometric NiO_(x) due to its low carrier concentration and conductivity,silver-doped nickel oxide(NiO_(x):Ag)hole transport layers with high carrier concentrations were prepared by co-sputtering high-purity silver sheets and pure NiO_(x) *** improved electrical conductivity of NiO_(x) was attributed to the holes generated by the Ag^(+)substituents for Ni^(2+),and moreover,the introduction of Ag^(+)also increased the amount of Ni^(3+)present,both of which increased the carrier concentration in NiO_(x).Ag^(+)doping also reduced the c-Si/NiO_(x) contact resistivity and improved the hole-selective contact with NiO_(x).Furthermore,the problems of particle clusters and interfacial defects on the surfaces of NiO_(x):Ag films were solved by UV-ozone oxidation and high-temperature annealing,which facilitated separation and transport of carriers at the c-Si/NiO_(x) *** constructed c-Si/NiO_(x):Ag solar cell exhibited an increase in open-circuit voltage from 490 to 596 mV and achieved a conversion efficiency of 14.4%.

关键词： band alignment nickel oxide hole transport layer silver-doped nickel oxide UV-ozone

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Skill enhancement learning with knowledge distillation

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Science China(Information Sciences) 2024年第8期67卷 206-220页

作者： Naijun liu Fuchun SUN Bin FANG Huaping liu Department of Computer Science and Technology Tsinghua University

Skill learning through reinforcement learning has significantly progressed in recent years. However, it often struggles to efficiently find optimal or near-optimal policies due to the inherent trial-and-error exploration in reinforcement learning. Although algorithms have been proposed to enhance skill learning efficacy, there is still much room for improvement in terms of skill learning performance and training stability. In this paper, we propose an algorithm called skill enhancement learning with knowledge distillation(SELKD), which integrates multiple actors and multiple critics for skill learning. SELKD employs knowledge distillation to establish a mutual learning mechanism among actors. To mitigate critic overestimation bias,we introduce a novel target value calculation method. We also perform theoretical analysis to ensure the convergence of SELKD. Finally, experiments are conducted on several continuous control tasks, illustrating the effectiveness of the proposed algorithm.

关键词： skill learning enhancement learning reinforcement learning knowledge distillation

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A stable staggered-grid finite-difference scheme for acoustic modeling beyond conventional stability limit

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Petroleum Science 2024年第1期21卷 182-194页

作者： Jing-Yi Xu Yang liu National Key Laboratory of Petroleum Resources and Engineering China University of Petroleum(Beijing)Beijing 102249China China University of Petroleum(Beijing) Karamay CampusKaramay 834000XinjiangChina

Staggered-grid finite-difference(SGFD)schemes have been widely used in acoustic wave modeling for geophysical *** improved methods are proposed to enhance the accuracy of numerical ***,these methods are inevitably limited by the maximum Courant-Friedrichs-Lewy(CFL)numbers,making them unstable when modeling with large time sampling intervals or small grid *** solve this problem,we extend a stable SGFD scheme by controlling SGFD dispersion relations and maximizing the maximum CFL ***,to improve modeling stability,we minimize the error between the FD dispersion relation and the exact relation in the given wave-number region,and make the FD dispersion approach a given function outside the given wave-number area,thus breaking the conventional limits of the maximum CFL ***,to obtain high modeling accuracy,we use the SGFD scheme based on the Remez algorithm to compute the FD *** addition,the hybrid absorbing boundary condition is adopted to suppress boundary reflections and we find a suitable weighting coefficient for the proposed *** derivation and numerical modeling demonstrate that the proposed scheme can maintain high accuracy in the modeling process and the value of the maximum CFL number of the proposed scheme can exceed that of the conventional SGFD scheme when adopting a small maximum effective wavenumber,indicating that the proposed scheme improves stability during the modeling.

关键词： Acoustic wave Staggered-grid finite-difference(SGFD) modeling Courant-friedrichs-lewy(CFL)number Stability

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A compact bimorph rotary piezoelectric actuator with customized small power supply

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Science China(Technological Sciences) 2024年第4期67卷 1185-1195页

作者： DENG Jie liu DaQing WANG WeiYi liu YingXiang School of Mechatronics and Engineering Harbin Institute of TechnologyHarbin 150001China

Inertial piezoelectric actuators are widely applied in precision devices with simple structure and accurate ***,existing inertial piezoelectric actuators still face the challenges of rollback motion and bulky power *** this work,an alternate excitation strategy and a customized small power supply for a bimorph rotary piezoelectric actuator(BRPA)are proposed to solve the *** BRPA prototype is designed with a bipedal symmetrical structure,measuring 35 mm in height and 32 mm in diameter,which has a maximum rotation velocity of 0.247 rad/s and a resolution of 0.66μ*** to the bipedal symmetrical structure,the friction directions between the driving feet and the rotor can be coordinated to suppress the *** rollback ratio is almost zero when the phase difference of the exciting signal is set as 180°.The customized power supply is designed and manufactured,whose size is 58 mm×56 mm×46 *** can output signals for the single step mode and the continuous mode,and they are adopted to excite BRPA to achieve a small stroke with one single step and a large stroke with continuous step,***,an experimental system for optical fiber alignment is developed based on the BRPA and the customized small power supply,the experiment has verified the practicability of this work in the precision fields,especially in the miniaturized precision systems.

关键词： inertial piezoelectric actuator customized small power supply single step mode continuous mode rollback suppression miniaturized precision system

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Data-driven evacuation and rescue traffic optimization with rescue contraflow control

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Journal of Safety Science and Resilience 2024年第1期5卷 1-12页

作者： Zheng liu Jialin liu Xuecheng Shang Xingang Li School of Management Engineering Zhengzhou University of AeronauticsZhengzhou 450046China Collaborative Innovation Center for Aviation Economy Development of Henan Province Zhengzhou University of AeronauticsZhengzhou 450046China School of Systems science Beijing Jiaotong UniversityBeijing 100044China Key Laboratory of Transport Industry of Big Data Application Technologies for Comprehensive Transport Beijing Jiaotong UniversityBeijing 100044China School of Transportation Engineering Shandong Jianzhu UniversityJinan 250101China

In response to local sudden disasters,e.g.,high-rise office or residential building fire disasters,road occupation can cause conflicts,and traffic directions may be opposite between evacuation vehicles and rescue vehicles;moreover,lane contraflow can be adopted to meet these surge traffic ***,lane contraflow that provides more roads for rescue vehicles reduces the traffic supply in the evacuation *** is unclear how to control the number of contraflow roads used by rescue vehicles to coordinate evacuation and rescue traffic ***,we adjust the critical rescue traffic volume of reversing the normal road traffic direction to control rescue ***,we propose a multiobjective mixed integer linear programming formulation for evacuation and rescue traffic ***,considering that the upper limit of the critical rescue traffic volume is unknown and that the proposed formulation includes multiple objectives and multi-priority vehicle classes,a three-stage solving algorithm is ***,a large-scale evacuation and rescue traffic optimization result dataset is obtained for the Nguyen–Dupuis road network,and the impact of different rescue contraflow control plans on evacuation and rescue traffic is studied based on data-driven sta-tistical *** results show that by adjusting the optimal rescue traffic route,the critical rescue traffic volume for reversing the normal road traffic direction can reduce the interference of rescue traffic to evacuation traffic operation performance without reducing rescue traffic operation performance,and can be used to coor-dinate evacuation and rescue traffic operation under rescue contraflow.

关键词： Evacuation and rescue traffic optimization Rescue contraflow control Multiobjective mixed integer linear programming Three-stage solving algorithm Data-driven statistical analysis

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Deep Global Multiple-Scale and Local Patches Attention Dual-Branch Network for Pose-Invariant Facial Expression Recognition

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Computer Modeling in Engineering & Sciences 2024年第4期139卷 405-440页

作者： Chaoji liu Xingqiao liu Chong Chen Kang Zhou School of Electrical and Information Engineering Jiangsu UniversityZhenjiang212013China School of Electrical Engineering Yancheng Institute of TechnologyYancheng224051China

Pose-invariant facial expression recognition(FER)is an active but challenging research topic in computer *** with the involvement of diverse observation angles,FER makes the training parameter models inconsistent from one view to *** study develops a deep global multiple-scale and local patches attention(GMS-LPA)dual-branch network for pose-invariant FER to weaken the influence of pose variation and selfocclusion on recognition *** this research,the designed GMS-LPA network contains four main parts,i.e.,the feature extraction module,the global multiple-scale(GMS)module,the local patches attention(LPA)module,and the model-level fusion *** feature extraction module is designed to extract and normalize texture information to the same *** GMS model can extract deep global features with different receptive fields,releasing the sensitivity of deeper convolution layers to pose-variant and *** LPA module is built to force the network to focus on local salient features,which can lower the effect of pose variation and self-occlusion on recognition ***,the extracted features are fused with a model-level strategy to improve recognition *** experimentswere conducted on four public databases,and the recognition results demonstrated the feasibility and validity of the proposed methods.

关键词： Pose-invariant FER global multiple-scale(GMS) local patches attention(LPA) model-level fusion

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