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Thiazoloisoindigo-based Polymer Semiconductors: Synthesis,Structure-Property Relationship, Charge Carrier Polarity, and Field-Effect Transistor Performance

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Chinese Journal of Polymer Science 2024年第1期42卷 24-31,I0006页

作者： Bo-Wen Li Miao Xiong Mei-hua liu Zhi-Gao Li Long Sang Zi-Han Xiong Biao Xiao Jian Pei Xiao-Bo Wan Key Laboratory of Optoelectronic Chemical Materials and Devices Ministry of EducationSchoolofOptoelectronic Materials&TechnologyJianghan UniversityWuhan430056China Bejing National Laboratoryfor Molecular Sciences the Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Developing new polymeric semiconductors with excellent device performance is essential for organic electronics. Herein, we synthesized two new thiazoloisoindigo(Tz II)-based polymers, namely, P(Tz II-d Th-d Th) and P(Tz II-d Th-d Tz), by copolymerizing thiophene-flanked Tz II with bithiophene and bithiazole, respectively. Owing to the more electron-deficient nature of bithiazole than bithiophene, P(Tz II-d Th-d Tz)possesses deeper LUMO/HOMO levels of-3.45/-5.47 e V than P(Tz II-d Th-d Th)(-3.34/-5.32 e V). The organic field-effect transistor(OFET) devices based on P(Tz II-d Th-d Th) exhibited p-type behaviors with an average hole mobility value as high as 1.43 cm^(2)·V^(-1)·s^(-1), while P(Tz II-d Th-d Tz)showed typical ambipolar characteristics with average hole and electron mobilities of 0.38 and 0.56 cm^(2)·V^(-1)·s^(-1). In addition, we compared the performances of both polymers with other Tz II-based polymers reported in our previous work, and showed that the charge carrier polarity can be manipulated by adjusting the number of the thiophene units between the acceptor unit. As the increase of the number of thiophene rings,charge carrier polarity shifts from electron-dominated ambipolar transport to hole-dominated ambipolar transport and then to unipolar hole transport in OFETs, which provides an effective molecular design strategy for further optimization of polymer OFET performance.

关键词： Field-effect transistor Charge carrier polarity Thiazoloisoindigo

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Fine-mapping of a candidate gene for web blotch resistance in Arachis hypogaea L.

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Journal of Integrative Agriculture 2024年第5期23卷 1494-1506页

作者： Xiaohui Wu Mengyuan Zhang Zheng Zheng Ziqi Sun Feiyan Qi hua liu Juan Wang Mengmeng Wang Ruifang Zhao Yue Wu Xiao Wang Hongfei liu Wenzhao Dong Xinyou Zhang College of Agronomy Henan Agricultural UniversityZhengzhou 450046China Henan Academy of Agricultural Sciences/Henan Academy of Crop Molecular Breeding/Key Laboratory of Oil Crops in huang-huai-Hai Plain Ministry of Agriculture and Rural Affairs/Henan Provincial Key Laboratory for Oil Crop ImprovementZhengzhou 450002China The Shennong Laboratory Zhengzhou 450002China Shangqiu Academy of Agricultural and Forestry Sciences Shangqiu 476000China

Peanut(Arachis hypogaea L.)is a globally important oil *** blotch is one of the most important foliar diseases affecting peanut,which results in serious yield losses *** web blotch-resistant peanut varieties is the most effective and economically viable method for minimizing yield losses due to web *** the current study,a bulked segregant analysis with next-generation sequencing was used to analyze an F2:3 segregating population and identify candidate loci related to web blotch *** on the fine-mapping of the candidate genomic interval using kompetitive allele-specific PCR(KASP)markers,we identified a novel web blotch resistance-related locus spanning approximately 169 kb on chromosome *** region included four annotated genes,of which only Arahy.35VVQ3 had a non-synonymous single nucleotide polymorphism in the coding region between the two *** markers(Chr.16.12872635 and Chr.16.12966357)linked to this gene were shown to be co-segregated with the resistance of peanut web blotch by 72 randomly selected recombinant inbred lines(RIL),which could be used in marker-assisted breeding of resistant peanut varieties.

关键词： peanut web blotch bulked segregant analysis KAsP markers resistant gene

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Construction of wavelength-tunable DSE quinoline salt derivatives by regulating the hybridization form of the nitrogen atom and intramolecular torsion angle

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Chinese Chemical Letters 2024年第10期35卷 315-320页

作者： Kuan Deng Fei Yang Zhi-Qi Cheng Bi-Wen Ren hua liu Jiao Chen Meng-Yao She Le Yu Xiao-Gang liu Hai-Tao Feng Jian-Li Li Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education Shaanxi Key Laboratory for Carbon Neutral TechnologyCollege of Chemistry&Materials ScienceNorthwest UniversityXi'an710127China Key Laboratory of Resource Biology and Biotechnology in Western China Ministry of EducationBiomedicine Key Laboratory of Shaanxi ProvinceLab of Tissue Engineeringthe College of Life SciencesFaculty of Life Science&MedicineNorthwest UniversityXi'an 710069China Fluorescence Research Group Singapore University of Technology and DesignSingapore 487372Singapore Baoji AIE Research Center Shaanxi Key Laboratory of PhytochemistryCollege of Chemistry and Chemical EngineeringBaoji University of Arts and SciencesBaoji721013China

Dual-state emission(DSE)molecules displayed conspicuous fluorescent performance both in solid and solution ***,the construction of DSE molecules and the regulation of their emission wavelengths remains a great *** on the structure-function relationship of quinolinonitrile-type fluorophores,this work proposed a feasible strategy for modulating their fluorescent properties into DSE via limiting the torsion angle between the quinoline ring and C=C bond in the range of 4.7°to 30°.Based on this strategy,53 compounds were obtained which displayed tunable emission wavelengths from^(3)97 nm to 740 nm in solid-state and from 360 nm to 672 nm in *** feasibility of the strategy was supported by a series of theoretical calculations,optical characterizations,and crystal analysis,suggesting the compounds have great potential in imaging living cells and tissues with desired wavelengths.

关键词： Fluorescence Dual-state emission Structure-function relationship Wavelength regulation Fluorescent imaging

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Moyamoya syndrome may result from psoriasis: Four case reports

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World Journal of Clinical Cases 2024年第10期12卷 1830-1836页

作者： Zhi-Ying Chen Xiao-Qin Yu Yuan-Yuan Xiang Ling-hua liu Xiao-Ping Yin Department of Neurology The Affiliated Hospital of Jiujiang UniversityJiujiang 332000Jiangxi ProvinceChina Department of Dermatology The Affiliated Hospital of Jiujiang UniversityJiujiang 332000Jiangxi ProvinceChina

BACKGROUND Moyamoya syndrome(MMS)is a group of diseases that involves more than one underlying disease and is accompanied by moyamoya vascular *** is a chronic immune skin disease closely linked to high blood pressure and heart ***,psoriasis-related MMS has not been *** SUMMARY We collected data on patients with stroke due to MMS between January 2017 and December 2019 and identified four cases of *** histories,imaging,and hematological data were *** average age of the initial stroke onset was 58.25±11.52 years;three cases of hemorrhagic and one case of ischemic stroke were *** average duration from psoriasis confirmation to the initial MMS-mediated stroke onset was 17±3.56 *** MMS-related stenoses involved the bilateral cerebral arteries:Suzuki grade III in one case,grade IV in two cases,and grade V in one *** elevated plasma interleukin-6 levels were observed in four *** patients had abnormally elevated immunoglobulin E levels,and two had *** four patients received medication instead of *** an average follow-up time of 2 years,two causing transient ischemic attacks occurred in two patients,and no hemorrhagic events *** Psoriasis may be a potential risk factor for *** with psoriasis should be screened for MMS when they present with neurological symptoms.

关键词： Moyamoya syndrome Psoriasis Stroke Interleukin-6 Immune Hypertension Case report

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Analysis of the potential biological value of pyruvate dehydrogenase E1 subunitβin human cancer

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World Journal of Gastrointestinal Oncology 2024年第1期16卷 144-181页

作者： Yao Rong Song-hua liu Ming-Zheng Tang Zhi-Hang Wu Guo-Rong Ma Xiao-Feng Li Hui Cai First Clinical Medical College Gansu University of Chinese MedicineLanzhou 730000Gansu ProvinceChina General Surgery Clinical Medical Center Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina Key Laboratory of Molecular Diagnostics and Precision Medicine for Surgical Oncology in Gansu Province Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina NHC Key Laboratory of Diagnosis and Therapy of Gastrointestinal Tumor Gansu Provincial HospitalLanzhou 730000Gansu ProvinceChina

BACKGROUND The pyruvate dehydrogenase E1 subunitβ(PDHB)gene which regulates energy metabolism is located in ***,few studies have elucidated the role and mechanism of PDHB in different *** To comprehensive pan-cancer analysis of PDHB was performed based on bioinformatics approaches to explore its tumor diagnostic and prognostic value and tumor immune relevance in *** vitro experiments were performed to examine the biological regulation of PDHB in liver *** Pan-cancer data related to PDHB were obtained from the Cancer Genome Atlas(TCGA)*** of the gene expression profiles of PDHB was based on TCGA and Genotype Tissue Expression Dataset *** regression analysis and Kaplan-Meier methods were used to assess the correlation between PDHB expression and survival prognosis in cancer *** correlation between PDHB and receiver operating characteristic diagnostic curve,clinicopathological staging,somatic mutation,tumor mutation burden(TMB),microsatellite instability(MSI),DNA methylation,and drug susceptibility in pan-cancer was also *** algorithms were used to analyze the correlation between PDHB and immune cell infiltration and tumor chemotaxis environment,as well as the co-expression analysis of PDHB and immune checkpoint(ICP)*** expression and functional phenotype of PDHB in single tumor cells were studied by single-cell sequencing,and the functional enrichment analysis of PDHB-related genes was *** study also validated the level of mRNA or protein expression of PDHB in several ***,in vitro experiments verified the regulatory effect of PDHB on the proliferation,migration,and invasion of liver *** PDHB was significantly and differently expressed in most *** was significantly associated with prognosis in patients with a wide range of cancers,including kidney renal clear cell carcinoma,kidney renal papillary cell carcinoma,breast invasive carcinom

关键词： Cuprotosis Pyruvate dehydrogenase E1 subunitβ Pan-cancer Prognosis Liver cancer

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Role of hsa_circ_0007482 in pterygium development: insights into proliferation, apoptosis, and clinical correlations

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International Journal of Ophthalmology(English edition) 2024年第8期17卷 1387-1395页

作者： Li-Yun Zhang Xin liu Shuo Zheng Wen-Qun Xi Xue-Ping Wu Dan-Yao Nie Hui-Ling Hu Jian-Tao Wang Xin-hua liu Jing Zhang Shenzhen Eye Hospital Jinan UniversityShenzhen Eye InstituteShenzhen 518000Guangdong ProvinceChina

AIM:To investigate the impact of hsa_circ_0007482 on the proliferation and apoptosis of human pterygium fibroblasts(HPFs)and its correlation with the severity grades of ***:Pterygium and normal conjunctival tissues were collected from the superior area of the same patient’s eye(n=33).The correlation between pterygium severity and hsa_circ_0007482 expression using quantitative reversetranscription polymerase chain reaction(RT-qPCR)were *** distinct siRNA sequences targeting hsa_circ_0007482,along with a negative control sequence,were transfected into *** proliferation was assessed using the cell counting *** levels of Ki67,proliferating cell nuclear antigen(PCNA),Cyclin D1,Bax,B-cell lymphoma-2(Bcl-2),and Caspase-3 were measured via *** staining was employed to detect Ki67 and vimentin *** was evaluated using flow ***:Hsa_circ_0007482 expression was significantly higher in pterygium tissues compared to normal conjunctival tissues(P<0.001).Positive correlations were observed between hsa_circ_0007482 expression and pterygium severity,thickness,and vascular *** of hsa_circ_0007482 inhibited cell proliferation,reducing the mRNA expression of Ki67,PCNA,and Cyclin D1 in ***_circ_0007482 knockdown induced apoptosis,increasing mRNA expression levels of Bax and Caspase-3,while decreasing Bcl-2 expression in ***,hsa_circ_0007482 knockdown attenuated vimentin expression in ***:The downregulation of hsa_circ_0007482 effectively hampers cell proliferation and triggers apoptosis in *** are discernible positive correlations detected between the expression of hsa_circ_0007482 and the severity of pterygium.

关键词： hsa_circ_0007482 circular RNA pterygium cell proliferation apoptosis

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Binder-induced ultrafast ■-intercalation toward a high-voltage,high-power and long-cycling zinc–graphite dual-ion battery

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Rare Metals 2024年第10期43卷 5017-5029页

作者： Gen Li Xiao-Jun Shi Ting Dong Qian Yu Zhi-Fei Mao Xin-hua liu Rui Wang Bei-Bei He Jun Jin Yan-Sheng Gong huan-Wen Wang Engineering Research Center of Nano-Geomaterials of Ministry of Education Faculty of Material Science and ChemistryChina University of Geosciences College of Resources and Environment South-Central Minzu University School of Transportation Science and Engineering Beihang University

Metallic zinc is an ideal anode material owing to its high theoretical capacity (819 mAh·g-1),ecofriendliness,low cost and high safety,which have driven fast development of Zn-ion batteries （ZIBs）.However,the practical application of current ZIBs is significantly restricted by irregular dendrite growth of zinc anode and the low working voltage （usually<2 V） of cathode ***,we report a high-voltage Zn-based dualion battery （DIB）,which is constructed by a graphite cathode,a Zn anode,and 3 M LiPF6in the ethyl methyl carbonate （EMC） *** the corrosion interaction of Li+ions,Zn2+can be easily dissolved from Zn anode into the electrolyte to enable dendrite-free Zn2+plating/stripping at the ***,an aqueous carboxymethyl cellulose （CMC） binder is employed to generate a robust cathode electrolyte interface （CEI） layer on the graphite cathode,which renders ultrafast PF6--de-/intercalation into *** resultant Zn–graphite DIB operates stably at a high cut off voltage of 3.2 V,corresponding to an average output voltage of 2.2 *** 9000cycles at 5C,the high capacity retention of 95.9% can be achieved with～100%Coulomb *** on the mass of cathode material,our Zn–graphite battery exhibits ultrafast rate capability （60 C,a discharge time of 44 s） and high energy/power densities (208 Wh·kg-1at 214 W·kg-1;142 Wh·kg-1at 8692 W·kg-1),which holds great promise for large-scale energy storage.

关键词： Binder Graphite High-voltage PF6−-de-/intercalation Zn-ion batteries

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基于DMD的无掩模光刻图形精准性优化方法(特邀)

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中国激光 2024年第12期51卷 398-408页

作者：刘华黄龙刘雨晴东北师范大学物理学院先进光电功能材料研究中心紫外发射材料与技术教育部重点实验室国家实验物理教育示范中心吉林长春130024

基于数字微镜器件(DMD)的无掩模光刻技术作为一种新兴技术在光刻领域备受关注,该技术利用DMD实现光刻掩模的数字化控制,为微纳米加工和快速原型制作提供了一种全新的解决方案。然而,在DMD无掩模光刻技术中还存在着一些问题,如投影畸变... 详细信息

基于数字微镜器件(DMD)的无掩模光刻技术作为一种新兴技术在光刻领域备受关注,该技术利用DMD实现光刻掩模的数字化控制,为微纳米加工和快速原型制作提供了一种全新的解决方案。然而,在DMD无掩模光刻技术中还存在着一些问题,如投影畸变、像素化效应和邻近效应等,这些问题严重影响了光刻图形的精准性。本课题组基于多年的工作基础,全面分析了影响光刻图形质量的因素,并系统总结了几种提高光刻图案精准性的方法,包括数字掩模补偿法、像素叠加优化方法和飞秒局部修饰技术等。基于这些方法的相互配合,本课题组将投影畸变由37.7μm降低至1.7μm,将像素化效应降低为原来的1/6,将邻近效应造成的局部形变尺寸减小为1μm左右,制备出了高精准性的光刻图形。

关键词：投影光刻数字微镜器件光刻质量飞秒激光

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Construction and validation of a neovascular glaucoma nomogram in patients with diabetic retinopathy after pars plana vitrectomy

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World Journal of Diabetes 2024年第4期15卷 654-663页

作者： Yi Shi Yan-Xin Zhang Ming-Fei Jiao Xin-Jun Ren Bo-Jie Hu Ai-hua liu Xiao-Rong Li Surgical Retina Tianjin Key Laboratory of Retinal Functions and DiseasesTianjin Branch of National Clinical Research Center for Ocular DiseaseEye Institute and School of OptometryTianjin Medical University Eye HospitalTianjin 300384China Glaucoma Tianjin Key Laboratory of Retinal Functions and DiseasesTianjin Branch of National Clinical Research Center for Ocular DiseaseEye Institute and School of OptometryTianjin Medical University Eye HospitalTianjin 300384China Ocular Trauma Tianjin Key Laboratory of Retinal Functions and DiseasesTianjin Branch of National Clinical Research Center for Ocular DiseaseEye Institute and School of OptometryTianjin Medical University Eye HospitalTianjin 300384China

BACKGROUND Neovascular glaucoma(NVG)is likely to occur after pars plana vitrectomy(PPV)for diabetic retinopathy(DR)in some patients,thus reducing the expected *** the risk factors for NVG occurrence and building effective risk prediction models are currently required for clinical *** To develop a visual risk profile model to explore factors influencing DR after *** We retrospectively selected 151 patients with DR undergoing *** patients were divided into the NVG(NVG occurrence)and No-NVG(No NVG occurrence)groups according to the occurrence of NVG within 6 months after *** risk factors for postoperative NVG were screened by logistic regression.A nomogram prediction model was established using R software,and the model’s prediction accuracy was verified internally and externally,involving the receiver operator characteristic curve and correction *** After importing the data into a logistic regression model,we concluded that a posterior capsular defect,preoperative vascular endothelial growth factor≥302.90 pg/mL,glycosylated hemoglobin≥9.05%,aqueous fluid interleukin 6(IL-6)≥53.27 pg/mL,and aqueous fluid IL-10≥9.11 pg/mL were independent risk factors for postoperative NVG in patients with DR(P<0.05).A nomogram model was established based on the aforementioned independent risk factors,and a computer simulation repeated sampling method was used to internally and externally verify the nomogram *** area under the curve(AUC),sensitivity,and specificity of the model were 0.962[95%confidence interval(95%CI):0.932-0.991],91.5%,and 82.3%,*** AUC,sensitivity,and specificity of the external validation were 0.878(95%CI:0.746-0.982),66.7%,and 95.7%,*** A nomogram constructed based on the risk factors for postoperative NVG in patients with DR has a high prediction *** study can help formulate relevant preventive and treatment measures.

关键词： Diabetic retinopathy Retinopathy Neovascular Glaucoma Risk factors Nomogram

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海底火山喷发大气冲击波激发的轴对称海啸波数值模型

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力学学报 2024年第7期56卷 2015-2028页

作者：吴蓓蓓刘桦上海交通大学工程力学系水动力学教育部重点实验室上海200240

海底火山喷发引发海啸具有多源激发机制,包括水下爆炸、边坡失稳、火山口坍塌、碎屑流、地震以及大气扰动.为了深入认识轴对称移动气压扰动激发海啸的机理,探究气压扰动参数对水波形态的影响规律,本文在柱面孤立波Boussinesq模型的基础... 详细信息

海底火山喷发引发海啸具有多源激发机制,包括水下爆炸、边坡失稳、火山口坍塌、碎屑流、地震以及大气扰动.为了深入认识轴对称移动气压扰动激发海啸的机理,探究气压扰动参数对水波形态的影响规律,本文在柱面孤立波Boussinesq模型的基础上,考虑水面移动气压扰动作用,建立了由火山喷发激发的轴对称移动气压场所驱动的海啸波数值模型.利用不同地形上柱面波的传播算例验证了本模型的精确性与稳定性.数值模拟了2022年汤加火山喷发大气扰动激发海啸事件,并与太平洋DART浮标实测数据比较,较好地复演了大气扰动驱动海啸波的远场传播过程,并讨论了波动在深水区的色散行为.研究了轴对称气压扰动的径向移速、强度及尺度对波动演化特征的影响,结果显示:气压移速与浅水波速的相对大小显著影响波形,当二者接近时将激发Proudman共振.在共振条件下,波幅与径向传播距离呈近似线性增长关系,波幅放大因子随气压尺度增大而减小.在远离共振条件时,气压强度和尺度对波幅放大因子的影响相对较小,受波能流守恒约束柱面自由波幅则沿程衰减,受迫波幅值近似按气压衰减规律变化.

关键词：移动气压扰动柱面波 Boussinesq方程 Proudman共振汤加火山海啸

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