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Journal of Geographical Sciences 2025年第1期35卷 189-212页

作者： LIU Meiying MIN Leilei WU lin ZHANG Yucui QI Yongqing wang Shiqin LIU Binbin GENG Di SHEN Yanjun Hebei Key Laboratory of Water-Saving Agriculture Key Laboratory of Agricultural Water ResourcesCenter for Agricultural Resources ResearchInstitute of Genetics and Developmental BiologyCAS School of Advanced Agricultural Sciences University of Chinese Academy of Sciences

Nitrate （NO3-） accumulation and transport processes in the thick vadose zone affect the evolution of the groundwater NO3-content in intensive agricultural *** land-use change （ALUC）,typically accompanied by substantial alterations in nitrogen fertilizer application and irrigation practices,is an important influencing *** study evaluated the changes in NO3-accumulation and transport in the deep vadose zone （DVZ,below the root zone）,and the groundwater NO3-content associated with ALUC from grain to vegetable fields in the North China Plain （NCP）.The ALUC from grain to vegetable resulted in nitrate–nitrogen （NO3--N） accumulation in DVZ increased by 235.5 kg ha-1m-1（163.2%） in the piedmont plain and 224.9 kg ha-1m-1（102.7%） in the central plain,*** change accelerated downward transport velocity in the DVZ (from 0.81±0.47 to 0.89±0.55 m yr-1in the piedmont plain,and from 0.24±0.12 to 0.92±0.12 m yr-1in the central plain) and increased NO3-leaching *** transport velocity and leaching fluxes resulted in chemical N-fertilizer entering the aquifer in several areas in the piedmont *** impact of the agricultural activity intensity changes,accompanied by the ALUC,on groundwater quantity and quality should be considered in similar regions.

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Engineering N3C vacancies in hierarchical porous carbon nitride nanosheets for room temperature ultradeep photocatalytic aerobic oxidative desulfurization

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Science China Chemistry 2025年

作者： Yina Nie Weijie Yang Xin wang Xiang Li Lele Wei Xiaolin Bai lin Liu Feng Fu Jun Wan College of Chemistry & Chemical Engineering Research Institute of Comprehensive Energy Industrial Technology Shaanxi Key Laboratory of Chemical Reaction Engineering Yan'an University Anhui Engineering Research Center of Carbon Neutrality College of Chemistry and Materials Science Anhui Normal University

The production of ultra-low sulfur clean fuels holds global significance for improving energy efficiency and reducing environmental pollution. Photocatalytic aerobic oxidative desulfurization（PODS） offers an attractive approach to efficiently remove refractory heterocyclic aromatic sulfur compounds under mild conditions. However, the sluggish charge dynamics,insufficient molecule activation, and slow mass transfer within photocatalysts restrict the overall desulfurization efficiency,hindering the widespread application of this technology. Herein, we developed a defective g-C3N4（M1U3CN） photocatalyst with bridged N3Cvacancies and hierarchical porous structures to address these limitations. This catalyst not only demonstrates outstanding dibenzothiophene（DBT） removal efficiency of 99.6% for model oil with high conversion and selectivity but also achieves complete sulfur removal from gasoline as well as 96.7% sulfur removal for distilled diesel at room temperature,successfully achieving ultradeep aerobic oxidative desulfurization. The introduction of rich N3Cvacancies and abundant micromeso-macroporous distribution in M1U3CN enhances kinetic efficiencies by promoting charge carrier separation, mass transfer,and molecular activation simultaneously; resulting in exceptional PODS performance. This work provides a collaborative strategy to overcome kinetic challenges in aerobic oxidative desulfurization via defect and structural engineering of the catalyst.

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南疆绿洲-荒漠过渡带“肥岛”的养分特征分析

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西南农业学报 2017年第7期30卷 1625-1628页

作者：查向浩林宁王晶张文河李有文喀什大学化学与环境科学学院新疆喀什844000 新疆生物类固废资源化工程技术研究中心新疆喀什844000

【目的】为了分析和检验塔克拉玛干沙漠边缘绿洲-荒漠中灌木"肥岛"效应对荒漠土壤肥力的作用强度。【方法】采用野外取样和室内实验分析相结合的方法,测定了胡杨(Populos euphraticu)灌丛林及周边过渡带中不同深度土壤养分含量;通过计... 详细信息

【目的】为了分析和检验塔克拉玛干沙漠边缘绿洲-荒漠中灌木"肥岛"效应对荒漠土壤肥力的作用强度。【方法】采用野外取样和室内实验分析相结合的方法,测定了胡杨(Populos euphraticu)灌丛林及周边过渡带中不同深度土壤养分含量;通过计算富集率和构建土壤肥力指数模型评价南疆绿洲-荒漠过渡带的土壤肥力水平。【结果】过渡带和灌丛下的土壤p H均呈碱性,且随土壤深度增加碱性增强;土壤中全N、全P、全K和速效N、速效P、速效K含量都随着土壤深度的增加而降低。富集率表明,在胡杨灌丛,土壤OM、全N、全P、全K、和速效养分含量都表现为EB>1,且EB在垂直剖面上呈现先增大后减小的趋势,在20~40cm深度土壤聚集效果最为显著,其中有机质、全K、速效N、速效K富集率相对较大。SFI模型标明,绿洲-荒漠过渡带灌丛下的土壤肥力状况明显高于灌丛间过渡带。【结论】胡杨灌丛下存在典型的灌丛"肥岛"现象,灌木的长期生长能够增强土壤空间异质性的作用,改善灌丛下土壤养分结构和肥力水平,使土壤沙化程度得以缓解。

关键词：绿洲荒漠过渡带胡杨养分主成分分析土壤肥力

Stepwise assembly to construct stable copper(I) cluster-based circularly polarized luminescent MOFs

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Science China Chemistry 2025年

作者： jing-Wen Xie Meng-Ting wang Yan Jin Si Li Jian-Hua Qin Shuang-Quan Zang Tomas C.W.Mak College of Chemistry Henan Key Laboratory of Crystalline Molecular Functional Materials Zhengzhou University College of Chemistry and Chemical Engineering Luoyang Normal University Department of Chemistry The Chinese University of Hong Kong

Circularly polarized luminescence （CPL） materials have been extensively studied in recent years owing to their widespread applications in 3D display,optical storage,optical anti-counterfeiting,and biological imaging,***（I） clusters have emerged as a promising candidate for CPL materials,driven by their cost-effectiveness,superior luminescent properties,precise structure,and low ***,the poor environmental stability of copper（I） clusters renders their synthesis and preservation challenging,thereby significantly impeding their ***,we have designed and synthesised a chiral double-coordinated ligand in order to construct copper（I） cluster nodes that can be further *** anticipated,by utilizing stepwise assembly strategy,a Cu4cluster node co-modified by chiral alkynyl ligands and triphenylphosphine was further assembled with Cd2+ions to obtain 2D layers structure,L/*** L/D-Cu4-Cd exhibits excellent stability and optical properties,including bright yellow emission,solvent-responsive luminescence,and CPL activity with a maximum glumup to 2.0×10-3,which shows potential applications in the WLED and *** interestingly,the material also exhibits deflection ability towards different wavelengths of linearly polarized light,showing certain potential in the preparation of circular polarizer.

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Content of the anti-DNA antibody in the serum of BXSB mouse and suppressive effect of BXSB mouse serum on lymphocyte proliferation

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Acta Pharmacologica Sinica 1999年第5期 92-92页

作者： MEI lin, wang jing-Xue, DANG Hong-Fe, DING Gui-Feng, FAN Shao-Guang(Department of Physiology, Department of Immunology, Beijing Medical University, Beijing 100083, China)

The content of the anti-DNA antibody in BXSB mouse serum and the effect of the sere from BXSB mice on lymphocyte proliferation of normal mouse were ***-linked immunosorbent assay (ELISA) and ~3H-thymidine incorporation were *** content of anti-DNA antibody in male BXSB mouse serum increased from the age of 3 month and reached to the

关键词： DNA Content of the anti-DNA antibody in the serum of BXSB mouse and suppressive effect of BXSB mouse serum on lymphocyte proliferation

甲醇在CM-3-1催化剂上脱水生成二甲醚的本征动力学

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燃料化学学报 1997年第3期25卷 271-276页

作者：房鼎业薛从军林荆陈鹏王小勤华东理工大学化学工程系化工部西南化工研究院

采用等温积分反应器研究了常压下甲醇在ＣＭ３１催化剂上脱水生成二甲醚反应的本征动力学，得到Ｌａｎｇｍｉｕｒ均匀吸附双曲型动力学方程：ｒＭ＝１．５８７×１０１２ｅｘｐ１２２９８４ＲＴＰＭ１ＰＤＰＷＫＰ２Ｍ１＋１．１０３×... 详细信息

采用等温积分反应器研究了常压下甲醇在ＣＭ３１催化剂上脱水生成二甲醚反应的本征动力学，得到Ｌａｎｇｍｉｕｒ均匀吸附双曲型动力学方程：ｒＭ＝１．５８７×１０１２ｅｘｐ１２２９８４ＲＴＰＭ１ＰＤＰＷＫＰ２Ｍ１＋１．１０３×１０９ｅｘｐ８１７６０ＲＴＰＭ２，ｍｏｌ／（ｇ·ｈ）

关键词：二甲醚甲醇动力学催化剂脱水甲醚

Growth behavior and electronic regulation of Pt on various Mo-based supports for hydrogen evolution electrocatalysis

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Science China Chemistry 2025年

作者： Lulu Chen Yichao Huang Jiajun wang Meihong Liao Zhiyuan Liu Meiqi Liu Hanqing Cai lin wang Lidong Gao Dawei Hu Lianming Zhao Ning Pu Zhuangjun Fan State Key Laboratory of Chemical Safety School of Materials Science and Engineering China University of Petroleum (East China) School of Mechanical and Electronic Engineering Qingdao Binhai University Qingdao Chuangqi New Energy Catalysis Technology Co.Ltd. Sinopec Research Institute of Petroleum Processing Co.Ltd. Institute of Energy Hefei Comprehensive National Science Center

Insight into the growth behavior and electronic regulation of platinum （Pt） on various transition metal supports is paramount in developing high-performing electrocatalysts for hydrogen evolution reactions （HER）.Herein,we studied the influence of molybdenum-based supports （MoX,X=C,N,P,and S） on the growth behavior and electronic regulation of *** found that the formation energy variations between Pt single atom and clusters on MoX supports play a pivotal role in the growth behavior of ***,the electronic regulation of Pt induced by metal-support interaction may reflect the valence changes of Pt in Pt-MoX/*** Pt-MoC/C catalyst with a moderate valence state of Pt exhibits the best HER activity with an overpotential of 12.0 mV at 10 mA cm-2and a mass activity of 27.1 A mgPt-1,12.3 times as high as that of commercial 20 wt% Pt/*** work provides constructive guidance for the design of high-performance HER catalysts.

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柴胡疏肝散合四物汤加减预防性治疗月经周期性偏头痛32例临床观察

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湖南中医杂志 2018年第3期34卷 11-13页

作者：吕芳张林全淑林王净净湖南中医药大学湖南长沙410208 湖南中医药大学第二附属医院湖南长沙410005

目的:观察柴胡疏肝散合四物汤加减预防性治疗月经周期性偏头痛的临床疗效。方法:选取肝郁血虚型月经周期性偏头痛患者64例,随机分为治疗组与对照组,每组32例。2组均于月经前10d开始服药,均以10d为1个疗程,连续服用3个疗程,于治疗后4、1... 详细信息

目的:观察柴胡疏肝散合四物汤加减预防性治疗月经周期性偏头痛的临床疗效。方法:选取肝郁血虚型月经周期性偏头痛患者64例,随机分为治疗组与对照组,每组32例。2组均于月经前10d开始服药,均以10d为1个疗程,连续服用3个疗程,于治疗后4、12周各随访1次。观察2组头痛VAS评分、发作次数及时间。结果:与治疗前比较,治疗后4、12周2组头痛VAS评分下降、头痛发作次数减少、发作时间缩短,差异均有统计学意义(P<0.01,P<0.05),且治疗组改善优于对照组(P<0.05)。结论:柴胡疏肝散合四物汤预防性治疗月经周期性偏头痛可明显缓解头痛,减少发作次数,缩短发作时间,其疗效优于口服氟桂利嗪胶囊治疗。

关键词：月经周期性偏头痛中医药疗法柴胡疏肝散四物汤

Mechanism of action of linggui Zhugan Decoction in treating non-alcoholic fatty liver disease using untargeted metabolomics approach

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Traditional Medicine Research 2025年第2期10卷 65-76页

作者： Huan Pei Ren-lin Li Xin-Ran Song Qian-Qian Wan Yu-Ming wang Han-Zhou Li Wei-Quan Xu Jia-Bao Liao Wei-Bo Wen jing Miao Huan-Tian Cui School of Basic Medicine Yunnan University of Chinese MedicineKunming 650599China School Clinical Medical College Yunnan University of Chinese MedicineKunming 650599China First School of Clinical Medicine Yunnan University of Chinese MedicineKunming 650599China School of Integrative Chinese and Western Medicine Tianjin University of Traditional Chinese MedicineTianjin 301617China Department of Pharmacy Tianjin Second People's HospitalTianjin 300192China

Background:Non-alcoholic fatty liver disease(NAFLD)is a liver disorder characterized by the accumulation and degeneration of fat in the liver cells,a condition that may further deteriorate and lead to cirrhosis and liver *** studies showed that metabolic dysfunction can promote NAFLD *** Zhugan Decoction(LGZGD)has therapeutic effects on *** mechanism of LGZGD still remains *** study was to examine the impact of LGZGD on the metabolic processes involved in the development of ***:A mice model of NAFLD was treated with *** therapeutic potential of LGZGD was evaluated by assessing the activity of transaminases,lipids levels of blood,and pathological changes in the liver of the mice model of ***,this study also evaluated the influence of LGZGD on liver inflammation and oxidative ***:The results of untargeted metabolomics analysis showed that LGZGD reduced the disordered lipid metabolism in NAFLD *** improved the oxidative stress and also reduced the levels of pro-inflammatory cytokines in the *** metabolomics analysis of liver samples revealed that LGZGD treatment improved metabolic disorders,including alanine,aspartate,glutamate,glycerophospholipid metabolism,and citrate *** RT-qPCR and Western blot results showed that LGZGD could regulate the expression of key enzymes in the metabolic pathway of the citrate cycle,including ATP-citrate lyase(ACLY),alanine-glyoxylate aminotransferase-2(AGXT2),phosphatidylethanolamine N-methyltransferase(PEMT),and succinate dehydrogenase(SDH).Conclusion:We found that LGZGD can treat NAFLD by reducing inflammatory responses,inhibiting oxidative stress,regulating alanine,aspartate,glutamate,and glycerophospholipid metabolism,and citrate cycle pathways.

关键词： NAFLD LGZGD untargeted metabolomics glycerophospholipid metabolism citrate cycle

莆田黑猪不同组织DNA甲基化的MSAP分析

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福建农林大学学报（自然科学版） 2017年第3期46卷 305-310页

作者：胡宇平张金耀林瑞意林威敏陈静汪稳肖天放福建农林大学动物科学学院福建福州350002

为研究莆田黑猪不同组织间基因组DNA甲基化水平差异及各组织甲基化水平在不同生长发育阶段之间的变化规律,采用甲基化敏感扩增片段多态性(MSAP)方法检测了1、25和210日龄莆田黑猪的心脏、肝脏、肌肉、脂肪、耳和尾6个组织基因组DNA的甲... 详细信息

为研究莆田黑猪不同组织间基因组DNA甲基化水平差异及各组织甲基化水平在不同生长发育阶段之间的变化规律,采用甲基化敏感扩增片段多态性(MSAP)方法检测了1、25和210日龄莆田黑猪的心脏、肝脏、肌肉、脂肪、耳和尾6个组织基因组DNA的甲基化水平.结果表明:心脏和肝脏组织的甲基化水平随日龄增长呈下降趋势,且日龄间的甲基化水平差异显著(P0.05),但显著高于210日龄(P0.05);3个日龄的肝脏与脂肪组织之间、肝脏与耳组织之间的甲基化水平均存在显著差异(P<0.05),表明DNA甲基化在肝脏与脂肪组织之间、肝脏与耳组织之间存在组织特异性.

关键词： DNA甲基化组织甲基化敏感扩增多态性(MSAP) 莆田黑猪