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Prussian Blue Analogue‑Templated Nanocomposites for Alkali‑Ion Batteries:Progress and Perspective

Nano-Micro Letters 2025年第1期17卷 216-261页

作者： Jian‑En Zhou yilin Li Xiaoming lin Jiaye ye Key Laboratory of Theoretical Chemistry of Environment Ministry of EducationSchool of ChemistrySouth China Normal UniversityGuangzhou 510006People’s Republic of China School of Chemistry and Physics Faculty of ScienceQueensland University of Technology2 George StreetBrisbaneQLD 4000Australia Centre for Materials Science Queensland University of Technology2 George StreetBrisbaneQLD 4000Australia

Lithium-ion batteries(LIBs)have dominated the portable electronic and electrochemical energy markets since their commercialisation,whose high cost and lithium scarcity have prompted the development of other alkali-ion batteries(AIBs)including sodium-ion batteries(SIBs)and potassium-ion batteries(PIBs).Owing to larger ion sizes of Na^(+)and K^(+)compared with Li^(+),nanocomposites with excellent crystallinity orientation and well-developed porosity show unprecedented potential for advanced lithium/sodium/potassium *** enticing open rigid framework structures,Prussian blue analogues(PBAs)remain promising self-sacrificial templates for the preparation of various nanocomposites,whose appeal originates from the well-retained porous structures and exceptional electrochemical activities after thermal *** review focuses on the recent progress of PBA-derived nanocomposites from their fabrication,lithium/sodium/potassium storage mechanism,and applications in AIBs(LIBs,SIBs,and PIBs).To distinguish various PBA derivatives,the working mechanism and applications of PBA-templated metal oxides,metal chalcogenides,metal phosphides,and other nanocomposites are systematically evaluated,facilitating the establishment of a structure–activity correlation for these *** on the fruitful achievements of PBA-derived nanocomposites,perspectives for their future development are envisioned,aiming to narrow down the gap between laboratory study and industrial reality.

关键词： Prussian blue analogues Self-sacrificial template Lithium-ion batteries Sodium-ion batteries Potassium-ion batteries

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High Fe‑Loading Single‑Atom Catalyst Boosts ROS Production by Density Effect for Efficient Antibacterial Therapy

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Nano-Micro Letters 2025年第2期17卷 187-203页

作者： Si Chen Fang Huang Lijie Mao Zhimin Zhang Han lin Qixin yan Xiangyu Lu Jianlin Shi Department of Cardiology Shanghai Tenth People’s HospitalSchool of MedicineTongji UniversityShanghai 200092People’s Republic of China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050People’s Republic of China Shanghai Frontiers Science Center of Nanocatalytic Medicine School of MedicineTongji UniversityShanghai 200092People’s Republic of China

The current single-atom catalysts(SACs)for medicine still suffer from the limited active site ***,we develop a synthetic method capable of increasing both the metal loading and mass-specific activity of SACs by exchanging zinc with *** constructed iron SACs(h^(3)-FNC)with a high metal loading of 6.27 wt%and an optimized adjacent Fe distance of~4 A exhibit excellent oxidase-like catalytic performance without significant activity decay after being stored for six months and promising antibacterial ***,a“density effect”has been found at a high-enough metal doping amount,at which individual active sites become close enough to interact with each other and alter the electronic structure,resulting in significantly boosted intrinsic activity of single-atomic iron sites in h^(3)-FNCs by 2.3 times compared to low-and medium-loading ***,the overall catalytic activity of h^(3)-FNC is highly improved,with mass activity and metal mass-specific activity that are,respectively,66 and 315 times higher than those of commercial Pt/*** addition,h^(3)-FNCs demonstrate efficiently enhanced capability in catalyzing oxygen reduction into superoxide anion(O_(2)·^(−))and glutathione(GSH)*** in vitro and in vivo assays demonstrate the superior antibacterial efficacy of h^(3)-FNCs in promoting wound *** work presents an intriguing activity-enhancement effect in catalysts and exhibits impressive therapeutic efficacy in combating bacterial infections.

关键词： Nanocatalytic medicine Single-atom catalysts Reactive oxygen species(ROS) High metal loading Oxidase catalysis

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Evaluation of solubility of polycyclic aromatic hydrocarbons in ethyl lactate/water versus ethanol/water mixtures for contaminated soil remediation applications

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Journal of Environmental Sciences 2012年第6期24卷 1064-1075页

作者： Chiew lin yap Suyin Gan Hoon Kiat ng Department of Chemical and Environmental Engineering The University of Nottingham Malaysia CampusJalan Broga43500 SemenyihSelangor Darul EhsanMalaysia Department of Mechanical Materials and Manufacturing Engineering The University of Nottingham l~lalaysia Campus Jalan Broga 43500 Semenyih Selangor Darul Ehsan Malaysia

Solubility data of recalcitrant contaminants in cosolvents is essential to determine their potential applications in enhanced soil *** solubilities of phenanthrene,anthracene,fluoranthene and benzo[a]pyrene in ethyl lactate/water and ethanol/water mixtures were measured using equilibrium *** cosolvency powers derived from solubility data were then applied to the model developed from the solvophobic approach to predict the capability of ethyl lactate and ethanol in enhancing the desorption of contaminants from *** ethyl lactate and ethanol cosolvents were shown to be able to enhance the solubilisation of the tested four polycyclic aromatic hydrocarbons by 〉 4 orders of magnitude above the levels obtained with water ***,ethyl lactate demonstrated a greater capacity to enhance PAH solubility than *** cosolvency powers of ethyl lactate/water system obtained from the end-to-end slope （σ） and the end-to-half slope （σ 0.5） of the solubilisation curve were 1.0-1.5 and 2.0-2.9 higher than ethanol/water system *** line with this,ethyl lactate/water was demonstrated to enhance the desorption of contaminants from soil by 20%-37% and 18%-61% higher compared to ethanol/water system in low organic content and high organic content soils respectively,with a 2：1 （V/W） ratio of solution：soil and with cosolvent fraction as low as *** the exception of benzo[a]pyrene,the experimental desorption results agreed fairly with the predicted values,under an applied solution：soil ratio that was enough to hold the capacity of released contaminants.

关键词： polycyclic aromatic hydrocarbon solubility desorption ethyl lactate ethanol

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Alkali and Silane Treatments towards Exemplary Mechanical Properties of Kenaf and Pineapple Leaf Fibre-reinforced Composites

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Journal of Bionic Engineering 2020年第2期17卷 380-392页

作者： ng lin Feng Sivakumar Dhar Malingam Nadlene Razali Sivarao Subramonian Centre for Advanced Research on Energy Fakulti Kejuruteraan MekanikalUniversiti Teknikal Malaysia MelakaMelaka 76100Malaysia Fakulti Kejuruteraan Pembuatan Universiti Teknikal Malaysia MelakaMelaka 76100Malaysia

Following the contemporary research trend of exploring the potential of eco-friendly natural fibres,this work studies the effects of alkali and silane treatments,with vary.ng concentrations,on the mechanical characterization of composites reinforced with kenaf and pineapple leaf fibre(PALF).Kenaf-and PALF-based composites were fabricated through the heat compression *** mechanical characterization was then performed to evaluate the tensile,flexural and impact *** findings concluded that chemical treatments indeed enhanced the mechanical properties of composite materials.5%NaOH and 3%silane treatments can respectively provide the optimum mechanical properties to the kenaf fibre and PALF reinforced *** treatment results evidenced that silane-treated composites exhibit higher mechanical properties compared to the NaOH-treated *** comparing the mechanical properties of kenaf-and PALF-reinforced polypropylene composites,the overall results show that composites based on PALF have superior mechanical properties.

关键词： natural fibres kenaf fibre pineapple leaf fibre chemical treatment mechanical properties

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Hepatocellular Tumors:Immunohistochemical Analyses for Classification and Prognostication

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Chinese Journal of Cancer Research 2011年第4期23卷 245-253页

作者： Regina Cheuk-Lam Lo Irene Oi-lin ng Department of Pathology and State Key Laboratory for Liver Research The University of Hong Kong

Following the classification of hepatocellular nodules by the International Working Party in 1995 and further elaboration by the International Consensus Group for Hepatocellular Neoplasia in 2009, entities under the spectrum of hepatocellular nodules have been better characterized. Research work hence has been done to answer questions such as distinguishing high-grade dysplastic nodules from early hepatocellular carcinoma (HCC), delineating the tumor cell origin of HCC, identify.ng its prognostic markers, and subtyping hepatocellular adenomas. As a result, a copious amount of data at immunohistochemical and molecular levels has emerged. A panel of immunohistochemical markers including glypican-3, heat shock protein 70 and glutamine synthetase has been found to be of use in the diagnosis of small, well differentiated hepatocellular tumors and particularly of HCC. The use of liver fatty acid binding protein (L-FABP), β-catenin, glutamine synthetase, serum amyloid protein and C-reactive protein is found to be helpful in the subtyping of hepatocellular adenomas. The role of tissue biomarkers for prognostication in HCC and the use of biomarkers in subclassify.ng HCC based on tumor cell origin are also discussed.

关键词： Hepatocellular tumors Immunohistochemical Classification

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Reconstructing shock front of unstable detonations based on multi-layer perceptron

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Acta Mechanica Sinica 2021年第11期37卷 1610-1623,I0001页

作者： lin Zhou Honghui Teng Hoi Dick ng Pengfei y.ng Zonglin Jiang School of Aerospace Engineering Beijing Institute of TechnologyBeijing100081China State Key Laboratory of Laser Propulsion and Application Beijing Power Machinery InstituteBeijing100074China Department of Mechanical Industrial and Aerospace EngineeringConcordia UniversityMontrealQCH3G 1M8Canada State Key Laboratory of High Temperature Gas Dynamics Institute of MechanicsChinese Academy of SciencesBeijing100190China School of Engineering Sciences University of Chinese Academy of SciencesBeijing100049China

The dynamics of frontal and transverse shocks in gaseous detonation waves is a complex phenomenon bringing many difficulties to both numerical and experimental *** laser-optical visualization of detonation structure may provide certain information of its reactive front,but the corresponding lead shock needs to be reconstructed building the complete flow *** the multi-layer perceptron(MLP)approach,we propose a shock front reconstruction method which can predict evolution of the lead shock wavefront from the state of the reactive *** method is verified through the numerical results of one-and two-dimensional unstable detonations based on the reactive Euler equations with a one-step irreversible chemical reaction *** show that the accuracy of the proposed method depends on the activation energy of the reactive mixture,which influences prominently the cellular detonation instability and hence,the distortion of the lead shock *** select the input variables for training and evaluate their influence on the effectiveness of the proposed method,five groups,one with six variables,and the other with four variables,are tested and analyzed in the MLP *** trained MLP is tested in the cases with different activation energies,demonstrates the inspiring generalization *** paper offers a universal framework for predicting detonation frontal evolution and provides a novel way to interpret numerical and experimental results of detonation waves.

关键词： Cellular detonation Lead shock evolution Multi-layer perceptron Numerical simulations

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Impact of ozone assisted ultrasonication pre-treatment on anaerobic digestibility of sewage sludge

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Journal of Environmental Sciences 2015年第7期27卷 29-38页

作者： Xinbo Tian Antoine Prandota Trzcinski Li Leonard lin Wun Jern ng Advanced Environmental Biotechnology Centre Nanyang Environment and Water Research Institute Nanyang Technological University School of Civil and Environmental Engineering Nanyang Technological University Public Utilities Board Water Reclamation (Plants) Department Nany.ng Environment and Water Research Institute Nanyang Technological University

Impact of ultrasonication（ULS） and ultrasonication-ozonation（ULS-Ozone） pre-treatment on the anaerobic digestibility of sewage sludge was investigated with semi-continuous anaerobic reactors at solid retention time（SRT） of 10 and 20 days. The control, ULS and ULS-Ozone reactors produced 256, 309 and 348 m L biogas/g CODfedand the volatile solid（VS） removals were 35.6%, 38.3% and 42.1%, respectively at SRT of 10 days. At SRT of20 days, the biogas yields reached 313, 337 and 393 m L biogas/g CODfedand the VS removal rates were 37.3%, 40.9% and 45.3% in the control, ULS and ULS-Ozone reactors, ***-Ozone pre-treatment increased the residual organic amount in the digested *** soluble residual organics were found to contain macromolecules with molecular weights（MW） larger than 500 k Da and smaller polymeric products with MW around 19.4and 7.7 k Da. These compounds were further characterized to be humic acid-like substances with fluorescent spectroscopy analysis.

关键词： Sewage sludge Ultrasound Ozone Pre-treatment Molecular weight Anaerobic digestion

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Insights on the solubilization products after combined alkaline and ultrasonic pre-treatment of sewage sludge

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Journal of Environmental Sciences 2015年第3期27卷 97-105页

作者： Xinbo Tian Chong Wang Antoine Prandota Trzcinski Leonard lin Wun Jern ng Advanced Environmental Biotechnology Centre Nanyang Environment and Water Research Institute Nanyang Technological University School of Civil and Environmental Engineering Nanyang Technological University Public Utilities Board Water Reclamation (Plants) Department Nany.ng Environment and Water Research Institute Nanyang Technological University

This work provides insights on the solubilization products after a simultaneous combination of alkaline and ultrasonic （ALK ＋ ULS） pre-treatment of sewage sludge. Soluble chemical oxygen demand （SCOD） increased from 1200 to 11,000 mg/L after such treatment. Organics with molecular weight around 5.6 kDa were solubilized because of the synergistic effect of ultrasound and alkali. Organics with molecular weight larger than 300 kDa increased from 7.8% to 60%, 16% and 42.3% after ULS, ALK and ALK ＋ ULS treatment, respectively. Excitation emission matrix fluorescence spectroscopy analysis identified soluble microbial product-like and humic acid-like matters as the main solubilization products. Sludge anaerobic biodegradability was significantly enhanced with the simultaneous application of ALK ＋ ULS pre-treatment. ALK ＋ ULS pre-treatment resulted in 37.8% biodegradability increase compared to the untreated sludge. This value was higher compared to the biodegradability increase induced by individual ALK pre-treatment （5.7%） or individual ULS pre-treatment （20.7%） under the same conditions applied.

关键词： Ultrasound AlkaliSewage sludge Molecular weight Excitation emission matrix (EEM) Anaerobic biodegradability

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you shall never walk alone:burnout and depression amongst healthcare professionals

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Hepatobiliary Surgery and Nutrition 2021年第5期10卷 678-681页

作者： Kelvin lin Chieh ng Chen Liu Institute of Mental Health SingaporeSingapore United Family Hospital BeijingChina

There are two stages of tsunami,first is the earthquake in deep sea,followed by *** are three waves of pandemic,the death toll,economic and social disruption,and a psychological storm that is looming in the distance *** this time of worldwide COVID-19 pandemic,to date,we have seen over 200 million cases worldwide,and the death toll is in excess of 4 million,and there are various news reports coming in about devastating economic and social ***,numerous studies report that the public,as well as the healthcare professionals are at heightened risk mental health problems in the short and longer term from pandemic.

关键词： storm earthquake alone

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Photoluminescence of ZnS Clusters in Zeolite-y

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Journal of Materials Science & Technology 1997年第5期13卷 397-404页

作者： Chen, W Wang, ZG lin, ZJ Xu, y lin, Ly Lab. of Semiconductor Materials Sciences Institute of Semiconductors Chinese Academy of Sciences Beijing 100083 China

Two obvious emissions are observed from the ZnS clusters encapsulated in zeolite-y. The emission around 355 nm is sharp and weak, locating at the onset of the absorption edge. The band around 535 nm is broad, strong and Stokes-shifted. Both the two emissions shift to blue and their intensities firstly increase then decrease as the loading of ZnS in zeolite-y or clusters size decreases. Through investigation, the former is attributed to the excitonic fluorescence, and the latter to the trapped luminescence from surface states. The cluster size-dependence of the luminescence may be explained qualitatively by considering both the carrier recombination and the nonradiative recombination rates. Four peaks appearing in the excitation spectra are assigned to the transitions of 1S-1S, 1S-1P, 1S-1D and surface state, respectively. The excitation spectra of the clusters do not coincide with their absorption spectra. The states splitted by quantum-size confinement are detected in the excitation spectra, but could not be differentiated in the optical absorption spectra due to inhomogeneous broadening. The size-dependence of the excitation spectra is similar to that of the absorption spectra. Both the excitation spectra of excitonic and of trapped emissions are similar, but change in relative intensity and shift in position are observed.

关键词： Zeolites

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