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Improving benzene catalytic oxidation on Ag/Co_(3)O_(4) by regulating the chemical states of Co and Ag

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Journal of Environmental Sciences 2024年第9期143卷 201-212页

作者： hao Guo Tao Guo Mengqi Zhao Yaxin Zhang Wenfeng Shangguan Yinnian liao State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources Xinjiang UniversityXinjiang 830017China Xinjiang Key Laboratory of Coal Clean Conversion&Chemical Engineering Process Xinjiang UniversityXinjiang 830017China School of Chemical Engineering and Technology Xinjiang UniversityXinjiang 830017China Research Center for Combustion and Environmental Technology Shanghai Jiao Tong UniversityShanghai 200240China School of Applied Chemistry and Materials Zhuhai College of Science and TechnologyGuangdong 519041China

Silver(9 wt.%)was loaded on Co_(3)O_(4)-nanofiber using reduction and impregnation methods,*** to the stronger electronegativity of silver,the ratios of surface Co^(3+)/Co^(2+) on Ag/Co_(3)O_(4) were higher than on Co_(3)O_(4),which further led to more adsorbed oxygen species as a result of the charge ***,the introducing of silver also obviously improved the reducibility of Co_(3)O_(4).Hence the Ag/Co_(3)O_(4) showed better catalytic performance than Co_(3)O_(4) in benzene *** with the Ag/Co_(3)O_(4) synthesized via impregnation method,the one prepared using reduction method(named as Ag Co-R)exhibited higher contents of surface Co^(3+) and adsorbed oxygen species,stronger reducibility,as well as more active surface lattice oxygen ***,Ag Co-R showed lowest T_(90) value of 183℃,admirable catalytic stability,largest normalized reaction rate of1.36×10^(-4)mol/(h·m^(2))(150℃),and lowest apparent activation energy(E_(a))of 63.2 kJ/*** analyzing of in-situ DRIFTS indicated benzene molecules were successively oxidized to phenol,o-benzoquinone,small molecular intermediates,and finally to CO_(2) and water on the surface of Ag *** last,potential reaction pathways including five detailed steps were proposed.

关键词： Reduction method Co_(3)O_(4)-supported Ag catalyst,VOCs Benzene oxidation Reaction mechanism

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光伏电站落尘影响分析及清扫机器人提效研究

现代工业经济和信息化 2024年第1期14卷 144-146页

作者：廖皓单诗涵刘聪周楚昂田维生中国电建集团成都勘测设计研究院有限公司四川成都610000

不同的光伏电站落尘清扫方式用以提升光伏电站的发电量。通过对国内外对落尘影响光伏发电量进行了阐释,对传统清扫设备及清扫机器人清扫方式进行了描述,并结合工程案例进行了清扫机器人清扫提效试验研究。

关键词：新能源光伏运维清扫发电量提效

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燃烧喷焰的红外辐射特性分析

光学与光电技术 2024年第2期22卷 122-130页

作者：廖鹏昊汪玉琴李佳文张蓉竹四川大学电子信息学院四川成都610065

在探测燃烧形成的火焰目标时,由于不同红外波段辐射特性不同,不同波段下成像效果差异明显。以喷枪火焰为研究对象,用仿真与实验相结合分析了其在近红外(0.9~1.7μm)、中红外(3.8~4.7μm)、远红外(7.5~13μm)三个波段下的红外辐射特性。... 详细信息

在探测燃烧形成的火焰目标时,由于不同红外波段辐射特性不同,不同波段下成像效果差异明显。以喷枪火焰为研究对象,用仿真与实验相结合分析了其在近红外(0.9~1.7μm)、中红外(3.8~4.7μm)、远红外(7.5~13μm)三个波段下的红外辐射特性。从气体辐射理论出发,根据辐射传输方程对喷焰在0.9~1.7μm、3.8~4.7μm、7.5~13μm三个波段下的红外辐射特性进行了计算和比较。通过辐射成像实验,对响应波段的辐射图像信息进行了采集,并与仿真计算结果进行了比对分析。结果表明:在640×512分辨率下火焰的中波红外成像目标像素约10000个,包含了最多的信息量,其红外辐射强度最大,长波红外有效目标像素约7000个,但其红外辐射分布最广且受环境影响最小,近红外成像像素约3400个。为各类动力目标的探测和识别以及图像的融合、信息增强等提供了依据。

关键词：红外辐射喷枪火焰辐射出射度红外成像图像融合

A Privacy Preservation Method for Attributed Social Network Based on Negative Representation of Information

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Computer Modeling in Engineering & Sciences 2024年第7期140卷 1045-1075页

作者： hao Jiang Yuerong liao Dongdong Zhao Wenjian Luo Xingyi Zhang Key Laboratory of Intelligent Computing and Signal Processing of Ministry of Education School of Computer Science and TechnologyAnhui UniversityHefei230601China Chongqing Research Institute School of Computer Science and Artificial IntelligenceWuhan University of TechnologyWuhan430070China Guangdong Provincial Key Laboratory of Novel Security Intelligence Technologies School of Computer Science and TechnologyHarbin Institute of TechnologyShenzhen518055China

Due to the presence of a large amount of personal sensitive information in social networks,privacy preservation issues in social networks have attracted the attention of many *** by the self-nonself discrimination paradigmin the biological immune system,the negative representation of information indicates features such as simplicity and efficiency,which is very suitable for preserving social network ***,we suggest a method to preserve the topology privacy and node attribute privacy of attribute social networks,called ***,a negative survey-based method is developed to disturb the relationship between nodes in the social network so that the topology structure can be kept ***,a negative database-based method is proposed to hide node attributes,so that the privacy of node attributes can be preserved while supporting the similarity estimation between different node attributes,which is crucial to the analysis of social *** evaluate the performance of the AttNetNRI,empirical studies have been conducted on various attribute social networks and compared with several state-of-the-art methods tailored to preserve the privacy of social *** experimental results show the superiority of the developed method in preserving the privacy of attribute social networks and demonstrate the effectiveness of the topology disturbing and attribute hiding *** experimental results show the superiority of the developed methods in preserving the privacy of attribute social networks and demonstrate the effectiveness of the topological interference and attribute-hiding components.

关键词： Attributed social network topology privacy node attribute privacy negative representation of information negative survey negative database

Publication-level analysis of Journal of Plant Ecology during 2018-2022

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Journal of Plant Ecology 2024年第4期17卷 197-201页

作者： Yu liao Pu Wang Lijuan Liu Wen-hao Zhang National Science Library Chinese Academy of SciencesBeijing 100190China Center for Documentation and Information Institute of BotanyChinese Academy of SciencesBeijing 100093China State Key Laboratory of Vegetation and Environmental Change Institute of BotanyChinese Academy of SciencesBeijing 100093China

Journal of Plant Ecology(JPE)was established in 2008 and is sponsored by the Botanical Society of China and the Institute of Botany,Chinese Academy of *** by Oxford University Press,UK,JPE encompasses a wide range of article types within the expansive field of plant *** of July 2021,JPE has transitioned to fully Open Access,ensuring unrestricted access to the full text for both readers and *** shift enhances the journal’s role as a crucial platform for plant ecologists worldwide to disseminate their research findings.

关键词： Open Plant Access

A Stable Copper-based Metal-Azolate Framework for Efficient Electroreduction of CO_(2)to C_(2+)Products

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Chemical Research in Chinese Universities 2024年第4期40卷 664-669页

作者： LIU Yuan-Yuan ZHU hao-Lin liao Pei-Qin CHEN Xiao-Ming Key Laboratory of Bioinorganic and Synthetic Chemistry Ministry of EducationGBRCE for Functional Molecular EngineeringSchool of ChemistryIGCMESun Yat-sen UniversityGuangzhou510275P.R.China Chemistry and Chemical Engineering Guangdong Laboratory Shantou515031P.R.China

Driven by renewable or excess electrical energy,electrochemical CO_(2)reduction reaction(eCO_(2)RR)represents a promising carbon-neutral approach to generating valuable low-carbon fuels by consuming CO_(2)and H_(2)O.C_(2+)products are one of the most economically valuable products among the reduction species of eCO_(2)RR,but there are still some challenges,such as low selectivity or low current *** this work,we showed that a copper-based metal-azolate framework(MAF),denoted as MAF-203,exhibits the high performance of eCO_(2)RR to yield C_(2+)products with the Faradaic efficiency(C_(2+))of 52.5%and a current density of 660 mA/cm^(2)at-1.2 V *** in a flow cell device under alkaline *** experiment,in situ infrared spectroscopy and the density functional theory(DFT)calculations showed that the electron donating effect of methyl substituents on organic ligands of the copper-based MAF could enhance the ligand field and activation of key intermediates(*CO and*CHO species),thus promoting the coupling of*CO and*CHO for yielding C_(2+)products.

关键词： Metal-organic framework Carbon dioxide Electroreduction C_(2+)product Metal-azolate framework

Harnessing innate immune pathways for therapeutic advancement in cancer

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Signal Transduction and Targeted Therapy 2024年第4期9卷 1506-1564页

作者： Ankang Hu Li Sun hao Lin Yuheng liao Hui Yang Ying Mao Department of Neurosurgery Huashan HospitalFudan UniversityShanghaiP.R.China Institute for Translational Brain Research Shanghai Medical CollegeFudan University ShanghaiPR.China National Center for Neurological Disorders Huashan HospitalShanghai Medical CollegeFudan UniversityShanghaiP.R.China Shanghai Key Laboratory of Brain Function Restoration and Neural Regeneration Shanghai Clinical Medical Center of NeurosurgeryNeurosurgical Institute of Fudan UniversityHuashan HospitalShanghai Medical CollegeFudan UniversityShanghaiP.R.China State Key Laboratory of Medical Neurobiology and MOE Frontiers Center for Brain Science and MOE Frontiers Center for Brain Science Institutes of Brain ScienceShanghai Medical CollegeFudan UniversityShanghaiP.R.China Shanghai Key Laboratory of Medical Epigenetics International Co-laboratory of Medical Epigenetics and Metabolism(Ministry of Science and Technology)and Key Laboratory of Metabolism and Molecular Medicine(Ministry of Education)and Molecular and Cell Biology LabInstitutes of Biomedical SciencesShanghai Medical College of Fudan UniversityShanghaiP.R.China

The innate immune pathway is receiving increasing attention in cancer *** pathway is ubiquitous across various cell types,not only in innate immune cells but also in adaptive immune cells,tumor cells,and stromal *** targeting the innate immune pathway have shown profound changes in the tumor microenvironment(TME)and improved tumor prognosis in preclinical ***,to date,the clinical success of drugs targeting the innate immune pathway remains ***,recent studies have shown that activation of the innate immune pathway can paradoxically promote tumor *** uncertainty surrounding the therapeutic effectiveness of targeted drugs for the innate immune pathway is a critical issue that needs immediate *** this review,we observe that the role of the innate immune pathway demonstrates heterogeneity,linked to the tumor development stage,pathway status,and specific cell *** propose that within the TME,the innate immune pathway exhibits multidimensional *** diversity is fundamentally rooted in cellular heterogeneity and is manifested as a variety of signaling *** pro-tumor effect of innate immune pathway activation essentially reflects the suppression of classical pathways and the activation of potential pro-tumor alternative *** our understanding of the tumor's innate immune pathway network and employing appropriate targeting strategies can enhance our ability to harness the anti-tumor potential of the innate immune pathway and ultimately bridge the gap from preclinical to clinicalapplication.

关键词： drugs therapeutic innate

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异辛醇胺化合成三异辛胺镍铜基催化剂的研究

安徽化工 2024年第1期50卷 46-50页

作者：蔡佳欣王嘉怡廖浩枫覃承文王琪合肥工业大学化学与化工学院高值催化转化与反应工程安徽省重点实验室安徽合肥230009

采用浸渍法制备了不同镍铜比的镍基催化剂。采用氢气程序升温还原(H2-TPR)、氨气程序升温脱附(NH3-TPD)、X射线粉末衍射(XRD)对催化剂进行表征,并考查其催化异辛醇氨化合成三异辛胺的活性。结果表明,还原态催化剂表面检测出明显的Cu衍射... 详细信息

采用浸渍法制备了不同镍铜比的镍基催化剂。采用氢气程序升温还原(H2-TPR)、氨气程序升温脱附(NH3-TPD)、X射线粉末衍射(XRD)对催化剂进行表征,并考查其催化异辛醇氨化合成三异辛胺的活性。结果表明,还原态催化剂表面检测出明显的Cu衍射峰,Ni的衍射峰较弱,说明Ni物种更为分散。H2-TPR表征显示,铜的添加促进了镍的还原,使得催化剂表面还原态Ni和Cu物种增多,增加了催化剂加氢、脱氢能力;NH3-TPD显示,镍对NH3有更好的吸附活化作用,铜与镍对NH3形成了协同吸附。Cu1.5Ni1/A300催化剂体现出较好的催化活性,胺化反应4 h,异辛醇转化率达82.69%,三异辛胺选择性达到63.28%。

关键词：镍铜基催化剂异辛醇三异辛胺

Evaluation of Multi-Temporal-Spatial Scale Adjustment Capability and Cluster Optimization Operation Method for Distribution Networks with Distributed Photovoltaics

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Energy Engineering 2024年第9期121卷 2655-2680页

作者： Jiaxin Qiao Yuchen hao Yingqi liao Fang Liang Jing Bian Northeast Electric Power University Key Laboratory of Modern Power System Simulation and Control&Renewable Energy TechnologyMinistry of EducationJilin132011China State Grid Jiangsu Electric Power Co. Ltd.Power Dispatch Control CenterNanjing210017China State Grid Jiangsu Electric Power Co. Ltd.Nanjing Power Supply BranchPower Dispatch Control CenterNanjing210019China

Themassive integration of high-proportioned distributed photovoltaics into distribution networks poses significant challenges to the flexible regulation capabilities of distribution *** accurately assess the flexible regulation capabilities of distribution stations,amulti-temporal and spatial scale regulation capability assessment technique is proposed for distribution station areas with distributed photovoltaics,considering different geographical locations,coverage areas,and response ***,the multi-temporal scale regulation characteristics and response capabilities of different regulation resources in distribution station areas are analyzed,and a resource regulation capability model is established to quantify the adjustable range of different regulation *** this basis,considering the limitations of line transmission capacity,a regulation capability assessment index for distribution stations is proposed to evaluate their regulation ***,considering different geographical locations and coverage areas,a comprehensive performance index based on electrical distance modularity and active power balance is established,and a cluster division method based on genetic algorithms is proposed to fully leverage the coordination and complementarity among nodes and improve the active power matching degree within ***,an economic optimization model with the objective of minimizing the economic cost of the distribution station is established,comprehensively considering the safety constraints of the distribution network and the regulation constraints of *** model can provide scientific guidance for the economic dispatch of the distribution station ***,case studies demonstrate that the proposed assessment and optimization methods effectively evaluate the regulation capabilities of distribution stations,facilitate the consumption of distributed photovoltaics,and enhance the economic efficiency of th

关键词： Distributed photovoltaic distribution station area assessment of adjustment capacity line transmission capacity economic optimization