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A new 4-Ti-added polyoxometalate

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Tungsten 2024年第2期6卷 465-471页

作者： Hai-Lou Li chen lian.Guo-Yu Yang MOE Key Laboratory of cluster Science School of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 102488China

A new inorganic–organic hybrid 4-Ti-added polyoxometalate:[H_(2)N(cH_(3))_(2)]_(2)Na_(3)H_(5)[{Ti(c_(2)O_(4))(H_(2)O)}_(2){Ti(c_(2)O_(4))}_(2)(B-β-SbW_(9)O_(33))_(2)]·22H_(2)O(1)has been successfully made and further characterized by infrared spectroscopy,thermogravimetric analysis,powder X-ray diff raction and single-crystal X-ray diff *** polyoxoanion of 1 exhibits a Krebs-type structure that is constructed from two[B-β-SbW_(9)O_(33)]^(9)−fragments fused together by a belt of four additional Ti atoms decorated by oxalate ***,1 as a heterogeneous catalyst exhibits high activity for Knoevenagel condensation under mild reaction conditions.

关键词： Polyoxometalate Ti-added POM Krebs-type structure Knoevenagel condensation

Simulation Study on constraining Gravitational Wave Propagation Speed by Gravitational Wave and Gamma-ray Burst Joint Observation on Binary Neutron Star Mergers

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Research in Astronomy and Astrophysics 2024年第8期24卷 42-51页

作者： Jin-Hui Rao Shu-Xu Yi lian.Tao Qing-Wen Tang Department of Physics School of Physics and Materials ScienceNanchang UniversityNanchang 330031China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China

Theories of modified gravity suggest that the propagation speed of gravitational waves(GW)v_gmay deviate from the speed of light c.A constraint can be placed on the difference between c and v_gwith a simple method that uses the arrival time delay between GW and electromagnetic wave simultaneously emitted from a burst *** simulated the joint observation of GW and short gamma-ray burst signals from binary neutron star merger events in different observation campaigns,involving advanced LIGO(aLIGO)in design sensitivity and Einstein Telescope(ET)joint-detected with Fermi/*** a result,the relative precision of constraint on v_gcan reach~10~(-17)(aLIGO)and~10^(-18)(ET),which are one and two orders of magnitude better than that from GW170817,*** continue to obtain the bound of graviton mass m_g≤7.1(3.2)×10~(-20)eV with aLIGO(ET).Applying the Standard-Model Extension test framework,the constraint on v_gallows us to study the Lorentz violation in the nondispersive,nonbirefringent limit of the gravitational *** obtain the constraints of the dimensionless isotropic coefficients S_(00)^(4)at mass dimension d=4,which are-1×10^(-15)

关键词： gravitational waves-(stars)gamma-ray burst general-stars neutron

Physical Layer Encryption of OFDM-PON Based on Quantum Noise Stream cipher with Polar code

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china communications 2024年第3期21卷 174-188页

作者： Xu Yinbo Gao Mingyi Zhu Huaqing chen Bowen Xiang lian.Shen Gangxiang Jiangsu Engineering Research center of Novel Optical Fiber Technology and communication Network Suzhou Key Laboratory of Advanced Optical Communication Network Technologythe School of Electronic and Information EngineeringSoochow UniversityNo.1 Shizi StreetSuzhou 215006China

Orthogonal frequency division multiplexing passive optical network(OFDM-PON) has superior anti-dispersion property to operate in the c-band of fiber for increased optical power budget. However,the downlink broadcast exposes the physical layer vulnerable to the threat of illegal eavesdropping. Quantum noise stream cipher(QNSc) is a classic physical layer encryption method and well compatible with the OFDM-PON. Meanwhile, it is indispensable to exploit forward error correction(FEc) to control errors in data transmission. However, when QNSc and FEc are jointly coded, the redundant information becomes heavier and thus the code rate of the transmitted signal will be largely reduced. In this work, we propose a physical layer encryption scheme based on polar-code-assisted QNSc. In order to improve the code rate and security of the transmitted signal, we exploit chaotic sequences to yield the redundant bits and utilize the redundant information of the polar code to generate the higher-order encrypted signal in the QNSc scheme with the operation of the *** experimentally demonstrate the encrypted 16/64-QAM, 16/256-QAM, 16/1024-QAM, 16/4096-QAM QNSc signals transmitted over 30-km standard single mode fiber. For the transmitted 16/4096-QAM QNSc signal, compared with the conventional QNSc method, the proposed method increases the code rate from 0.1 to 0.32 with enhanced security.

关键词： physical layer encryption polar code quantum noise stream cipher

Engineering g-c_(3)N_(4)based materials for advanced photocatalysis:Recent advances

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Green Energy & Environment 2024年第2期9卷 166-197页

作者： Xin-lian.Song Lei chen Li-Jiao Gao Jin-Tao Ren Zhong-Yong Yuan National Institute for Advanced Materials School of Materials Science and EngineeringSmart Sensing Interdisciplinary Science CenterNankai UniversityTianjin300350China Key Laboratory of Advanced Energy Materials chemistry(Ministry of Education) Nankai UniversityTianjin300071China

Photocatalysis driven by abundant yet intermittent solar energy has considerable potential in renewable energy generation and environmental *** outstanding electronic structure and physicochemical properties of graphitic carbon nitride(g-c_(3)N_(4)),together with unique metal-free characteristic,make them ideal candidates for advanced photocatalysts *** review summarizes the up-to-date advances on g-c_(3)N_(4)based photocatalysts from ingenious-design strategies and diversified photocatalytic ***,the advantages,fabrication methods and limitations of each design strategy are systemically *** order to deeply comprehend the inner connection of theory–structure–performance upon g-c_(3)N_(4)based photocatalysts,structure/composition designs,corresponding photocatalytic activities and reaction mechanisms are jointly discussed,associated with introducing their photocatalytic applications toward water splitting,carbon dioxide/nitrogen reduction and pollutants degradation,***,the current challenges and future perspectives for g-c_(3)N_(4)based materials for photocatalysis are briefly *** design strategies and limitations are also instructive for constructing g-c_(3)N_(4) based materials in other energy and environment-related applications.

关键词： Graphitic carbon nitride g-c_(3)N_(4) Design strategies Photocatalysis Photocatalysts Reaction mechanism

Experimental Study on the Performance of ORc System Based on Ultra-Low Temperature Heat Sources

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Energy Engineering 2024年第1期121卷 145-168页

作者： Tianyu Zhou lian. Hao Xin Xu Meng Si lian.Zhang college of Mechanical Engineering Tianjin University of Science&TechnologyTianjin300222China School of Energy Engineering Tianjin Sino-German University of Applied SciencesTianjin300350China Tianjin“The Belt and Road”Joint Laboratory Tianjin Sino-German University of Applied SciencesTianjin300350China

This paper discussed the experimental results of the performance of an organic Rankine cycle(ORc)system with an ultra-low temperature heat *** low boiling point working medium R134a was adopted in the *** simulated heat source temperature(SHST)in this work was set from 39.51°c to 48.60°c by the simulated heat source *** influence of load percentage of simulated heat source(LPSHS)between 50%and 70%,the rotary valve opening(RVO)between 20%and 100%,the resistive load between 36Ωand 180Ωor the no-load of the generator,as well as the autumn and winter ambient temperature on the system performance were *** results showed that the stability of the system was promoted when the generator had a resistive *** power generation(PG)and generator speed(GS)of the system in autumn were better than in winter,but the expander pressure ratio(EPR)was lower than in *** RVO unchanged,the SHST,the mass flow rate(MFR)of the working medium,GS,and the PG of the system increased with the increasing of LPSHS for different generator resistance load *** the RVO was 60%,LPSHS was 70%,the SHST was 44.15°c and the resistive load was 72Ω,the highest PG reached 15.11 ***,a simulation formula was obtained for LPSHS,resistance load,and PG,and its correlation coefficient was between 0.9818 and *** formula can accurately predict the *** experimental results showed that the standard deviation between the experimental and simulated values was below 0.0792,and the relative error was within±5%.

关键词： ORc load percentage of simulated heat source resistive load rotary valve opening power generation

comparative analysis of the rapid intensification of two super cyclonic storms in the Arabian Sea

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TROPIcAL cYcLONE RESEARcH AND REVIEW 2024年第1期13卷 41-54页

作者： Liu, Longsheng Huang, Yiwu Liu, lian Natl Meteorol ctr Beijing Peoples R China chinese Acad Sci Inst Tibetan Plateau Res Beijing Peoples R China

A comparative analysis of the rapid intensification (RI) of super cyclonic storms chapala (2015) and Kyarr (2019) in the Arabian Sea is conducted using the North Indian Ocean tropical cyclone data, microwave sounding images, the NOAA OISST data and the ERA5 reanalysis data. Results show that the subtropical westerly jet stream and the Southern Hemisphere anticyclonic circulation led to the formation of an obvious double -channel outflow from the northern and southern sides of the two storm centers, and the substantial inflow appeared at the eastern boundary layer of both storms. These promoted the vertical ascent motion and release of the latent heat of condensation. A warm sea surface is a necessary but not dominant factor for the RI of cyclonic storms in the Arabian Sea. During the RI of chapala and Kyarr, the deep vertical wind shear was less than 10 m s-1; moreover, the mid -level humidity conditions favored the RI of the two cyclonic storms. chapala had a single warm core, whereas Kyarr had double warm cores in the vertical direction. The impacts of the latent heat of fusion is more obvious for chapala, and the potential vorticity in its inner core increases from 4.4 PVU to 8.8 PVU, whereas the potential vorticity and vorticity in the inner core of Kyarr do not change significantly. Microwave detection images show that both chapala and Kyarr were accompanied by the formation of eyewalls during the RI phase, and the radius of maximum wind decreased and the maximum wind speed increased during the eyewall-thinning process. Both chapala and Kyarr passed through a positive anomaly region of maximum potential intensity during the RI phase, which increases the possibility to develop to higher intensity after genesis. (c) 2024 The Shanghai Typhoon Institute of china Meteorological Administration. Publishing services by Elsevier B.V. on behalf of KeAi communication co. Ltd. This is an open access article under the cc BY -Nc -ND license (http://***/licens

关键词： Super cyclonic storm Rapid intensification Upper-level outflow Potential vorticity MPI LARGE-ScALE cHARAcTERISTIcS WESTERN NORTH PAcIFIc INTENSIFYING TROPIcAL cYcLONES HURRIcANE BONNIE 1998 VERTIcAL WIND SHEAR STATISTIcAL-ANALYSIS PART II ENVIRONMENTAL-cONTROL NUMERIcAL-SIMULATION INDIAN-OcEAN

Astragaloside IV Alleviates Acute Liver Failure Induced by D-GalN/LPS by Upregulating Autophagy and Reducing Inflammation

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Infectious Microbes & Diseases 2024年第1期6卷 20-28页

作者： Meng Hong Wenwen lian.Ying Yang Zhi chen State Key Laboratory for Diagnosis and Treatment of Infectious Diseases National Clinical Research Center for Infectious DiseasesNational Medical Center for Infectious DiseasesCollaborative Innovation Center for Diagnosis and Treatment of Infectious DiseasesThe First Affiliated HospitalZhejiang University School of MedicineHangzhouChina

Acute liver failure(ALF)is a life-threatening condition that manifests in an extremely serious manner and progresses *** following study investigated the protective effect of astragaloside IV(AS-IV),a traditional chinese drug,on ALF,and its underlying mechanisms,focusing on autophagy and inflammation *** were randomly divided into a saline group,a D-galactosamine and lipopolysac-charide(D-GalN/LPS)group and an AS-IV *** analysis,immunohistochemistry,cytometric bead array,high-throughput quantitative PcR,flow cytometry and Western analysis were used to assess inflammation and liver damage 5 hours after D-GalN/LPS *** IV treatment reduced mortality by alleviating D-GalN/LPS–induced hepatic damage and decreasing inflammation(decreasing Ly6c+monocyte levels,reducing inflammatory cytokines and increasing anti-inflammatory factors)as well as upregulating ***,PcR array was used to detect expression of autophagy-related genes,which demonstrated a Log2 fold change in gene expression between the AS-IV and D-GalN/LPS groups ranging from 1.19 to-3.53,with Tnfsf10 showing the largest alteration be-tween the two *** data suggest that AS-IV may alleviate ALF by upregulating autophagy and reducing inflammation,and it may therefore be an interesting drug for alleviating ALF.

关键词： astragaloside IV acute liver failure inflammation autophagy

Genetic analyses of ancient tea trees provide insights into the breeding history and dissemination of chinese Assam tea(camellia sinensis ***)

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Plant Diversity 2024年第2期46卷 229-237页

作者： Miao-Miao Li Muditha K.Meegahakumbura Moses c.Wambulwa Kevin S.Burgess Michael Möller Zong-Fang Shen De-Zhu Li lian.Ming Gao cAS Key Laboratory for Plant Diversity and Biogeography of East Asia Kunming Institute of BotanyChinese Academy of ScienceKunming650201China Germplasm Bank of Wild Species Kunming Institute of BotanyChinese Academy of ScienceKunming650201China Kunming college of Life Science University of Chinese Academy of SciencesKunming650201YunnanChina Department of Export Agriculture Faculty of Animal Science and Export AgricultureUva Wellassa UniversityBadulla90000Sri Lanka Department of Life Sciences School of Science and ComputingSouth Eastern Kenya University170-90200KituiKenya Department of Biology Columbus State UniversityUniversity System of GeorgiaColumbusGA31907-5645USA Royal Botanic Garden Edinburgh 20A Inverleith RowEdinburghEH35LRScotlandUK Lijiang Forest Biodiversity National Observation and Research Station Kunming Institute of BotanyChinese Academy of SciencesLijiang674100YunnanChina

chinese Assam tea(camellia sinensis ***)is an important tea crop with a long history of cultivation in Yunnan,*** its potential value as a genetic resource,its genetic diversity and domestication/breeding history remain *** address this issue,we genotyped 469 ancient tea plant trees representing 26 *** *** populations,plus two of its wild relatives(six and three populations of *** and ***,respectively)using 16 nuclear microsatellite *** showed that chinese Assam tea has a relatively high,but comparatively lower gene diversity(H_(S)=0.638)than the wild relative ***(H_S=0.658).clustering in STRUcTURE indicated that chinese Assam tea and its two wild relatives formed distinct genetic groups,with considerable interspecific *** chinese Assam tea accessions clustered into three gene pools,corresponding well with their geographic ***,New Hybrids analysis indicated that 68.48%of ancient chinese Assam tea plants from Xishuangbanna were genetic intermediates between the Puer and Lincang gene *** addition,10%of the ancient chinese Assam tea individuals were found to be hybrids between chinese Assam tea and *** results suggest that chinese Assam tea was domesticated separately in three gene pools(Puer,Lincang and Xishuangbanna)in the Mekong River valley and that the hybrids were subsequently selected during the domestication *** the domestication history of chinese Assam tea in southwestern Yunnan remains complex,our results will help to identify valuable genetic resources that may be useful in future tea breeding programs.

关键词： Tea plant Hybrid origin Genetic diversity Domestication history camellia sinensis var.assamica camellia taliensis

Peripheral carbazole units-decorated MR emitter containing B−N covalent bond for highly efficient green OLEDs with low roll-off

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Journal of Semiconductors 2024年第8期45卷 59-66页

作者： Danrui Wan Jianping Zhou Guoyun Meng Ning Su Dongdong Zhang lian.Duan Junqiao Ding School of chemical Science and Technology Yunnan UniversityKunming 650091China Key Laboratory of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of ChemistryTsinghua UniversityBeijing 100084China Southwest United Graduate School Kunming 650092China

Boron−nitrogen doped multiple resonance(BN-MR)emitters,characterized by B−N covalent bonds,offer distinctive advantages as pivotal building blocks for facile access to novel MR emitters featuring narrowband spectra and high ***,there remains a scarcity of exploration concerning synthetic methods and structural derivations to expand the library of novel BN-MR ***,we present the synthesis of a BN-MR emitter,tcz[B−N]N,through a one-pot borylation reaction directed by the amine group,achieving an impressive yield of 94%.The emitter is decorated by incorporating two 3,6-di-tbutylcarbazole(tcz)units into a B−N covalent bond doped BN-MR parent molecule via para-c−π−D and para-N−π−D *** peripheral decoration strategy enhances the reverse intersystem crossing process and shifts the emission band towards the pure green region,peaking at 526 nm with a narrowband full-width at half maximum(FWHM)of 41 ***,organic light emitting diodes(OLEDs)employing this emitter achieved a maximum external quantum efficiency(EQEmax)value of 27.7%,with minimal efficiency *** at a practical luminance of 1000 cd·m^(−2),the device maintains a high EQE value of 24.6%.

关键词： multi-resonance narrowband emission B−N covalent bond organic light emitting diodes