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Flexible molecules dedicate to release strain of inverted inorganic perovskite solar cell

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Journal of Energy Chemistry 2025年第1期100卷 87-93页

作者： Hongrui Sun Sanlong Wang Pengyang Wang Yali Liu Shanshan Qi biao Shi Ying zhao Xiaodan Zhang Institute of Photoelectronic Thin Film Devices and Technology Renewable Energy Conversion and Storage Center State Key Laboratory of Photovoltaic Materials and CellsNankai University Key Laboratory of Photoelectronic Thin Film Devices and Technology of Tianjin Haihe Laboratory of Sustainable Chemical Transformations Engineering Research Center of Thin Film Photoelectronic Technology of Ministry of Education Collaborative Innovation Center of Chemical Science and Engineering (Tianjin)

The tensile strain in inorganic perovskite films induced by thermal annealing is one of the primary factors contributing to the inefficiency and instability of inorganic perovskite solar cells （IPSCs）,which reduces the defect formation ***,a flexible molecule 5-maleimidovaleric acid （5-MVA） was introduced as a strain buffer to release the residual strain of *** anhydride and carboxyl groups in 5-MVA interact strongly with the uncoordinated Pb2+through Lewis acid-base reaction,thus tightly“pull”the perovskite *** in-between soft carbon chain increased the structural flexibility of CsPbI2.85Br0.15perovskite materials,which effectively relieved the intrinsic internal strain of CsPbI2.85Br0.15,resisted the corrosion of external strain,and also reduced the formation of defects such as VIand *** addition,the introduction of 5-MVA improved crystal quality,passivated residual defects,and narrowed energy level ***,power conversion efficiency （PCE） of NiOxbased inverted IPSCs increased from 19.25% to 20.82% with the open-circuit voltage enhanced from 1.164 V to 1.230 *** release of strain also improved the stability of CsPbI2.85Br0.15perovskite films and devices.

关键词： Perovskite solar cells

Multifunctional Nacre‑Like Nanocomposite Papers for Electromagnetic Interference Shielding via Heterocyclic Aramid/MXene Template‑Assisted In‑Situ Polypyrrole Assembly

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Nano-Micro Letters 2025年第3期17卷 37-54页

作者： Jinhua Xiong Xu zhao Zonglin Liu He Chen Qian Yan Huanxin lian Yunxiang Chen Qingyu Peng Xiaodong He National Key Laboratory of Science and Technology On Advanced Composites in Special Environments Center for Composite Materials and StructuresHarbin Institute of TechnologyHarbin 150080People’s Republic of China

Robust, ultra-flexible, and multifunctional MXene-basedelectromagnetic interference (EMI) shielding nanocomposite filmsexhibit enormous potential for applications in artificial intelligence,wireless telecommunication, and portable/wearable electronic *** this work, a nacre-inspired multifunctional heterocyclic aramid(HA)/MXene@polypyrrole (PPy) (HMP) nanocomposite paper withlarge-scale, high strength, super toughness, and excellent tolerance tocomplex conditions is fabricated through the strategy of HA/MXenehydrogel template-assisted in-situ assembly of PPy. Benefiting from the"brick-and-mortar" layered structure and the strong hydrogen-bondinginteractions among MXene, HA, and PPy, the paper exhibits remarkable mechanical performances, including high tensile strength (309.7 MPa),outstanding toughness (57.6 MJ m−3), exceptional foldability, and structural stability against ultrasonication. By using the template effect ofHA/MXene to guide the assembly of conductive polymers, the synthesized paper obtains excellent electronic conductivity. More importantly,the highly continuous conductive path enables the nanocomposite paper to achieve a splendid EMI shielding effectiveness (EMI SE) of 54.1 dBat an ultra-thin thickness (25.4 μm) and a high specific EMI SE of 17,204.7 dB cm2g−1. In addition, the papers also have excellent applicationsin electromagnetic protection, electro-/photothermal de-icing, thermal therapy, and fire safety. These findings broaden the ideas for developinghigh-performance and multifunctional MXene-based films with enormous application potential in EMI shielding and thermal management.

关键词： MXene Remarkable mechanical properties Heterocyclic aramid Electromagnetic interference shielding Polypyrrole Multifunctionality

Exploring the impacts of major events on the systemic risk of the international energy market

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Petroleum Science 2024年第2期21卷 1444-1457页

作者： Ming-Tao zhao Su-Wan Lu lian-biao Cui School of Statistics and Applied Mathematics Anhui University of Finance and EconomicsBengbu233030AnhuiChina Anhui Province Key Laboratory of Philosophy and Social Science of Low-Carbon Development and Carbon Finance Anhui University of Finance and EconomicsBengbu233030AnhuiChina

This study examines the systemic risk caused by major events in the international energy market(IEM)and proposes a management strategy to mitigate it. Using the tail-event driven network(TENET)method, this study constructed a tail-risk spillover network(TRSN) of IEM and simulated the dynamic spillover tail-risk process through the cascading failure mechanism. The study found that renewable energy markets contributed more to systemic risk during the Paris Agreement and the COVID-19pandemic, while fossil energy markets played a larger role during the Russia-Ukraine conflict. This study identifies systemically important markets(SM) and critical tail-risk spillover paths as potential sources of systemic risk. The research confirms that cutting off the IEM risk spillover path can greatly reduce systemic risk and the influence of SM. This study offers insights into the management of systemic risk in IEM and provides policy recommendations to reduce the impact of shock events.

关键词： International energy market Tail-risk spillover Cascading failure mechanism Systemic risk management

Antiosteoporosis and bone protective effect of alpinumisoflavone in steroid-induced osteoporosis rats via alteration of apoptosis,inflammatory and RANK/RANKL/OPG signaling pathway

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Asian Pacific Journal of Tropical Biomedicine 2024年第10期14卷 436-447页

作者： Jie lian Jun-Long Qu Guo-Wei zhao Xu-biao Ji Department of Orthopaedics Luzhou Traditional Chinese Medicine HospitalLuzhouSichuan646000China Department of Orthopedic Rehabilitation Shengli Oilfield Central HospitalDongyingShandong257000China Department of Spinal Surgery Changzhou Wujin People's HospitalWujin Hospital Affiliated with Jiangsu UniversityChangzhouJiangsu213000China

Objective:To estimate the bone protective effect of alpinumisoflavone,a natural prenylated isoflavonoid,against glucocorticoid-induced osteoporosis in ***:Male Wistar rats received intramuscular administration of dexamethasone(4 mg/mL)at a dose level of 7 mg/kg for 5 weeks,and then alpinumisoflavone(5,10,and 15 mg/kg)and alendronate(2 mg/kg)from 2 *** body weight and organ weight(femoral,vagina,and uterus)were *** analysis,bone turnover markers,bone parameters,oxidative stress parameters,and inflammatory cytokines were *** expressions of related genes were also ***:Alpinumisoflavone remarkably boosted body weight and organ weight(ureters and vagina),improved microCT analysis parameters,and boosted levels of bone ***,alpinumisoflavone considerably(P<0.001)restored the level of bone turnover markers and oxidative stress parameters,remarkably suppressed the level of cytokines such as interleukin-1β,interleukin-6,tumor necrosis factor-α,and increased transforming growth factor-βand insulin-like growth *** also significantly restored the osteoprotegerin(OPG,RANKL,and OPG/RANKL ratio)levels and the mRNA expression of Caspase(3,6,7,9),BMPs,OPN,ALP,RUNX2,and ***:The current result suggests the bone protective effect of alpinumisoflavone against glucocorticoid-induced osteoporosis in rats.

关键词： Osteoporosis Alpinumisoflavone Bone parameters Inflammation Oxidative stress

Quantum-classical correspondence in integrable systems

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Science China(Physics,Mechanics & Astronomy) 2019年第9期62卷 95-103页

作者： Yiqiang zhao biao Wu International Center for Quantum Materials School of PhysicsPeking UniversityBeijing 100871China Collaborative Innovation Center of Quantum Matter Beijing 100871China Wilczek Quantum Center School of Physics and Astronomy Shanghai Jiao Tong UniversityShanghai 200240China

We find that the quantum-classical correspondence in integrable systems is characterized by two time scales. One is the Ehrenfest time below which the system is classical;the other is the quantum revival time beyond which the system is fully quantum. In between, the quantum system can be well approximated by classical ensemble distribution in phase space. These results can be summarized in a diagram which we call Ehrenfest diagram. We derive an analytical expression for Ehrenfest time, which is proportional to h-1/2. According to our formula, the Ehrenfest time for the solar-earth system is about 1026 times of the age of the solar system. We also find an analytical expression for the quantum revival time, which is proportional to h-1. Both time scales involve ω(I), the classical frequency as a function of classical action. Our results are numerically illustrated with two simple integrable models. In addition, we show that similar results exist for Bose gases, where 1/N serves as an effective Planck constant.

关键词： quantum-classical correspondence Ehrenfest time quantum revival time integrable systems

Highly luminescent zero-dimensional lead-free manganese halides forβ-ray scintillation

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Nano Research 2022年第9期15卷 8486-8492页

作者： Linyuan lian Wei Qi Huaiyi Ding Hao Tian Qi Ye Yong-biao zhao Long zhao Jianbo Gao Daoli Zhang Jianbing Zhang School of Optical and Electronic Information Huazhong University of Science and Technology1037 Luoyu RoadWuhan 430074China Hubei Key Laboratory of Bioinorganic Chemistry&Materia Medica School of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Yunnan Provincial Higher Education Institutions for Optoelectronics Device Engineering School of Physics and AstronomyYunnan UniversityKunming 650504China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China Department of Physics and Astronomy Ultrafast Photophysics of Quantum Devices LaboratoryClemson UniversityClemsonSC 29634USA Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China Shenzhen Huazhong University of Science and Technology Research Institute Shenzhen 518057China

Because of their moderate penetration power,β-rays(high-energy electrons)are a useful signal for evaluating the surface contamination of nuclear ***,the development ofβ-ray scintillators,which convert the absorbed high-energy electrons into visible photons,is hindered by the limitations of materials ***,we report two highly luminescent zerodimensional(0D)organic-inorganic lead-free metal halide hybrids,(C_(13)H_(30)N)_(2)MnBr_(4)and(C_(19)H_(34)N)_(2)MnBr_(4),as scintillators exhibiting efficientβ-ray *** hybrid scintillators combine the superior properties of organic and inorganic *** example,organic components that contain light elements C,H,and N enhance the capturing efficiency ofβparticles;isolated inorganic[MnBr_(4)]2−tetrahedrons serve as highly localized emitting centers to emit intense radioluminescence(RL)underβ-ray *** hybrids show a narrow-band green emission peaked at 518 nm with photoluminescence quantum efficiencies(PLQEs)of 81.3%for(C_(13)H_(30)N)_(2)MnBr_(4)and 86.4%for(C_(19)H_(34)N)_(2)MnBr_(4),*** enable the solution processing of this promising metal halide hybrid,we successfully synthesized(C_(13)H_(30)N)_(2)MnBr_(4)colloidal nanocrystals for the first *** excited byβ-rays,(C_(13)H_(30)N)_(2)MnBr_(4)scintillators show a linear response toβ-ray dose rate over a broad range from 400 to 2,800 Gy·s^(−1),and also display robust radiation resistance that 80%of the initial RL intensity can be maintained after an ultrahigh accumulated radiation dose of 240 *** work will open up a new route for the development ofβ-ray scintillators.

关键词： zero-dimensional metal halide hybrids radiation sterilization β-ray scintillation nanocrystals

基于改进DeblurGAN-v2的运动模糊农作物害虫图像复原方法

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光电子·激光 2025年第1期36卷 46-52页

作者：赵辉黄镖王红君岳有军天津理工大学电气工程与自动化学院天津市复杂系统控制理论与应用重点实验室

为对巡检机器人在巡检过程中产生的运动模糊图像进行高效精准识别，提出了一种基于改进DeblurGAN-v2的运动模糊农作物害虫图像复原方法。为有效提取图像重要特征，该方法将通道注意力(channel attention, CA)机制集成到DeblurGAN-v2主... 详细信息

为对巡检机器人在巡检过程中产生的运动模糊图像进行高效精准识别，提出了一种基于改进DeblurGAN-v2的运动模糊农作物害虫图像复原方法。为有效提取图像重要特征，该方法将通道注意力(channel attention, CA)机制集成到DeblurGAN-v2主干网格中，使模型更加关注细节特征，提高对运动模糊图像的复原能力；此外，在原模型特征提取网络顶层引入空间金字塔池化(spatial pryamid pooling, SPP)缓解图像多尺度变化造成对图像复原的负面影响，提高模型对图像复原的性能。基于实际农田环境建立的数据集所做的实验结果表明，改进后算法的PSNR、SSIM指标分别为26.281 8 dB、0.947 3,较原模型提升了8、7.2个百分点。与其他主流模型的对比实验结果表明，本文方法对模糊图像的实际复原效果更优，对解决运动模糊农作物害虫的图像复原问题具有实际应用价值。

关键词：运动模糊深度学习图像复原 DeblurGAN-v2 通道注意力(CA)机制空间金字塔池化(SPP)模块

DESIGN AND ANALYSIS OF THE GREEN CLIMATE FUND

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Journal of Systems Science and Systems Engineering 2014年第3期23卷 266-299页

作者： lian-biao CUI Lei ZHU Marco SPRINGMANN Ying FAN Center for Energy and Environmental Policy Research Institute of Policy and ManagementChinese Academy of Sciences Department of Economics University of Oldenburg

The Green Climate Fund （GCF） has been one of the core issues of the world climate summits under the United Nations Framework Convention on Climate Change （UNFCCC） in recent years. However, the GCF has not progressed smoothly, and currently there are no satisfactory schemes for raising and distributing the fund. This paper first discusses how to finance the GCF among Annex II countries. It introduces the ＇preference score compromises＇（PSC） approach which is based on environmental responsibility and economic capacity, with historical emissions as an indicator for environmental responsibility and GDP as indicator for economic capacity. The results show that the United States and the European Union are the two largest contributors to the GCF, sponsoring more than 80% of the funds. Second, we discuss how to allocate the funds among non-Annex II parties. The ＇adaptation needs＇（AN） approach, which takes account of economic strength and climate damages, is proposed to achieve the adaptation purpose of the GCF, and the results reveal that African countries with high levels of climate vulnerability could get most funds, with a share of almost 30%. Regarding the mitigation purpose of the GCF, this research introduces two approaches： the ＇carbon reduction contribution＇（CC） approach and the ＇incremental cost＇（IC） approach. Both approaches could achieve significant reductions in carbon emissions in non-Annex II parties, whereas the latter may provide limited adaptation finance but result in more mitigation effects. This paper also develops a method to combine abatement efficiency and adaptation fairness of the GCF, and we find that with an equal split between the AN and CC （or AN and IC） approaches, the amount of USD 100 billion could finance an emissions reduction of 1613 MtCO2 （2477 MtCO2）, while allocating USD 16 （or USD 9） per capita for adaptation in non-Annex II parties. The schemes proposed may be useful for promoting the development of the GCF in the future.

关键词： Climate change green climate fund preference score compromises carbon reductioncontribution mitigation and adaptation

Intrinsic mechanism and multiphysics analysis of electromagnetic wave absorbing materials: New horizons and breakthrough

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Journal of Materials Science & Technology 2022年第35期130卷 136-156页

作者： Long Xia Yuming Feng biao zhao School of Materials Science and Engineering Harbin Institute of Technology at WeihaiWeihai 264209China School of Microelectronics Fudan UniversityShanghai 200433China

Electromagnetic absorbers(EMA) have driven the development of Electromagnetic(EM) technology and advanced EM devices. Utilizing the EM energy conversion of EM absorbers to design various devices is attractive and promising, especially in personal protection and healthcare. In this review article, the simulation and numerical analysis of EM materials are reviewed, from numerical analysis of dielectric parameters, simulation of wave absorbing performance, electromagnetic performance improvement, and structural construction optimization. For the EM response mechanism, radiation-dependent relaxation and charge transport energy transitions are dissected. For the EM calculation section, two leading roles are highlighted, including the purposeful design of EM and the provision of theoretical guidance for optimizing electromagnetic absorption performance. In addition, this work points out the current problems and potential opportunities in the numerical simulation of absorbing materials, points out the new development direction, and proposes prospects.

关键词： Microwave absorption Multiphysics simulation Dielectric parameters EMA Properties optimization