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Additives strategies to improving cycling stability of li metal batteries by modifying electrode electrolyte interphases

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Progress in Natural Science:Materials international 2024年第2期34卷 338-344页

作者： Yuan li Pengfei Huang Chunyu Cui Xiaoyuan Ma li Chen Zekun li linhai li Yuhong Tian School of Biological and Chemical Engineering Guangxi University of Science and Technology School of College of Chemistry and Chemical Engineering Hunan University isky future Energy institute

li metal batteries（LMBs） have attracted much attention due to the ultra-high theoretical capacity of the li metal anode（LMA）.However,the uncontrollable dendrites growth and low coulombic efficiency hinder their practical ***,we explore 3,5-difluoropyridine（2f-BD） as a novel electrolyte additive to enable highperformance *** 2f-BD additive participates in and modifies the solvation structure of li ions by reducing the coordinated number of Pf6-at the electrode surface,leading to the formation of a lif and li3N-rich solid electrolyte interphase（SEi）.The lif component increases the robustness of SEi and suppresses the formation of li dendrites,while the li3N component facilitates the transportation and reaction kinetics of li *** a result,the li‖li symmetric cell presents a stable cycling performance of up to 500 h at a current density of 1 mA *** coupling with lifePO4cathode,the obtained full cell achieves high specific capacities of 106.06 mA h g-1and 84.98 mA h g-1at 2.55 mA cm-2and 5.10 mA cm-2,respectively,and maintains a high capacity retention of84.0% after 1000 cycles at 0.13 mA cm-2,with an average cycling CE of 99.58%.

关键词： li metal batteries li dendrites Electrolyte additive

Rainbow Pancyclicity in a Collection of Graphs Under the Dirac-type Condition

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 269-274页

作者： Lu-yi li Ping li Xue-liang li Center for Combinatorics and LPMC Nankai UniversityTianjin 300071China School of Mathematics and Statistics Shaanxi Normal UniversityXi’an 710062China

Let G={gi:i∈[n]} be a collection of not necessarily distinct n-vertex graphs with the same vertex set V,where G can be seen as an edge-colored(multi)graph and each gi is the set of edges with color i.A graph f on V is called rainbow if any two edges of f come from different gis’.We say that G is rainbow pancyclic if there is a rainbow cycle Cℓof lengthℓin G for each integerℓ2[3,n].in 2020,Joos and Kim proved a rainbow version of Dirac’s theorem:ifδ(gi)≥2/n for each i∈[n],then there is a rainbow Hamiltonian cycle in *** this paper,under the same condition,we show that G is rainbow pancyclic except that n is even and G consists of n copies of Kn/2,n/*** result supports the famous meta-conjecture posed by Bondy.

关键词： rainbow Hamiltonian cycle rainbow pancyclic meta-conjecture

Long-term integration Ability of the Submillimeter Wave Astronomy Satellite(SWAS)Spectral line Receivers

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Research in Astronomy and Astrophysics 2024年第6期24卷 315-322页

作者： Bing-Ru Wang Di li Paul f.Goldsmith Jingwen Wu Chao-Wei Tsai Rudolf Schieder Gary J.Melnick National Astronomical Observatories Chinese Academy of SciencesBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China Research Center for Astronomical Computing Zhejiang LaboratoryHangzhou 311100China Jet Propulsion Laboratory California Institute of TechnologyPasadenaCA 91109USA institute for frontiers in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China KOSMA I.Physik.InstitutUniversität zu KölnZülpicher Str.7750937 KölnGermany Center for Astrophysics|Harvard&Smithsonian 60 Garden StreetMS 66CambridgeMA 02138USA

The Submillimeter Wave Astronomy Satellite(SWAS)was the first space telescope capable of high spectral resolution observations of terahertz spectral *** have investigated the integration ability of its two receivers and spectrometer during five and a half years of on-orbit *** Ci,O_(2),H_(2)O,and^(13)CO spectra taken toward all observed Galactic sources were *** present results are based on spectra with a total integration time of up to 2.72×10~4hr(■10~8s).The noise in the spectra is generally consistent with that expected from the radiometer equation,without any sign of approaching a noise *** noise performance reflects the extremely stable performance of the passively cooled front end as well as other relevant components in the SWAS instrument throughout its mission lifetime.

关键词： telescopes space vehicles:instruments instrumentation:miscellaneous iSM:lines and bands

Machine Learning-based identification of Contaminated images in light Curve Data Preprocessing

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Research in Astronomy and Astrophysics 2024年第4期24卷 287-295页

作者： Hui li Rong-Wang li Peng Shu Yu-Qiang li Yunnan Observatories Chinese Academy of SciencesKunming 650216China University of Chinese Academy of Sciences Beijing 100049China Key Laboratory of Space Object and Debris Observation Chinese Academy of SciencesNanjing 210023China

Attitude is one of the crucial parameters for space objects and plays a vital role in collision prediction and debris *** light curves to determine attitude is the most commonly used *** photometric observations,outliers may exist in the obtained light curves due to various ***,preprocessing is required to remove these outliers to obtain high quality light *** statistical analysis,the reasons leading to outliers can be categorized into two main types:first,the brightness of the object significantly increases due to the passage of a star nearby,referred to as“stellar contamination,”and second,the brightness markedly decreases due to cloudy cover,referred to as“cloudy contamination.”The traditional approach of manually inspecting images for contamination is time-consuming and ***,we propose the utilization of machine learning methods as a *** Neural Networks and SVMs are employed to identify cases of stellar contamination and cloudy contamination,achieving f1 scores of 1.00 and 0.98 on a test set,*** also explore other machine learning methods such as ResNet-18 and light Gradient Boosting Machine,then conduct comparative analyses of the results.

关键词： techniques:image processing methods:data analysis light pollution

Precise separation and efficient recovery of Pd(Ⅱ) from high-level liquid waste by XAD-based adsorbents

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Rare Metals 2024年第10期43卷 5372-5390页

作者： Hao-Ran Dong Shun-Yan Ning Zeng-Yuan li Si-Zhi Xu feng-Tao Hu feng Gao You-Bin Wang li-feng Chen Xiang-Biao Yin Toyohisa fujita Mohammed f.Hamza Yue-Zhou Wei School of Resources Environment and MaterialsGuangxi University School of Nuclear Science and Technology University of South China

Efficient separation of palladium (Pd（ii）) from high-level liquid waste （HLLW） not only helps the safe disposal of nuclear waste,but also is a vital importan supplement to Pd（ii） ***,16 kinds of nove Amberlite XAD resins-based adsorbents were prepared by vacuum impregnation method for the separation of Pd（ii）from simulated HLLW,and the MMBT/XAD7HP prepared using 4-methyl-2-mercaptobenzothiazole （MMBT） as ligand and Amberlite XAD7HP resin （XAD7HP） as the carrier was selected as the optimal research *** analysis experiments proved the successful preparation of MMBT/XAD7HP,which exhibited ultrahigh adsorption selectivity for Pd（ii）(distribution coefficient （Kd）≥12584.5 ml·g-1,separation factor (SfPd/M)≥2818.4) and superior adsorption capacity(Q≥130.1 mg·g-1).The adsorption kinetics and adsorption isotherms for Pd（ii） matched with pseudo-secondorder （PSO） kinetics model and Langmuir model,indicating that the adsorption mode for Pd（ii） by MMBT/XAD7 HP was monolayer chemical *** dynamic column experiments showed that MMBT/XAD7 HP achieved efficiently separation of Pd（ii） from simulated HLLW,and the recovery rate was nearly 100% The adsorption mechanism was analyzed by fourier transform infrared spectroscopy （fTiR）,X-ray photoelectron spectroscopy （XPS） and density functional theory（DfT）,and the ultrahigh selectivity of MMBT/XAD7 HP is attributed to the preferred affinity of the soft-N,S donor atoms in MMBT for Pd（ii）.MMBT has the shortest frontline molecular orbital energy band gap （HOMO–LUMO） among the four ligands,which makes it easier to become an electron donor to attract Pd2+to participate in ***3-participates in the adsorption to keep charge *** summary,MMBT/XAD7 HP has broad application prospects for the treatment of Pd（ii） in HLLW

关键词： Adsorption Column experiments HLLW Palladium XAD

Towards efficient strain engineering of 2D materials:A four-points bending approach for compressive strain

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Nano Research 2024年第6期17卷 5317-5325页

作者： Hao li félix Carrascoso Ana Borrás Gloria P.Moreno francisco J.Aparicio Ángel Barranco Andrés Castellanos Gómez Campus de Cantoblanco Instituto de Ciencia de Materiales de MadridC.Sor Juana Inés de la Cruz328049 MadridSpain Nanotechnology on Surfaces and Plasma Lab Instituto de Ciencia de Materiales de Sevilla(CSIC-Universidad de Sevilla).C/Americo Vespucio 49E-41092 SevilleSpain Departamento de física Aplicada i Escuela Politécnica SuperiorUniversidad de Sevillac/Virgen deÁfrica 7E-41011 SevilleSpain

Strain engineering,as a powerful strategy to tune the optical and electrical properties of two-dimensional(2D)materials by deforming their crystal lattice,has attracted significant interest in recent years.2D materials can sustain ultra-high strains,even up to 10%,due to the lack of dangling bonds on their surface,making them ideal brittle *** remarkable mechanical resilience,together with a strong strain-tunable band structure,endows 2D materials with a broad optical and electrical response upon ***,strain engineering based on 2D materials is restricted by their nanoscale and strain quantification *** this study,we have modified a homebuilt three-points bending apparatus to transform it into a four-points bending apparatus that allows for the application of both compressive and tensile strains on 2D *** approach allows for the efficient and reproducible construction of a strain system and minimizes the buckling effect caused by the van der Waals interaction by adamantane encapsulation *** results demonstrate the feasibility of introducing compressive strain on 2D materials and the potential for tuning their optical and physical properties through this approach.

关键词： uniaxial compressive strain polymer encapsulation differential reflectance spectroscopy exciton tunability

Leaching kinetics of fluorine during the aluminum removal from spent li-ion battery cathode materials

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Journal of Environmental Sciences 2024年第4期138卷 312-325页

作者： Shengjie li Jianxin Zhu Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

The high content of aluminum(Al)impurity in the recycled cathode powder seriously affects the extraction efficiency of Nickel,Cobalt,Manganese,and lithium resources and the actual commercial value of recycled materials,so Al removal is crucially important to conform to the industrial standard of spent li-ion battery cathode *** this work,we systematically investigated the leaching process and optimum conditions associated with Al removal from the cathode powder materials collected in a wet cathode-powder peeling and recycling production line of spent li-ion batteries(liBs).Moreover,we specifically studied the leaching of fluorine(f)synergistically happened along with the removal process of Al,which was not concerned about in other studies,but one of the key factors affecting pollution prevention in the recovery *** mechanism of the whole process including the leaching of Al and f from the cathode powder was indicated by using NMR,fTiR,and XPS,and a defluoridation process was preli.i.arily investigated in this *** leaching kinetics of Al could be successfully described by the shrinking core model,controlled by the diffusion process and the activation energy was 11.14 kJ/***,the leaching of f was attributed to the dissolution of liPf6and decomposition of PVDf,and the kinetics associated was described by Avrami *** interaction of Al and f is advantageous to realize the defluoridation to some *** is expected that our investigation will provide theoretical support for the large-scale recycling of spent liBs.

关键词： Al removal f leaching Cathode powder Heating alkali leaching Leaching kinetics

A Novel Tensor Decomposition-Based Efficient Detector for Low-Altitude Aerial Objects With Knowledge Distillation Scheme

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iEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 487-501页

作者： Nianyin Zeng Xinyu li Peishu Wu Han li Xin Luo Department of instrumental and Electrical Engineering Xiamen UniversityXiamen 361005China iEEE College of Computer and information Science Southwest UniversityChongqing 400715China

Unmanned aerial vehicles(UAVs) have gained significant attention in practical applications, especially the low-altitude aerial(LAA) object detection imposes stringent requirements on recognition accuracy and computational resources. in this paper, the LAA images-oriented tensor decomposition and knowledge distillation-based network(TDKD-Net) is proposed,where the TT-format TD(tensor decomposition) and equalweighted response-based KD(knowledge distillation) methods are designed to minimize redundant parameters while ensuring comparable performance. Moreover, some robust network structures are developed, including the small object detection head and the dual-domain attention mechanism, which enable the model to leverage the learned knowledge from small-scale targets and selectively focus on salient features. Considering the imbalance of bounding box regression samples and the inaccuracy of regression geometric factors, the focal and efficient ioU(intersection of union) loss with optimal transport assignment(f-EioU-OTA)mechanism is proposed to improve the detection accuracy. The proposed TDKD-Net is comprehensively evaluated through extensive experiments, and the results have demonstrated the effectiveness and superiority of the developed methods in comparison to other advanced detection algorithms, which also present high generalization and strong robustness. As a resource-efficient precise network, the complex detection of small and occluded LAA objects is also well addressed by TDKD-Net, which provides useful insights on handling imbalanced issues and realizing domain adaptation.

关键词： Attention mechanism knowledge distillation(KD) object detection tensor decomposition(TD) unmanned aerial vehicles(UAVs)

Joint fuzzy background and adaptive foreground model for moving target detection

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frontiers of Computer Science 2024年第2期18卷 93-106页

作者： Dawei ZHANG Peng WANG Yongfeng DONG linhao li Xin li School of Artificial intelligence Hebei University of TechnologyTianjin 300401China Lane Department of Computer Science and Electrical Engineering West Virginia UniversityMorgantownWV 26506-6109USA

Moving target detection is one of the most basic tasks in computer *** conventional wisdom,the problem is solved by iterative optimization under either Matrix Decomposition(MD)or Matrix factorization(Mf)*** utilizes foreground information to facilitate background *** uses noise-based weights to fine-tune the *** both noise and foreground information contribute to the recovery of the *** jointly exploit their advantages,inspired by two framework complementary characteristics,we propose to simultaneously exploit the advantages of these two optimizing approaches in a unified framework called Joint Matrix Decomposition and factorization(JMDf).To improve background extraction,a fuzzy factorization is *** fuzzy membership of the background/foreground association is calculated during the factorization process to distinguish their contributions of both to background *** describe the spatio-temporal continuity of foreground more accurately,we propose to incorporate the first order temporal difference into the group sparsity constraint *** temporal constraint is adjusted *** foreground and the background are jointly estimated through an effective alternate optimization process,and the noise can be modeled with the specific probability *** experimental results of vast real videos illustrate the effectiveness of our *** with the current state-of-the-art technology,our method can usually form the clearer background and extract the more accurate ***-noise experiments show the noise robustness of our method.

关键词： matrixdecomposition matrix factorization generalized sparsity noise modeling