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fabrication of heteroatom-doped cobalt oxide yolk–shell microsphere using recycled solution from waste materials and their excellent electrochemical properties as an anode material for lithium-ion batteries

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Rare Metals 2024年第10期43卷 4934-4947页

作者： Yeong Beom Kim Chanho Kim Seung-Hyun Kim Yun Chan Kang Dongju Lee gi Dae Park Department of Advanced Materials Engineering Chungbuk National University Department of Materials Science and Engineering Korea University Research institute YKSintering Co.Ltd.

Heteroatom-doped transition metal oxides have attracted great attention as advanced anode materials for lithium-ion batteries due to their high theoretical capacity and superior ***,the limited resource availability has led to a substantial rise in prices for valuable metals such as Ni and Co,posing a significant challenge for their *** address this issue,recycling of these metals from waste materials have gained prominence,and particularly the recovery of Co has been mostly focused on its economic ***,we introduced a novel recycling strategy for fabrication of heteroatomdoped CoOx（comprising mainly Co3O4with a minor CoO phase） anode with a yolk–shell structure for lithium-ion batteries,by separating Co from cemented tungsten carbide *** employing a simple leaching process and subsequent spray pyrolysis,the yolk–shell structured microsphere comprising CoOxwas successfully ***,the presence of other waste metals in the leachate facilitated multi-heteroatom doping during ***,the introduction of various dopants into CoOxinduced oxygen vacancy formation,thereby enhancing the electrochemical properties of the *** a result,compared with the phase-pure （undoped） CoOxyolk–shell,the heteroatom-doped CoOxyolk–shell exhibited robust cycling stability (602 mAh·g-1for 200 cycles at 1 A·g-1) and excellent rate capability(210 mAh·g-1at 10 A·g-1).

关键词： Anode Cobalt oxide Heteroatom doping lithium-ion batteries Recycling

An intrinsically self-healing and anti-freezing molecular chains induced polyacrylamide-based hydrogel electrolytes for zinc manganese dioxide batteries

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Journal of Energy Chemistry 2024年第2期89卷 565-578,I0013页

作者： Haiyang liao Wenzhao Zhong Chen li Jieling Han Xiao Sun Xinhui Xia Ting li Abolhassan Noori Mir f.Mousavi Xin liu Yongqi Zhang institute of fundamental and frontier Sciences University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina School of Mechanical Engineering Hunan University of TechnologyZhuzhou 412007HunanChina School of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014ZhejiangChina Department of Chemistry Faculty of Basic SciencesTarbiat Modares UniversityTehran 14117-13116Iran State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200HubeiChina

The anti-freezing strategy of hydrogels and their self-healing structure are often contradictory,it is vital to break through the molecular structure to design and construct hydrogels with intrinsic anti-freezing/self-healing for meeting the rapid development of flexible and wearable devices in diverse service ***,we design a new hydrogel electrolyte(Af/SH-Hydrogel)with intrinsic anti-freezing/self-healing capabilities by introducing ethylene glycol molecules,dynamic chemical bonding(disulfide bond),and supramolecular interaction(multi-hydrogen bond)into the polyacrylamide molecular *** to the exceptional freeze resistance(84%capacity retention at-20℃)and intrinsic self-healing capabilities(95%capacity retention after 5 cutting/self-healing cycles),the obtained Af/SH-Hydrogel makes the zinc||manganese dioxide cell an economically feasible battery for the state-of-the-art *** Zn||Af/SH-Hydrogel||MnO_(2)device offers a near-theoretical specific capacity of 285 m A h g^(-1)at 0.1 A g^(-1)(Coulombic efficiency≈100%),as well as good self-healing capability and mechanical flexibility in an ice *** work provides insight that can be utilized to develop multifunctional hydrogel electrolytes for application in next generation of self-healable and freeze-resistance smart aqueous energy storage devices.

关键词： flexible aqueous battery Hydrogel electrolyte Anti-freezing Self-healing Dual-dynamic reversible bond

Microstructure evolution and shape memory behaviors of Ni_(47)Ti_(44)Nb_(9)alloy subjected to multistep thermomechanical loading with different prestrain levels

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Journal of Materials Science & Technology 2024年第4期171卷 80-93页

作者： Y.H.Zhang H.li Z.W.Yang X.liu Q.f.Gu State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Shaanxi Key Laboratory of High-Performance Precision forming Technology and Equipment Northwestern Polytechnical UniversityXi’an 710072China

Ni_(47)Ti_(44)Nb_(9)shape memory alloy(SMA)is a promising material in the aerospace field due to its wide transformation *** application of shape memory effect depends on multistep thermomechan-ical loading,viz.,low-temperature deformation and subsequent heating to ***-temperature deformation prestrain plays a pivotal role in shape memory properties tailoring of SMA ***,microstructure evolution and deformation mechanisms of Ni_(47)Ti_(44)Nb_(9)SMA subjected to vari-ous prestrain levels are still *** this end,microstructure evolution and shape memory behaviors of Ni_(47)Ti_(44)Nb_(9)alloy subjected to multistep thermomechanical loading with prestrain levels of 8%-16%at-28℃(M_(s)+30℃)were *** results demonstrate that the stress-strain curve of the specimen exhibits four distinct stages at a maximal prestrain of 16%.Whereas stageⅡand stageⅢend at prestrains of∼8%and∼12%,*** stageⅡ,the stress-induced martensitic transformation is accompanied by the dislocation slip of the NiTi matrix andβ-Nb *** stageⅢ,in addition to the higher density of dislocations and further growth of stress-induced martensite variants(SiMVs),(001)compound twins are introduced as a result of the(001)deformation twinning in stress-induced ***{20-1}martensite twins are gradually introduced in stageⅣ.Correspondingly,after subsequent unloading and heating,a higher density ofiaustenite twins form in the specimen with a larger prestrain of 16%.With increasing prestrain from 8%to 16%,the recoverable strainε_(re)^(T)upon heating increases first and then ***ε_(re)^(T)obtains a maximum of 7.03%at 10%prestrain and de-creases to 6.17%at 16%*** increase ofε_(re)^(T)can be attributed to the formation of new SiMVs,the further growth of existing SiMVs,and the recoverable(001)compound *** the decrease ofε_(re)^(T)is mainly associated with the irrecoverable strain by{20−1}martensite *** effe

关键词： Ni_(47)Ti_(44)Nb_(9)shape memory alloy Wide transformation hysteresis Thermomechanical loading Microstructure evolution Shape memory behaviors Stress-induced martensitic transformation Deformation twinning

A review:the mechanism of plant-derived polysaccharides on osteoblasts and osteoclasts

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未来食品学报(英文) 2024年第3期4卷 183-192页

作者： Mengjie Ren Adel f.Ahmed Meng li Menghan li Zhiruo Yan Jinmei Wang National R&D Center for Edible fungus Processing Technology Henan UniversityKaifeng 475004China Joint international Research Laboratory of food&Medicine Resource function Henan ProvinceKaifeng 475004China Medicinal and Aromatic Plants Researches Department Horticulture Research InstituteAgricultural Research CenterGiza 12511Egypt

Bone loss and deterioration of bone microarchitecture would increase the bone fragility and fracture risk,leading to the *** and more evidences proved that plant-derived polysaccharides could have a remarkable influence on osteoblasts and osteoclasts,exerting anti-osteoporosis *** to the previous research,the extract of Cibotium barumoz,Achyranthes bidentata,Curculigo orchioides,Epimedium brevicornum,Angelica sinensis,Polygonatum sibiricum,Dendrobium officinale,Morinda officinalis,Nelumbo mucifera,Diospyros kaki,Hordeum vulgare,Cistanche deserticola,Commiphora Myrrha and other plant-derived polysaccharides could benefit to the osteoblasts and *** essential mechanisms are mainly related to the activation or inhibition of many factors,including runt-related transcription factor 2(Runx2),B-catenin,osterix(Osx),activator protein-1(AP-1),osteocalcin(OCN/BGP),alkaline phosphatase(ALP),osteopontin(OPN),bone morphogenetic protein(BMP),phosphatidylinositol 3-kinase(Pi3K)/C-Jun N-terminal kinase(JNK)/extracellular regulated protein kinase(ERK),osteoprotegerin(OPG),receptor activator of nuclear factor-kB(RANK),monocyte/macrophage colony-stimulating factor(M-CSf),tumor necrosis factor receptor-associated factor 6(TRAf-6),receptor activator of nuclear factor(Nf)-KB ligand(RANKL),nuclear factor of activated T cells 1(NfATc1),c-fos,matrix metallopeptidase-9(MMP-9),glycogen synthase kinase 3β(GSK3B)/B-catenin,nuclear factor E2-related factor 2(Nf2),as well as these related pathways,such as Wnt/p-catenin,BMP-2/SMAD1/5/8,Pi3K/AKT,OPG/RANKL/RANK,Nf-κB,MAPKs,*** plant-derived polysaccharides could improve the dynamic balance of bone formation and resorption through promoting the differentiation and maturation of osteoblast or inhibiting its *** reviewed plant-derived polysaccharides and their regulating mechanisms on the osteoclasts and osteoblasts provide the evidences for the development of osteoporosis therapeutics.

关键词： Osteoporosis Plant-derived polysaccharides Osteogenesis promotion Osteoclasts inhibition

fast efficient photon deceleration in plasmas by using two laser pulses at different frequencies

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Matter and Radiation at Extremes 2024年第3期9卷 11-18页

作者： Y.X.Wang X.L.Zhu S.M.Weng P.li X.f.li H.Ai H.R.Pan Z.M.Sheng Key Laboratory for Laser Plasmas(moe) School of Physics and AstronomyShanghai Jiao Tong UniversityShanghai 200240China Collaborative innovation Center of ifSA Shanghai Jiao Tong UniversityShanghai 200240China Research Center of Laser fusion of China Academy of Engineering Physics MianyangSichuan 621900China State key Laboratory of High field Laser Physics Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Tsung-dao Lee institute Shanghai Jiao Tong UniversityShanghai 200240China

The generation of ultrashort high-power light sources in the mid-infrared(mid-iR)to terahertz(THz)range is of interest for applications in a number of fields,from fundamental research to biology and *** conventional laser technology,photon deceleration in plasma wakes provides an alternative approach to the generation of ultrashort mid-iR or THz ***,we present a photon deceleration scheme for the efficient generation of ultrashort mid-iR or THz pulses by using an intense driver laser pulse with a relatively short wavelength and a signal laser pulse with a relatively long *** signal pulse trails the driver pulse with an appropriate time delay such that it sits at the front of the second wake bubble that is driven by the driver *** to its relatively long wavelength,the signal pulse will be subjected to a large gradient of the refractive index in the plasma wake ***,the photon deceleration in the plasma wake becomes faster and more efficient for signal pulses with longer *** greatly enhances the capacity and efficiency of photon deceleration in the generation of ultrashort high-power light sources in the long-wavelength iR and THz spectral ranges.

关键词： laser ultrashort photon

Genetic characteristics of H1N1 influenza virus outbreak in China in early 2023

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Virologica Sinica 2024年第3期39卷 520-523页

作者： Xuanxuan li Zefeng Dong Jiaming li Chuanran Dou Deyu Tian Zhenghai Ma Wenjun liu George f.Gao Yuhai Bi College of life Science and Technology Xinjiang UniversityUrumchi830046China CAS Key Laboratory of Pathogen Microbiology and immunology Institute of MicrobiologyCenter for Influenza Research and Early-warning(CASCIRE)CAS-TWAS Center of Excellence for Emerging Infectious Diseases(CEEID)Chinese Academy of SciencesBeijing100101China Suzhou Center for Disease Control and Prevention Suzhou215004China Lafayette College EastonPA 18042USA University of Chinese Academy of Sciences Beijing100049China D.H.Chen School of Universal Health Zhejiang UniversityHangzhou 310058China

Dear Editor,influenza A virus(iAV)exhibits rapid mutability and antigenic *** the 20th century,iAV has caused at least four pandemics(Yang et al.,2022).Presently,seasonal H_(3)N_(2)and H1N1 are the prevailing human-adaptive iAV subvariants responsible for human *** implementation of public health interventions since the commencement of the COViD-19 pandemic has effectively curtailed global influenza circulation(Olsen et al.,2021).following the downregulation of the prevention and control strategies against COViD-19,global influenza activity is showing a recovery.

关键词： influenza prevention H1N1

Editorial for Special issue on Artificial intelligence for Art

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Machine intelligence Research 2024年第1期21卷 1-3页

作者： Luntian Mou feng Gao Zijin li Jiaying liu Hongxun Yao Johan f.Hoorn Beijing University of Technology China Peking University China Central Conservatory of Music China Harbin institute of Technology China The Hong Kong Polytechnic University China

As an innovative engine for digital content generation,Ai-generated content(AiGC)has drawn more and more attention from academic fields as well as *** in the area of art creation,Ai has demonstrated its great potential and gained increasing *** are greatly impressed by Ai painting,composing,writing,virtual hosting,fashion,and ***,Ai is also becoming capable of understanding art,evaluating the aesthetic value of art,and protecting the copyright of art as *** has not only exhibited creativity to some extent,but also served as an enabling tool to discover the principles underneath creativity and imagination,which are traditional challenges for neuroscience,cognitive science,and *** all these promising features of Ai for art,we still have to face the many challenges such as the explainability of generative models and the copyright issues of Ai art works.

关键词： gained becoming spite

Guidance strategy of motion camouflage for spacecraft pursuit-evasion game

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Chinese Journal of Aeronautics 2024年第3期37卷 312-319页

作者： Jianqing li Chaoyong li Yonghe ZHANG Space information Research institute Hangzhou Dianzi UniversityHangzhou 310018China College of Electrical Engineering Zhejiang UniversityHangzhou 310027China Key Lab of Microsatellites Chinese Academy of SciencesShanghai 201210China

This work is inspired by a stealth pursuit behavior called motion camouflage whereby a pursuer approaches an evader while the pursuer camouflages itself against a predetermined *** formulate the spacecraft pursuit-evasion problem as a stealth pursuit strategy of motion camouflage,in which the pursuer tries to minimize a motion camouflage index defined in this *** Euler-Hill reference frame whose origin is set on the circular reference orbit is used to describe the *** on the rule of motion camouflage,a guidance strategy in open-loop form to achieve motion camouflage index is derived in which the pursuer lies on the camouflage constraint line connecting the central spacecraft and *** order to dispose of the dependence on the evader acceleration in the open-loop guidance strategy,we further consider the motion camouflage pursuit problem within an infinite-horizon nonlinear quadratic differential *** saddle point solution to the game is derived by using the state-dependent Riccati equation method,and the resulting closed-loop guidance strategy is effective in achieving motion *** are performed to demonstrate the capabilities of the proposed guidance strategies for the pursuit–evasion game scenario.

关键词： Pursuit-evasion problem Motion camouflage Differential game Guidance strategy Orbit control

Amelioration of habitat since the early Holocene contributed to the origin of agriculture in the farming-pastoral zone of northern China

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Science China Earth Sciences 2024年第8期67卷 2535-2546页

作者： Xin JiA Zhiping ZHANG Yonggang SUN Runqi JiANG Shuangwen Yi Wei CHEN Jue SUN Guoqiang li Shuzhi WANG Enrui li Xiaonong HU Qingchun BAO Harry f.LEE Huayu LU Jiangsu Center for Collaborative innovation in Geographical information Resource Development and Application Nanjing 210023China Schlool of History and Culture Chifeng UniversityChifeng 024000China School of Geography and Ocean Science Nanjing UniversityNanjing 210023China State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and PalaeontologyChinese Academy of SciencesNanjing 210008China Key Laboratory of Western China’s Environmental Systems(Ministry of Education) College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China institute of Archaeology Chinese Academy of Social SciencesBeijing 100710China Ulanqab Museum Ulanqab 012000China The institute of Cultural Relics and Archaeology Hohhot 010011China Department of Geography and Resource Management The Chinese University of Hong KongHong Kong 999077China Key Laboratory of Virtual Geographic Environment(Ministry of Education of PRC) Nanjing Normal UniversityNanjing 210023China School of Geography Nanjing Normal UniversityNanjing 210023China institute of Environmental Archaeology Nanjing Normal UniversityNanjing 210023China

The origin of agriculture in the farming-pastoral zone of northern China remains in *** central region of the inner Mongolia Plateau is located in the core area of the farming-pastoral zone;thus,it is a critical region for exploring the origin of the dryland farming system in northern *** study selected the Yumin Site and Banan Site,which belong to the Yumin Culture-the beginning of Neolithic culture in inner Mongolia-as the research *** on the quartz optically stimulated luminescence(OSL)dating on the sedimentary sections from the Yumin site(YM)and Banan site(BN1 and BN2),the Holocene chronology framework of each section was *** that,by identifying carbonized grains in the Yumin site and the multi-proxy analysis of each section,we investigated the relationship between the origin of agriculture and climate change in this *** results revealed that the timing of the origin of agriculture recorded in the Yumin site lagged behind the timing of a significant increase of precipitation during the early Holocene but coincided with the timing of a significant increase of vegetation around 8.4 *** phenomenon was further confirmed by the published high-resolution paleoenvironmental records from the surrounding area of the Yumin *** propose that with the gradual amelioration of hydrothermal conditions since the beginning of the Holocene,the regional ecosystem had been improved,resulting in the gradual conversion of the land surface from infertile sand to organic-rich soil,providing an appropriate environmental foundation for the origin of dryland farming in northern China around 8.4 *** study highlighted that the“accumulative environmental effects”during the early Holocene played a vital role in the origin of agriculture in northern China and provided a reference for agricultural management in the context of future climate change.

关键词： Origin of agriculture Accumulative environmental effects Yumin Culture Northern China Holocene