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Deciphering Water Oxidation Catalysts: The Dominant Role of Surface Chemistry over Reconstruction Degree in Activity Promotion

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NANO-MICRO LETTERS 2025年第1期17卷 1-15页

作者： An, li li, Jianyi sun, Yuanmiao Zhu, Jiamin Seow, Justin Zhu Yeow Zhang, Hong Zhang, Nan Xi, Pinxian Xu, Zhichuan J. Yan, Chun-Hua Lanzhou Univ Frontiers Sci Ctr Rare Isotopes Key Lab Nonferrous Met Chem & Resources Utilizat G State Key Lab Appl Organ ChemColl Chem & Chem Eng Lanzhou 730000 Peoples R China Nanyang Technol Univ Sch Mat Sci & Engn Singapore 639798 Singapore Chinese Acad Sci Fac Mat Sci & Energy Engn Shenzhen Inst Adv Technol Inst Technol Carbon Neutral Shenzhen 518055 Peoples R China Yunnan Univ Natl Ctr Int Res Photoelect & Energy Mat Electron Microscopy Ctr Sch Mat & EnergyKey Lab Electromagnet Mat & Devic Kunming 650091 Peoples R China Baotou Res Inst Rare Earths State Key Lab Baiyunobo Rare Earth Resource Res & Baotou 014030 Peoples R China Peking Univ Beijing Natl Lab Mol Sci State Key Lab Rare Earth Mat Chem & Applicat PKU HKU Joint Lab Rare Earth Mat & Bioinorgan Chem Beijing 100871 Peoples R China

Demonstrate that the key factor to determine the activity of reconstructed surfaces is the surface chemistry, instead of reconstruction degree using the popular perovskite LaNi1-xFexO3 oxides as model *** content can influence both the surface reconstruction degree, the activation degree, and the activity of reconstructed *** oxygen evolution reaction activity of reconstructed catalysts is primarily governed by the chemistry of the reconstructed surface species. Water splitting hinges crucially on the availability of electrocatalysts for the oxygen evolution reaction. The surface reconstruction has been widely observed in perovskite catalysts, and the reconstruction degree has been often correlated with the activity enhancement. Here, a systematic study on the roles of Fe substitution in activation of perovskite LaNiO3 is reported. The substituting Fe content influences both current change tendency and surface reconstruction degree. LaNi0.9Fe0.1O3 is found exhibiting a volcano-peak intrinsic activity in both pristine and reconstructed among all substituted perovskites in the LaNi1-xFexO3 (x = 0.00, 0.10, 0.25, 0.50, 0.75, 1.00) series. The reconstructed LaNi0.9Fe0.1O3 shows a higher intrinsic activity than most reported NiFe-based catalysts. Besides, density functional theory calculations reveal that Fe substitution can lower the O 2p level, which thus stabilize lattice oxygen in LaNi0.9Fe0.1O3 and ensure its long-term stability. Furthermore, it is vital interesting that activity of the reconstructed catalysts relied more on the surface chemistry rather than the reconstruction degree. The effect of Fe on the degree of surface reconstruction of the perovskite is decoupled from that on its activity enhancement after surface reconstruction. This finding showcases the importance to customize the surface chemistry of reconstructed catalysts for water oxidation.

关键词： Oxygen evolution reaction Perovskite oxides Doping Activation and reconstruction

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Low‑Temperature Oxidation Induced Phase Evolution with Gradient Magnetic Heterointerfaces for Superior Electromagnetic Wave Absorption

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Nano-Micro Letters 2025年第1期17卷 191-204页

作者： Zizhuang He lingzi Shi Ran sun lianfei Ding Mukun He Jiaming li Hua Guo Tiande Gao Panbo liu School of Chemistry and Chemical Engineering Northwestern Polytechnical UniversityXi’an 710129People’s Republic of China School of Marine Science and Technology Northwestern Polytechnical UniversityXi’an 710072People’s Republic of China

Gradient magnetic heterointerfaces have injected infinite vitality in optimizing impedance matching,adjusting dielectric/magnetic resonance and promoting electromagnetic(EM)wave absorption,but still exist a significant challenging in regulating local phase ***,accordion-shaped Co/Co_(3)O_(4)@N-doped carbon nanosheets(Co/Co_(3)O_(4)@NC)with gradient magnetic heterointerfaces have been fabricated via the cooperative high-temperature carbonization and lowtemperature oxidation *** results indicate that the surface epitaxial growth of crystal Co_(3)O_(4) domains on local Co nanoparticles realizes the adjustment of magnetic-heteroatomic components,which are beneficial for optimizing impedance matching and interfacial ***,gradient magnetic heterointerfaces simultaneously realize magnetic coupling,and long-range magnetic ***,the synthesized Co/Co_(3)O_(4)@NC absorbents display the strong electromagnetic wave attenuation capability of−53.5 dB at a thickness of 3.0 mm with an effective absorption bandwidth of 5.36 GHz,both are superior to those of single magnetic domains embedded in carbon *** design concept provides us an inspiration in optimizing interfacial polarization,regulating magnetic coupling and promoting electromagnetic wave absorption.

关键词： Magnetic heterointerfaces Phase evolution Interfacial polarization Magnetic coupling Electromagnetic wave absorption

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基于EKC假设的出口贸易低碳化实证研究——以江苏省为例

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系统工程 2017年第10期35卷 49-58页

作者：赵桂梅陈丽珍孙华平赵桂芹江苏大学财经学院江苏镇江212013 江苏大学京江学院江苏镇江212013

"十三五"时期绿色发展将成为生态文明建设的主基调,文章构建时间序列的出口贸易碳排放动态计量模型,以经济结构具有典型性的江苏省数据为基础,实证检验碳排放与出口贸易之间的短期动态关系以及长期均衡关系。研究表明:出口贸易碳排放EK... 详细信息

"十三五"时期绿色发展将成为生态文明建设的主基调,文章构建时间序列的出口贸易碳排放动态计量模型,以经济结构具有典型性的江苏省数据为基础,实证检验碳排放与出口贸易之间的短期动态关系以及长期均衡关系。研究表明:出口贸易碳排放EKC假设不成立,二氧化碳排放量与出口额之间存在长期协整关系,快速增长的外贸出口是碳排放增长的重要的驱动因素,而且影响日益增大。进一步提出应对温室气体排放,实现低碳化的绿色经济,应从优化外贸结构角度探讨减排的新途径,构建全球价值链体系,加强政府引导作用。

关键词： EKC假设出口贸易碳排放全球价值链绿色发展理念

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miRNA-21-5p is an important contributor to the promotion of injured peripheral nerve regeneration using hypoxia-pretreated bone marrow-derived neural crest cells

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Neural Regeneration Research 2025年第1期20卷 277-290页

作者： Meng Cong Jing-Jing Hu Yan Yu Xiao-li li Xiao-Ting sun li-Ting Wang Xia Wu ling-Jie Zhu Xiao-Jia Yang Qian-Ru He Fei Ding Hai-Yan Shi School of Medicine Nantong UniversityNantongJiangsu ProvinceChina Key Laboratory of Neuroregeneration of Jiangsu and Ministry of Education and Coinnovation Center of Neuroregeneration Nantong UniversityNantongJiangsu ProvinceChina Department of Physiology Jiangsu Health Vocational CollegeNanjingJiangsu ProvinceChina Department of Pathology Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina Jiangsu Clinical Medicine Center of Tissue Engineering and Nerve Injury Repair Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina

Our previous study found that rat bone marrow–derived neural crest cells(acting as Schwann cell progenitors)have the potential to promote long-distance nerve ***-based therapy can enhance peripheral nerve repair and regeneration through paracrine bioactive factors and intercellular ***,the complex contributions of various types of soluble cytokines and extracellular vesicle cargos to the secretome remain *** investigate the role of the secretome and extracellular vesicles in repairing damaged peripheral nerves,we collected conditioned culture medium from hypoxia-pretreated neural crest cells,and found that it significantly promoted the repair of sensory neurons damaged by oxygen-glucose *** mRNA expression of trophic factors was highly expressed in hypoxia-pretreated neural crest *** performed RNA sequencing and bioinformatics analysis and found that miR-21-5p was enriched in hypoxia-pretreated extracellular vesicles of neural crest ***,to further clarify the role of hypoxia-pretreated neural crest cell extracellular vesicles rich in miR-21-5p in axonal growth and regeneration of sensory neurons,we used a microfluidic axonal dissociation model of sensory neurons in vitro,and found that hypoxia-pretreated neural crest cell extracellular vesicles promoted axonal growth and regeneration of sensory neurons,which was greatly dependent on loaded ***,we constructed a miR-21-5p-loaded neural conduit to repair the sciatic nerve defect in rats and found that the motor and sensory functions of injured rat hind limb,as well as muscle tissue morphology of the hind limbs,were obviously *** findings suggest that hypoxia-pretreated neural crest extracellular vesicles are natural nanoparticles rich in ***-21-5p is one of the main contributors to promoting nerve regeneration by the neural crest cell *** helps to explain the mechanism of action of the secretome and e

关键词： axotomy cell-free therapy conditioned medium extracellular vesicles hypoxic preconditioning microRNA oxygen-glucose deprivation peripheral nerve injury Schwann cell precursors

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Inter-Skeleton Conductive Routes Tuning Multifunctional Conductive Foam for Electromagnetic Interference Shielding, Sensing and Thermal Management

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NANO-MICRO LETTERS 2025年第1期17卷 1-18页

作者： li, Xufeng Chen, Chunyan li, zhenyang Yi, Peng Zou, Haihan Deng, Gao Fang, Ming He, Junzhe sun, Xin Yu, Ronghai Shui, Jianglan Pan, Caofeng liu, Xiaofang Beihang Univ Sch Mat Sci & Engn Beijing 100191 Peoples R China Beihang Univ Inst Atom Mfg Beijing 100191 Peoples R China Tianmushan Lab Xixi Octagon City Hangzhou 310023 Peoples R China Beijing Inst Environm Features Sci & Technol Electromagnet Scattering Lab Beijing 100854 Peoples R China

Unique inter-skeleton conductive films are constructed in polymer *** resistance change of the foam can reach four orders of magnitude under *** foam exhibits strain-adaptive electromagnetic interference shielding performance, anti-interference pressure sensor with high sensitivity over a wide pressure range and compression-regulated Joule heating function. Conductive polymer foam (CPF) with excellent compressibility and variable resistance has promising applications in electromagnetic interference (EMI) shielding and other integrated functions for wearable electronics. However, its insufficient change amplitude of resistance with compressive strain generally leads to a degradation of shielding performance during deformation. Here, an innovative loading strategy of conductive materials on polymer foam is proposed to significantly increase the contact probability and contact area of conductive components under compression. Unique inter-skeleton conductive films are constructed by loading alginate-decorated magnetic liquid metal on the polymethacrylate films hanged between the foam skeleton (denoted as AMLM-PM foam). Traditional point contact between conductive skeletons under compression is upgraded to planar contact between conductive films. Therefore, the resistance change of AMLM-PM reaches four orders of magnitude under compression. Moreover, the inter-skeleton conductive films can improve the mechanical strength of foam, prevent the leakage of liquid metal and increase the scattering area of EM wave. AMLM-PM foam has strain-adaptive EMI shielding performance and shows compression-enhanced shielding effectiveness, solving the problem of traditional CPFs upon compression. The upgrade of resistance response also enables foam to achieve sensitive pressure sensing over a wide pressure range and compression-regulated Joule heating function.

关键词： Inter-skeleton conductive films Conductive polymer foam liquid metal Electromagnetic interference shielding

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An Unprecedented Efficiency with Approaching 21%Enabled by Additive‑Assisted Layer‑by‑Layer Processing in Organic Solar Cells

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Nano-Micro Letters 2025年第2期17卷 372-375页

作者： Shuai Xu Youdi Zhang Yanna sun Pei Cheng Zhaoyang Yao Ning li Long Ye lijian Zuo Ke Gao Key Laboratory of Advanced Green Functional Materials College of ChemistryChangchun Normal UniversityChangchun 130032People’s Republic of China Shandong Provincial Key Laboratory for Science of Material Creation and Energy Conversion School of Chemistry and Chemical EngineeringShandong UniversityQingdao 266237People’s Republic of China College of Polymer Science and Engineering Sichuan UniversityChengdu 610065People’s Republic of China State Key Laboratory and Institute of Elemento‑Organic Chemistry Centre of Nanoscale Science and Technology and Key Laboratory of Functional Polymer MaterialsRenewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071People’s Republic of China Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and Devices South China University of TechnologyGuangzhou 510640People’s Republic of China Tianjin Key Laboratory of Molecular Optoelectronic Sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300350People’s Republic of China State Key Laboratory of Silicon Materials MOE Key Laboratory of Macromolecular Synthesis and FunctionalizationDepartment of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China

Recently published in Joule,Feng liu and colleagues from Shanghai Jiaotong University reported a record-breaking 20.8%power conversion efficiency in organic solar cells(OSCs)with an interpenetrating fibril network active layer morphology,featuring a bulk p-in structure and proper vertical segregation achieved through additive-assisted layer-by-layer *** optimized hierarchical gradient fibrillar morphology and optical management synergistically facilitates exciton diffusion,reduces recombination losses,and enhances light capture *** approach not only offers a solution to achieving high-efficiency devices but also demonstrates the potential for commercial applications of OSCs.

关键词： Organic solar cells Additive-assisted layer-by-layer processing Three-dimensional fibril morphology Bulk p-i-n structure Optical management

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移动ICU转运模式应用于危重症患者转运中的临床效果

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临床医学研究与实践 2017年第23期2卷 140-142页

作者：李兴珍孙媛苏晓丽杜工亮陕西省人民医院急诊外科陕西西安710068

目的探讨院内展开移动ICU转运模式对危重症患者转运的影响和临床效果。方法回顾性分析2015年2月至2015年8月陕西省人民医院重症医学科收治的242例患者的临床资料,将其按照转运方式的不同分为对照组(117例)及观察组(125例)。对照组患者... 详细信息

目的探讨院内展开移动ICU转运模式对危重症患者转运的影响和临床效果。方法回顾性分析2015年2月至2015年8月陕西省人民医院重症医学科收治的242例患者的临床资料,将其按照转运方式的不同分为对照组(117例)及观察组(125例)。对照组患者采用传统转运方式,观察组患者则采用移动ICU转运模式,比较两组患者转运过程中不良事件发生率及相关因素。结果观察组中不良事件共发生12例,不良事件发生率为9.6%,对照组中不良事件共发生32例,不良事件发生率为27.4%,观察组患者的不良事件发生率明显低于对照组,差异有统计学意义(P0.05)。结论移动ICU转运模式可有效减少人为因素导致的不良事件发生,有效降低不良事件发生率,提高重症患者转运的安全性和实效性,值得临床推广及应用。

关键词：危重症患者移动ICU 转运模式

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食品安全国家标准GB 2763—2016对葡萄的新要求

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浙江农业学报 2018年第5期30卷 840-847页

作者：李真孙彩霞戴芬郑蔚然于国光姚佳蓉王强浙江省农业科学院农产品质量标准研究所浙江杭州310021

《食品安全国家标准食品中农药最大残留限量》(GB 2763—2016)对食品中农药残留的种类、最大残留限量及检测方法均提出了较多的新要求。对新标准中涉及葡萄或浆果类水果规定的变化进行了归纳,并与国际上的相关标准进行对比,旨在为有关... 详细信息

《食品安全国家标准食品中农药最大残留限量》(GB 2763—2016)对食品中农药残留的种类、最大残留限量及检测方法均提出了较多的新要求。对新标准中涉及葡萄或浆果类水果规定的变化进行了归纳,并与国际上的相关标准进行对比,旨在为有关产业的发展提供参考。

关键词：农产品质量安全农药残留国家标准

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改性方法对豆渣膳食纤维的结构影响研究

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食品科技 2011年第1期36卷 143-147页

作者：周丽珍孙海燕刘冬李艳唐旭蔚李世敏深圳职业技术学院应用化学与生物技术学院深圳518055

采用X射线衍射(XRD)和红外光谱技术,考察酶解改性、高温蒸煮改性以及高温蒸煮结合酶解改性对豆渣膳食纤维(DF)结构的影响。结合几种改性方法制备豆渣DF,运用XRD及红外光谱技术检测DF的结构特性。结果表明:酶解、高温蒸煮及其结合改性方... 详细信息

采用X射线衍射(XRD)和红外光谱技术,考察酶解改性、高温蒸煮改性以及高温蒸煮结合酶解改性对豆渣膳食纤维(DF)结构的影响。结合几种改性方法制备豆渣DF,运用XRD及红外光谱技术检测DF的结构特性。结果表明:酶解、高温蒸煮及其结合改性方法主要都是影响豆渣DF中的非结晶区结构,或部分破坏结晶区结构,使这些结构组分溶出或转化为水溶性成分溶出,从而达到改性目的;改性方法对豆渣DF的结晶区结构不会完全破坏。此外,XRD技术和红外光谱技术相结合,可作为研究DF的有效技术手段。

关键词：改性膳食纤维 X射线衍射(XRD) 红外光谱

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基于BIM的智慧农业温室大棚建模分析

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农机化研究 2025年第3期47卷 217-221页

作者：李祯庄卓河南工业职业技术学院河南南阳473000

智慧农业是当前农业发展的趋势,而温室大棚作为重要的农业生产设施,对其进行建模分析具有重要意义。为此,基于BIM技术,对Venlo智慧农业温室大棚进行了建模分析。首先,对温室大棚的设计流程进行分析;然后,对BIM工作流做介绍和分析,并对... 详细信息

智慧农业是当前农业发展的趋势,而温室大棚作为重要的农业生产设施,对其进行建模分析具有重要意义。为此,基于BIM技术,对Venlo智慧农业温室大棚进行了建模分析。首先,对温室大棚的设计流程进行分析;然后,对BIM工作流做介绍和分析,并对建筑结构和节点进行深化分析;最后,设计了一栋智慧农业温室大棚,并利用BIM软件对其进行三维建模和分析。实例设计表明:基于BIM技术的智慧农业温室大棚建模分析具有较高的准确性和可操作性,可为农业生产提供重要支持。

关键词：智慧农业 Venlo温室大棚 BIM技术建筑结构三维建模

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