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Food Science and Human Wellness 2024年第4期13卷 2152-2160页

作者： Mingming li Qiujin zhu Chao Qu Xiaohui Gong Yunhan Zhang xin Zhang Shouwei Wang China Meat Research Center Beijing 100068China Guizhou Provincial Key Laboratory of Agricultural and Animal Products Storage and Processing School of Liquor&Food EngineeringGuizhou UniversityGuiyang 550025China Beijing Academy of Food Sciences Beijing 100068China

Dry-cured meat products are considerably popular around the world due to unique *** is one of the enzymatic reactions from which flavor substances are derived,which is affected by endogenous *** purpose aimed to reveal the potential relationship between endogenous proteases and key flavor substances in dry-cured pork coppa in this *** dynamic changes of endogenous proteases activity,free amino acids,and volatiles during dry-cured pork coppa processing were *** results showed that 5 kinds of free amino acids,Glu,Lys,Val,Ala,and Leu,were identified as significant contributors to ***,key volatiles,such as hexanal,nonanal,octanal,benzaldehyde,3-methyl butanoic acid,2-methyl propanoic acid,and ethyl octanoate,greatly contributed to the flavor characteristics of dry-cured pork *** partial correlation analysis was performed to better elucidate the relationship among *** results revealed that close relationship between endogenous proteases and key *** not only significantly affected the accumulation of key active-amino acids,but also affected the accumulation of ethyl octanoate,2,3-pentanedione,and 2,3-octanedione by regulating the accumulation of octanoic acid and *** addition,cathepsin B and D,DPP II,DPP IV and RAP notably affected accumulation of hexanal.

关键词： Dry-cured pork coppa Endogenous proteases Proteolysis Key taste-active amino acids Volatile compounds

Novel wreck salvaging method using curved rectangular pipe basing method:A case study of"Yangtze River EstuaryⅡ"ancient shipwreck salvage project

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Underground Space 2024年第5期18卷 97-113页

作者： Qianwei zhuang Guofang Gong Dongrong Zhou Chi Zhang xin Huang Xiaodong zhu Weihao Yuan Deng li School of Mechanical Engineering Zhejiang UniversityHangzhou 310030China Shanghai Tunnel Engineering Co.Ltd. Shanghai 200137China Department of Geotechnical Engineering College of Civil EngineeringTongji UniversityShanghai 200092China College of Civil Engineering and Architecture Xinjiang UniversityUrumqi 830047China Shanghai Salvage Company Shanghai 200090China

Shipwreck salvage is a risky,time-consuming,and expensive *** there are many sunken ships along coastlines and in the open seas,the salvage process of a sunken ship has rarely been *** integrated salvage of the"Yangtze River EstuaryⅡ"shipwreck used a novel method with 22 closely locked curved rectangular pipes to form a watertight base that wrapped the shipwreck *** basing was lifted out of the water using a powerful crane situated on an engineering *** the first time,the tunneling method was used in a shipwreck salvage project,significantly reducing the disturbance to the shipwreck and its stowage,thereby preserving the original state and integrity of the shipwreck to the greatest *** this study,the basic concepts of the salvage method and process are *** to critical issues in the new salvage method are provided,including jacking force prediction and major considerations for the structural design of the salvage *** design of the salvage system and salvage process of the"Yangtze River EstuaryⅡ"shipwreck are *** monitored jacking force,pipe deformation,and observed water-tightness verified that the proposed method was effective and *** possible application scenarios for the proposed method are presented at the end.

关键词： Pipe jacking Shipwreck salvage Yangtze River EstuaryⅡ Structural design

High-Performance and Large-Area Inverted Perovskite Solar Cells Based on NiO_(x) Films Enabled with A Novel Microstructure-Control Technology

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Energy & Environmental Materials 2024年第1期7卷 153-159页

作者： Guibin Shen xin li Yuqin Zou Hongye Dong Dongping zhu Yanglin Jiang xin Ren Ng Fen lin Peter Müller-Buschbaum Cheng Mu Key Laboratory of Advanced light Conversion Materials and Biophotonics Department of ChemistryRenmin University of ChinaBeijing 100872China Solar Energy Research Institute of Singapore(SERIS) National University of SingaporeSingapore 117574Singapore Physik-Department Lehrstuhl für Funktionelle MaterialienTechnische Universität MünchenJames-Franck-Straße 185748Garching Germany Heinz Maier-Leibnitz Zentrum(MLZ) Technische Universität MünchenLichtenbergstr.185748Garching Germany

The improvement in the efficiency of inverted perovskite solar cells(PSCs)is significantly limited by undesirable contact at the NiO_(x)/perovskite *** this study,a novel microstructure-control technology is proposed for fabrication of porous NiO_(x)films using Pluronic P123 as the structure-directing agent and acetylacetone(AcAc)as the coordination *** synthesized porous NiO_(x)films enhanced the hole extraction efficiency and reduced recombination defects at the NiO_(x)/perovskite ***,without any modification,the power conversion efficiency(PCE)of the PSC with MAPbl_(3)as the absorber layer improved from 16.50%to 19.08%.Moreover,the PCE of the device composed of perovskite Cs0.05(MA_(0.15)FA_(0.85))_(0.95)Pb(I_(0.85)Br_(0.15))_(3)improved from 17.49%to 21.42%.Furthermore,the application of the fabricated porous NiO_(x)on fluorine-doped tin oxide(FTO)substrates enabled the fabrication of large-area PSCs(1.2 cm^(2))with a PCE of 19.63%.This study provides a novel strategy for improving the contact at the NiO_(x)/perovskite interface for the fabrication of high-performance large-area perovskite solar cells.

关键词： interfacial contact inverted and large-area perovskite solar cells photovoltaic materials porous NiO_(x)films renewable energy

A long-term daily gridded snow depth dataset for the Northern Hemisphere from 1980 to 2019 based on machine learning

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Big Earth Data 2024年第2期8卷 274-301页

作者： Yanxing Hu Tao Che liyun Dai Yu zhu lin Xiao Jie Deng xin li Key Laboratory of Remote Sensing of Gansu Province Heihe Remote Sensing Experimental Research StationNorthwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhouChina College of Resources and Environment University of Chinese Academy of SciencesBeijingChina State Key Laboratory of Tibetan Plateau Earth System Resources and Environment(TPESRE)Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijingChina Yunnan Key Laboratory of International Rivers and Transboundary Eco-Security Institute of International Rivers and Eco-SecurityYunnan UniversityKunmingChina National Forestry and Grassland Administration Key Laboratory of Forest Resource Conservation and Ecological Safety on the Upper Reaches of the Yangtze River Sichuan Province Key Laboratory of Ecological Forestry Engineering on the Upper Reaches of the Yangtze RiverCollege of ForestrySichuan Agricultural UniversityChengduChina

A high-quality snow depth product is very import for cryospheric science and its related *** long time-series snow depth products covering the Northern Hemisphere can be divided into two categories:remote sensing snow depth products and reana-lysis snow depth ***,existing gridded snow depth products have some *** sensing-derived snow depth products are temporally and spatially discontinuous and tend to underestimate snow depth,while reanalysis snow depth products have coarse spatial resolutions and great *** overcome these problems,in our previous work we proposed a novel data fusion framework based on Random Forest Regression of snow products from Advanced Microwave Scanning Radiometer for the Earth Observing System(AMSR-E),Advanced Microwave Scanning Radiometer-2(AMSR2),Global Snow Monitoring for Climate Research(GlobSnow),the Northern Hemisphere Snow Depth(NHSD),ERA-Interim,and Modern-Era Retrospective Analysis for Research and Applications,ver-sion 2(MERRA-2),incorporating geolocation(latitude and longitude),and topographic data(elevation),which were used as input indepen-dent *** than 30,000 ground observation sites were used as the dependent variable to train and validate the model in different time *** fusion framework resulted in a long time series of continuous daily snow depth product over the Northern Hemisphere with a spatial resolution of 0.25°.Here,we compared the fused snow depth and the original gridded snow depth products with 13,272 observation sites,showing an improved precision of our *** evaluation indices of the fused(best original)dataset yielded a coeffi-cient of determination R2 of 0.81(0.23),Root Mean Squared Error(RMSE)of 7.69(15.86)cm,and Mean Absolute Error(MAE)of 2.74(6.14)*** of the bias(88.31%)between the fused snow depth and in situ observations was in the range of−5 cm to 5 *** accuracy assessment of independent snow observation sites-Sodank

关键词： Snow depth datasets machine learning data fusion Northern Hemisphere

Organic ligand nanoarchitectonics for BiVO_(4) photoanodes surface passivation and cocatalyst grafting

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Nano Research 2024年第5期17卷 3667-3674页

作者： Jingyi lin xin li Zhiliang Wang Runlu liu Hui Pan Yixin Zhao lingti Kong Yao li Shenmin zhu lianzhou Wang State Key Laboratory of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Nanomaterials Centre School of Chemical Engineering and Australian Institute for Bioengineering and Nanotechnologythe University of QueenslandQLD 4072Australia School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Wuhan Institute of TechnologyWuhan 430205China

Bismuth vanadate(BiVO_(4))is a promising photoanode material for efficient photoelectrochemical(PEC)water splitting,whereas its performance is inhibited by detrimental surface *** solve the problem,herein,a low-cost organic molecule 1,3,5-benzenetricarboxylic acid(BTC)is selected for surface passivation of BiVO_(4) photoanodes(BVOs),which also provides bonding sites for Co^(2+)to anchor,resulting in a Co-BTC-BVO *** to its strong coordination with metal ions,BTC not only passivates surface states of BVO,but also provides bonding between BVO and catalytic active sites(Co^(2+))to form a molecular *** study and interfacial charge kinetic investigation reveal that chemical bonding formed at the interface greatly suppresses charge recombination and accelerates charge *** obtained Co-BTC-BVO photoanode exhibits a photocurrent density of 4.82 mA/cm^(2) at 1.23 V *** hydrogen electrode(RHE)and a low onset potential of 0.22 VRHE under AM 1.5 G illumination,which ranks among the best photoanodes coupled with Co-based *** work presents a novel selection of passivation layers and emphasizes the significance of interfacial chemical bonding for the construction of efficient photoanodes.

关键词： bismuth vanadate photoanode water splitting surface passivation bridging ligands

Effects of NLRP3 Inflammasome Mediated Pyroptosis on Cardiovascular Diseases and Intervention Mechanism of Chinese Medicine

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Chinese Journal of Integrative Medicine 2024年第5期30卷 468-479页

作者： ZHONG Yi li xin-yue liANG Tian-jun DING Bao-zhu MA Ke-xin REN Wen-xuan liANG Wen-jie College of Integrated Traditional Chinese and Western Medicine Hebei University of Chinese MedicineHebei Key Laboratory of Integrated Traditional Chinese and Western Medicine in Liver and Kidney DiseasesInstitute of Integrated Traditional Chinese and Western MedicineShijiazhuang 050200China Department of Cardiovascular Internal Medicine the Second Affiliated Hospital of Jiujiang UniversityJiujiangJiangxi Province 332000China Graduate School Hebei Medical UniversityShijiazhuang 050017China Rural Physician College Hebei Medical UniversityShijazhuang 050017China Medical Department the First Hospital of Hebei Medical UniversityShijiazhuang 050030China

Activation of the NOD-like receptor protein 3(NLRP3)inflammasome signaling pathway is an important mechanism underlying myocardial pyroptosis and plays an important role in inflammatory damage to myocardial tissue in patients with cardiovascular diseases(CVDs),such as diabetic cardiomyopathy,ischemia/reperfusion injury,myocardial infarction,heart failure and *** RNAs(nc RNAs)are important regulatory *** Chinese medicine(CM)compounds,including their effective components,can regulate pyroptosis and exert myocardium-protecting *** mechanisms underlying this protection include inhibition of inflammasome protein expression,Toll-like receptor 4–NF-κB signal pathway activation,oxidative stress,endoplasmic reticulum stress(ERS),and mixed lineage kinase 3 expression and the regulation of silent information regulator *** NLRP3 protein is an important regulatory target for CVD prevention and treatment with *** the effects of the interventions mediated by CM and the related mechanisms provides new ideas and perspectives for CVD prevention and treatment.

关键词： pyroptosis cardiovascular diseases Chinese medicine NOD-like receptor protein 3 mechanisms

Leaching kinetics of fluorine during the aluminum removal from spent li-ion battery cathode materials

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Journal of Environmental Sciences 2024年第4期138卷 312-325页

作者： Shengjie li Jianxin zhu Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

The high content of aluminum(Al)impurity in the recycled cathode powder seriously affects the extraction efficiency of Nickel,Cobalt,Manganese,and lithium resources and the actual commercial value of recycled materials,so Al removal is crucially important to conform to the industrial standard of spent li-ion battery cathode *** this work,we systematically investigated the leaching process and optimum conditions associated with Al removal from the cathode powder materials collected in a wet cathode-powder peeling and recycling production line of spent li-ion batteries(liBs).Moreover,we specifically studied the leaching of fluorine(F)synergistically happened along with the removal process of Al,which was not concerned about in other studies,but one of the key factors affecting pollution prevention in the recovery *** mechanism of the whole process including the leaching of Al and F from the cathode powder was indicated by using NMR,FTIR,and XPS,and a defluoridation process was preliminarily investigated in this *** leaching kinetics of Al could be successfully described by the shrinking core model,controlled by the diffusion process and the activation energy was 11.14 kJ/***,the leaching of F was attributed to the dissolution of liPF6and decomposition of PVDF,and the kinetics associated was described by Avrami *** interaction of Al and F is advantageous to realize the defluoridation to some *** is expected that our investigation will provide theoretical support for the large-scale recycling of spent liBs.

关键词： Al removal F leaching Cathode powder Heating alkali leaching Leaching kinetics

Online diagnosis platform for tomato seedling diseases in greenhouse production

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International Journal of Agricultural and Biological Engineering 2024年第1期17卷 80-89页

作者： xin Jin Xiaowu zhu Jiangtao Ji Mingyong li Xiaolin Xie Bo Zhao College of Agricultural Equipment Engineering Henan University of Science and TechnologyLuoyang 471003HenanChina Science&Technology Innovation Center for Completed Set Equipment Longmen LaboratoryLuoyang 471023HenanChina Institute of Mechatronics Technology and Application China Mechanized Agriculture Science Research Institute Group Co.LtdBeijing 100020China

The facility-based production method is an important stage in the development of modern agriculture,lifting natural light and temperature restrictions and helping to improve agricultural production *** address the problems of difficulty and low accuracy in detecting pests and diseases in the dense production environment of tomato facilities,an online diagnosis platform for tomato plant diseases based on deep learning and cluster fusion was proposed by collecting images of eight major prevalent pests and diseases during the growing period of tomatoes in a facility-based *** diagnostic platform consists of three main parts:pest and disease information detection,clustering and decision-making of detection results,and platform diagnostic ***,based on the You Only Look Once(YOLO)algorithm,the key information of the disease was extracted by adding attention module(CBAM),multi-scale feature fusion was performed using weighted bi-directional feature pyramid network(BiFPN),and the overall construction was designed to be compressed and lightweight;Secondly,the k-means clustering algorithm is used to fuse with the deep learning results to output pest identification decision values to further improve the accuracy of identification applications;Finally,a detection platform was designed and developed using Python,including the front-end,back-end,and database of the system to realize online diagnosis and interaction of tomato plant pests and *** experiment shows that the algorithm detects tomato plant diseases and insect pests with mAP(mean Average Precision)of 92.7%,weights of 12.8 Megabyte(M),inference time of 33.6 *** with the current mainstream single-stage detection series algorithms,the improved algorithm model has achieved better performance;The accuracy rate of the platform diagnosis output pests and diseases information of 91.2%for images and 95.2%for *** is a great significance to tomato pest control research and t

关键词： pest and disease detection YOLO diagnosis platform k-means clustering facility production base

GhATL68b regulates cotton fiber cell development by ubiquitinating the enzyme required forβ-oxidation of polyunsaturated fatty acids

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Plant Communications 2024年第10期5卷 139-153页

作者： xin li Gai Huang Yifan Zhou Kun Wang Yuxian zhu College of life Sciences Wuhan UniversityWuhan 430072China Institute for Advanced Studies Wuhan UniversityWuhan 430072China Hubei Hongshan Laboratory Wuhan 430072China TaiKang Center for life and Medical Sciences Wuhan UniversityWuhan 430072China State Key Laboratory of Plant Genomics and National Center for Plant Gene Research Institute of Genetics and Developmental BiologyChinese Academy of SciencesBeijing 100101China

E3 ligases are key enzymes required for protein ***,we identified a C3H2C3 RING domaincontaining E3 ubiquitin ligase gene named *** is preferentially and highly expressed in developing cotton fiber cells and shows greater conservation in plants than in animals or *** four orthologous copies of this gene in various diploid cottons and eight in the allotetraploid *** were found to have originated from a single common ancestor that can be traced back to Chlamydomonas reinhardtii at about 992 million years *** variations in the GhATL68b promoter regions of ***,***,***,and *** are correlated with significantly different methylation pat*** CRISPR-Cas9 knockout cotton lines exhibit significant reductions in fiber quality traits,including upper-half mean length,elongation at break,uniformity,and mature fiber *** vitro ubiquitination and cell-free protein degradation assays revealed that GhATL68b modulates the homeostasis of 2,4-dienoyl-CoA reductase,a rate-limiting enzyme for theβ-oxidation of polyunsaturated fatty acids(PUFAs),via the ubiquitin proteasome *** cells harvested from these knockout mutants contain significantly lower levels of PUFAs important for production of glycerophospholipids and regulation of plasma membrane *** fiber growth defects of the mutant can be fully rescued by the addition of linolenic acid(C18:3),the most abundant type of PUFA,to the ovule culture *** experimentally characterized C3H2C3 type E3 ubiquitin ligase involved in regulating fiber cell elongation may provide us with a new genetic target for improved cotton lint production.

关键词： Gossypium hirsutum E3 ligases polyunsaturated fatty acids β-oxidation fiber development

High-rate CH_(4)-to-C_(2)H_(6) photoconversion enabled by Au/ZnO porous nanosheets under oxygen-free system

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Science China Chemistry 2024年第3期67卷 869-875页

作者： Kai Zheng Xiaojing Zhang Jun Hu Chengbin Xu Juncheng zhu Jing li Mingyu Wu Shan zhu li li Shumin Wang Yumei Lv xin He Ming Zuo Chengyuan liu Yang Pan Junfa zhu Yongfu Sun Yi Xie Hefei National Laboratory for Physical Sciences at Microscale National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230026China Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China State Grid Anhui Electric Power Research Institute Hefei 230601China

Photocatalytic CH_(4) coupling into high-valued C_(2)H_(6) is highly attractive,whereas the photosynthetic rate,especially under oxygen-free system,is still ***,we designed the negatively charged metal supported on metal oxide nanosheets to activate the inert C-H bond in CH_(4)and hence accelerate CH_(4) coupling *** an example,the synthetic Au/ZnO porous nanosheets exhibit the C_(2)H_(6) photosynthetic rate of 1,121.6μmol g^(-1)_(cat)h^(-1)and the CH_(4) conversion rate of 2,374.6μmol g^(-1)_(cat)h^(-1) under oxygen-free system,2 orders of magnitude higher than those of previously reported *** virtue of several in situ spectroscopic techniques,it is established that the generated Au^(δ-)and O^-species together polarized the C-H bond,while the Au^(δ-)and O^-species jointly stabilized the CH_(3) intermediates,which favored the coupling of CH_(3) intermediate to photosynthesize C_(2)H_(6) instead of overoxidation into CO_(x).Thus,the design of dual active species is beneficial for achieving high-efficient CH_(4)-to-C_(2)H_(6) photoconversion.

关键词： dual surface-active sites selective methane coupling ethane room temperature