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Investigation on coal damage and fracture extension law of liquid nitrogen injection pre-cooling and fracturing under true triaxial stress

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International Journal of Mining Science and Technology 2025年第2期35卷 213-229页

作者： Botao li Haifei lin Jianping wei Hongtu Zhang Shugang li Zongyong wei Lei Qin Pei Wang Rongwei Luo Zeran liu School of Safety Science and Engineering Henan Polytechnic UniversityJiaozuo 454003China State Key Laboratory Cultivation Base for Gas Geology and Gas Control Henan Polytechnic UniversityJiaozuo 454003China State Collaborative Innovation Center of Coal Work Safety and Clean-efficiency Utilization Henan Polytechnic UniversityJiaozuo 454003China College of Safety Science and Engineering Xi’an University of Science and TechnologyXi’an 710054China Key Laboratory of Shaanxi Province Universities of Gas Disaster Prevention and Control in Western Coal Mines Xi’an 710054China

To more accurately describe the coal damage and fracture evolution law during liquid nitrogen(LN_(2))fracturing under true triaxial stress,a thermal-hydraulic-mechanical-damage(THMD)coupling model for LN_(2) fracturing coal was developed,considering the coal heterogeneity and thermophysical parameters of *** accuracy and applicability of model were verified by comparing with LN_(2) injection pre-cooling and fracturing experimental *** effects of different pre-cooling times and horizontal stress ratios on coal damage evolution,permeability,temperature distribution,and fracture characteristics were *** results show that the permeability and damage of the coal increase exponentially,while the temperature decreases exponentially during the fracturing *** the pre-cooling time increases,the damage range of the coal expands,and the fracture propagation becomes more *** initiation pressure and rupture pressure decrease and tend to stabilize with longer precooling *** the horizontal stress ratio increases,fractures preferentially extend along the direction of maximum horizontal principal stress,leading to a significant decrease in both initiation and rupture *** a horizontal stress ratio of 3,the initiation pressure drops by 48.07%,and the rupture pressure decreases by 41.36%.The results provide a theoretical basis for optimizing LN_(2) fracturing techniques and improving coal seam modification.

关键词： liquid nitrogen fracturing Thermal–hydraulic-mechanical-damage coupling Heterogeneous coal True triaxial stress Fracture morphology

Single-atom“surgery”on chiral all-dialkynyl-protected superatomic silver nanoclusters

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Science Bulletin 2025年第3期70卷 365-372页

作者： Chengkai Zhang wei-Dan Si wei-Dong Tian Wan-Jun Xiao Zhi-Yong gao Zhi Wang Chen-Ho Tung Di Sun School of Chemistry and Chemical Engineering State Key Laboratory of Crystal MaterialsShandong UniversityJinan 250100China School of Chemistry and Chemical Engineering Henan Normal UniversityXinxiang 453007China

The manipulation of single atom within the metallic kernel of nanoclusters has attracted considerable attention due to its potentials to elucidate kernel-based structure-property relationships at the single-atom ***,new-designed chiral bialkynyl ligands,have been chosen as protective agents to isolate two pairs of 8-electron superatomic silver nanoclusters,R/S-Ag39 and R/S-Ag40.X-ray diffraction analysis reveals that Ag39 and Ag40 with the same number of chiral ligands,possess a closely analogous silver skeleton but a single-atomic *** incorporation of an extra Ag40th atom into Ag40 evokes two significant changes of structure and property compared to Ag39:(i)a reduction in the symmetry of the entire nanocluster,resulting in an enhancement of kernel-related asymmetry g-factor;(ii)a regulation of the transitions(1P→1D and ligand(π)→1D)of excited state,leading to a second near-infrared(NIR-II,1000-1700 nm)phosphorescent emission red-shift from 1088 to 1150 *** work not only provides vital insights into the relationship between structures and ground/excited states chiroptical activities at the single-atom level,but also presents bialkynyl as a promising stabilizing agent for building superatomic metal nanoclusters.

关键词： Single atom manipulation Chiral bialkynyl ligands Superatomic silver nanoclusters NIR-Il phosphorescence

Adaptive-basis decomposition-based low-rank network for efficient non-uniform motion deblurring

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Optoelectronics Letters 2025年第1期21卷 43-50页

作者： CHEN Lei XIONG Qingbo ZHANG wei li Runde School of Software Henan UniversityKaifeng 475004China School of Applied Technology China University of Labor RelationsBeijing 100048China

In this study,we present a unified sparsity-driven framework that significantly enhances motion deblurring performance by integrating two key components:a custom-designed dataset and a low-rank module(LRM).This framework leverages the inherent sparsity of per-pixel blur kernels to bolster both deblurring accuracy and model ***,we propose an adaptive-basis decomposition-based deblurring(ADD)approach,which constructs a tailored training dataset to enhance the generalization capacity of the deblurring *** ADD framework adaptively decomposes motion blur into sparse basis elements,effectively addressing the intricacies associated with non-uniform ***,an LRM is proposed to improve the interpretability of deblurring models as a plug-and-play module,primarily designed to identify and harness the intrinsic sparse features in sharp images.A series of ablation studies have been conducted to substantiate the synergistic advantages of combining the proposed ADD with the LRM for overall improvement in deblurring ***,we empirically demonstrate through rigorous experimentation that incorporating the LRM into an existing Uformer network leads to substantial enhancement in reconstruction *** integration yields a sparsity-guided low-rank network(SGLRN).Operating under the overarching principle of sparsity,SGLRN consistently outperforms state-of-the-art methods across multiple standard deblurring *** experimental results,assessed through quantitative metrics and qualitative visual evaluations,provide compelling evidence of its *** overall deblurring results are available at Google Drive.

关键词： network motion uniform

SpaGRA:Graph augmentation facilitates domain identification for spatially resolved transcriptomics

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Journal of Genetics and Genomics 2025年第1期52卷 93-104页

作者： Xue Sun wei Zhang Wenrui li Na Yu Daoliang Zhang Qi Zou Qiongye Dong Xianglin Zhang Zhiping liu Zhiyuan Yuan Rui gao Center of Intelligent Medicine School of Control Science and EngineeringShandong UniversityJinanShandong 250061China MOE Key Lab of Bioinformatics and Bioinformatics Division of BNRIST Department of AutomationTsinghua UniversityBeijing 100084China Institute of Precision Medicine Peking University Shenzhen HospitalShenzhenGuangdong 518036China Department of Clinical Laboratory The Second HospitalCheeloo College of MedicineShandong UniversityJinanShandong 250033China Institute of Science and Technology for Brain-Inspired Intelligence Center for Medical Research and InnovationShanghai Pudong HospitalFudan University Pudong Medical CenterFudan UniversityShanghai 200433China

Recent advances in spatially resolved transcriptomics(SRT)have provided new opportunities for characterizing spatial structures of various ***-based geometric deep learning has gained widespread adoption for spatial domain identification ***,most methods define adjacency relation between cells or spots by their spatial distance in SRT data,which overlooks key biological interactions like gene expression similarities,and leads to inaccuracies in spatial domain *** tackle this challenge,we propose a novel method,SpaGRA(https://***/sunxue-yy/SpaGRA),for automatic multi-relationship construction based on graph *** uses spatial distance as prior knowledge and dynamically adjusts edge weights with multi-head graph attention networks(GATs).This helps SpaGRA to uncover diverse node relationships and enhance message passing in geometric contrastive ***,SpaGRA uses these multi-view relationships to construct negative samples,addressing sampling bias posed by random *** results show that SpaGRA presents superior domain identification performance on multiple datasets generated from different *** SpaGRA,we analyze the functional regions in the mouse hypothalamus,identify key genes related to heart development in mouse embryos,and observe cancer-associated fibroblasts enveloping cancer cells in the latest Visium HD ***,SpaGRA can effectively characterize spatial structures across diverse SRT datasets.

关键词： Spatial domain identification Spatially resolved transcriptomics Multi-head graph attention networks Graph augmentation Geometric contrastive learning

Travelling characteristics of road vehicles on single-level rail-cum-road bridge under the dynamic and aerodynamic impact of travelling trains

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Earthquake Engineering and Engineering Vibration 2025年第1期24卷 235-256页

作者： He Jiajun Lu Jun Guo wei Dong lianjie Bai Xue li Yongle Southwest Municipal Design&Research Institute of China Chengdu 610299China Southwest Jiaotong University Chengdu 610031China

Aerodynamic and dynamic interference from trains is a key issue of concern for the safety of road vehicles travelling on single-level rail-cum road *** on the wind-road vehicle-train-bridge(WRTB)coupled vibration system developed herein,this study examines the dynamic characteristics when road vehicles meet trains in this *** influence of load combination,vehicle type and vehicle location is analyzed.A method to obtain the aerodynamic load of road vehicles encountering the train at an arbitrary wind speed is *** results show that due to the windproof facilities and the large line distance between the railway and highway,the aerodynamic and dynamic influence of trains on road vehicles is slight,and the vibration of road vehicles depends on the road *** the road vehicles discussed,the bus is the easiest to rollover,and the truck-trailer is the easiest to *** with the aerodynamic impact of trains,the crosswind has a more significant influence on road *** first peak/valley value of aerodynamic loads determines the maximum dynamic response,and the quick method is optimized based on this *** cases show that the optimized method can produce conservative results and can be used for relevant research or engineering applications.

关键词： single-level rail-cum-road bridge vehicle-bridge coupled vibration dynamic characteristic aerodynamic impact road vehicle

Na_2S_2O_8促进硫醇的直接硫氰化:一个合成硫氰化合物的实用方法

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有机化学 2017年第2期37卷 480-484页

作者：李伟杨超高国林夏吾炯哈尔滨工业大学深圳研究生院城市水资源和环境国家重点实验室哈尔滨150080 哈尔滨商业大学食品科学工程重点实验室哈尔滨150076

报道了一种无金属催化制备硫氰化物的方法,利用Na_2S_2O_8/1,5-二氮杂二环[5.4.0]十一-5-烯(DBU)促进硫醇与Na CN直接硫氰基化得到硫氰化物.该反应条件温和,可获得产率31%～78%.

关键词：硫氰化合物过硫酸钠无金属硫醇

Combustion aerosols and suspended dust with controlled processes in Lhasa:Elemental analysis and size distribution characteristics

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Journal of Environmental Sciences 2025年第2期148卷 591-601页

作者： Jinglin li Zhuoga Deqing Jie liang Tao Guo Jian Yao wei liu Shanghai Institute of Applied Physics Chinese Academy of ScienceShanghai 201800China University of Chinese Academy of Science Beijing 100049China Meteorological Bureau of Tibet Autonomous Region Lhasa 850000China

To explore air contamination resulting from special biomass combustion and suspended dust in Lhasa,the present study focused on the size distribution and chemical characteristics of particulate matter(PM)emission resulting from 7 types of non-fossil pollution *** investigated the concentration and size distribution of trace elements from 7 pollution sources collected in *** Lhasa’s atmospheric particulate matter data,enrichment factors(EFs)have been calculated to examine the potential impact of those pollution sources on the atmosphere quality of *** highest mass concentration of total elements of biomass combustion appeared at PM_(0.4),and the second highest concentration existed in the size fraction 0.4-1μm;the higher proportion(12%)of toxicmetals was produced by biomass *** elemental composition of suspended dust and atmospheric particulate matter was close(except for As and Cd);the highest concentration of elements was all noted in PM_(2.5-10)(PM3-10).Potassium was found to be one of the main biomass *** proportion of Cu in suspended dust is significantly lower than that of atmospheric particulate matter(0.53%and 3.75%),which indicates that there are other anthropogenic *** EFs analysis showed that the Cr,Cu,Zn,and Pb produced by biomass combustion were highly enriched(EFs>100)in all particle *** EFs of most trace elements increased with decreasing particle size,indicating the greater influence of humanfactors on smaller particles.

关键词： Size distribution Trace elements Particulate matter Enrichment factors Lhasa

Broadband low-frequency sound absorption of multifunctional composite metastructure

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Science China(Technological Sciences) 2025年第2期68卷 114-124页

作者： Yilong YANG Shanshan liU Yan li Tong gao Yongdong PAN Yong li Yabin JIN School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai 200092China State International Joint Research Center of Aerospace Design and Additive Manufacturing Northwestern Polytechnical UniversityXi’an 710072China Institute of Acoustics School of Physics Science and EngineeringTongji UniversityShanghai 200092China Shanghai Key Laboratory of Intelligent Sensing and Detection Technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237China Shanghai Institute of Aircraft Mechanics and Control Shanghai 200092China

In this study,we fabricated multifunctional metastructures from carbon fiber-reinforced plastic composites using additive manufacturing *** metastructures are characterized by their lightweight,load-bearing capacity,and broadband low-frequency sound absorption *** metastructure consists of 36 unit cells,and non-local coupling mechanism was considered for designing the sound absorption *** developed an acoustic impedance theory tailored for the metastructure,facilitating an analysis of thermal and viscous dissipation *** is proven theoretically and experimentally that the proposed composite metastructure can achieve a noise reduction with an average sound absorption coefficient greater than 0.9 across frequencies in the rage of 330-1500 *** also studied the metastructure’s quasi-static and cyclic compression performance,confirming its efficient absorption capabilities after cyclic *** proposed design and additive manufacturing method for composite metastructures provides a novel pathway for creating lightweight,multifunctional structures with diverse applications,such as aerospace engineering.

关键词： composite metastructure broadband sound absorption additive manufacturing

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Highly anticipated natural diterpenoids as an important source of new drugs in 2013-2023

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Chinese Chemical Letters 2025年第1期36卷 119-136页

作者： Yingjie Wang Peng Tang Wenchao Tu Qi gao Cuizhu Wang Luying Tan lixin Zhao Hongye Han liefeng Ma Kouharu Otsuki weilie Xiao Wenli Wang Jinping liu Yong li Zhajun Zhan wei li Xianli Zhou Ning li School of Traditional Chinese Materia Medica Key Laboratory of Innovative Traditional Chinese Medicine for Major Chronic Diseases of Liaoning provinceKey Laboratory for TCM Material Basis Study and Innovative Drug Development of Shenyang CityShenyang Pharmaceutical UniversityShenyang 110016China Key Laboratory of Medicinal Chemistry for Natural Resource Ministry of EducationYunnan Characteristic Plant Extraction LaboratoryYunnan Key Laboratory of Research and Development for Natural ProductsSchool of Pharmacy and School of Chemical Science and TechnologyState Key Laboratory for Conservation and Utilization of Bio-Resources in YunnanYunnan UniversityKunming 650091China School of Pharmacy Nantong UniversityNantong 226001China School of Pharmaceutical Sciences Jilin UniversityChangchun 130021China State Key Laboratory of Bioactive Substance and Function of Natural Medicines Institute of Materia MedicaChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100050China College of Pharmaceutical Sciences Zhejiang University of TechnologyHangzhou 310014China Faculty of Pharmaceutical Sciences Toho UniversityFunabashiChiba 274-8510Japan School of life Science and Engineering Southwest Jiaotong UniversityChengdu 610031China

This review covers the structures of diterpenoids,including chain(72),monocyclic(9),labdane-type(67),clerodane-type(127)abietane-type(716),ent-kaurane-type(89),grayanane-type(331),ingenanetype(55),tigliane-type(154),daphnane-type(237),and aconitine-type diterpene alkaloids(265)with rich biological activities reported in *** the drugs in clinical use or under clinical investigation of diterpenoids and leading compounds were summarized.

关键词： Natural diterpenoids Structures Bioactivities Druggability Leading compounds New drugs