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Local Adaptive Gradient Variance Attack for Deep Fake Fingerprint Detection

Computers, Materials & Continua 2024年第1期78卷 899-914页

作者： Chengsheng Yuan Baojie cui Zhili Zhou Xinting li Qingming Jonathan Wu Engineering Research Center of Digital Forensics Ministry of EducationNanjing University of Information Science and TechnologyNanjing210044China School of Computer Science Nanjing University of Information Science and TechnologyNanjing210044China Institute of Artificial Intelligence and Blockchain Guangzhou UniversityGuangzhou510006China School of International Relations National University of Defense TechnologyNanjing210039China Department of Electrical and Computer Engineering University of WindsorWindsorN9B 3P4Canada

In recent years,deep learning has been the mainstream technology for fingerprint liveness detection(FLD)tasks because of its remarkable ***,recent studies have shown that these deep fake fingerprint detection(DFFD)models are not resistant to attacks by adversarial examples,which are generated by the introduction of subtle perturbations in the fingerprint image,allowing the model to make fake *** of the existing adversarial example generation methods are based on gradient optimization,which is easy to fall into local optimal,resulting in poor transferability of adversarial *** addition,the perturbation added to the blank area of the fingerprint image is easily perceived by the human eye,leading to poor visual *** response to the above challenges,this paper proposes a novel adversarial attack method based on local adaptive gradient variance for *** ridge texture area within the fingerprint image has been identified and designated as the region for perturbation ***,the images are fed into the targeted white-box model,and the gradient direction is optimized to compute gradient ***,an adaptive parameter search method is proposed using stochastic gradient ascent to explore the parameter values during adversarial example generation,aiming to maximize adversarial attack *** results on two publicly available fingerprint datasets show that ourmethod achieves higher attack transferability and robustness than existing methods,and the perturbation is harder to perceive.

关键词： FLD adversarial attacks adversarial examples gradient optimization transferability

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Single-atom alloys prepared by two-step thermal evaporation

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Nano Research 2024年第4期17卷 2808-2813页

作者： Honglin Wang jing li Meirong Huang Jizhe cui Zhiying Cheng Rong Yu Hongwei Zhu State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China State Key Lab of Solid Waste Reuse for Building Materials Beijing Building Materials Academy of Science ResearchBeijing 100041China

Single-atom alloys(SAAs)have gained significant attention due to their remarkable atomic utilization efficiency,interactions between single atoms(SAs)and metal supports,and free-atom-like electronic structure of dopant *** this work,we observed the formation of SAs in pre-deposited metal particles by a two-step thermal evaporation technique,thereby establishing the first instance of discovering SAAs by thermal *** discovery of SAAs by thermal evaporation extends the range of SAAs preparation methods to include this traditional synthetic technique,which offers convenience,cost-efficiency,and *** formation mechanism of SAAs prepared using this technique was elucidated by density functional theory *** was demonstrated that thermal evaporation can be utilized to prepare SAAs with multiple SAs,further highlighting its universal applicability.

关键词： single-atom alloys thermal evaporation density functional theory

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Phosphotungstic acid immobilized on amino-functionalized TS-1 zeolite as a solid acid catalyst for the synthesis of tributyl citrate

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Chinese Journal of Chemical Engineering 2024年第6期70卷 199-210页

作者： Pei li Bianfang Shi Junyao Shen Ran cui Wenze Guo ling Zhao Zhenhao Xi State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationEast China University of Science and TechnologyShanghai 200237China

The amino-functionalization of TS-1 zeolite followed by immobilization of phosphotungstic acid(HPW)was presented to prepare a strong solid acid catalyst for the synthesis of bio-based tributyl citrate from the esterification of citric acid and n-butanol.γ-Aminopropyltriethoxysilane(APTES)was first grafted on the TS-1 zeolite via the condensation reactions with surface hydroxyl groups,and subsequently the HPW was immobilized via the reaction between the amino groups and the protons from HPW-forming strong ionic *** Keggin structure of HPW and MFI topology of TS-1 zeolite were well maintained after the *** amino-functionalization generated abundant uniformly distributed active sites on TS-1 for HPW immobilization,which promoted the dispersity,abundance,as well as the stability of the acid *** tetrahedrally coordinated framework titanium and non-framework titania behaved as weak Lewis acid sites,and the protons from the immobilized HPW acted as the moderate or strong Brønsted acid *** optimized TBC yield of 96.2%(mol)with a conversion of-COOH of 98.1%(mol)was achieved at 150℃for 6 h over the HPW immobilized on amino-functionalized *** catalyst exhibited good stability after four consecutive reaction runs,where the activity leveled off at still a relatively high level after somewhat deactivation possibly caused by the leaching of a small portion of weakly anchored APTES or HPW.

关键词： Amino-functionalization Phosphotungstic acid TS-1 zeolite Esterification Tributyl citrate

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Optimization of mixing speed and time to disperse the composite conductive agent composed of carbon black and graphene in lithium-ion battery slurry

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Particuology 2024年第9期92卷 1-12页

作者： Zhilong Wang Jialong Tu Xinhao Yu Feixiang li Zhenzhen Zhao Yahui cui Tong Zhao Faculty of Mechanical and Precision Instrument Engineering Xi'an University of TechnologyXi'an710048China

This paper proposed an optimal approach to disperse the composite conductive agent which is composed of carbon black(CB)and graphene(Gr)within lithium-ion battery(liB)slurry with different mixing speeds and mixing *** internal structures of liB slurry are characterized by Electrochemical Impedance Spectroscopy,Scanning Electron Microscopy,and Raman ***,a composite conductive solution is prepared by mixing the composite conductive agent with NMP solvent under the conditions of five different mixing speeds n_(1)(n_(1)=1000,1100,1200,1300,1400 rpm)in the case of mixing time t_(1)=10 ***,liB slurry is prepared by blending the composite conductive solution,liCoO_(2)and PVDF-NMP solution under the conditions of five different mixing speeds n_(2)(n_(2)=1000±280,1100±280,1200±280,1300±280,1400±280 rpm)in the case of mixing time t_(2)=6 *** analyzing the internal structure of different liB slurries,it shows that in the case of n_(1)=n_(2)=1200 rpm,a conductive network structure is well formed within liB ***,in order to determine the optimal time to prepare the composite conductive solution for liB slurry,nine different t_(1)(t_(1)=0,10,20,30,40,50,60,70,80 min)are *** analyzing the internal structure of different liB slurries,a well-formed conductive network structure and a uniformly distributed composite conductive agent are deduced in liB slurry when t_(1)=50 ***,it can be concluded that the composite conductive agent composed of CB and Gr is able to be uniformly dispersed in liB slurry by establishing a well-formed conductive network structure under the optimal mixing speed n_(1)=n_(2)=1200 rpm and the optimal mixing time t_(1)=50 min,t_(2)=6 *** kind of the internal structure has the potential to be used to further analyze the dispersion characterizations of liB slurry under different composite conductive agent and CB/Gr ratios with the aim of improving the final performance of liB.

关键词： lithium-ion battery slurry Composite conductive agent Carbon black Graphene

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Influence of crystal-transforming agent on the performance and mechanism ofα-high-strength gypsum prepared from FGD gypsum

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Particuology 2024年第4期87卷 37-45页

作者： Zhuoyue Xu Xiao Wang Biao jin Dawang Zhang Hui li College of Materials Science and Engineering Xi'an University of Architecture and TechnologyXi'an710055China Schoolof Materials and Chemical Engineering Henan University of Urban ConstructionPingdingshan46736China

This paper investigates the impact of flue gas desulfurization(FGD)gypsum's crystal modifier on the characteristics and microcosmic mechanism ofα-high strength *** results demonstrate that all three crystal modifiers can convert FGD gypsum toα-high-strength *** acid(CA)has the most significant influence onα-high-strength gypsum,and the preparedα-high-strength gypsum is short columnar,with an aspect ratio in the range of 1-3,and has a faster setting time,a larger specific surface area,and a smaller standard consistency,higher compressive strength,greater surface hardness,and smaller crystal particle *** initial setting time of theα-high-strength gypsum manufactured with CA crystal modifier was decreased by 36%compared to the blank sample,the final setting time was lowered by 37.5%,and the water consumption of the standard consistency was reduced by 8%.The maximum strength is 32 MPa after 2 h,the absolute dry compressive strength is up to 38 MPa,and the surface hardness is improved by 24.43%.

关键词： Flue gas desulfurization gypsum Crystal modifier Microscopic mechanism α-high-strength gypsum

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Temperature-sensing array using the metal-to-insulator transition of Nd_(x)Sm_(1-x)NiO_(3)

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1694-1700页

作者： Fengbo Yan Ziang li Hao Zhang Yuchen cui Kaiqi Nie Nuofu Chen Jikun Chen School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China School of Renewable Energy North China Electric Power UniversityBeijing 102206China Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China

Rare-earth nickelates(RENiO_(3))show widely tunable metal-to-insulator transition(MIT)properties with ignorable variations in lattice constants and small latent heat across the critical temperature(TMIT).Particularly,it is worth noting that compared with the more commonly investigated vanadium oxides,the MIT of RENiO_(3)is less abrupt but usually across a wider range of *** sheds light on their alternative applications as negative temperature coefficient resistance(NTCR)thermistors with high sensitivity compared with the current NTCR thermistors,other than their expected use as critical temperature resistance *** this work,we demonstrate the NTCR thermistor functionality for using the adjustable MIT of Nd_(x)Sm_(1-x)NiO_(3)within 200–400 K,which displays larger magnitudes of NTCR(e.g.,more than 7%/K)that is unattainable in traditional NTCR thermistor *** temperature dependence of resistance(R–T)shows sharp variation during the MIT of Nd_(x)Sm_(1-x)NiO_(3)with no hysteresis via decreasing the Nd content(e.g.,x≤0.8),and such a R–T tendency can be linearized by introducing an optimum parallel *** sensitive range of temperature can be further extended to 210–360 K by combining a series of Nd_(x)Sm_(1-x)NiO_(3)with eight rare-earth co-occupation ratios as an array,with a high magnitude of NTCR(e.g.,7%–14%/K)covering the entire range of temperatures.

关键词： rare-earth nickelates metal-to-insulator transition correlated oxides perovskites

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Molecular simulation study on the evolution process of hydrate residual structures into hydrate

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Chinese Journal of Chemical Engineering 2024年第5期69卷 79-91页

作者： liwei Cheng Yunfei li jinlong cui Huibo Qin Fulong Ning Bei liu Guangjin Chen Faculty of Engineering China University of GeosciencesWuhan 430074China State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China College of Science Nanchang Institute of TechnologyNanchang 330099China School of Chemical Engineering Guangdong University of Petrochemical TechnologyMaoming 525000China National Center for International Research on Deep Earth Drilling and Resource Development China University of Geosciences(Wuhan)Wuhan 430074China

The clathrate hydrate memory effect is a fascinating phenomenon with potential applications in carbon capture,utilization and storage(CCUS),gas separation,and gas storage as it can accelerate the secondary formation of clathrate ***,the underlying mechanism of this effect remains *** gain a better understanding of the mechanism,we conducted molecular dynamic simulations to simulate the initial formation and reformation processes of methane *** this work,we showed the evolution process of hydrate residual structures into hydrate *** simulation results indicate that the residual structures are closely related to the existence of hydrate memory effect,and the higher the contribution of hydrate dissociated water to the hydrate nucleation process,the faster the hydrate *** hydrate dissociation,the locally ordered structures still exist after hydrate dissociation and can promote the formation of cluster structures,thus accelerating hydrate ***,the nucleation process of hydrate and the formation process of clusters are *** size of clusters composed of cup-cage structures is critical for hydrate *** residence time at high temperature after hydrate decomposition will affect the strength of the hydrate memory *** simulation results provide microscopic insights into the occurrence of the hydrate memory effect and shed light on the hydrate reformation process at the molecular scale.

关键词： Memory effect Molecular simulation Hydrate reformation Residual structures

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A novel interpretable multilevel wavelet decomposition deep network for actual heartbeat classification

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Science China(Technological Sciences) 2024年第6期67卷 1842-1854页

作者： jin YanRui li ZhiYuan TIAN YuanYuan WEI XiaoYang liU Chengliang School of Mechanical Engineering Shanghai Jiao Tong UniversityShanghai200240China

Arrhythmias may lead to sudden cardiac death if not detected and treated in time.A supraventricular premature beat(SPB)and premature ventricular contraction(PVC)are important categories of arrhythmia ***,deep learning methods have been applied to the PVC/SPB heartbeats ***,most researchers have focused on time-domain information of the electrocardiogram and there has been a lack of exploration of the interpretability of the *** this study,we design an interpretable and accurate PVC/SPB recognition algorithm,called the interpretable multilevel wavelet decomposition deep network(IMWDDN).Wavelet decomposition is introduced into the deep network and the squeeze and excitation(SE)-Residual block is designed for extracting time-domain and frequency-domain ***,inspired by the idea of residual learning,we construct a novel loss function for the constant updating of the multilevel wavelet decomposition ***,the IMWDDN is evaluated on the Third China Physiological Signal Challenge Dataset and the MIT-BIH Arrhythmia *** comparison results show IMWDDN has better detection performance with 98.51%accuracy and a 93.75%F1-macro on average,and its areas of concern are similar to those of an expert diagnosis to a certain ***,the IMWDDN has good application value in the clinical screening of PVC/SPB heartbeats.

关键词： actual heartbeat classification electrocardiogram interpretable deep network multilevel discrete wavelet decomposition layer SE-Residual block

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Spatial-temporal heterogeneity of ecological quality changes across the Qinghai-Tibet Plateau under the influence of climate factors and human activities

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Research in Cold and Arid Regions 2024年第3期16卷 129-140页

作者： ZiPing Zhang YuWei cui WenJia Tang Sen li Qinghai Province Ecological and Environmental Monitoring Center XiningQinghai 810007China Key Laboratory of Desert and Desertification Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhouGansu 730000China University of Chinese Academy of Sciences Beijing 100049China

Over the last few decades,the ecological quality of the Qinghai–Tibet Plateau(QTP)has significantly changed due to climate warming,humidification,and increasing human ***,evaluating this region's ecological quality and dominant factors is crucial for sustainable *** this study,the changes in the ecological quality on the QTP from 2000 to 2020 were evaluated based on aggregated indices and Sen–MK trend analyses,and the dominant factors affecting the ecological quality of the QTP were quantitatively analyzed using decision tree *** results revealed that(1)the ecological quality of the QTP exhibited an overall high trend in the east and a low pattern in the west;(2)the ecological quality of the QTP significantly increased from 2000 to 2020,and human activities were the dominant factors causing this change;and(3)the changes in the ecological quality and dominant factors exhibited obvious spatiotemporal *** area with an improved ecological quality occurred mainly in the northern QTP *** was governed by human activities and *** contrast,the area with a deteriorated ecological quality occurred largely in the southern QTP region and was dominated by human activities and *** 2000–2010 period was the most significant period of heterogeneity regarding of ecological quality and its driving factors.(4)The change in the ecological quality was mainly affected by the synergistic relationship between human activities and climate change in this region,which encompassed multiple dominant *** study provides important information on the spatiotemporal heterogeneity of ecological quality change and its dominant factors on the QTP and offers systematic guidance for the planning and implementation of ecological protection projects.

关键词： Remote sensing-based ecological index(RSEI) Dominant factors Synergies and trade-offs Qinghai‒Tibet Plateau

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Time-domain dynamic constitutive model suitable for mucky soil site seismic response

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Earthquake Engineering and Engineering Vibration 2024年第1期23卷 1-13页

作者： Dong Qing Chen Su jin liguo Zhou Zhenghua li Xiaojun Architectural Engineering Institute Huaiyin Institute of TechnologyHuai’an 223600China Key Laboratory of Urban Security and Disaster Engineering of Ministry of Education Beijing University of TechnologyBeijing 100020China Institute of Geophysics China Earthquake AdministrationBeijing 100089China College of Transportation Science and Engineering Nanjing Tech UniversityNanjing 211816China

Soil nonlinear behavior displays noticeable effects on the site seismic *** study proposes a new functional expression of the skeleton curve to replace the hyperbolic skeleton *** integrating shear modulus and combining the dynamic skeleton curve and the damping degradation coefficient,the constitutive equation of the logarithmic dynamic skeleton can be obtained,which considers the damping effect in a soil dynamics *** on the finite difference method and the multi-transmitting boundary condition,a 1D site seismic response analysis program called Soilresp1D has been developed herein and used to analyze the time-domain seismic response in three types of *** the same time,this study also provides numerical simulation results based on the hyperbolic constitutive model and the equivalent linear *** results verify the rationality of the new soil dynamic constitutive *** can analyze the mucky soil site nonlinear seismic response,reflecting the deformation characteristics and damping effect of the silty *** hysteresis loop area is more extensive,and the residual strain is evident.

关键词： seismic response time-domain dynamic constitutive model logarithmic dynamic skeleton dampening effect mucky soil

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