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经皮椎体成形联合增强椎弓钉治疗Ⅲ期Kummell病

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中国矫形外科杂志 2024年第19期32卷 1740-1746页

作者：钟炯彪孟旭东许胤李佳福杨帆彭佳睿袁野王佩珊湖南师范大学岳阳市人民医院脊柱外科

[目的]评价经皮椎体成形（percutaneous vertebroplasty, PVP）联合增强椎弓钉（augmented pedicle screw, APS）治疗III期Kummell病的临床疗效。[方法]回顾性分析2019年3月—2021年8月本院手术治疗无神经症状III期Kummell病76例患者的临床资料。根据医患沟通结果，32例采用单纯PVP(PVP组)，21例采用PVP-椎弓钉（pedicle screw, PS）(PVP-PS组)，23例采用PVP-增强椎弓钉（PVP-APS组），比较三组患者围术期、随访和影像资料。[结果]PVP组在手术时间、术中透视次数、穿刺调整次数、骨水泥注入量、术中出血量、下地行走时间、住院时间均显著少于PVP-PS组和PVP-APS组（P<0.05）。随访时间均超过1年，随时间推移，三组VAS、ODI评分均显著减少（P<0.05）；末次随访时，PVP-PS组和PVP-APS组的VAS [(2.7±0.6) vs(2.4±0.6) vs (3.3±0.4), P<0.001]以及ODI评分[(22.6±4.3) vs (25.0±4.8) vs (30.1±5.8), P<0.001]均显著优于PVP组。影像方面，末次随访时，PVP-PS组和PVP-APS组的矢状面指数（sagittal index, SI）[(88.4±3.6)%vs (93.2±3.7)%vs (46.2±3.6)%, P<0.001]、局部后凸Cobb角[(17.6±4.2)°vs (10.7±3.5)°vs (27.6±4.6)°, P<0.001]以及椎管狭窄率[(14.4±3.6)%vs (9.1±3.2)%vs (25.2±4.8)%, P<0.001]显著优于PVP组，且PVP-APS组显著优于PVP-PS组（P<0.05）。[结论]采取经皮骨水泥螺钉短节段固定联合病椎PVP术治疗无神经症状III期Kummell病，能有效恢复病椎高度、矫正后凸畸形、改善椎管狭窄，短期临床疗效满意，长期疗效仍待随访观察。

关键词： Kummell病经皮椎体成形术经皮椎弓根螺钉骨水泥强化

Optical edge-to-screw singularity state conversions

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Photonics Research 2024年第8期12卷 1689-1695页

作者： HAOliN liN JUNHUI jia GUOHUA liU YANWEN HU ZHEN li ZHENQIANG CHEN SHENHE fu Department of Optoelectronic Engineering Jinan UniversityGuangzhou 510632China Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications Guangzhou 510632China Guangdong Provincial Engineering Research Center of Crystal and Laser Technology Guangzhou 510632China

Optical singularity states,which significantly affect propagation properties of light in free space or optical medium,can be geometrically classified into screw and edge *** different types of singularity states do not exhibit direct connection,being decoupled from each other in the absence of external *** we demonstrate a novel optical process in which a higher-order edge singularity state initially nested in the propagating Gaussian light field gradually involves into a screw singularity with a new-born topological charge determined by order of the edge *** considered edge state comprises an equal superposition of oppositely charged vortex and antivortex *** theoretically and experimentally realize this edge-to-screw conversion process by introducing intrinsic vortex–antivortex *** also present a geometrical representation for mapping this dynamical process,based on the higher-order orbital Poincaré*** this framework,the edge-to-screw conversion is explained by a mapping of state evolution from the equator to the north or south pole of the Poincaré*** demonstration provides a novel approach for manipulating singularity state by the intrinsic vortex–antivortex *** presented phenomenon can be also generalized to other wave systems such as matter wave,water wave,and acoustic wave.

关键词： interaction Poincaré wave

A Class of m-Complex Symmetric Operators on Hardy Space

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Journal of Mathematical Research with Applications 2024年第1期44卷 63-80页

作者： jia fu Xinmei li Ran li School of Mathematics Liaoning Normal University

In this paper,we study the necessary and sufficient condition that the Toeplitz operators with respect to the conjugations of one permutation are 2-complex ***,we introduce a class of conjugations called the conjugations of one permutations on the classical Hardy ***,Toeplitz operators are completely characterized as 2-complex symmetric structure under this class of *** matrix representation of Toeplitz operators in the classical regular orthogonal basis on Hardy space is used to describe this class of 2-complex symmetric Toeplitz ***,we add two preconditions fn=-f-nand fn=f-nrespectively to the Toeplitz operators,and we get more simplified *** the second condition,we study the 3-complex symmetry of Toeplitz operators,and we get the same result for Tfis a 3-CSO with the conjugation C((i,j)) and 2-CSO’s.

关键词： m-complex symmetric operator Toeplitz operator Hardy space

An AIEgen nano-assembly for simultaneous detection of ATP and H_(2)S

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Chinese Chemical Letters 2024年第6期35卷 376-379页

作者： jia-Mei Qin Xue li Wei Lang fu-Hao Zhang Qian-Yong Cao School of Chemistry and Chemical Engineering Nanchang UniversityNanchang 330031China

A new aggregation-induced emission(AIE)-based fluorescence sensor,TPEPy-SS-C14,for simultaneous recognition of adenosine triphosphate(ATP)and hydrogen sulfide(H_(2)S)has been reported via the aggregation-disaggregation *** probe self-assembles nano-structure aggregations in aqueous *** shows fluorescence turn-on response toward ATP for the complexation-enhanced aggregation,but leads to fluorescence quenching of H_(2)S for cleavage the aggregations.

关键词： AIE-based ATP detection H_(2)S detection Fluorescent sensor Cell imaging

Photoinduced Dehalocyclization to Access Oxindoles Using Formate as a Reductant

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Chinese Journal of Chemistry 2024年第11期42卷 1203-1208页

作者： Wei Ge jia-Xin Wang Ming-Chen fu Yao fu Hefei National Research Center for Physical Sciences at the Microscale iChEMCAS Key Laboratory of Urban Pollutant ConversionAnhui Province Key Laboratory of Biomass Clean EnergyUniversity of Science and Technology of ChinaHefeiAnhui230026 China Anhui Province Key Laboratory of Value-Added Catalytic Conversion and Reaction Engineering Hefei University of TechnologyHefeiAnhui230009 China

Herein,we report an efficient and practical protocol for the photoinduced dehalocyclization of ortho-halophenylacrylamides with formate by the engagement of a CO_(2) radical anion to access substituted *** method proceeds smoothly under mild conditions and exhibits a wide range of substrate as well as remarkable functional group compatibility.

关键词： Formate CO_(2)Radical ions Oxindole Photocatalysts Cyclization Organohalides

Two-dimensional ballistic transistors for advanced-node integrated circuits

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National Science Review 2024年第3期11卷 9-10页

作者： jia li Xidong Duan Hunan Provincial Key Laboratory of Two-Dimensional Materials State Key Laboratory for Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University

As the feature size of metal-oxide-semiconductor-field-effect-transistors(MOSFETs) in integrated circuits(ICs)is reduced to sub-10-nm, the traditional channel materials are plagued by enhanced scattering and short-cha... 详细信息

关键词： CONTACT

Significantly Enhanced Melt Memory Effect of Metallocene-made Isotactic Polypropylene Containing Talc

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Chinese Journal of Polymer Science 2024年第2期42卷 213-222,I0008页

作者： Hong-Wen Sun fu-Shan Wang Yan Gao fu-Qing Wei jia-Chun Feng State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai200433China Lanzhou Petrochemical Corporation of PetroChina Lanzhou730060China Lanzhou Petrochemical Research Center Petrochemical Research Institute of PetroChinaLanzhou730060China

The melt memory effect is a widely observed phenomenon in semi-crystalline polymers. In practical applications, various additives are usually introduced into polymers, which may affect their melt memory behavior. In this work, the effect of talc on the melt memory effect of metallocene-made isotactic polypropylene(M-PP) was investigated in detail by using the differential scanning calorimetry. The results indicated that the introduction of talc significantly strengthened the melt memory effect of M-PP. Specifically, the upper limit temperature of Domain II increased from 161 ℃ to 174 ℃, resulting in a substantial widening of the temperature range of Domain IIa from 1 ℃ to 14 ℃. Analysis of the crystal orientation of the M-PP containing talc cooled from various Ts suggested that the remarkably enhanced melt memory effect could be ascribed to the stabilization of oriented nuclei facilitated by talc. This stabilizing effect was likely attributable to the prefreezing effect or the sorption interaction between talc and the M-PP chains.

关键词： Metallocene-made isotactic polypropylene Talc Melt memory effect Crystal orientation

Nitric oxide assists nitrogen reduction reaction on 2D MBene: A theoretical study

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Chinese Chemical Letters 2024年第5期35卷 428-433页

作者： Chaozheng He jia Wang ling fu Wei Wei Henan Engineering Center of New Energy Battery Materials College of Chemistry and Chemical EngineeringShangqiu Normal UniversityShangqiu 476000China School of Chemistry and Chemical Engineering Shandong Provincial Key Laboratory/Collaborative Innovation Center of Chemical Energy Storage&Novel Cell TechnologyLiaocheng UniversityLiaocheng 252059China Institute of Environment and Energy Catalysis Shaanxi Key Laboratory of Optoelectronic Functional Materials and DevicesSchool of Materials Science and Chemical EngineeringXi’an Technological UniversityXi’an 710021China College of Resources and Environmental Engineering Tianshui Normal UniversityTianshui 741001China

Electrocatalytic synthesis of ammonia as an environment-friendly and sustainable development method has received widespread attention in recent ***-dimensional(2D)materials are a promising catalyst for ammonia synthesis due to their large surface *** this work,we have constructed a series of 2D metal borides(MBenes)with transition metal(TM)defects(TMd-MBenes)and comprehensively calculated the reactivity of electrocatalytic synthesis of ammonia-based on density functional *** results have demonstrated that the TMd-MBenes can effectively activate nitrogen oxide(NO)and nitrogen(N2)molecules *** interesting,the co-chemisorption of O atoms,dissociated from NO,can facilitate the spilled of the inert N2 molecules into single N atoms,which can further hydrogenate into ammonia easily with an ultralow limiting potential of 0.59 V on *** research has not only provided clues for catalyst design for experimental study but also paved the way for the industrial application of electrocatalytic ammonia synthesis.

关键词： 2D mbenes Nitrogen electro-reduction DFT N_(2)activation Ammonia synthesis

High-throughput screening system of citrus bacterial cankerassociated transcription factors and its application to the regulation of citrus canker resistance

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Journal of Integrative Agriculture 2024年第1期23卷 155-165页

作者： jia fu Jie Fan Chenxi Zhang Yongyao fu Baohang Xian Qiyuan Yu Xin Huang Wen Yang Shanchun Chen Yongrui He Qiang li Integrative Science Center of Germplasm Creation in Western China(Chongqing)Science City Citrus Research InstituteSouthwest UniversityChongqing 400712China School of Advanced Agriculture and Bioengineering Yangtze Normal UniversityChongqing 408100China National Citrus Engineering Research Center Chongqing 400712China

One of the main diseases that adversely impacts the global citrus industry is citrus bacterial canker(CBC),caused by the bacteria Xanthomonas citri ***(Xcc).Response to CBC is a complex process,with both proteinDNA as well as protein–protein interactions for the regulatory *** detect such interactions in CBC resistant regulation,a citrus high-throughput screening system with 203 CBC-inducible transcription factors(TFs),were *** the upstream regulators of target by yeast-one hybrid(Y1H)methods was also performed.A regulatory module of CBC resistance was identified based on this *** TF(CsDOF5.8)was explored due to its interactions with the 1-kb promoter fragment of CsPrx25,a resistant gene of CBC involved in reactive oxygen species(ROS)homeostasis *** mobility shift assay(EMSA),dual-LUC assays,as well as transient overexpression of CsDOF5.8,further validated the interactions and transcriptional *** CsDOF5.8–CsPrx25 promoter interaction revealed a complex pathway that governs the regulation of CBC resistance via *** high-throughput Y1H/Y2H screening system could be an efficient tool for studying regulatory pathways or network of CBC resistance *** addition,it could highlight the potential of these candidate genes as targets for efforts to breed CBC-resistant citrus varieties.

关键词： citrus bacterial canker(CBC) high-throughput screening system transcription factor(TF) yeast-one hybrid(Y1H) CsPrx25