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铝碳微电解技术净化聚合氯化铝的研究

价值工程 2015年第4期34卷 295-296页

作者：李荣寨浙江传化股份有限公司杭州311215

铝矿粉与副产盐酸生产的聚合氯化铝中重金属杂质和有机杂质往往较多,借鉴铁碳微电解原理,人为投加活性炭,创造铝碳微电解条件,用来去除聚合氯化铝中的重金属和有机杂质。在采用铝碳比1:1,动态操作,停留时间在1小时的控制参数,处理费用约... 详细信息

铝矿粉与副产盐酸生产的聚合氯化铝中重金属杂质和有机杂质往往较多,借鉴铁碳微电解原理,人为投加活性炭,创造铝碳微电解条件,用来去除聚合氯化铝中的重金属和有机杂质。在采用铝碳比1:1,动态操作,停留时间在1小时的控制参数,处理费用约6.67元/吨的条件下,原液铅Pb2+含量23.3ppm,处理后铅Pb2+含量下降到5.8ppm,低于国标10ppm的要求。

关键词：铝碳微电解聚合氯化铝重金属铅去除

Designing Electronic Structures of Multiscale Helical Converters for Tailored Ultrabroad Electromagnetic Absorption

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Nano-Micro Letters 2025年第1期17卷 439-455页

作者： Zhaobo Feng Chongbo liu Xin li Guangsheng Luo Naixin zhai Ruizhe Hu Jing lin Jinbin Peng Yuhui Peng Renchao Che Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle School of Environmental and Chemical EngineeringNanchang Hangkong UniversityNanchang 330063People’s Republic of China School of Physics and Materials Nanchang UniversityNanchang 330031People’s Republic of China Key Laboratory of Nondestructive Testing Ministry of EducationNanchang Hangkong UniversityNanchang 330063People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering and TechnologyFudan UniversityShanghai 200438People’s Republic of China

Atomic-scale doping strategies and structure design play pivotal roles in tailoring the electronic structure and physicochemical property of electromagnetic wave absorption(EMWA)***,the relationship between configuration and electromagnetic(EM)loss mechanism has remained ***,drawing inspiration from the DNA transcription process,we report the successful synthesis of novel in situ Mn/N co-doped helical carbon nanotubes with ultrabroad EMWA *** calculation and EM simulation confirm that the orbital coupling and spin polarization of the Mn–N4–C configuration,along with cross polarization generated by the helical structure,endow the helical converters with enhanced EM *** a result,HMC-8 demonstrates outstanding EMWA performance,achieving a minimum reflection loss of−63.13 dB at an ultralow thickness of 1.29 *** precise tuning of the graphite domain size,HMC-7 achieves an effective absorption bandwidth(EAB)of 6.08 GHz at 2.02 mm ***,constructing macroscale gradient metamaterials enables an ultrabroadband EAB of 12.16 GHz at a thickness of only 5.00 mm,with the maximum radar cross section reduction value reaching 36.4 dB *** innovative approach not only advances the understanding of metal–nonmetal co-doping but also realizes broadband EMWA,thus contributing to the development of EMWA mechanisms and applications.

关键词： Metal-nonmetal co-doping 3d-2p orbital coupling Spin polarization Helical structure Broadband EM wave absorption

Situation-adaptive neural network for fast pre-computing image enhancement

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Science China(Information Sciences) 2025年

作者： Xinyue li Huiyu DUAN Jia WANG Xiaohong liU Yitong CHEN Guangtao zhai Institute of Image Communication and Network Engineering Department of Electronic EngineeringShanghai Jiao Tong University

As intelligent vision tasks become more widespread, enhancing image quality before further computational analysis is crucial. Recently, deep learning has shown potential for automated pre-computing enhancement, but it typically requires substantial computational resources and is hard to adapt to in multiple situations without *** practice, image enhancement often demands flexible adjustments based on different situations and subsequent computation devices, such as optical computing. Therefore,we propose SAEnhancer, a situation-adaptive neural network for fast pre-computing image enhancement. It learns from a small sample set to achieve personalized and adaptive enhancements for various situations without re-training,using semantic-aware embedding for precise color adjustments, surpassing traditional 3D lookup tables (LUTs), and enhancing computational effectiveness in intelligent vision applications.

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A self-adaptive inorganic in-situ separator by particle crosslinking for nonflammable lithium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 469-480页

作者： Jiarui Yang Jiuzhou liu Wenrui Cai Ziyu Zhao Shan Wang Lu He Shanshan Lv Zhiwei Zhu Zhongfeng Ji Guojiang Wen Hua li Yuanming zhai Xuewei Fu Wei Yang Yu Wang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University

All-safe liquid-state lithium-ion batteries(ASLS-liBs) is of great interest as they can potentially combine the safety of all-solid-state batteries with the high performance and low manufacturing cost of traditional liquid-state liBs. However, the practical success of ASLS-liBs is bottlenecked by the lack of advanced separator technology that can simultaneously realize high performances in puncturing-tolerability,fire-resistance, and importantly, wetting-capability with non-flammable liquid-electrolytes. Here, we propose a concept of inorganic in-situ separator(IISS) by hybrid-sol physical crosslinking directly onto the electrode surface to address the above challenges. Particularly, the hybrid-sol is designed with silica nanoparticles as the building block and poly(vinylidene difluoride) nanoparticles as the crosslinking agent. The critical factors for controlling the IISS microstructures and properties have been systematically investigated. The advantages of the IISS have been confirmed by its fast wetting with various fireresistant liquid-electrolytes, customizable thickness and porous structures, robust interface with planar or three-dimensional(3D)-structured electrodes, and importantly, unexpected self-adaptability against puncturing. Enabled by the above merits, a fire-resistant ASLS-liB is successfully assembled and demonstrated with stable electrochemical performance. This sol-crosslinked IISS may open an avenue for the studies on the next-generation separator technology, cell assembling, solid electrolyte processing as well as non-flammable secondary batteries.

关键词： Silica nanoparticles

Spontaneous Orientation Polarization of Anisotropic Equivalent Dipoles Harnessed by Entropy Engineering for Ultra‑Thin Electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： Honghan Wang Xinyu Xiao Shangru zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao Che Junye Cheng liaoning Key Lab of lignocellulose Chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China Department of Mechanical Engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and Engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HEAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HEAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HEAs and construction of emblematic shell-core CCF/HEAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HEAs composite prepared by 35%molar ratio of Mn element(CCP/HEAs-Mn_(2.15))achieves efficient electromagnetic wave(EMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HEAs-based EMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes Emblematic shell-core heterointerfaces Ultra-thin thickness

Gradient‑Layered MXene/Hollow lignin Nanospheres Architecture Design for Flexible and Stretchable Supercapacitors

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Nano-Micro Letters 2025年第2期17卷 447-462页

作者： Haonan Zhang Cheng Hao Tongtong Fu Dian Yu Jane Howe Kaiwen Chen Ning Yan Hao Ren Huamin zhai Jiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass Materials NanJing Forestry UniversityNanjing 210037People’s Republic of China Department of Chemical Engineering and Applied Chemistry University of Toronto200 College StreetTorontoON M5S 3E5Canada Department of Materials Science and Engineering University of Toronto184 College StreetTorontoON M5S 3E4Canada College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037People’s Republic of China

With the rapid development of flexible wearable electronics,the demand for stretchable energy storage devices has *** this work,a novel gradient-layered architecture was design based on single-pore hollow lignin nanospheres(HLNPs)-intercalated two-dimensional transition metal carbide(Ti_(3)C_(2)T_(x) MXene)for fabricating highly stretchable and durable *** depositing and inserting HLNPs in the MXene layers with a bottom-up decreasing gradient,a multilayered porous MXene structure with smooth ion channels was constructed by reducing the overstacking of MXene ***,the micro-chamber architecture of thin-walled lignin nanospheres effectively extended the contact area between lignin and MXene to improve ion and electron accessibility,thus better utilizing the pseudocapacitive property of *** these strategies effectively enhanced the capacitive performance of the *** addition,HLNPs,which acted as a protective phase for MXene layer,enhanced mechanical properties of the wrinkled stretchable electrodes by releasing stress through slip and deformation during the stretch-release cycling and greatly improved the structural integrity and capacitive stability of the *** electrodes and symmetric flexible all-solid-state supercapacitors capable of enduring 600%uniaxial tensile strain were developed with high specific capacitances of 1273 mF cm^(−2)(241 F g^(−1))and 514 mF cm^(−2)(95 F g^(−1)),***,their capacitances were well preserved after 1000 times of 600%stretch-release *** study showcased new possibilities of incorporating biobased lignin nanospheres in energy storage devices to fabricate stretchable devices leveraging synergies among various two-dimensional nanomaterials.

关键词： Hollow lignin nanospheres MXene Gradient-layered architecture Wrinkled electrodes Stretchable supercapacitors

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马氏体时效钢离子氮化工艺和渗层的研究

钢铁研究总院学报 1985年第2期 159-165页

作者：吴佩芝李荣翟中生李焱刘宏

本文对超高强度18Ni马氏体时效钢离子氮化前后的尺寸稳定性和渗层进行了研究。预时效和氮化工艺选择恰当使氮化前后有高度的尺寸稳定性。通过金相,X光相分析,俄歇谱仪,扫描电镜和透射电镜等,研究了渗层的组织、结构及相成分。采用了单... 详细信息

本文对超高强度18Ni马氏体时效钢离子氮化前后的尺寸稳定性和渗层进行了研究。预时效和氮化工艺选择恰当使氮化前后有高度的尺寸稳定性。通过金相,X光相分析,俄歇谱仪,扫描电镜和透射电镜等,研究了渗层的组织、结构及相成分。采用了单侧减薄的制膜技术,观察了化合物的精细结构。18Ni马氏体时效钢经离子氮化后,表面硬度可达HRC62以上,渗层深度大于0.2mm,扩散层内除有分布均匀的氮化物外,还有细而密的Ni3Mo存在,表面化合物层是由晶粒细小,且有一定方向性的γ′相组成。

关键词：离子氮化氮化工艺预时效渗氮马氏体时效钢高强度钢渗层

Controllably elevating the initial Coulombic efficiency of li3VO4 anode via a facile electrode pre-lithiation technique for lithium-ion batteries

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Science China Chemistry 2025年

作者： Haoyue liang Xingguo Zhong Guxin Huang Wenpan liu Yao liu Shuhao Wang Deyu Wang Hao liu Hao Wang Tianyou zhai Huiqiao li State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Shenzhen Research Institute of Huazhong University of Science and Technology Key Laboratory of Optoelectronic Chemical Materials and Devices (Ministry of Education) School of Optoelectronic Materials &Technology Jianghan University Centre for Clean Energy Technology Faculty of Science University of Technology Sydney Yichang Brunp Recycling Technology Co. Ltd.

li3VO4has been a promising insertion anode material for li-ion batteries,which has high theoretical capacity (up to～600 mAh g-1) and safe li insertion voltage （0.5–1 V ***/li+）.However,the low initial Coulombic efficiency （ICE） has always been the bottleneck limiting its ***,we propose a facile pre-lithiation method to controllably elevate the ICE by the post-treatment of the prepared li3VO4composite electrode based on an immersion *** this process,the whole electrode was immersed in the liquid li source,via which the ICE of the li3VO4electrode can be controllably elevated from 80%to over 100%within 5 min of *** than the traditional powder treatment for pre-lithiation,this process we proposed minimizes the impact of pre-lithiation on the battery assembly ***,we further investigated the effect of this pre-lithiation process on the functional components in the *** the first time the ICE of li3VO4electrode was elevated to 100%.As a result,the initial reversible capacity of liFePO4||li3VO4full cell was improved from 44.0 to146.3 m Ah g-1,demonstrating the feasibility and great potential of the process.

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Changes in Summer Persistent Precipitation over the Middle–Lower Reaches of the Yangtze River and Associated Atmospheric Circulation Patterns

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Journal of Meteorological Research 2021年第3期35卷 393-401页

作者： rong YU Panmao zhai State Key Laboratory of Severe Weather Chinese Academy of Meteorological SciencesChina Meteorological AdministrationBeijing 100081

Persistence is an important property of precipitation and its related impacts. However, changes in persistent precipitation and the possible underlying mechanisms in the context of global warming have not yet been discussed in sufficient depth. In this study, the changes in persistent precipitation in summer and related atmospheric circulation patterns over the middle–lower reaches of the Yangtze River(MLRYZR)—a typical monsoon region frequently hit by consecutive rainfall events—are analyzed based on observed daily precipitation and NCEP/NCAR reanalysis data from 1961 to 2019. The results reveal that persistent precipitation events(PPs) tend to happen in a more persistent way, with increased frequency and intensity in the MLRYZR region. Mechanism analyses show that persistent precipitation has happened along with simultaneous enhancement of some large-scale atmospheric circulation patterns,including the Lake Baikal blocking(BB), the Okhotsk Sea blocking(OB), and the western Pacific subtropical high(WPSH). Such enhanced anomalous circulation patterns could persistently reinforce the convergence and supply of water vapor in the MLRYZR region, contributing to the increase in PPs in this region. Based on the above results, we are able to offer some new insights into the long-term changes in precipitation structure and the possible causes. This study is also expected to support attribution studies on regional precipitation changes in the future.

关键词： persistent precipitation precipitation change atmospheric circulation pattern