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Integration of urchin-like MnCo_(2)O_(4)@C core–shell nanowire arrays within porous copper current collector for superior performance li-ion battery anodes

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Rare Metals 2024年第2期43卷 599-611页

作者： Xue-Ru Zhang Qiong wu Yong Zhang Xi-fei li Ting Xie Yu-Cheng wu Instrumental Analysis Center Hefei University of TechnologyHefei230009China Key Laboratory of Advanced Functional Materials and Devices of Anhui Province Hefei230009China School of Materials Science and Engineering Hefei University of TechnologyHefei230009China Institute of Advanced Electrochemical Energy Xi’an University of TechnologyXi’an710048China

Spinel MnCo_(2)O_(4) is a promising energy storage candidate as anode materials in lithium-ion batteries owing to synergistic effects of two intrinsic solid-state redox ***,low conductivity,poor rate capacity and rapid capacity fading have seriously impaired its practical *** overcome the inferiorities,urchin-like MnCo_(2)O_(4)@C core–shell nanowire arrays have been fabricated directly within a porous copper current collector via a facile hydrothermal method followed by a chemical vapor deposition carbonization *** a typical nanowire,the core is composed of interconnected MnCo_(2)O_(4)nanoparticles and the shell shows as a thin amorphous carbon *** integrated MnCo_(2)O_(4)@C/Cu structure could act as working anodes without using additives or polymer *** MnCo_(2)O_(4)@C/Cu possesses slightly longer li-ion insertion/desertion pathway than that of MnCo_(2)O_(4)/Cu,the carbon shell could effectively prevent the pulverization of MnCo_(2)O_(4) and lower down charge transfer resistance and actively participate in li-ion *** rearrangement of carbon atoms during lithiation/delithiation cycling could inhibit the formation of passive solid electrolyte interphase *** a result,the MnCo_(2)O_(4)@C/Cu electrode presents superior rate capacity(600 mAh·g^(−1) at 1 A·g^(−1)) and better stability(797 mAh·g^(−1) after 200 cycles at 100 mA·g^(−1)).The excellent reversible li ion storage capacity,cycling stability and rate capacity endow MnCo_(2)O_(4)@C/Cu great potential as stable and high output integrated anode materials in li-ion batteries.

关键词： MnCo_(2)O_(4)@C Urchin-like nanowire arrays Core-shell Integrated anode materials lithium-ion batteries

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A quantum federated learning framework for classical clients

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Science China(Physics,Mechanics & Astronomy) 2024年第5期67卷 1-10页

作者： Yanqi Song Yusen wu Shengyao wu Dandan li Qiaoyan Wen Sujuan Qin fei Gao State Key Laboratory of Networking and Switching Technology Beijing University of Posts and TelecommunicationsBeijing 00876China Department of Physics The University of Western AustraliaPerthWA 6009Australia School of Computer Science(National Pilot Software Engineering School) Beijing University of Posts and TelecommunicationsBeijing100876China

Quantum federated learning(QFL)enables collaborative training of a quantum machine learning(QML)model among multiple clients possessing quantum computing capabilities,without the need to share their respective local ***,the limited availability of quantum computing resources poses a challenge for each client to acquire quantum computing *** raises a natural question:Can quantum computing capabilities be deployed on the server instead?In this paper,we propose a QFL framework specifically designed for classical clients,referred to as CC-QFL,in response to this *** each iteration,the collaborative training of the QML model is assisted by the shadow tomography technique,eliminating the need for quantum computing capabilities of ***,the server constructs a classical representation of the QML model and transmits it to the *** clients encode their local data onto observables and use this classical representation to calculate local *** local gradients are then utilized to update the parameters of the QML *** evaluate the effectiveness of our framework through extensive numerical simulations using handwritten digit images from the MNIST *** framework provides valuable insights into QFL,particularly in scenarios where quantum computing resources are scarce.

关键词： client server quantum

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A novel box-counting method for quantitative fractal analysis of threedimensional pore characteristics in sandstone

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International Journal of Mining Science and Technology 2024年第4期34卷 479-489页

作者： Huiqing liu Heping Xie fei wu Cunbao li Renbo Gao State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400030China School of Resources and Safety Engineering Chongqing UniversityChongqing 400030China Guangdong Provincial Key Laboratory of Deep Earth Sciences and Geothermal Energy Exploitation and Utilization Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Deep Underground Engineering Sciences and Green Energy College of Civil and Transportation EngineeringShenzhen UniversityShenzhen 518060China

Fractal theory offers a powerful tool for the precise description and quantification of the complex pore structures in reservoir rocks,crucial for understanding the storage and migration characteristics of media within these *** with the challenge of calculating the three-dimensional fractal dimensions of rock porosity,this study proposes an innovative computational process that directly calculates the three-dimensional fractal dimensions from a geometric *** employing a composite denoising approach that integrates Fourier transform(FT)and wavelet transform(WT),coupled with multimodal pore extraction techniques such as threshold segmentation,top-hat transformation,and membrane enhancement,we successfully crafted accurate digital rock *** improved box-counting method was then applied to analyze the voxel data of these digital rocks,accurately calculating the fractal dimensions of the rock pore *** numerical simulations of permeability experiments were conducted to explore the physical correlations between the rock pore fractal dimensions,porosity,and absolute *** results reveal that rocks with higher fractal dimensions exhibit more complex pore connectivity pathways and a wider,more uneven pore distribution,suggesting that the ideal rock samples should possess lower fractal dimensions and higher effective porosity rates to achieve optimal fluid transmission *** methodology and conclusions of this study provide new tools and insights for the quantitative analysis of complex pores in rocks and contribute to the exploration of the fractal transport properties of media within rocks.

关键词： 3D fractal analysis Fractal dimension Rock pore structure Box-counting method Permeability simulation Computational geosciences

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Hole-Transporting Materials with Rational Combination of Pyridine and Dibenzo[a,c]phenazine as Electron Acceptor for Dopant-Free Perovskite Solar Cells

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Chinese Journal of Chemistry 2024年第10期42卷 1100-1106页

作者： Weidong ling fei wu Wentao Yuan linna Zhu Qianqian li Zhen li Hubei Key Lab on Organic and Polymeric Opto-Electronic Materials Department of ChemistryWuhan UniversityWuhanHubei 430072China Chongqing Key Laboratory for Advanced Materials and Technologies of Clean Energy Faculty of Materials&EnergySouthwest UniversityChongqing400715China TaiKang Center for life and Medical Sciences Wuhan UniversityWuhanHubei 430072China

Perovskite solar cells(PSCs)have been proven to be a promising option for photovoltaic *** the aim to achieve efficient and stable PSCs,it is essential to explore dopant-free hole-transporting materials(HTMs)with high hole ***,HTMs bearing electron donor(D)-electron acceptor(A)-electron donor(D)structures have been constructed with strong intramolecular charge transfer(ICT)effect,based on rational combination of dibenzo[a,c]phenazine and pyridine as electronic acceptors and anchoring groups to perovskite ***,high hole mobility(7.31×10^(-5) cm^(2)·V^(-1)·s^(-1))and photoelectric conversion efficiency(20.45%)have been achieved by dopant-free DPyP-based *** afforded an efficient way to design HTMs with high hole mobility by adjustment of molecular configurations and electronic property of conjugated systems.

关键词： Perovskite solar cell Charge transfer Donor-acceptor systems Energy conversion Hole mobility

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Homer1a reduces inflammatory response after retinal ischemia/reperfusion injury

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Neural Regeneration Research 2024年第7期19卷 1608-1617页

作者： Yanan Dou Xiaowei fei Xin He Yu Huan Jialiang Wei Xiuquan wu Weihao Lyu Zhou fei Xia li fei fei Department of Neurosurgery Xijing HospitalAir Force Military Medical UniversityXi’anShaanxi ProvinceChina Department of Ophthalmology Xijing HospitalAir Force Military Medical UniversityXi’anShaanxi ProvinceChina

Elevated intraocular pressure(IOP)is one of the causes of retinal ischemia/reperfusion injury,which results in NRP3 inflammasome activation and leads to visual *** is repo rted to play a protective role in neuroinflammation in the ***,the effects of Homerla on NLRP3inflammasomes in retinal ischemia/reperfusion injury caused by elevated IOP remain *** our study,animal models we re constructed using C57BL/6J and Homer1^(flox/-)/Homerla^(+/-)/Nestin-Cre^(+/-)mice with elevated IOP-induced retinal ischemia/repe rfusion *** in vitro expe riments,the oxygen-glucose deprivation/repe rfusion injury model was constructed with M uller *** found that Homerla ove rexpression amelio rated the decreases in retinal thickness and Muller cell viability after ischemia/reperfusion ***,Homerla knockdown promoted NF-κB P65^(Ser536)activation via caspase-8,NF-κB P65 nuclear translocation,NLRP3 inflammasome formation,and the production and processing of interleukin-1βand inte *** opposite results we re observed with Homerla ove ***,the combined administration of Homerla protein and JSH-23 significantly inhibited the reduction in retinal thickness in Homer1^(flox/-)Homer1a^(+/-)/Nestin-Cre^(+/-)mice and apoptosis in M uller cells after ischemia/reperfusion *** together,these studies demonstrate that Homer1a exerts protective effects on retinal tissue and M uller cells via the caspase-8/NF-KB P65/NLRP3 pathway after I/R injury.

关键词： caspase-8 Homer1a interleukin-18 interleukin-1β intraocular pressure ischemia/reperfusion injury JSH-23 Müller cells NLRP3 nuclear factor-kB p65 retina

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Self-assembly of perovskite nanocrystals:From driving forces to applications

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Journal of Energy Chemistry 2024年第1期88卷 561-578,I0013页

作者： Yi li fei Zhang School of Chemical Engineering and Technology Tianjin UniversityTianjin 300072China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) Tianjin 300072China

Self-assembly of metal halide perovskite nanocrystals(NCs)into superlattices can exhibit unique collective properties,which have significant application values in the display,detector,and solar cell *** review discusses the driving forces behind the self-assembly process of perovskite NCs,and the commonly used self-assembly methods and different self-assembly structures are ***,we summarize the collective optoelectronic properties and application areas of perovskite superlattice ***,we conclude with an outlook on the potential issues and future challenges in developing perovskite NCs.

关键词： Self-assembly Metal halide perovskite Nanocrystals Driving forces

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The significance of long non-coding RNAs in the pathogenesis,diagnosis and treatment of inflammatory bowel disease

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Precision Clinical Medicine 2024年第1期7卷 34-53页

作者： fei Jiang Min wu Rongpeng li Jiangsu Province Engineering Research Center of Cardiovascular Drugs Targeting Endothelial Cells School of Life SciencesJiangsu Normal UniversityXuzhou 221000China Department of Laboratory Medicine the Affiliated Hospital of Xuzhou Medical UniversityXuzhou 221000China Drug Discovery Section Wenzhou InstituteUniversity of Chinese Academy of SciencesWenzhou 325000China Department of Neurology Medical College of WisconsinMilwaukeeWI 53226USA

Inflammatory bowel diseases(IBD)are a group of chronic relapsing gastrointestinal inflammatory diseases with significant global *** the pathomechanism of IBD has been extensively investigated,several aspects of its pathogenesis remain *** non-coding RNAs(lncRNAs)are transcripts with more than 200 nucleotides in length that have potential protein-coding *** play important roles in biological processes such as epigenetic modification,transcriptional regulation and posttranscriptional *** this review,we summarize recent advances in research on IBD-related lncRNAs from the perspective of the overall intestinal microenvironment,as well as their potential roles as immune regulators,diagnostic biomarkers and therapeutic targets or agents for IBD.

关键词： lncRNAs inflammatory bowel diseases intestinal barrier intestinal microenvironment immune regulator diagnostic biomarker therapeutic target

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Synthesis,Characterization of Polyethylene Ionomers and Their Antibacterial Properties

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Chinese Journal of Polymer Science 2024年第8期42卷 1077-1084页

作者： Jia-Jia wu fei Wang Peng-Qi Wan li Pan Chun-Sheng Xiao Zhe Ma Yue-Sheng li Tianjin Key Lab Composite&Functional Materials School of Materials Science and EngineeringTianjin UniversityTianjin 300350China Key Lab Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China

Owing to its high production volume and wide range of application s,polyethylene has gained a great deal of attention,but its low surface energy and non-polar nature have limited its application in some important *** this study,ethylene/11-iodo-1-undecene copolymers were prepared and used as the intermediates to afford a series of imidazolium-based ionomers bearing methanesulfonate(CH_(3)SO_(3)^(-)),trifluoromethanesulfonate(CF_(3)SO_(3)^(-)),or bis(trifluoromethane)sulfonimide(Tf_(2)N^(-))*** tensile test results showed that the stress-at-break(7.8-25.6 MPa)and the elongation-at-break(445%-847%)of the ionomers could be adjusted by changing the counterion species and the ionic group *** importantly,the ionomers exhibited marvelous antibacterial activities against Staphylococcus aureus(***)and Escherichia coli(***).The ionomers bearing Tf_(2)N^(-)exhibited antibacterial activities>99%against both *** and *** when ionic content reached 9.1%.The imidazolium-based ionomers prepared in this work demonstrated excellent comprehensive properties,especially highefficient and broad-spectrum antibacterial ability,exhibiting the potential fo r the application as the antibacterial materials in packaging,medical,and other fields.

关键词： Polyethylene Ionomer Polymerization catalysis Imidazolium Antibacterial material

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A Difference Scheme with Intrinsic Parallelism for Fractional Diffusion-wave Equation with Damping

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Acta Mathematicae Applicatae Sinica 2021年第3期37卷 602-616页

作者： li-fei wu Xiao-Zhong YANG Min li School of Mathematics and Physics North China Electric Power UniversityBeijing 102206China

Anomalous diffusion is a widespread physical phenomenon,and numerical methods of fractional diffusion models are of important scientific significance and engineering application *** time fractional diffusion-wave equation with damping,a difference(ASC-N,alternating segment Crank-Nicolson)scheme with intrinsic parallelism is *** on alternating technology,the ASC-N scheme is constructed with four kinds of Saul’yev asymmetric schemes and Crank-Nicolson(C-N)*** unconditional stability and convergence are rigorously *** theoretical analysis and numerical experiments show that the ASC-N scheme is effective for solving time fractional diffusion-wave equation.

关键词： time fractional diffusion-wave equation with damping intrinsic parallelism ASC-N scheme stability parallel computing

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Considering solid shear stress in MP-PIC simulation of a CFB riser

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Particuology 2024年第6期89卷 79-87页

作者： Tagir Kadyrov fei li Atta Ullah Nature-inspired Engineering Center University of TyumenTyumen 625003Russia Laboratory of Theory and Optimization of Chemical and Technological Processes University of TyumenTyumen625003Russia State Key Laboratory of Multi-phase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Department of Chemical Engineering Pakistan Institute of Engineering&Applied SciencesIslamabad 45650Pakistan

To enable successful multi-phase particle-in-cell(MP-PIC)simulations of circulating fluidized beds(CFBs),both the interphase drag force and interparticle collisions need to be carefully *** collisions are usually represented by the solid stress consisting of the normal and shear components,in which the normal stress was found to have a leading role in the numerical stability of MP-PIC simulations,whereas the impact of the shear stress has seldom been *** this work,the effects of the solid shear stress are investigated by using two-dimensional simulations of the moderately dense laboratory-scale CFB riser with in-house MP-PIC code implemented on MFIX open-source *** including only normal solid stress and those considering both normal and shear solid stresses are *** results of solids flux,axial and radial solids profiles are compared with available experimental *** results show that the solid shear stress plays a minor role on the accuracy of simulation,and the increase of PPP(number particles per parcel)leads to a lower accuracy of simulation.

关键词： Simulation Fluidization Multiphase particle-in-cell(MP-PIC) Solid shear stress

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