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Hydrothermal synthesis mechanism and electrochemical performance of liMn_(0.6)Fe_(0.4)PO_4 cathode material

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Rare Metals 2019年第1期38卷 29-34页

作者： Chang-Chang Xu Ying Wang li li Yi-Jing Wang li-fang jiao Hua-Tang Yuan Institute of New Energy Material Chemistry Nankai University Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) Nankai University Key Laboratory of Advanced Energy Materials Chemistry Nankai University Tianjin Key Laboratory on Metal and Molecule-based Material Chemistry Nankai University

Monocrystal liMn_(0. 6)Fe_(0. 4)PO_4 cathode material was obtained via hydrothermal method at 180℃ for 10 h without any surfactant. The effects of hydrothermal time on the phase and morphology of the material were *** controlling the reaction solutions, the rodlike, flowerlike,and strawlike liMn_(0.6)Fe_(0.4)PO_4 cathode materials were synthesized. Electrochemical performances show that the rodlike liMn_(0. 6)Fe_(0. 4)PO_4 has the best electrochemical properties. The initial discharge capacity of the rodlike structure is 106.4 mAh·g^(-1), which is higher than those of flowerlike and strawlike materials.

关键词： liMn0.6Fe0.4PO4 Hydrothermal method Cathode material lithium-ion batteries Synthesis mechanism

Advances in the Development of Gradient Scaffolds Made of Nano-Micromaterials for Musculoskeletal Tissue Regeneration

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NANO-MICRO LETTERS 2025年第1期17卷 1-46页

作者： fang, Lei lin, Xiaoqi Xu, Ruian liu, Lu Zhang, Yu Tian, Feng li, jiao jiao Xue, Jiajia Beijing Univ Chem Technol Beijing Lab Biomed Mat Beijing 100029 Peoples R China Beijing Univ Chem Technol State Key Lab Organ Inorgan Composites Beijing 100029 Peoples R China Univ Technol Sydney Fac Engn & IT Sch Biomed Engn Sydney NSW 2007 Australia

This review highlights the gradient variations in the structural composition of musculoskeletal tissues and comprehensively examines recent progress in the fabrication and application of biomimetic gradient scaffolds for musculoskeletal *** challenges and prospects of gradient scaffolds for clinical application are discussed. The intricate hierarchical structure of musculoskeletal tissues, including bone and interface tissues, necessitates the use of complex scaffold designs and material structures to serve as tissue-engineered substitutes. This has led to growing interest in the development of gradient bone scaffolds with hierarchical structures mimicking the extracellular matrix of native tissues to achieve improved therapeutic outcomes. Building on the anatomical characteristics of bone and interfacial tissues, this review provides a summary of current strategies used to design and fabricate biomimetic gradient scaffolds for repairing musculoskeletal tissues, specifically focusing on methods used to construct compositional and structural gradients within the scaffolds. The latest applications of gradient scaffolds for the regeneration of bone, osteochondral, and tendon-to-bone interfaces are presented. Furthermore, the current progress of testing gradient scaffolds in physiologically relevant animal models of skeletal repair is discussed, as well as the challenges and prospects of moving these scaffolds into clinical application for treating musculoskeletal injuries.

关键词： Gradient scaffolds Musculoskeletal tissues Advanced manufacturing Biomaterials Tissue regeneration

IMPROVED MLV FILTER TO REMOVE MULTIPliCATIVE NOISE

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Journal of Electronics(China) 2006年第1期23卷 85-88页

作者： li Weibin liu fang jiao licheng Zhang Shuling li Zongling Institute of Graphics and lmage Processing Xiangyang Normal University Xianyang 712000 China National Key Laboratory for Radar Signal Processing Xidian University Xi＇an 710071 China Insititute of lntelligent Information Processing Xidian University Xi＇an 710071China

More methods can be used to remove the additive noise, such as the Mean of Least Variance (MLV) filter. When the signal is noised by the multiplicative noise, it is difficult to remove. The paper presents an improved filter to remove multiplicative noise by changing the multiplicative noise to the additive noise, and then using the MLV-like to remove the additive noise. The simulation results show that the performance is better than Minimum Coefficient of Variation (MCV) filter and MLV filter. Both one-dimension and image experiments demonstrate its theoretical performance.

关键词： Denoising Minimum Coefficient of Variation (MCV) Mean of Least Variance (MLV)

The autophagy-lysosome pathway:a potential target in the chemical and gene therapeutic strategies for Parkinson’s disease

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Neural Regeneration Research 2025年第1期20卷 139-158页

作者： Fengjuan jiao lingyan Meng Kang Du Xuezhi li School of Mental Health Jining Medical UniversityJiningShandong ProvinceChina Shandong Collaborative Innovation Center for Diagnosis Treatment and Behavioral Interventions of Mental DisordersInstitute of Mental HealthJining Medical UniversityJiningShandong ProvinceChina

Parkinson’s disease is a common neurodegenerative disease with movement disorders associated with the intracytoplasmic deposition of aggregate proteins such asα-synuclein in *** one of the major intracellular degradation pathways,the autophagy-lysosome pathway plays an important role in eliminating these *** evidence has shown that upregulation of the autophagy-lysosome pathway may contribute to the clearance ofα-synuclein aggregates and protect against degeneration of dopaminergic neurons in Parkinson’s ***,multiple genes associated with the pathogenesis of Parkinson’s disease are intimately linked to alterations in the autophagy-lysosome ***,this pathway appears to be a promising therapeutic target for treatment of Parkinson’s *** this review,we briefly introduce the machinery of ***,we provide a description of the effects of Parkinson’s disease–related genes on the autophagy-lysosome ***,we highlight the potential chemical and genetic therapeutic strategies targeting the autophagy–lysosome pathway and their applications in Parkinson’s disease.

关键词： autophagy chemical therapy gene therapy Parkinson’s disease α-synuclein

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实用医学杂志 2016年第18期32卷 3044-3046页

作者：李兰芳曾姣娥湖北省荆州中心医院内分泌科 434020

目的:探讨分泌型卷曲相关蛋白5(Sfrp5)与2型糖尿病(T2DM)大血管病变的相关性及羟苯磺酸钙的干预作用。方法:T2DM患者分为实验组(IMT≥0.90 mm)65例和对照组(IMT0.05)。A组IMT下降幅度高于B组(P<0.05)。结论 :Sfrp5与大血管病变呈负相关... 详细信息

目的:探讨分泌型卷曲相关蛋白5(Sfrp5)与2型糖尿病(T2DM)大血管病变的相关性及羟苯磺酸钙的干预作用。方法:T2DM患者分为实验组(IMT≥0.90 mm)65例和对照组(IMT0.05)。A组IMT下降幅度高于B组(P<0.05)。结论 :Sfrp5与大血管病变呈负相关,羟苯磺酸钙可升高Sfrp5、IL-10水平,延缓大血管病变的进展。

关键词： 2型糖尿病大血管病变分泌型卷曲相关蛋白5 白介素-10 羟苯磺酸钙

High-energy-density lithium manganese iron phosphate for lithium-ion batteries: Progresses, challenges, and prospects

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Journal of Energy Chemistry 2025年第1期100卷 1-17页

作者： Bokun Zhang Xiaoyun Wang Shuai Wang Yan li libo Chen Handong jiao Zhijing Yu Jiguo Tu State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing Research Institute for Intelligent Wearable Systems The Hong Kong Polytechnic University Institute of Advanced Structure Technology Beijing Institute of Technology

The soaring demand for smart portable electronics and electric vehicles is propelling the advancements in high-energy–density lithium-ion *** manganese iron phosphate (liMnxFe1-xPO4) has garnered significant attention as a promising positive electrode material for lithium-ion batteries due to its advantages of low cost,high safety,long cycle life,high voltage,good high-temperature performance,and high energy *** liMnxFe1-xPO4has made significant breakthroughs in the past few decades,there are still facing great challenges in poor electronic conductivity and li-ion diffusion,manganese dissolution affecting battery cycling performance,as well as low tap *** review systematically summarizes the reaction mechanisms,various synthesis methods,and electrochemical properties of liMnxFe1-xPO4to analyze reaction processes accurately and guide material ***,the main challenges currently faced are concluded,and the corresponding various modification strategies are discussed to enhance the reaction kinetics and electrochemical performance of liMnxFe1-xPO4,including multi-scale particle regulation,heteroatom doping,surface coating,as well as microscopic morphology ***,in view of the current research challenges faced by intrinsic reaction processes,kinetics,and energy storage applications,the promising research directions are *** importantly,it is expected to provide key insights into the development of high-performance and stable liMnxFe1-xPO4materials,to achieve practical energy storage requirements.

关键词： lithium manganese iron phosphate High energy density lithium-ion batteries Reaction mechanism Tap density

α-MnO_2 nanoneedle-based hollow microspheres coated with Pd nanoparticles as a novel catalyst for rechargeable lithium-air batteries

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Transactions of Nonferrous Metals Society of China 2014年第1期24卷 164-170页

作者：张明徐强桑林丁飞刘兴江焦丽芳天津大学化工学院天津300072 天津电源研究所化学与物理电源重点实验室天津300384 南开大学先进能源材料化学教育部重点实验室天津300071

The hollow α-MnO2 nanoneedle-based microspheres coated with Pd nanoparticles were reported as a novel catalyst for rechargeable lithium-air batteries. The hollow microspheres are composed ofα-MnO2 nanoneedles. Pd nanoparticles are deposited on the hollow microspheres through an aqueous-solution reduction of PdCl2 with NaBH4 at room temperature. The results of TEM, XRD, and EDS show that the Pd nanoparticles are coated on the surface ofα-MnO2 nanoneedles uniformly and the mass fraction of Pd in the Pd-coated α-MnO2 catalyst is about 8.88%. Compared with the counterpart of the hollow α-MnO2 catalyst, the hollow Pd-coated α-MnO2 catalyst improves the energy conversion efficiency and the charge-discharge cycling performance of the air electrode. The initial specific discharge capacity of an air electrode composed of Super P carbon and the as-prepared Pd-coatedα-MnO2 catalyst is 1220 mA＆#183;h/g （based on the total electrode mass） at a current density of 0.1 mA/cm2, and the capacity retention rate is about 47.3% after 13 charge-discharge cycles. The results of charge-discharge cycling tests demonstrate that this novel Pd-coatedα-MnO2 catalyst with a hierarchical core-shell structure is a promising catalyst for the lithium-air battery.

关键词： lithium-air battery composite catalyst nanoneedle-based hollow microsphere core-shell structure

Interfacial Zn2+-solvation regulator towards reversible and stable Zn anode

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Journal of Energy Chemistry 2025年第1期100卷 684-692页

作者： Miao Zhou Xiongbin Luo Hang li Shan Guo Zhuang Tong Xiaotao Zhou Xu li Zhaohui Hou Shuquan liang Guozhao fang College of Mechanical Engineering Key Laboratory of Hunan Province for Advanced Carbon-based Functional Materials Hunan Institute of Science and Technology School of Materials Science and Engineering Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province Central South University College of Materials and Metallurgy Guizhou University National Energy Metal Resources and New Materials Key Laboratory Central South University

Aqueous zinc-ion batteries （AZIBs） are fundamentally challenged by the instability of the electrode/electrolyte interface,predominantly due to irreversible zinc （Zn） deposition and hydrogen ***,the intricate mechanisms behind the electrochemical discrepancies induced by interfacial Zn2+-solvation and deposition behavior demand comprehensive *** molecules endowed with special functional groups （such as hydroxyl,carboxyl,etc.） have the potential to significantly optimize the solvation structure of Zn2+and regulate the interfacial electric double layer （EDL）.By increasing nucleation overpotential and decreasing interfacial free energy,these functional groups facilitate a lower critical nucleation radius,thereby forming an asymptotic nucleation model to promote uniform Zn ***,this study presents a pioneering approach by introducing trace amounts of n-butanol as solvation regulators to engineer the homogenized Zn （H-Zn） anode with a uniform and dense *** interfacial reaction and structure evolution are explored by in/ex-situ experimental techniques,indicating that the H-Zn anode exhibits dendrite-free growth,no by-products,and weak hydrogen evolution,in sharp contrast to the bare ***,the H-Zn anode achieves a remarkable Zn utilization rate of approximately 20% and simultaneously sustains a prolonged cycle life exceeding 500 ***,the H-Zn//NH4V4O10（NVO） full battery showcases exceptional cycle stability,retaining 95.04%capacity retention after 400 cycles at a large current density of 5 A *** study enlightens solvation-regulated additives to develop Zn anode with superior utilization efficiency and extended operational lifespan.

关键词： Aqueous zinc-ion batteries Interfacial reaction Asymptotic nucleation model Reversible and stable Zn anode

The low-latitude sodium layer:comparative data from lidar observations at Hainan,China and São Paulo,Brazil

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Earth and Planetary Physics 2025年第1期9卷 39-53页

作者： fang Wu Jing jiao GuoTao Yang lifang Du ZhengKuan liu HaoRan Zheng JiXin Guo ShaoHua Gong YaJun Zhu State Key Laboratory of Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China Hainan National Field Science Observation and Research Observatory for Space Weather National Space Science CenterChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China China-Brazil Joint Laboratory for Space Weather NSSC/INPESão Josédos Campos 12227-010Brazil School of Physics and Electronics Engineering Hainan Normal UniversityHaikou 571158China

Physical and chemical processes observed in the mesosphere and thermosphere above the Earth’s low latitudes are complex and highly interrelated to activity in the low-latitude *** sodium detected by lidar can yield clues to dynamic and chemical processes in these spatial layers above the Earth’s *** paper is based on sodium layer data collected at two low-latitude stations,one in the northern hemisphere and one in the *** low-latitude sodium layer exhibits conspicuous seasonal variations in shape,density,and altitude;these variations are similar between Earth’s hemispheres:sodium layer density at both stations reaches its seasonal maximum in autumn and minimum in ***,maximal Na density over Brazil is greater than that over *** variations of Na density above the two low-latitude stations are also similar;at both,maxima are observed before *** variations of the Na layer over Brazil that differ from those observed in the northern hemisphere may be related to the South Atlantic Magnetic Anomaly(SAMA)or fountain *** suggest that low-latitude Na layer data may provide useful additional evidence that could significantly improve the low-latitude part of the WACCM-Na model.

关键词： metallic sodium layer seasonal variation nocturnal variation lidar