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Facile fabrication of graphene/g-C_(3)N_(4) for electromagnetic wave absorption

Nano Research 2024年第3期17卷 1687-1698页

作者： Qiang Su Yunfei He Dongdong liu Daguang li Long Xia Xiaoxiao Huang Bo zhong School of Materials Science and Engineering Harbin Institute of Technology WeihaiWeihai 264209China Weihai Yunshan Technology Co. Ltd.Weihai 264200China State Key Laboratory on Integrated Optoelectronics College of Electronic Science&EngineeringJilin UniversityChangchun 130012China School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China

With the development of the miniaturization of electronic equipment and lightweight weapon equipment,there are new requirements for electromagnetic wave absorption material(EMWAM).EMWAM has outstanding electromagnetic wave absorption properties and lightweight characteristics become an important direction of *** this study,graphene/g-C_(3)N_(4)(GGCN)EMWAM was first synthesized in situ by simple heat treatment,in which the g-C_(3)N_(4) had a porous structure and dispersed on the surface of *** impedance matching of the GGCN was well adjusted by decreasing the dielectric constant and attenuation constant due to the g-C_(3)N_(4) semiconductor property and the graphite-like *** EMW loss mechanism of GGCN was also analyzed by simulating GGCN’s electric field mode distribution and resistance loss power *** analysis result shows that the distribution of g-C_(3)N_(4) among GGCN sheets can produce more polarization effects and relaxation effects by increasing the lamellar ***,the polarization loss of GGCN could be increased successfully by porous g-C_(3)N_(4).Ultimately,the EMW absorption property of GGCN is optimized significantly,and GGCN exhibits excellent EMW absorption *** the thickness is 2 mm,the effective absorption bandwidth(EAB)can reach 4.6 GHz,and when the thickness is 4.5 mm,the minimum reflection loss(RLmin)at 4.56 GHz can reach-34.69 ***,the practical application of EMWAM was studied by radar cross-section(RCS)simulation,showing that GGCN has a good application prospect.

关键词： graphene/g-C_(3)N_(4) impedance matching simulation analysis dielectric loss excellent electromagnetic wave absorption

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Regulation of aqueous electrolyte interface via electrolyte strategies for uniform zinc deposition

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Nano Research 2024年第10期17卷 8678-8693页

作者： Wei zhong Chaoqiang Tan Laixi li Shichao Zhang Xinyang Wang Hao Cheng Yingying Lu Institute of Wenzhou Zhejiang UniversityWenzhou 325006China State Key Laboratory of Chemical Engineering Institute of Pharmaceutical EngineeringCollege of Chemical and Biological EngineeringZhejiang UniversityHangzhou 310027China ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang UniversityHangzhou 311215China Zhejiang Huayou Cobalt Company limited Tongxiang 314500China

Aqueous zinc ion batteries(AZIBs),renowned for their high theoretical energy density,safety,cost-effectiveness and ecofriendliness,offer immense potential in the realm of energy storage and conversion,finding applications in renewable energy and portable ***,the development of AZIBs still faces several challenges related to the electrochemical behavior of zinc anodes in aqueous electrolytes,primarily zinc dendrite formation,which emphasize the critical need for a fundamental understanding of the interfacial phenomena between the electrode and *** review focuses on the three models:the electric double layer(EDL)model,the solvation structure model,and the Zn/electrolyte interface *** guide the design of the electrolyte system in *** models provide a comprehensive understanding of the interactions between the electrode,electrolyte,and the solvated ions in the *** optimizing the salt types,salt concentrations,solvents and additives based on these models,it is possible to enhance the performance of AZIBs,including their energy density,cycle life,and *** review also highlights recent research progress in electrolyte modification of AZIBs for understanding battery behavior,along with perspectives for the direction of further investigations.

关键词： aqueous zinc ion batteries electric double layer solvation structure electrolyte optimization

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Contrasting strategies of optimizing carrier concentration in bulk InSe for enhanced thermoelectric performance

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Rare Metals 2024年第9期43卷 4425-4432页

作者： Hao-Nan Shi Shu-lin Bai Yu-Ping Wang li-zhong Su Qian Cao Cheng Chang li-Dong Zhao School of Materials Science and Engineering Beihang UniversityBeijing 100191China School of Materials Science and Engineering Taiyuan University of Science and TechnologyTaiyuan 030024China Huabei Cooling Device Co.Ltd. Hebei 065400China

Indium selenide(InSe),as a wide-bandgap semiconductor,has received extensive attention in the flexible electronics field in recent years due to its exceptional plasticity and promising thermoelectric ***,the low carrier concentration severely limits its thermoelectric performance *** this work,we conducted contrasting strategies that can be employed to increase the carrier concentration of InSe,including bandgap narrowing and heterovalent ***,the carrier concentration initially increases as a result of the reduced bandgap upon Te alloying and then slightly decreases due to the weak electronegativity of *** Br doping realizes high carrier concentration by pushing the Fermi level into the conduction bands and activating the multiple *** the other hand,both Te and Br obviously suppress the thermal conductivity due to the point defect *** contrast,Br doping realizes a higher thermoelectric performance with a maximum ZT of~0.13 at 773 K benefiting from the better optimization of carrier *** work elucidates the strategies for enhancing carrier concentration at anion sites and demonstrates the high efficiency of halogen doping in ***,the carrier concentration of InSe is promising to be further optimized,and future work should focus on employing approaches such as cation doping or secondphase compositing.

关键词： Thermoelectric InSe Carrier concentration Bandgap Heterovalent doping

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基于深度迁移学习的复杂机场场景飞机目标检测方法

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光子学报 2024年第4期53卷 221-231页

作者：钟聃李铁虎李诚西北工业大学自动化学院西安710129 西北工业大学材料学院西安710072 中国科学院西安光学精密机械研究所西安710119

提出了一种改进的深度学习模型,旨在解决检测问题。首先基于迁移学习,微调预训练模型,提高了模型在有限的飞机数据集中的特征提取能力。其次,融入调整模块以增加深层特征图的感受野,提升模型的鲁棒性。引入特征金字塔网络,融合不同尺度... 详细信息

提出了一种改进的深度学习模型,旨在解决检测问题。首先基于迁移学习,微调预训练模型,提高了模型在有限的飞机数据集中的特征提取能力。其次,融入调整模块以增加深层特征图的感受野,提升模型的鲁棒性。引入特征金字塔网络,融合不同尺度的特征信息,进一步增强多尺度特征提取能力。最后,优化了检测头,融合轻量化的分类和回归并行分支,平衡了目标检测的准确性和实时性。构建了易于拓展的Aeroplane数据集,并对所提方法进行了实验验证。结果表明,所提模型在单架飞机、相互遮挡的飞机和小飞机的检测中平均精度分别提高了4.9%、4.0%和4.4%。所提方法在不同环境下表现优于其他经典方法,包括各类遮挡和夜间、雾天等复杂场景,具有良好的场景鲁棒性。

关键词：深度学习飞机目标检测迁移学习机场场面特征金字塔网络

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C_(Ar)-Br bond cleavage via cooperative EnT/NHC catalysis: mild access to indolines

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Science China Chemistry 2024年第3期67卷 922-927页

作者： Yi-Xiong Dong Cao-Bo li Ming-Lei Jin zhong-Hua Gao Song Ye Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Molecular Recognition and FunctionCAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

The cooperative visible-light mediated and NHC-catalyzed dearomative arylation-acylation of N-(2-bromobenzoyl)indoles with aldehydes was developed, affording the corresponding highly functionalized polycyclic indolines in moderate to good yields with exclusive diastereoselectivities. Mechanism investigations support the activation of CAr-Br bond via visible-light mediated energy transfer(EnT) and the following single-electron-transfer(SET) with Breslow intermediate under NHC catalysis to give key aryl radical and ketyl radical. This protocol demonstrates the cleavage of CAr-Br bond under mild cooperative EnT/NHC catalysis.

关键词： energy transfer N-heterocyclic carbenes photocatalysis aryl radicals indolines

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Prediction of contact resistance of electrical contact wear using different machine learning algorithms

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Friction 2024年第6期12卷 1250-1271页

作者： Zhen-bing CAI Chun-lin li Lei YOU Xu-dong CHEN li-ping HE zhong-qing CAO Zhi-nan ZHANG Tribology Research Institute Southwest Jiaotong UniversityChengdu 610031China State Key Laboratory of Mechanical System and Vibration Shanghai Jiao Tong UniversityShanghai 200240China

H62 brass material is one of the important materials in the process of electrical energy transmission and signal transmission,and has excellent performance in all *** the wear behavior of electrical contact pairs is particularly complex when they are in service,we evaluated the effects of load,sliding velocity,displacement amplitude,current intensity,and surface roughness on the changes in contact *** learning(ML)algorithms were used to predict the electrical contact performance of different factors after wear to determine the correlation between different factors and contact *** forest(RF),support vector regression(SVR)and BP neural network(BPNN)algorithms were used to establish RF,SVR and BPNN models,respectively,and the experimental data were trained and *** was proved that BP neural network model could better predict the stable mean resistance of H62 brass alloy after *** analysis shows that the load and current have great influence on the predicted electrical contact *** wear behavior of electrical contacts is influenced by factors such as load,sliding speed,displacement amplitude,current intensity,and surface roughness during *** learning algorithms can predict the electrical contact performance after wear caused by these *** results indicate that an increase in load,current,and surface roughness leads to a decrease in stable mean resistance,while an increase in displacement amplitude and frequency results in an increase in stable mean resistance,leading to a decline in electrical contact *** reduce testing time and costs and quickly obtain the electrical contact performance of H62 brass alloy after wear caused by different factors,three algorithms(random forest(RF),support vector regression(SVR),and BP neural network(BPNN))were used to train and test experimental results,resulting in a machine learning model suitable for predicting the stable mean

关键词： electrical contact wear contact resistance machine learning(ML) neural network

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MP-3 microperimeter in early primary open angle glaucoma with a new pattern

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International Journal of Ophthalmology(English edition) 2024年第5期17卷 861-868页

作者： Shuang liang li-Tao Wang Xiao-li liu Jia-liang Duan dan-Yan liu Department of Ophthalmology of the Second Hospital of Hebei Medical University Shijiazhuang 050000Hebei ProvinceChina Department of Ophthalmology Shijiazhuang People’s HospitalShijiazhuang 050000Hebei ProvinceChina

AIM:To investigate macular microperimetry in patients with early primary open angle glaucoma(POAG)using a new custom-made pattern,and analyze the characteristics of macular ***:This case-control study included 38 patients with POAG,who were divided into pre-perimetric glaucoma(18 eyes of 18 patients),early-stage(20 eyes of 20 patients),and control(20 eyes of 20 patients)*** subjects underwent standard 24-2 humphrey visual field *** MP-3 microperimeter with a new custom-made pattern(28 testing points distributed in four quadrants,covering the central 10°of the retina)was used to evaluate macular *** cell complex(GCC)thicknesses were examined using an RS-3000 Advance OCT *** features of structure and function were analysed per ***:The pre-perimetric glaucoma group had significantly lower inferior hemifield macular sensitivity compared to controls(Plier than conventional perimetry,particularly in pre-perimetric glaucoma cases in which it might be undetectable by conventional me

关键词： early primary open angle glaucoma macular sensitivity microperimetry optical coherence tomography ganglion cell complex

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Highly active organocatalyst from a trivalent phosphazenium salt for ring-opening copolymerization of epoxides and cyclic anhydrides enhanced by hydrogen bonding interactions

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Science China Chemistry 2024年第9期67卷 3111-3120页

作者： Chunhuan Jiang Junqi Wang Xiaoyu liu Xiaoxia You Ronglin zhong Chuanli Ren Zhibo li Key Laboratory of Biobased Polymer Materials Shandong Provincial Education DepartmentCollege of Polymer Science and EngineeringQingdao University of Science and TechnologyQingdao 266042China College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042China Laboratory of Theoretical and Computational Chemistry Institute of Theoretical ChemistryCollege of ChemistryJilin UniversityChangchun 130012China

It is highly desirable to develop simple organocatalysts for the controlled ring-opening alternating copolymerization(ROAC)of epoxides and cyclic anhydrides,leading to high molecular weight ***,a phosphazenium salt,namely tri[tris(dimethylamino)phosphoranylidenamino]phosphonium chloride(P_(4)^(+)Cl^(-)),is developed as a catalyst for the ROAC of epoxides and cyclic ***,the combination of P_(4)^(+)Cl^(-)with a protonic initiator,such as 1,4-benzenedimethanol(BDM)exhibited high efficiency in the copolymerization of propylene oxide(PO)and phthalic anhydride(PA).This led to the production of polyester with an exceptional high molecular weight(M_n)of up to 126 k Da,which represented a rare example of poly(PO-alt-PA)with Mnsurpassing 100 k *** that the core P atom is trivalent status and the tris[tris(dimethylamino)]phosphoranyl group will share one proton in the P_(4)^(+)Cl^(-)*** combined with protonic species,the P_(4)^(+)Cl^(-)will not only serve as a proton acceptor but also as a hydrogen bonding donor for the cyclic ***,it was assumed that the P_(4)^(+)plus proton served dual role in mimic of base/urea pair to effectively catalyze ROAC,which was supported by density functional theory(DFT)calculations.

关键词： ring-opening copolymerization organocatalyst epoxides cyclic anhydrides phosphazenium salt

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Low-cost dopant-free fluoranthene-based branched hole transporting materials for efficient and stable n-i-p perovskite solar cells

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Chinese Chemical Letters 2024年第10期35卷 187-193页

作者： Xinyu Yu Fei Wu Xianglang Sun linna Zhu Baoyu Xia zhong'an li Key Laboratory for Material Chemistry of Energy Conversion and Storage Ministry of EducationHubei Key Laboratory of Material Chemistry and Service FailureSchool of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhan 430074China Chongqing Key Laboratory for Advanced Materials and Technologies of Clean Energy Faculty of Materials&EnergySouthwest UniversityChongqing 400715China

It has been widely recognized that hole transporting materials(HTMs)play a key role in the rapid progress of perovskite solar cells(PVSCs).However,common organic HTMs such as spiro-OMe TAD not only suffer from high synthetic costs,but also usually require the additional chemical doping process to improve their hole transport ability,which unfortunately induces the terrible stability ***,it is urgent to develop low-cost dopant-free HTMs for efficient and stable *** this work,we have successfully developed a new class of efficient dopant-free fluoranthene-based HTMs(TPF1–5)with quite low lab synthetic costs by combining donor-acceptor and branched structure *** detailed structure-property study revealed that tuning the twisted arms at different substitution sites would regulate the intermolecular interactions and film-forming ability,thereby significantly affecting the performance of the *** applying these HTMs in conventional PVSCs,the dopant-free TPF1-based devices not only achieved the best efficiency of 21.76%,which is comparable to that of the doped spiro-OMeTAD control devices,but also showed much better operational stability,which maintained over 87%of the initial efficiency under maximum power point tracking after 1038 h.

关键词： Perovskite solar cells Holetransporting materials Dopant-free Fluoranthene Low-cost

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The Influential Mechanisms of Theory of Mind on Prosocial Behavior and the Effect of Mindfulness Intervention

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International Journal of Mental Health Promotion 2024年第9期26卷 679-695页

作者： Sisi li Nailiang zhong Qingke Guo Department of Psychology Guangxi Normal UniversityGuilin541006China School of Teacher Education Hechi UniversityHechi546300China South China Normal University liru Senior High School Xinyi525300China

Background:Theory of Mind(ToM)and empathy are crucial cognitive and emotional capacities that influence social *** their role in promoting prosocial behavior has been established,the potential moderating effect of mindfulness on this relationship remains *** these complex interactions is vital for developing effective interventions to foster prosocial behavior among college *** study examines the influence of ToM on college students’prosocial behavior and explores the moderating role of mindfulness in this ***:A mixed-methods approach combining questionnaires and experimental design was *** 1:A survey of 759 college students(mean age 22.03 years;477 females)was conducted using the ToM Scale,Interpersonal Reactivity Index,Prosocial Behavior Tendency Scale,and Mindfulness Awareness *** were analyzed using correlation and moderated mediation *** 2:An 8-week mindfulness attention training program was implemented for the intervention group and compared with a control *** training served as a moderating variable to validate Model 59 from Study ***:*** 1 found:(a)ToM was significantly positively correlated with prosocial behavior(r=0.31,plidity of the moderated mediation model 59 from Study 1 w

关键词： Prosocial behavior Theory of Mind trait mindfulness empathy mindfulness intervention

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