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Hexagonal boron nitride based slippery liquid infused porous surface with anti-corrosion, anti-contaminant and anti-icing properties for protecting magnesium alloy

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Chinese Chemical Letters 2024年第4期35卷 532-538页

作者： Wenhao Yan Shuaiya xue xuerui Zhao Wei Zhang Jian li Key Laboratory of Eco-Functional Polymer Materials of the Ministry of Education College of Chemistry and Chemical EngineeringNorthwest Normal UniversityLanzhou 730070China

In an era where the concept of green development is deeply rooted, magnesium(Mg) alloy as a light metal has a long-term development prospect in the process of energy saving, emission reduction and environmental improvement. However, anti-corrosion performance of Mg alloy is poor due to the high chemical activity and low equilibrium potential, which limits the development of Mg alloy ***, three-dimensional mesopore hollow polypyrrole spheres(MHPS) were prepared, and the MHPS was inserted into the middle of the stacked hexagon boron nitride(h-BN) lamellae, which allowed the hBN to be separated forming a further composite with abundant pore structure. Subsequently, the MHPS/hBN-OH composite was uniformly sprayed on the Mg alloy surface via simple spraying method to form the superhydrophobic surface(SHS). Finally, the slippery liquid infused porous surface(SliPS) was successfully fabricated by applying drops of silicone lubricant on the superhydrophobic coating surface. After a series of characterization and testing, the results showed that the stacking of h-BN lamellae was significantly reduced after h-BN was successfully embedded by MHPS. In addition, the fabricated SliPS have excellent self-cleaning, mechanical stability, anti-icing and anti-corrosion properties. Therefore, the method of embedding polymer microspheres not only offers a new strategy for h-BN exfoliation, but also the successful prepared SliPS largely retards the corrosion of Mg alloy while providing new ideas for the development of SliPS.

关键词： Anti-corrosion Mg alloy Hexagon boron nitride Polypyrrole SliPS

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Acid-rock reaction kinetics in a two-scale model based on reaction order correction

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Petroleum Science 2024年第3期21卷 2089-2101页

作者： xue-Song li Ning Qi Ze-Hui Zhang lian liu Xia-Qing li Xu-Hang Su School of Petroleum Engineering China University of Petroleum(East China)Qingdao266580ShandongChina Key Lab of Unconventional Oil&Gas Development Ministry of EducationChina University of Petroleum(East China)Qingdao26650ShandongChina SINOPEC Northwest Oilfield Branch Company Urumqi830011XinjiangChina Petroleum Engineering technology Research Institute SINOPEC Shengli Oilfield CompanyDongying257000ShandongChina

The reaction order plays a crucial role in evaluating the response rate of ***,the conventional two-scale model typically assumes that the reaction order is constant as one,which can lead to significant deviations from *** address this issue,this study proposes a novel multi-order dynamic model for acid-rock reaction by combining rotating disk experimental data with theoretical *** numerical simulations,this model allows for the investigation of the impact of acidification conditions on different orders of reaction,thereby providing valuable insights for on-site *** analysis reveals that higher response orders require higher optimal acid liquid flow rates,and lower optimal H+diffusion coefficients,and demonstrate no significant correlation with acid ***,it is recommended to increase the displacement and use high-viscosity acid for reservoirs with high calcite content,while reducing the displacement and using low-viscosity acid for reservoirs with high dolomite content.

关键词： Reaction order Two-scale model Wormhole propagation Carbonate rocks Numerical simulation

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Progress of semitransparent emerging photovoltaics for building integrated applications

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Green Energy & Environment 2024年第6期9卷 992-1015页

作者： Zhisheng Zhou Zhangyu Yuan Zhipeng Yin Qifan xue Ning li Fei Huang State Key Laboratory of Luminescent Materials and Devices School of Materials Science and EngineeringSouth China University of TechnologyGuangzhou510640China Pazhou Lab Guangzhou510320China

With the rapid development of emerging photovoltaics technology in recent years,the application of building-integrated photovoltaics(BIPVs)has attracted the research interest of photovoltaic *** meet the practical application requirements of BIPVs,in addition to the evaluation indicator of power conversion efficiency(PCE),other key performance indicators such as heat-insulating ability,average visible light transmittance(AVT),color properties,and integrability are equally *** traditional Si-based photovoltaic technology is typically limited by its opaque properties for application scenarios where transparency is *** emerging PV technologies,such as organic and perovskite photovoltaics are promising candidates for BIPV applications,owing to their advantages such as high PCE,high AVT,and tunable *** present,the PCE of semitransparent perovskite solar cells(ST-PSCs)has attained 14%with AVT of 22–25%;for semitransparent organic solar cells(ST-OSCs),the PCE reached 13%with AVT of almost 40%.In this review article,we summarize recent advances in material selection,optical engineering,and device architecture design for high-performance semitransparent emerging PV devices,and discuss the application of optical modeling,as well as the challenges of commercializing these semitransparent solar cells for building-integrated applications.

关键词： Building integrated photovoltaics Emerging photovoltaics Semitransparent solar cells Perovskite solar cells Organic solar cells

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Analysis of Tidal Current Energy Potential in the Major Channels of the Bohai Strait Based on Delft3D

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Journal of Ocean university of China 2024年第4期23卷 859-870页

作者： MA Pengcheng SHI Hongyuan xue Huaiyuan li Pingping SUN Yongkang School of Hydraulic Engineering Ludong University of ChinaYantai 264025China Institute of Coastal Research Ludong University of ChinaYantai 264025China Yantai Kekan Marine technology Co. Ltd.Yantai 264025China

The utilization and development of tidal current energy can help alleviate the current energy shortage,improve the global ecological environment,and maintain sustainable *** this study,numerical simulation is carried out on a rectangular grid using *** tidal current energy potential of the major channels in the Bohai Strait is further simulated and estimated by comparing the simulated and measured *** show that the flow module in Delft3D has good modeling ability for the assessment of tidal current energy *** average flow velocity,maximum flow velocity,and energy flow density are *** Laotieshan Channel,located in the northern part of the Bohai Strait,shows a large tidal current energy *** maximum flow velocity of this channel can reach 2 m s-1,and the maximum energy flow density can exceed 500 W *** tidal current energy in the Laotieshan Channel is more than 10 times that in other ***,this study advocates for the continued exploration and exploitation of the tidal current energy resources in the Laotieshan Channel.

关键词： Delft3D Bohai Strait tidal current energy numerical simulation power density

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Effect of Bimodal Quasicrystal Phase on the Dynamic Recrystallization of Mg–Zn–Gd Alloy during High-Pressure Torsion

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Acta Metallurgica Sinica(English Letters) 2024年第7期37卷 1128-1134页

作者： Ping li Shuangwu Xia Junfu Dong liangwei Dai Zhicheng Luo Kemin xue School of Material Science and Engineering Hefei University of TechnologyHefei230009China

The Mg–Zn–Gd alloy with quasicrystal icosahedral phase was processed by high-pressure torsion (HPT). The effect of bimodal I-phase on the dynamic recrystallization was analyzed by transmission electron microscopy. The results showed that the block I-phase can stimulate obvious particle-stimulated nucleation and dynamic recrystallization (DRX) grains were preferentially formed after HPT for 5 turns, while the granular I-phase only promoted the generation of sub-grains. The orientation relationship was determined as twofold//[1210] and fivefold//(0002)_(Mg). Moreover, after HPT for 9 turns, the DRX grains induced by block I-phase appeared to grow up and coarsened. Compared with block I-phase, the grains induced by granular I-phase presented much smaller size and distributed more homogeneous due to the strong pinning effect.

关键词： High-pressure torsion(HPT)-Quasicrystal phase Dynamic recrystallization Particle-stimulated nucleation Orientation relationship

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Facile molybdenum and aluminum recovery from spent hydrogenation catalyst

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Chinese Journal of Chemical Engineering 2024年第5期69卷 72-78页

作者： Zhenhui Lv Jianan li Dong xue Tao Yang Gang Wang Chong Peng State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyDalian 116024China Dalian Research Institute of Petroleum and Petrochemicals SINOPECDalian 116041China

Industrial catalyst waste has emerged as a hazardous pollutant that requires safe and proper disposal after the unloading *** a valuable and sustainable strategy for its treatment is a significant challenge compared to traditional *** this study,we present a facile method for the recovery of molybdenum and aluminum contents from spent Mo-Ni/Al_(2)O_(3) hydrogenation catalysts through crystallization separation and ***,the recovered molybdenum and aluminum are utilized as active metals and carriers for the preparation of new *** properties were thoroughly analyzed and investigated using various characterization *** hydrogenation activity of these newly prepared catalysts was evaluated on a fixed-bed small-scale device and compared with a reference catalyst synthesized from commercial raw ***,the hydrogenation activity of the catalysts was further assessed by using the entire distillate oil of coal liquefaction as the raw oil,specifically focusing on denitrogenation and aromatic *** work not only offers an effective solution for recycling catalysts but also promotes sustainable development.

关键词： Waste treatment Alumina Hydrogenation Catalyst Crystallization Precipitation

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Experimental investigation on coal pore-fracture variation and fractal characteristics synergistically affected by solvents for improving clean gas extraction

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International Journal of Mining Science and technology 2024年第3期34卷 413-425页

作者： Feilin Han Sheng xue Chunshan Zheng Zhongwei Chen Guofu li Bingyou Jiang Key Laboratory of Safe and Effective Coal Mining of Ministry of Education Anhui University of Science and TechnologyHuainan 232001China School of Safety Science and Engineering Anhui University of Science and TechnologyHuainan 232001China School of Mechanical and Mining Engineering University of QueenslandQLD 4072Australia State Key Laboratory of Coal and Coalbed Methane Co-Mining Jincheng 048012China

Chemical solvents instead of pure water being as hydraulic fracturing fluid could effectively increase permeability and improve clean methane extraction ***,pore-fracture variation features of lean coal synergistically affected by solvents have not been fully *** testing,nuclear magnetic resonance analysis,liquid phase mass spectrometry was adopted to comprehensively analyze pore-fracture change characteristics of lean coal treated by combined solvent(NMP and CS_(2)).Meanwhile,quantitative characterization of above changing properties was conducted using geometric fractal *** model between permeability,fractal dimension and porosity were *** indicate that the end face fractures of coal are well developed after CS2and combined solvent treatments,of which,end face box-counting fractal dimensions range from 1.1227 to *** decreases in ultrasonic longitudinal wave velocity of coal affected by NMP,CS_(2)and combined solvent are 2.700%,20.521%,22.454%,*** treatments could lead to increasing amount of both mesopores and *** ratio of fractal dimension Dsis 0.259%–2.159%,while permeability increases ratio of NMR ranges from 0.1904 to ***,combined solvent could dissolve coal polar and non-polar small molecules and expand flow *** could provide reference for solvent selection and parameter optimization of permeability-enhancement technology.

关键词： Clean gas extraction Chemical solvent Experimental investigation Fractal characteristics Pore fracture

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Improving strength-ductility synchronously of Electron beam welded Ti600/Ti2AlNb joint through isothermal forging

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Progress in Natural Science:Materials International 2024年第3期34卷 532-539页

作者： Yongqiang Zhang Xiangyi xue Guoming Zheng Jingli Zhang Huiming li Shewei Xin State Key Laboratory of Solidification Processing Northwestern Polytechnical University Xi'an Qin Ti Intelligent Manufacturing Technologies Co.Ltd. Northwest Institute for Nonferrous Metal Research Xi'an university of Science and technology Avic Xi'an Aircraft Industry Group Company Ltd.

Different alloys can be flexibly combined to meet the performance needs of different parts of the compressor disc by welding process. However, achieving a good combination of dissimilar alloys with different mechanical properties has always been a research difficulty. In this work, a Ti600/Ti2AlNb joint was fabricated through electron beam welding and an isothermal forging was used to optimized its microstructure and mechanical performance. The isothermal forging process increases the ultimate tensile strength（UST） and yield strength（YS）of the Ti600/Ti2AlNb joint by ～18 %, while ～2.5 times the ductility. It is indicated that before forging, the Ti600/Ti2AlNb joint exhibits a much lower strength than that of Ti600 matrix, whereas the opposite is true after isothermal forging. The isothermal forging broken the coarse columnar grains of Ti600/Ti2AlNb joint and render to an equiaxed B2 structure in which the acicular α2and O phase are precipitated, resulting a synchronous enhancement of strength and ductility. This work may pave an effective routine for improving the comprehensive mechanical properties of dissimilar metal welding joint.

关键词： Electron beam welding Isothermal forging Mechanical performance Ti600/Ti2AlNb joint

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Magnetic behaviors and magnetocaloric effects in rare earth high-entropy amorphous/nanocrystalline alloys

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Journal of Rare Earths 2024年第1期42卷 129-136,I0005页

作者： lin xue liliang Shao Baosen Zhang Zongzhen li Jiangbo Cheng Baolong Shen College of Mechanics and Materials Hohai UniversityNanjing211106China School of Materials Science and Engineering Jiangsu Key Laboratory of Advanced Metallic MaterialsSoutheast UniversityNanjing211189China School of Materials Science and Engineering Nanjing Institute of TechnologyNanjing211167China Jiangsu JITRI Advanced Energy Materials Research Institute Co. Ltd.Changzhou213000China

Rare earth high-entropy alloys(RE-HEAs)exhibit great potential to be applied as refrigerants due to their good comprehensive magnetocaloric *** this work,octary GdTbDyHoErTmCoAl and GdTbDyHoErTmCoNi RE-HEAs with amorphous/nanocrystalline structure exhibiting comparable magnetocaloric effect were *** RE-HEAs show a second-order magnetic phase transition in the temperature range of hydrogen *** to the complex magnetic interactions,a spin glasslike behavior at low temperatures is observed in the RE-HEAs.A superior magnetocaloric effect is obtained in the nanocrystalline GdTbDyHoErTmCoNi high-entropy alloy that is multiphase attributed to a stronger magnetic exchange interaction when compared with the other that exhibits single amorphous *** heterogeneous microstructure,homogeneous chemical distributions are observed in the partially crystallized high-entropy *** addition,the magnetocaloric effect and magnetic transition behavior of rare earth medium-and high-entropy alloys,including the RE-HEAs in this study,are summarized and *** results in this work provide a helpful guide for the design of RE-HEAs for hydrogen liquefaction applications with excellent magnetocaloric effects.

关键词： Rare earths High-entropy alloy Metallic glass Magnetocaloric effect

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Accelerated aging and frailty in cardiovascular diseases

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Journal of Geriatric Cardiology 2024年第8期21卷 828-830页

作者： xue-Hua CHENG Tao WU li HAN Department of Traditional Chinese Medicine Geriatrics Huadong Hospital Affiliated to Fudan UniversityShanghaiChina

Aging is the greatest risk factor for cardiovascular disease(CVD),which is the most common cause of death in European countries.[1]It is estimated that during the period from 2020 to 2022,there were 9.0%more excess deaths from CVD than expected.[2]By 2030,approximately 20%of the population will be aged 65 years and older,and CVD will account for 40%of deaths in this age group,[3]imposing a significant burden on the healthcare system and society as a *** is related to frailty,which represents the dynamic progression of physical and physiological decline in older *** limits an individual’s ability to recover from acute stressors and serves as a predictor of clinical adverse *** the uncertainties in screening,assessing,and managing frailty in clinical practice,emphasizing the connections between frailty,aging,and CVD will provide new insights for the prediction,prevention and management of CVD in the aging population.

关键词： aging prevention prediction

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