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Investigating missing sources of glyoxal over China using a regional air quality model (RAmS-CmAQ)

Journal of Environmental Sciences 2018年第9期30卷 108-118页

作者： Jialin Li meigen Zhang Guiqian Tang Fangkun Wu leonardo m.a. alvarado mihalis Vrekoussis Andreas Richter John P. Burrows State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPQ) Institute of Atmospheric Physics (IAP)Chinese Academy of Sciences (CAS) Beijing 100029 China University of Chinese Academy of Sciences Beijing 100049 China Center for Excellence in Urban Atmospheric Environment Institute of Urban Environment Chinese Academy of Sciences Xiamen 361021 China Institute of Environmental Physics and Remote Sensing IUP University of Bremen D-28203 Bremen Germany Center of marine Environmental Sciences MARUM University of Bremen D-28203 Bremen Germany Energy Environment and Water Research Center the Cyprus Institute CY2121 Nicosia Cyprus

Currently, modeling studies tend to significantly underestimate observed space-based glyoxal （CHOCHO） vertical column densities （VCDs）, implying the existence of missing sources of giyoxal. Several recent studies suggest that the emissions of aromatic compounds and molar yields of glyoxal in the chemical mechanisms may both be underestimated, which can affect the simulated glyoxal concentrations. In this study, the influences of these two factors on glyoxal amounts over China were investigated using the RAmS-CmAQ modeling system for January and July 2014. Four sensitivity simulations were performed, and the results were com.a.ed to satellite observations. These results demonstrated significant im.a.ts on glyoxal concentrations from these two factors. In case 1, where the emissions of aromatic compounds were increased three-fold, improvements to glyoxal VCDs were seen in high anthropogenic emissions regions. In case 2, where molar yields of glyoxal from isoprene were increased five-fold, the resulted concentrations in July were B-B-fold higher, achieving closer agreement between the modeled and m.a.ured glyoxal VCDs. The combined changes from both cases 1 and 2 were applied in case B, and the model succeeded in further reducing the underestimations of glyoxal VCDs. However, the results over most of the regions with pronounced anthropogenic emissions were still underestimated. So the molar yields of giyoxal from.a.thropogenic precursors were considered in case 4. With these additional mole yield changes （a two-fold increase）, the improved concentrations agreed better with the m.a.urements in regions of the lower reaches of the Yangtze River and Yellow River in January but not in July.

关键词： Glyoxal Volatile organic compounds molar yields RAmS-CmAQ China

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Characterization of Arroyo Verde Epithermal Deposit:Paragenesis,mineral Geochemistry,Geochronology and Fluid Inclusions in Lower Chon Aike Volcanism.a.gentina

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Journal of Earth Science 2024年第1期35卷 62-84页

作者： Cecilia Pavón Pivetta leonardo Benedini Paulo marcos ma.Agustina Cócola mercedes Virginia Barros Daniel Gregori leonardo Strazzere Anderson Costa dos Santos mauro C.Geraldes Instituto Geologico del Sur(INGEOSUR) Universidad Nacional del Sur(UNS)-Consejo Nacional de Investigaciones Cientificas y Tecnicas(CONICET)Bahia Blanca 8000Argentina Dpto.de Geologia Universidad Nacional del Sur(UNS)Bahia Blanca 8000Argentina Universidad Nacional de Rio Negro Instituto de Investigacion en Paleobiologia y GeologiaGeneral Roca 8332Argentina Universidade do Estado do Rio de Janeiro Faculdade de GeologiaDepartamento de Mineralogia e Petrologia igneaRiodeJaneiro20559-900Brazil Geobiotec Departamento de GeocienciasUniversidade de AveiroAveiro 3800-002Portuga

Arroyo Verde epithermal deposit,in the North Patagonia region of Argentina,is located within the Lower Chon Aike volcanism.a.d is developed between 192.6±2.5 ma(mineralization host rock)and 189.5±2.6 ma(overlying lava).marifil volcanic complex is the host rock for these veins,veinlets and breccias.This particular small deposit has developed low to intermediate sulphidation characteristics,with gangue mineral textures associated with several ore minerals.Electron probe microanalysis determines electrum,silver minerals such as acanthite,and tetrahedrite,related Ag-Cu minerals like jalpaite,mckinstryite,stromeyerite,and base metals like chalcopyrite,sphalerite,galena and pyrite.Fluid inclusions in quartz of two out of five events indicate that these Low Jurassic veins were formed due to subtle boiling and dilution mechanisms and by low-salinity(3.4 wt.%to 6.7 wt.%NaCl Eq)magmatic-hydrothermal fluid at 225 to 310℃.The fluid inclusion m.a.urements that indicate boiling(Event 3)were plotted,and based on this data,we interpret that the Arroyo Verde deposit has been eroded between 550 and 700 m.This particular character has not been previously recorded for other sectors of the eastern north Patagonian region.

关键词： epithermal deposit Ag minerals mineral geochemistry fluid inclusions Chon Aike geochronology

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Pulsed electromagnetic field stimulation enhances neurite outgrowth in neural cells and modulates inflam.a.ion in macrophages

Engineered Regeneration

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Engineered Regeneration 2024年第1期5卷 80-91页

作者： Francesco Fontana Andrea Cafarelli Francesco Iacoponi Soria Gasparini Tiziano Pratellesi Abigail NKoppes leonardo Ricotti The BioRobotics Institute Scuola Superiore Sant’Anna56127 PisaItaly Department of Excellence in Robotics&AI Scuola Superiore Sant’Anna56127 PisaItaly BAC Technology s.r.l. 50063 FlorenceItaly Department of Chemical Engineering Northeastern UniversityBostonMA 02115USA Department of Bioengineering Northeastern UniversityBostonMA 02115USA Department of Biology Northeastern UniversityBostonMA 02115USA

Nerve regeneration following traumas remains an unmet challenge.The application of pulsed electromagnetic field(PEmF)stimulation has gained traction for a minimally invasive regeneration of nerves.However,a sys-tematic exploration of different PEmF parameters influencing neuron function at a cellular level is not available.In this study,we exposed neuroblastoma F11 cells to PEmF to trigger beneficial effects on neurite outgrowth.Different carrier frequencies,pulse repetition frequencies,and duty cycles were screened with a custom.a. hoc setup to find the most influential parameters values.A carrier frequency of 13.5 mHz,a pulse repetition frequency of 20 Hz,and a duty cycle of 10%allowed maximal neurite outgrowth,with unaltered viability with respect to non-stimulated controls.Furthermore,in a longer-term.a.alysis,such optimal conditions were also able to in-crease the gene expression of neuronal expression markers NeuN and Tuj-1 and transcription factor Ngn1.Finally,the same optimal stimulation conditions were also applied to THP-1 macrophages,and both pro-inflam.a.ory(TNF-𝛼,IL-1𝛽,IL-6,IL-8)and anti-inflam.a.ory cytokines(IL-10,CD206)were analyzed.The optimal PEmF stimulation parameters did not induce differentiation towards an m1 macrophage phenotype,decreased IL-1𝛽and IL-8 gene expression,decreased TNF-𝛼and IL-8 cytokine release in m1-differentiated cells,increased IL-10 and CD206 gene expression,as well as IL-10 cytokine release in m0 cells.The specific PEmF stimulation regime,which is optimal in vitro,might have a high potential for a future in vivo translation targeting neural regeneration and anti-inflam.a.ory action for treating peripheral nerve injuries.

关键词： Nerve regeneration Biophysical stimulation Pulsed electromagnetic fields(PEmF) Neurite outgrowth Anti-inflam.a.ory Peripheral nerve injuries

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Dendritic spine degeneration:a primary mechanism in the aging process

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Neural Regeneration Research 2025年第6期20卷 1696-1698页

作者： Gonzalo Flores leonardo Aguilar-Hernández Fernado García-Dolores Humberto Nicolini Andrea Judith Vázquez-Hernández Hiram Tendilla-Beltrán Instituto de Fisiología Benemérita Universidad Autónoma de Puebla(BUAP)PueblaMexico Instituto de Ciencias Forenses(INCIFO) Tribunal Superior de Justicia de la Ciudad de México(TSJCDMX).Mexico CityMexico Instituto Nacional de medicina Genómica(INmEGEN) Mexico CityMexico

Recent reports suggest that aging is not solely a physiological process in living beings;instead, it should be considered a pathological process or disease(Amorim et al., 2022). Consequently, this process involves a wide range of factors, spanning from genetic to environmental factors, and even includes the gut microbiome(Gm)(mayer et al., 2022). All these processes coincide at some point in the inflam.a.ory process, oxidative stress, and apoptosis, at different degrees in various organs and systems that constitute a living organism(mayer et al., 2022;AguilarHernández et al., 2023).

关键词： aging process stress

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Solar-driven CO_(2) conversion to methane and methanol using different nanostructured Cu_(2)O-based catalysts modified with Au nanoparticles

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Journal of Energy Chemistry 2024年第4期91卷 287-298页

作者： João Angelo Lima Perini Lilian D.moura Torquato Juliana Fde Brito Gustavo A.Andolpho mateus A.Gonçalves leonardo D.De Angelis Lucas D.Germano Susana I.Córdoba de Torresi Teodorico C.Ramalho maria V.Boldrin Zanoni São Paulo State University(UNESP) Institute of ChemistryRua Prof.Francisco Degni55AraraquaraSP 14800-060Brazil National Institute of Alternative Technologies for Detection Toxicological Evaluation and Removal of Micropollutants and Radioactive Substances(INCT-DATREM)São Paulo State University(UNESP)Institute of ChemistryRua Prof.Francisco Degni55AraraquaraSP 14800-060Brazil Laboratory of molecular modelling Department of ChemistryNatural Sciences InstituteFederal University of LavrasLavrasMG 37200-900Brazil Department of Chemistry Faculty of ScienceUniversity of Hradec KrálovéHradec Králové50003Czech Republic Instituto de Química Universidade de São PauloAv.Prof.Lineu Prestes 74805508-080São PauloSPBrazil

This work describes the use of TiO_(2)nanotubes-based electrodes(TNT)modified with Cu_(2)O nanostructures and gold nanoparticles for the photoelectroreduction of CO_(2)to produce value-added compounds.A thin layer of polydopamine was used as both an adherent agent and an electron transfer mediator,due to itsπ-conjugated electron system.The highest production yield was achieved using a TNT@PDA/Nc/Au40%electrode,with Faradaic efficiencies of 47.4%(110.5μm cm^(-2))and 27.8%(50.4μm cm^(-2))for methanol and methane,respectively.The performance of the photoelectrodes was shown to be Cu_(2)O facet-dependent,with cubic structures leading to greater conversion of CO_(2)to methanol(43%)and methane(27%),com.a.ed to the octahedral morphology,while a higher percentage of metallic gold on the nanostructured Cu_(2)O surface was mainly important for CH4production.Density functional theory(DFT)calculations supported these findings,attributing the superior photoelectrocatalytic performance of the TNT@PDA/Nc/Au40%electrode for CH4generation to the formation of an OCH3intermediate bonded to Au atoms.Studies using isotope-labeling and analysis by gas chromatograph-mass(GC-mS)demonstrated that13CO_(2)was the source for photoelectrocatalytic generation of13CH3OH and13CH313CH2OH.

关键词： Cu_(2)O nanocubes Photoelectrocatalysis Polydopamine CO_(2) photoelectroreduction DFT calculations

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Academic Stress Assessment Using Virtual Reality as an Educational Tool in Spine Surgery

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Open Journal of modern Neurosurgery 2024年第2期14卷 114-123页

作者： Diana Chávez Lizárraga Jesús Alberto Pérez Contreras Fernando alvarado Gómez Evelyn Quintero medina Em.a.uel Cantú Chávez Iván Ulises Sámano López Ana Sofía Peña Blesa Department of Neurosurgery ángeles Pedregal Ciudad de México México Department of Traumatology and Orthopedics Hospital Santa Fe Bogotá Colombia

Introduction: The evaluation of academic stress in medical students and residents is a topic of significant interest, given the considerable challenges they face during their learning process with traditional teaching methods. The use of technologies like virtual reality presents an opportunity to enhance their skills through simulations and training. The main objective of this study is to qualitatively assess the stress levels experienced by medical students and residents by integrating virtual reality into their current learning methods, aiming to improve their ability to manage stressors in their practice. material and methods: A questionnaire was conducted with 12 medical students and 12 Traumatology and orthopedics residents. The purpose of the questionnaire was to evaluate the levels of academic stress using the SISCO inventory. The stress levels were calculated by transforming average values into percentages, and the following criteria were assigned: 0 to 33% for mild Stress, 34 to 66% for moderate Stress, and 67 to 100% for Deep Stress. Then, a virtual reality class focused on spine surgery was provided. Both medical students and residents were trained using the Non Nocere SharpSurgeon software platform.a.d Oculus Quest 2 virtual reality glasses. At the end of the session, a second questionnaire related to the practice with virtual reality was conducted with the same evaluation criteria and a com.a.ative analysis was carried out. Results: 12 undergraduate students from Hospital Angeles mexico, CDmX and 12 traumatology and orthopedics residents at Hospital Santa Fe, Bogota were evaluated. The students in CDmX reported an average qualitative stress of 28.50% during habitual practices, which decreased to an average of 14.67% after virtual reality practice. Residents in Bogotá experienced an average qualitative stress of 30.50% with their current learning methods but this reduced to an average of 13.92% after using virtual reality. These findings indicate that the use of virtual reality has a positive im.a.t

关键词： Virtual Reality Academic Stress Learning Strategies Spine Surgery Training

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Evaluation of Clinical Characteristics and Plasma Cortisol Concentrations in Individuals with COVID-19 and Post-COVID Syndrome

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Case Reports in Clinical medicine 2024年第1期13卷 12-24页

作者： David Alejandro García López Stephania Ramos Hernández Yamile López-Hernández maría Argelia López Luna Elena Donaji Ramírez alvarado Rosa maría Ramírez Santoyo Sergio Hugo Sánchez Rodríguez Laboratorio de Biología Celular y Neurobiología Universidad Autónoma de Zacatecas México Zacatecas Unidad Académica de Ciencias Químicas Universidad Autónoma de Zacatecas México Zacatecas Laboratorio de metabolómica y Proteómica Universidad Autónoma de Zacatecas México Zacatecas Laboratorio de Bacterias y Hongos filamentosos Universidad Autónoma de Zacatecas México Zacatecas

COVID-19 generates systematic alterations in humans both in active stages of infection and over time, called post-COVID syndrome. Cortisol is a hormone that is overexpressed in inflam.a.ion and cellular stress processes. Its main function is to return to physiological homeostasis, so its evaluation together with other clinical parameters can allow us to determine the degree of systemic affectation by COVID-19. Objective: To evaluate changes in clinical parameters and plasma cortisol concentrations in patients with active COVID-19 and post-COVID syndrome. material and methods: Healthy patients, in stages of mild infection, critical and with post-COVID syndrome, were recruited, obtaining, through clinical diagnoses and interviews, their main clinical characteristics, in addition to plasma, in which cortisol concentrations were determined using competitive ELISA. Results: The critical stage group had higher frequencies of comorbidities, clinical symptoms, as well as more altered laboratory parameters com.a.ed to the other subgroups. In the post-COVID syndrome group after the initial infection, most laboratory parameters recovered, however, several clinical symptoms remained latent over time. The determination of cortisol showed an increase in its concentration, being higher in patients in critical stage and with post-COVID syndrome. Conclusion: COVID-19 disease generates clinical alterations that trigger an increase in plasma cortisol. These alterations increase as the stages of infection become more severe and some of them remain altered in patients with post-COVID syndrome.

关键词： COVID-19 Cortisol Post-COVID Syndrome

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Direct observation of the CO_(2) formation and C–H consumption of carbon electrode in an aqueous neutral electrolyte supercapacitor by in-situ FTIR and Raman

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Journal of Energy Chemistry 2022年第8期31卷 488-496,I0013页

作者： murilo m.a.aral Victor Y.Yukuhiro Rafael Vicentini Alfredo C.Peterlevitz leonardo m.Da Silva Pablo Fernandez Hudson Zanin Advanced Energy Storage Division State University of Campinas13083-852Av.Albert Einsten 400CampinasSPBrazil Chemistry Institute State University of Campinas13083-970Josue de Castro StreetCampinasSPBrazil Department of Chemistry Laboratory of Fundamental and Applied ElectrochemistryFederal University of Jequitinhonha and Mucuri’s ValleyRodovia MGT 367km 5835000Alto da Jacuba39100-000DiamantinaMGBrazil Center for Innovation on New Energies University of Campinas13083-841 CampinasSão PauloBrazil

Electrical double-layer capacitors(EDLCs)consist of energy storage devices that present high-power and moderate energy density.The electrolyte and electrode physicochemical properties are crucial for improving their overall energy storage capabilities.Therefore,the stability of the EDLCs’materials is the primary focus of this study.Since energy storage depends on the specific capacitance,and also on the square of the maximum capacitive cell voltage(UmCV).Thus,electrodes with high specific surface area(SSA)and electrolytes with excellent electrochemical stability are commonly reported in the literature.Aqueous electrolytes are safer and green devices com.a.ed to other organic-based solutions.On the other hand,their UmCVis reduced com.a.ed to other electrolytes(e.g.,organic-based and ionic liquids).In this sense,spanning the UmCVfor aqueous-based electrolytes is a’hot topic’research.Unfortunately,the lack of protocols to establish reliable UmCVvalues has culminated in the publishing of several conflicting results.Herein,we confirm that multiwalled carbon nanotubes(mWCNTs)housed in cells degrade and produce CO_(2) under abusive polarisation conditions.It is probed by employing electrochemical techniques,in-situ FTIR and in-situ Raman spectroscopies.From these considerations,the current study uses spectro-electrochemical techniques to support the correct determination of the electrode and electrolyte stability conditions as a function of the operating electrochemical parameters.

关键词： Electrode and electrolyte stabilities In-situ FTIR CO_(2)formation Carbon degradation Supercapacitor Aqueous electrolytes Carbon nanotubes

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First record of Odontaster penicillatus populations(Philippi,1870)(Echinodermata:Asteroidea)in the Atacama and Antofagasta regions,Chile(Southeast Pacific)

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Acta Oceanologica Sinica 2022年第12期41卷 152-155页

作者： leonardo Campos Fernando Berrios Brenda BHermosillo-Núñez marco Ortiz Departamento de Ciencias Acuáticas y Ambientales Universidad de Antofagasta ChileAntofagasta 1240000Chile Centro de Investigaciones Costeras Universidad de Atacama(CIC-UDA) Avenida Copayapu 485Copiapó1530000Chile Laboratorio de modelamiento de Sistemas Ecológicos Complejos(LAmSEC) Instituto AntofagastaUniversidad de AntofagastaAntofagasta 1240000Chile Instituto de Ciencias Naturales AvH Facultad de Ciencias del Mar y Recursos BiológicosUniversidad de AntofagastaAntofagasta 1240000Chile Centro de Investigación y Estudios Avanzados del maule Vicerrectoría de Investigación y PosgradoUniversidad Católica Del MauleCampus San MiguelTalca 3480094Chile

We report for the first time the presence of local populations of the starfish Odontaster penicillatus in the regions of Atacama and Antofagasta,Chile.This finding indicates an extension of the distribution limit of 500 km with respect to the last observation made in 2007 in Isla Grande de Atacama.A total of 121 specimens of O.penicillatus were recorded at depths of between 8 m.a.d 24 m.They were associated with rocky substrate and with different species of barnacles,sponges and bryozoans.The presence of O.penicillatus expands the knowledge of the benthic biodiversity of the region,and the development of studies on its ecological importance will be promoted.

关键词： Odontaster penicillatus new record Antofagasta Atacama South Pacific Ocean

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Rapid prototyping of a polymer mEmS dropletdispenser by laser-assisted 3D printing

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microsystems & Nanoengineering 2023年第4期9卷 211-221页

作者： Rémi Courson Oleksii Bratash Ali maziz CloéDesmet Ricardo alvarado meza Loïc Leroy Elodie Engel Arnaud Buhot Laurent malaquin Thierry Leïchlé LAAS-CNRS Universitéde ToulouseCNRS31400 ToulouseFrance UniversitéGrenoble Alpes CNRSCEAIRIGSyMMES38000 GrenobleFrance Georgia Tech−CNRS International Research Laboratory AtlantaGA 30332USA

In this work, we introduce a polymer version of a previously developed silicon mEmS drop deposition tool for surfacefunctionalization that consists of a microcantilever integrating an open fluidic channel and a reservoir. The device isfabricated by laser stereolithography, which offers the advantages of low-cost and fast prototyping. Additionally,thanks to the ability to process multiple materials, a magnetic base is incorporated into the cantilever for convenienthandling and attachment to the holder of a robotized stage used for spotting. Droplets with diameters ranging from∼50 μm to ∼300 μm.a.e printed upon direct contact of the cantilever tip with the surface to pattern. Liquid loading isachieved by fully immersing the cantilever into a reservoir drop, where a single load results in the deposition of morethan 200 droplets. The influences of the size and shape of the cantilever tip and the reservoir on the printing outcom.a.e studied. As a proof-of-concept of the biofunctionalization capability of this 3D printed droplet dispenser,microarrays of oligonucleotides and antibodies displaying high specificity and no cross-contamination are fabricated,and droplets are deposited at the tip of an optical fiber bundle.

关键词： cantilever reservoir printing

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