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Enhanced thermoelectric and mechanical properties of Bi_(0.5)Sb_(1.5)Te_(3) alloy with dispersed yttrium oxide ceramic nanoparticles

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Rare Metals 2024年第4期43卷 1758-1768页

作者： Cun-Cheng Li Ming-wei Zhang Ji-Wu Xin lei wei Wen-Yu Zhao School of Materials Science and Engineering Shandong University of TechnologyZibo255000China School of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore639798Singapore State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Reducing thermal conductivity while avoiding adverse interfacial reactions during sintering is crucial for improving the thermoelectric performance of Bi_(2)Te_(3)based *** ceramic nanoparticles are good candidates for achieving this *** this study,we designed and prepared a series of p-type Bi_(0.5)Sb_(1.5)Te_(3)nanocomposites decorated with Y_(2)O_(3)ceramic nanoparticles via ball-milling dispersion and spark-plasma *** to the chemical stability of the ceramics,no traces of atomic doping or interfacial reactions were *** measurements revealed that the Y_(2)O_(3)nanoparticles distributed along the grain boundaries acted as energy-dependent carrier-filtering centers to improve the scattering parameter and Seebeck coefficient,contributing to the elevated power factor even with a decreased electrical ***,the incorporated Y_(2)O_(3)nanoparticles and various defect structures they induced effectively strengthened the phonon scattering and suppressed the lattice thermal ***,a peak figure of merit(ZT)of 1.23 at 313 K was achieved for 0.4%Y_(2)O_(3)/Bi_(0.5)Sb_(1.5)Te_(3),which is 13%higher than that of the *** addition,the Vickers hardness of the composite material was 35%higher than that of the *** study demonstrates the effectiveness of ceramic nanoparticles in synergistic ally improving the thermoelectric and mechanical properties,which may be further extended to other thermoelectric systems.

关键词： Bi_(0.5)Sb_(1.5)Te_3 alloy Y_(2)O_(3) ceramic nanoparticles Microstructures Thermoelectric performance Mechanical properties

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Multilevel carbon architecture of subnanoscopic silicon for fast‐charging high‐energy‐density lithium‐ion batteries

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Carbon Energy 2024年第4期6卷 256-268页

作者： Meisheng Han Yongbiao Mu lei wei Lin Zeng Tianshou Zhao Shenzhen Key Laboratory of Advanced Energy Storage Southern University of Science and TechnologyShenzhenChina SUSTech Energy Institute for Carbon Neutrality Southern University of Science and TechnologyShenzhenChina Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhenChina

Silicon(Si)is widely used as a lithium‐ion‐battery anode owing to its high capacity and abundant crustal ***,large volume change upon cycling and poor conductivity of Si cause rapid capacity decay and poor fast‐charging capability limiting its commercial ***,we propose a multilevel carbon architecture with vertical graphene sheets(VGSs)grown on surfaces of subnanoscopically and homogeneously dispersed Si–C composite nanospheres,which are subsequently embedded into a carbon matrix(C/VGSs@Si–C).Subnanoscopic C in the Si–C nanospheres,VGSs,and carbon matrix form a three‐dimensional conductive and robust network,which significantly improves the conductivity and suppresses the volume expansion of Si,thereby boosting charge transport and improving electrode *** VGSs with vast exposed edges considerably increase the contact area with the carbon matrix and supply directional transport channels through the entire material,which boosts charge *** carbon matrix encapsulates VGSs@Si–C to decrease the specific surface area and increase tap density,thus yielding high first Coulombic efficiency and electrode compaction ***,C/VGSs@Si–C delivers excellent Li‐ion storage performances under industrial electrode *** particular,the full cells show high energy densities of 603.5 Wh kg^(−1)and 1685.5 Wh L^(−1)at 0.1 C and maintain 80.7%of the energy density at 3 C.

关键词： fast charging high energy densities lithium‐ion batteries multilevel carbon architecture subnanoscopic silicon anode

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Controlled fluorescent switch based on a cation grease/brake rotor system of pillar[5]arene

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Chinese Chemical Letters 2024年第3期35卷 5-7页

作者： wei-lei Zhou Siwei Wang Yong Chen College of Chemistry and Material Science Inner Mongolia Key Laboratory of Chemistry for Nature Products and Synthesis for Functional MoleculesInnovation Team of Optical Functional Molecular DevicesInner Mongolia Minzu UniversityTongliao 028000China College of Chemistry Nankai UniversityTianjin 300071China

In recent years,molecular shuttles,motors,pumps,and elevators,*** specifically respond external physical or chemical stimuli including light,temperature,pH,redox,solvent and chemical additive to change the structure a... 详细信息

关键词： additive system showing

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NeoHunter:Flexible software for systematically detecting neoantigens from sequencing data

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Quantitative Biology 2024年第1期12卷 70-84页

作者： Tianxing Ma Zetong Zhao Haochen Li lei wei Xuegong Zhang MOE Key Lab of Bioinformatics Bioinformatics Division of BNRIST and Department of AutomationTsinghua UniversityBeijingChina School of Medicine Tsinghua UniversityBeijingChina School of Life Sciences Tsinghua UniversityBeijingChina

Complicated molecular alterations in tumors generate various mutant *** of these mutant peptides can be presented to the cell surface and then elicit immune responses,and such mutant peptides are called *** detection of neoantigens could help to design personalized cancer *** some computational frameworks for neoantigen detection have been proposed,most of them can only detect SNV-and indel-derived *** addition,current frameworks adopt oversimplified neoantigen prioritization *** factors hinder the comprehensive and effective detection of *** developed NeoHunter,flexible software to systematically detect and prioritize neoantigens from sequencing data in different *** can detect not only SNV-and indel-derived neoantigens but also gene fusion-and aberrant splicing-derived *** supports both direct and indirect immunogenicity evaluation strategies to prioritize candidate *** strategies utilize binding characteristics,existing biological big data,and T-cell receptor specificity to ensure accurate detection and *** applied NeoHunter to the TESLA dataset,cohorts of melanoma and non-small cell lung cancer *** achieved high performance across the TESLA cancer patients and detected 79%(27 out of 34)of validated neoantigens in ***-and indel-derived neoantigens accounted for 90%of the top 100 candidate neoantigens while neoantigens from aberrant splicing accounted for 9%.Gene fusion-derived neoantigens were detected in one *** is a powerful tool to‘catch all’neoantigens and is available for free academic use on Github(XuegongLab/NeoHunter).

关键词： cancer vaccine molecular alteration neoantigen neoantigen prioritization

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Nano polystyrene microplastics could accumulate in Nile tilapia(Oreochromis niloticus):Negatively impacts on the intestinal and liver health through water exposure

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Journal of Environmental Sciences 2024年第3期137卷 604-614页

作者： Di Wu Xing Lu Li-Xue Dong Juan Tian Jin Deng lei wei Hua Wen Shan Zhong Ming Jiang School of Basic Medical Sciences Wuhan UniversityWuhan 430071China Key Laboratory of Freshwater Biodiversity Conservation Ministry of Agriculture and Rural AffairsYangtze River Fisheries Research InstituteChinese Academy of Fishery SciencesWuhan 430223China Hubei Province Key Laboratory of Allergy and Immunology Wuhan 430071China

Microplastics(MPs)have become a significant concern for their potential ***,the correlation between the size of plastic particles and their toxicity remains ***,we investigate the toxic effects of different sizes(80 nm,800 nm,8μm and 80μm)polystyrene MPs(PS-MPs)on the model organism Nile tilapia(Oreochromis niloticus).The results of bioluminescent imaging indicate that the 80 nm PS-MPs are more likely to invade the body.H&E staining shows severe damage on the intestinal villi and distinct hepatic steatosis in the 80 nm *** U labeling shows that the proliferation activity of intestinal and liver cells reduces significantly in the 80 nm *** gut microbiome analysis shows a severe imbalance of gut microbiota homeostasis in the 80 nm *** analysis of liver transcriptomics and metabolomics shows that the liver lipid metabolism is disordered in the 80 nm *** conclusion,this study confirms that the 80 nm PS-MPs are more likely to induce intestinal and liver *** the above lay the foundation for further study on the pathological damage of MPs to other organisms.

关键词： Microplastics(MPs) Intestinal toxicity Liver toxicity Gut microbiome Lipid metabolism

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Bioinspired Stretchable MXene Deformation-Insensitive Hydrogel Temperature Sensors for Plant and Skin Electronics

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Research 2024年第1期2023卷 389-401页

作者： Jun Wu Yinghui Li Shengshun Duan Zhehan Wang Xu Jing Yucheng Lin Di Zhu wei lei Qiongfeng Shi Li Tao Joint International Research Laboratory of Information Display and Visualization School of Electronic Science and EngineeringSoutheast UniversityNanjingJiangsu 210096China School of Materials Science and Engineering Southeast UniversityNanjingJiangsu 210096China Center of 2D Materials and Devices Southeast UniversityNanjingJiangsu 210096China

Temperature sensing is of high value in the wearable healthcare,robotics/prosthesis,and noncontact physiological ***,the common mechanic deformation,including pressing,bending,and stretching,usually causes undesirable feature size changes to the inner conductive network distribution of temperature sensors,which seriously influences the ***,inspired by the transient receptor potential mechanism of biological thermoreceptors that could work precisely under various skin contortions,we propose an MXene/Clay/poly(N-isopropylacrylamide)(PNIPAM)(MCP)hydrogel with high stretchability,spike response,and deformation *** dynamic spike response is triggered by the inner conductive network transformation from the 3-dimensional structure to the 2-dimensional surface after water being discharged at the threshold *** water discharge is solely determined by the thermosensitivity of PNIPAM,which is free from mechanical deformation,so the MCP hydrogels can perform precise threshold temperature(32℃)sensing under various deformation conditions,i.e.,pressing and 15%*** a proof of concept,we demonstrated the applications in plant electronics for the real-time surface temperature monitoring and skin electronics for communicating between human and *** research opens venues for the accurate temperature-threshold sensation on the complicated surface and mechanical conditions.

关键词： stretching proof precise

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A deep learning interatomic potential suitable for simulating radiation damage in bulk tungsten

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Tungsten 2024年第2期6卷 304-322页

作者： Chang-Jie Ding Ya-wei lei Xiao-Yang Wang Xiao-Lin Li Xiang-Yan Li Yan-Ge Zhang Yi-Chun Xu Chang-Song Liu Xue-Bang Wu Key Laboratory of Materials Physics Institute of Solid State PhysicsHFIPSChinese Academy of SciencesHefei 230031China Science Island University of Science and Technology of ChinaHefei 230026China Laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing 100088China

So far, it has been a challenge for existing interatomic potentials to accurately describe a wide range of physical properties and maintain reasonable efficiency. In this work, we develop an interatomic potential for simulating radiation damage in body-centered cubic tungsten by employing deep potential, a neural network-based deep learning model for representing the potential energy surface. The resulting potential predicts a variety of physical properties consistent with first-principles calculations, including phonon spectrum, thermal expansion, generalized stacking fault energies, energetics of free surfaces, point defects, vacancy clusters, and prismatic dislocation loops. Specifically, we investigated the elasticity-related properties of prismatic dislocation loops, i.e., their dipole tensors, relaxation volumes, and elastic interaction energies. This potential is found to predict the maximal elastic interaction energy between two 1/2 loops better than previous potentials, with a relative error of only 7.6%. The predicted threshold displacement energies are in reasonable agreement with experimental results, with an average of 128 eV. The efficiency of the present potential is also comparable to the tabulated gaussian approximation potentials and modified embedded atom method potentials, meanwhile, can be further accelerated by graphical processing units. Extensive benchmark tests indicate that this potential has a relatively good balance between accuracy, transferability, and efficiency.

关键词： Machine learning Deep learning Interatomic potential Radiation damage Tungsten

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Analysis of the Heavy Rainfall Process in Mangshi City on August 8, 2023

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Meteorological and Environmental Research 2024年第2期15卷 48-54,61页

作者： Yan YU Bowen LIU Wan GONG Shuxuan HE lei wei Dehong Meteorological Observatory Dehong 678400China Yunnan Meteorological Observatory Kunming 650034China Key Laboratory of Heavy Rainfall in River Basins China Meteorological AdministrationWuhan 430205China Research Center for Disastrous Weather over Hengduan Mountains&Low-Latitude Plateau China Meteorological AdministrationKunming 650034China Yunnan Institute of Geological Environment Monitoring Kunming 650216China

On August 7,2023,Mangshi City,Dehong Prefecture experienced a local heavy rainstorm,and the geological disaster caused by the heavy rainfall caused casualties and property *** on the real-time observation data of automatic stations,Doppler weather radar detection and meteorological risk warning products,the disaster situation,social impact,forecast and early warning service,causes of heavy precipitation and forecast and early warning inspection were summarized and *** results show that the heavy rainfall was prominent locally,lasted for a long time and accumulated a large amount of *** were biases in model products,and it was difficult for forecasters to make subjective corrections in complex *** analysis ideas and focus points of heavy rainfall forecast,the improvement ideas and technical schemes of forecast deviation,and the improvement ideas and suggestions of services were *** provides a reference for the forecast and early warning of severe weather in the future.

关键词： Heavy rainfall Low-pressure inverted trough Geological disaster Forecast deviation

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跨地方视角下非物质文化遗产地方性的多尺度建构

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地理学报 2024年第4期79卷 1068-1084页

作者：魏雷刘晓平朱竑杨蓉广州大学管理学院广州510006 广州大学地理科学与遥感学院广州510006 广州大学华南人文地理与城市发展中心广州510006

非物质文化遗产是源自特定社区、群体或个人的社会实践,地方性是非遗的主要特征。在全球化与地方化的相互作用下,非遗的地方性不仅被本土要素塑造,更是被超越本土的不同物质、知识技术和观念符号等共同建构。本文采用多源数据分析了3个... 详细信息

非物质文化遗产是源自特定社区、群体或个人的社会实践,地方性是非遗的主要特征。在全球化与地方化的相互作用下,非遗的地方性不仅被本土要素塑造,更是被超越本土的不同物质、知识技术和观念符号等共同建构。本文采用多源数据分析了3个服饰品牌对珠三角地区香云纱及其染整技艺的地方性表征。研究发现,由于在跨地方网络中的位置性差异,各个品牌采用不同的尺度策略形成了关于香云纱及其染整技艺地方性的多种叙事。具体来看:①本土化策略将品牌主理人的本土身份与本土文化资源的领域相对应,将传统非遗所包含的历史、气候、资源、文化等关键地方性要素定位为品牌市场运作的核心竞争力;②多重再地化策略是品牌在本土、区域和全球的多重尺度上进行资源整合,利用各层面机会进行品牌运作,同时将非遗实践与多尺度的议程连接起来;③地方杂糅策略在世界主义价值观的主导下,融合了不同地方的理念、话语和知识,将非遗实践塑造为全球多元文化的杂糅景观。本文诠释了在非遗实践中尺度是非层级的、网络化的。相应非遗的地方性是关系化的和情境化的,不是由边界所限定而成,而是被非遗实践所创造的地方之间的关联所塑造。

关键词：多尺度性跨地性本土化多重再地化地方杂糅

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时间反转OFDM系统中增强安全性能的功率分配与人工噪声设计

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电子学报 2024年第5期52卷 1570-1581页

作者：雷维嘉毕文佳雷宏江唐宏重庆邮电大学通信与信息工程学院重庆400065 重庆邮电大学移动通信技术重庆市重点实验室重庆400065

时间反转技术特有的时空聚焦特性使其具有抗窃听能力.本文对提高时间反转正交频分复用系统安全性能的优化方案进行研究.首先,通过应用时间反转预滤波的时空聚焦特性来提高合法接收端相对于窃听端的信号强度;然后,以最大化保密速率为目... 详细信息

时间反转技术特有的时空聚焦特性使其具有抗窃听能力.本文对提高时间反转正交频分复用系统安全性能的优化方案进行研究.首先,通过应用时间反转预滤波的时空聚焦特性来提高合法接收端相对于窃听端的信号强度;然后,以最大化保密速率为目标对子载波的功率分配进行优化.为进一步提升系统保密传输能力,利用循环前缀提供的自由度实现零空间人工噪声,在对窃听端形成有效干扰的同时,不对合法接收端造成影响.通过对子载波功率分配和人工噪声协方差阵进行联合优化,最大化系统的保密传输速率.仿真结果表明,所提优化方案能显著提高系统的保密速率.

关键词：物理层安全正交频分复用时间反转功率分配人工噪声

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