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International Journal of Modeling, Simulation, and Scientific Computing 2019年第2期10卷 142-155页

作者： lang-yang huang Zhi-Feng Weng Chao-Ying Lin Fujian Province University Key Laboratory of Computational Science School of Mathematical SciencesHuaqiao University Quanzhou 362021P.R.China Key Laboratory of Applied Mathematics(Putian University) Fujian Province University Fujian Putian 351100P.R.China

Combining symplectic algorithm,splitting technique and compact method,a compact splitting symplectic scheme is proposed to solve the fourth-order dispersive Schr¨odinger equation with cubic-quintic nonlinear *** scheme has fourth-order accuracy in space and second-order accuracy in *** discrete charge conservation law and stability of the scheme are *** examples are given to confirm the theoretical results.

关键词： Symplectic scheme Schr¨odinger equation compact splitting method conservation law

Oxygen-assisted zinc recovery from electric arc furnace dust using magnesium chloride

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International Journal of Minerals,Metallurgy and Materials 2024年第10期31卷 2300-2311页

作者： Jingdong huang Xiao yang School of Materials Science and Engineering Zhejiang UniversityHangzhou 310027China School of Engineering Westlake UniversityHangzhou 310030China

Electric arc furnace(EAF)dust is an important secondary resource containing metals,such as zinc(Zn)and iron(Fe).Recover-ing Zn from EAF dust can contribute to resource recycling and reduce environmental ***,the high chemical stability of ZnFe_(2)O_(4)in EAF dust poses challenges to Zn *** address this issue,a facile approach that involves oxygen-assisted chlorination using molten MgCl_(2)is *** work focused on elucidating the role of O2 in the reaction between ZnFe_(2)O_(4)and molten MgCl_(2).The results demonstrate that MgCl_(2)effectively broke down the ZnFe_(2)O_(4)structure,and the high O2 atmosphere considerably promoted the sep-aration of Zn from other components in the form of ZnCl_(2).The presence of O2 facilitated the formation of MgFe_(2)O_(4),which stabilized Fe and prevented its ***,the excessive use of MgCl_(2)resulted in increased evaporation loss,and high temperatures pro-moted the rapid separation of *** on these findings,we successfully extracted ZnCl_(2)-enriched volatiles from practical EAF dust through oxygen-assisted *** optimized conditions,this method achieved exceptional Zn chlorination percentage of over 97%within a short period,while Fe chlorination remained below 1%.The resulting volatiles contained 85wt%of ZnCl_(2),which can be further processed to produce metallic *** findings offer guidance for the selective recovery of valuable metals,particularly from solid wastes such as EAF dust.

关键词： electric arc furnace dust zinc oxygen magnesium chloride chlorination

Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao Li Lijinhong huang Bin Xiao Xiaoguang Duan Haike Li lang Li Wanfu huang Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

Ultrathin organic solvent nanofiltration membrane with polydopamine-HKUST-1 interlayer for organic solvent separation

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Journal of Environmental Sciences 2024年第7期141卷 182-193页

作者： Haike Li Xindong Li Guozai Ouyang Lijinhong huang lang Li Wenhao Li Wanfu huang Duokun Li Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou 341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou 341000China School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou 341000China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityWA 6845Australia School of Materials Science and Engineering Tiangong UniversityTianjin 300387China

Polydopamine(PDA)and metal-organic skeleton HKUST-1 were co-deposited on the base membrane of hexamethylenediamine(HDA)-crosslinked polyetherimide(PEI)ultrafiltration membrane as the interlayer,and high-throughput organic solvent nanofiltration membrane(OSN)was prepared by interfacial polymerization and solvent activation *** polyamide(PA)layer surface roughness from 28.4 nm in PA/PEI to 78.3 nm in PA/PDA-HKUST-10.6/PEI membrane,reduced the thickness of the separation layer from 79 to 14 nm,and significantly improved the hydrophilic,thermal and mechanical *** flux of the PA/PDA-HKUST-10.6/PEI membrane in a 0.1 g/L Congo Red(CR)ethanol solution at 0.6 MPa test pressure reached 21.8 L/(m^(2)·hr)and the rejection of CR was 92.8%.Solvent adsorption test,N,N-dimethylformamide(DMF)immersion experiment,and long-term operation test in ethanol showed that the membranes had high solvent *** solvent flux test demonstrated that,under the test pressure of 0.6 MPa,the flux of different solvents ranked as follows:methanol(56.9 L/(m^(2)·hr))>DMF(39.6 L/(m^(2)·hr))>ethanol(31.2 L/(m^(2)·hr))>IPA(4.5 L/(m^(2)·hr))>N-hexane(1.9 L/(m^(2)·hr)).The ability of the membranes to retain dyes in IPA/water dyes solution was also *** flux of the membrane was 30.4 L/(m^(2)·hr)and the rejection of CR was 91.6%when the IPA concentration reached 50%.This OSN membrane-making strategy is economical,environment-friendly and efficient,and has a great application prospect in organic solvent separation systems.

关键词： Interfacial polymerization Organic solvent nanofiltration Interlayer Metal-organic frameworks Polydopamine

Coupling effect of cement-stabilization and biopolymer-modification on the mechanical behavior of dredged sediment

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3284-3298页

作者： Lei lang Jiangshan Li Xiao huang Ping Wang Wei Zhang State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChinese Academy of SciencesWuhan430071China Hubei Provincial Key Laboratory of Contaminated Sludge and Soil Science and Engineering Wuhan430071China University of Chinese Academy of Sciences Beijing100049China

Nowadays,biopolymer stabilization as a promising eco-friendly approach in soft ground improvement has attracted wide ***,the feasibility of using biopolymer as a green additive of cementstabilized dredged sediment(CDS)with high water content is still *** this study,guar gum(GG)and xanthan gum(XG)were adopted as typical biopolymers,and a series of unconfined compressive strength(UCS),splitting tensile strength(STS)and scanning electron microscopy(SEM)tests were performed to evaluate the mechanical and microstructural properties of XG-and GG-modified CDSs considering several factors including biopolymer modification,binderesoil ratio and wateresolid ***,the micro-mechanisms revealing the evolutions of mechanical properties of biopolymermodified CDS were *** results indicate that the addition of XG can effectively improve the strength of CDS,while the GG has a side *** XG content of 9%was recommended,which can improve the 7 d-and 28 d-UCSs by 196%and 51.8%,together with the 7 d-and 28 d-STSs by 118.3%and 42.2%,*** the binderesoil ratio or decreasing the wateresolid ratio significantly improved the strength gaining but aggravated the brittleness characteristics of *** XG to CDS contributed to the formation of microstructure with more compactness and higher cementation degrees of ordinary Portland cement(OPC)-XG-stabilized DS(CXDS).The micro-mechanism models revealing the interactions of multiple media including OPC cementation,biopolymer film bonding and bridging effects inside CXDS were *** key findings confirm the feasibility of XG modification as a green and high-efficiency mean for improving the mechanical properties of CDS.

关键词： Dredged sediment(DS) Stabilization Biopolymer modification Mechanical properties Micro-mechanism

Single-atom catalysis:a promising avenue for precisely controlling reaction pathways

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Frontiers of Chemical Science and Engineering 2024年第7期18卷 97-120页

作者： Xiaobo yang Xuning Li Yanqiang huang State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China

Single-atom catalysts (SACs), characterized by exceptionally high atom efficiency, have garnered significant attention across various catalytic reactions. Recent studies have showcased SACs with robust capabilities for precise catalysis, specifically targeting reactions along designated pathways. This review focuses on the advances in the precise activation and reconstruction of chemical bonds on SACs, including precise activation of C–O and C–H bonds and selective couplings involving C–C and C–N bonds. Our discussion begins with a thorough exploration of the factors that render SACs skilled in precise catalytic processes, encompassing the narrow d-band electronic state of single atom site resulting in the adsorption tendency, isolate site resulting in unique adsorption structure, and synergy effect of a single atom site with its neighbors. Subsequently, we elaborate on the applications of SACs in electrocatalysis and thermocatalysis including four prominent reactions, namely, electrochemical CO_(2) reduction, urea electrochemical synthesis, CO_(2) hydrogenation, and CH4 activation. Then the concept of rational design of SACs for precisely controlling reaction pathways is discussed from the aspects of pore structure design, support-metal strong interaction, and support hydrophilic/hydrophobic. Finally, we summarize the challenges encountered by SACs in the field of precise catalytic processes and outline prospects for their further development in this domain.

关键词： single atom catalysts selective oxidation CO_(2)RR bond coupling

On-chip source-device-independent quantum random number generator

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Photonics Research 2024年第7期12卷 1379-1394页

作者： lang LI MINGLU CAI TAO WANG ZICONG TAN PENG huang KAN WU GUIHUA ZENG State Key Laboratory of Advanced Optical Communication Systems and Networks Shanghai Jiao Tong UniversityShanghai 200240China Institute of Quantum Sensing and Information Processing School of Sensing Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Shanghai Research Center for Quantum Sciences Hefei National LaboratoryShanghai 201315China Shanghai Xun Tai Quantech Co. Ltd.Shanghai 200241China

Quantum resources offer intrinsic randomness that is valuable for applications such as cryptography, scientific simulation, and computing. Silicon-based photonics chips present an excellent platform for the cost-effective deployment of next-generation quantum systems on a large scale, even at room temperature. Nevertheless,the potential susceptibility of these chips to hacker control poses a challenge in ensuring security for on-chip quantum random number generation, which is crucial for enabling extensive utilization of quantum resources.

关键词： temperature quantum random

Piecewise Acoustic Source Imaging with Unknown Speed of Sound Using a Level-Set Method

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Communications on Applied Mathematics and Computation 2024年第2期6卷 1070-1095页

作者： Guanghui huang Jianliang Qian yang yang Petroleum Geo-Services HoustonTX 77079USA Department of Mathematics Michigan State UniversityEast LansingMI 48824USA Department of Computational Mathematics Science and EngineeringMichigan State UniversityEastLansingMI48824USA

We investigate the following inverse problem:starting from the acoustic wave equation,reconstruct a piecewise constant passive acoustic source from a single boundary temporal measurement without knowing the speed of *** the amplitudes of the source are known a priori,we prove a unique determination result of the shape and propose a level set algorithm to reconstruct the *** the singularities of the source are known a priori,we show unique determination of the source amplitudes and propose a least-squares fitting algorithm to recover the source *** analysis bridges the low-frequency source inversion problem and the inverse problem of *** proposed algorithms are validated and quantitatively evaluated with numerical experiments in 2D and 3D.

关键词： Inverse gravimetry Acoustic source imaging Inversion of sound speed Level-set method Inverse problem

Bound-Preserving Discontinuous Galerkin Methods with Modified Patankar Time Integrations for Chemical Reacting Flows

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Communications on Applied Mathematics and Computation 2024年第1期6卷 190-217页

作者： Fangyao Zhu Juntao huang yang yang Department of Mathematical Sciences Michigan Technological UniversityHoughtonMI49931USA Department of Mathematics and Statistics Texas Tech UniversityLubbockTX79409USA

In this paper,we develop bound-preserving discontinuous Galerkin(DG)methods for chemical reactive *** are several difficulties in constructing suitable numerical *** of all,the density and internal energy are positive,and the mass fraction of each species is between 0 and ***,due to the rapid reaction rate,the system may contain stiff sources,and the strong-stability-preserving explicit Runge-Kutta method may result in limited time-step *** obtain physically relevant numerical approximations,we apply the bound-preserving technique to the DG *** traditional positivity-preserving techniques can successfully yield positive density,internal energy,and mass fractions,they may not enforce the upper bound 1 of the mass *** solve this problem,we need to(i)make sure the numerical fluxes in the equations of the mass fractions are consistent with that in the equation of the density;(ii)choose conservative time integrations,such that the summation of the mass fractions is *** the above two conditions,the positive mass fractions have summation 1,and then,they are all between 0 and *** time discretization,we apply the modified Runge-Kutta/multi-step Patankar methods,which are explicit for the flux while implicit for the *** methods can handle stiff sources with relatively large time steps,preserve the positivity of the target variables,and keep the summation of the mass fractions to be ***,it is not straightforward to combine the bound-preserving DG methods and the Patankar time *** positivity-preserving technique for DG methods requires positive numerical approximations at the cell interfaces,while Patankar methods can keep the positivity of the pre-selected point values of the target *** match the degree of freedom,we use polynomials on rectangular meshes for problems in two space *** evolve in time,we first read the polynomials at the Gaussian ***,suitable slope l

关键词： Compressible Euler equations Chemical reacting flows Bound-preserving Discontinuous Galerkin(DG)method Modified Patankar method

Friction Characteristics Between Marine Clay and Construction Materials

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Journal of Ocean University of China 2024年第2期23卷 427-437页

作者： KOU Hailei huang Jiaming CHENG yang College of Engineering Ocean University of ChinaQingdao 266100China Fourth Division Organization Department of the CPC Qingdao Municipal CommitteeQingdao 266100China

Structure-soil interface friction characteristics is of importance to investigate the interaction between engineering structures and soils,especially for offshore *** interface friction behavior between marine clay and structural materials with different roughness was studied in this paper by using 3D optical scanning tests,a modified direct shear device and numerical *** between the surface roughness of structures,water content and interface friction angle were presented by model *** increase of water contents decreased the interface friction *** interfaces with different roughness,the interface friction angles will be smaller than that of the soil when the water content exceeds a certain *** roughness of the interface and the water content of the soil are mutually coupled to influence the coefficient of friction(COF).This paper proposed a Finite Element Method(FEM)to simulate the interface direct shear tests of structures with different *** surface models with different roughness are established based on the structure data obtained by 3D *** Coupled Eulerian-Lagrangian(CEL)approach was employed to analyse soils sheared by irregular *** interface behavior for interfaces with different roughness under cyclic shear stresses was analyzed by FEM.

关键词： marine clay construction material interface friction behavior surface roughness Finite Element Method