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Research advances in enhanced coal seam gas extraction by controllable shock wave fracturing

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International Journal of Coal Science & Technology 2024年第3期11卷 1-31页

作者： Chaojun fan Hao Sun Sheng Li Lei Yang Bin Xiao Zhenhua Yang Mingkun luo Xiaofeng Jiang Lijun Zhou College of Mining Liaoning Technical UniversityFuxin123000China College of Safety Science and Engineering Liaoning Technical UniversityFuxin123000China Energy Business Department Shanxi Lu’an Chemical GroupChangzhi046200China

With the continuous increase of mining in depth,the gas extraction faces the challenges of low permeability,great ground stress,high temperature and large gas pressure in coal *** controllable shock wave(CSW),as a new method for enhancing permeability of coal seam to improve gas extraction,features in the advantages of high efficiency,eco-friendly,and low *** order to better utilize the CSW into gas extraction in coal mine,the mechanism and feasibility of CSW enhanced extraction need to be *** this paper,the basic principles,the experimental tests,the mathematical models,and the on-site tests of CSW fracturing coal seams are reviewed,thereby its future research directions are *** on the different media between electrodes,the CSW can be divided into three categories:hydraulic effect,wire explosion and excitation of energetic materials by detonating *** the process of propagation and attenuation of the high-energy shock wave in coal,the shock wave and bubble pulsation work together to produce an enhanced permeability effect on the coal *** stronger the strength of the CSW is,the more cracks created in the coal is,and the greater the length,width and area of the cracks *** repeated shock on the coal seam is conducive to the formation of complex network fracture system as well as the reduction of coal seam strength,but excessive shock frequency will also damage the coal structure,resulting in the limited effect of the enhanced gas *** the influence of ground stress,the crack propagation in coal seam will be *** difference of horizontal principal stress has a significant impact on the shape,propagation direction and connectivity of the CSW induced *** permeability enhancement effect of CSW is affected by the breakage degree of coal *** shock wave is absorbed by the broken coal,which may hinder the propagation of CSW,resulting in a poor effect of permeability *** arranging two a

关键词： Controllable shock wave Permeability enhancement Gas extraction Basic principle Experimental test Mathematical models On-site test

Effects of cyclodextrins on hydrolysis of malathion

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Journal of Environmental Sciences 2006年第3期18卷 572-576页

作者： ZHANG An-ping luo fan CHEN Sheng-wen LIU Wei-ping Institute of Environmental Science Zhejiang University Hangzhou 310029 China Research Center of Green Chirality College of Biological and Environmental Engineering Zhejiang University of Technology Hangzhou 310032 China

Cyclodextrins （CDs）, with hydrophobic interior cavity and hydrophilic external surface, are capable of accelerating or inhibiting chemical degradation of organophosphorus pesticides through forming inclusion complexes between CDs and pesticides. This work evaluated the effects of CDs on hydrolysis of malathion in an attempt to assess their potential application in environmental approach. β-CD and its two derivatives, randomly methylated β-CD （RAMEB） and hydroxypropyl β-CD （HP-β-CD）, were tested. It was found that RAMEB could inhibit the hydrolysis of malathion, and this was the function of pH and temperature, the inhibitory effects increase with increasing concentration of RAMEB and elevating temperature between 15 and 35℃. On the other hand, β-CD and HP-β-CD have little or no stabilizing effects on malathion at all pH and temperature studied, except that the large concentration of β-CD and HP- β-CD can mildly reduce hydrolysis of malathion. Both 2 mol/L and 5 mol/L urea increase the inhibitory effects of RAMEB on hydrolysis of malathion at 25℃, oH 9.0.

关键词： cyclodextrin malathion hydrolysis urea

维普期刊数据库

Phase reconfiguration of heterogeneous CoFeS/CoNiS nanoparticles for superior battery-type supercapacitors

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Journal of Energy Chemistry 2024年第9期96卷 217-225页

作者： Lina Ma fan Li Min Zhou Jidong Dong Hao luo Wei Zhang Wenchao Zhao Xinliang Li Zaixing Jiang Yudong Huang College of Chemistrynd Chemical Engineering Qingdao UniversityQingdao 266071ShandongChina School of Materials Sciencend Engineering Xiamen University of TechnologyXiamen 361024FujianChina Co-Innovation Center of Efficient Processingnd Utilization of Forest Resources College of Materials Sciencend EngineeringNanjing Forestry UniversityNanjing 210037JiangusChina Key Laboratory of Material Physics Ministry of EducationSchool of Physicsnd MicroelectronicsZhengzhou UniversityZhengzhou 450052HenanChina MIIT Key Laboratory of Critical Materials Technology for New Energy Conversionnd Storage State Key Laboratory of Urban Water Resourcend EnvironmentSchool of Chemistrynd Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HeilongjiangChina Material Sciencend Engineering College Northeast Forestry UniversityHarbin 150040HeilongjiangChina

Developing advanced battery-type materials with abundant active sites,high conductivity,versatile morphologies,and hierarchically porous structures is crucial for realizing high-quality hybrid ***,heterogeneous FeS@NiS is synthesized by cationic Co doping via surface-structure *** density functional theory(DFT)theoretical calculations are firstly performed to predict the advantages of Co dopant by improving the OH^(−)adsorption properties and adjusting electronic structure,benefiting ions/electron *** dynamic surface evolution is further explored which demonstrates that CoFeS@CoNiS could be quickly reconstructed to Ni(Co)Fe_(2)O_(4)during the charging process,while the unstable structure of the amorphous Ni(Co)Fe_(2)O_(4)results in partial conversion to Ni/Co/FeOOH at high potentials,which contributes to the more reactive active site and good structural ***,the free-standing electrode reveals excellent electrochemical performance with a superior capacity(335.6 mA h g^(−1),2684 F g^(−1))at 3 A g^(−1).Furthermore,the as-fabricated device shows a quality energy density of 78.1 W h kg^(−1)at a power density of 750 W kg^(−1)and excellent cycle life of 92.1%capacitance retention after 5000 *** work offers a facile strategy to construct versatile morphological structures using electrochemical activation and holds promising applications in energy-related fields.

关键词： In-situ reconfiguration Heterogeneous design Battery-type supercapacitors Superior performance Sulphide

3D inversion of audio-magnetotelluric data for mineral exploration:A case study of Layikeleke buried porphyry copper deposit,Xinjiang,China

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Applied Geophysics 2020年第4期17卷 576-588页

作者： Fu Guang-Ming Chen Hui Yu Hui luo fan luo Lei Tao Xin School of Geophysics and Measurement-control Technology East China University of TechnologyNanchang 330013China China Deep Exploration Center China Geological Survey&Chinese Academy of Geological SciencesBeijing 100037China

Layikeleke copper deposit is a large-scale porphyry copper polymetallic buried deposit,which has been discovered recently in the eastern Junggar area of *** occurred in the Late Silurian and Early Devonian with the copper body mainly confined to *** find new ore bodies,it is necessary to map the 3D spatial distribution of the *** this reason,we deployed audio-magnetotelluric(AMT)sounding in the research area,collected 26 profi les and 1198 measuring points,carried out 3D inversion calculations of off-diagonal elements in the impedance tensor data using the nonlinear conjugate gradient method,and obtained a 3D electrical structure *** electrical structure reveals two groups of NW-SE trending middle and middle low resistivity anomaly zones,which intersect the high resistivity bedrock area in the northwest of the study *** on the electrical data,it can be inferred that the medium low resistance tonalite in the northern part of the study area is the host rock of the porphyry copper polymetallic deposit,which has been verifi ed by borehole *** results of 3D AMT inversion depict the spatial distribution and depth variation characteristics of the tonalite electrical structure model,providing a basis for further prospecting and ***,this method of identifying lithology by 3D inversion can provide an important basis for mineral exploration and mining of buried rock masses,and is an effective prospecting method.

关键词： AMT 3D inversion Layikeleke porphyry copper mine

维普期刊数据库

Machine learning-based predictions of current and future susceptibility to retrogressive thaw slumps across the Northern Hemisphere

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Advances in Climate Change Research 2024年第2期15卷 253-264页

作者： Jing luo Guo-An YIN Fu-Jun NIU Tian-Chun DONG Ze-Yong GAO Ming-Hao LIU fan YU State Key Laboratory of Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China China Railway Qinghai-Tibet Group Co. LtdXining 810000China University of Chinese Academy of Sciences Beijing 100049China

Retrogressive thaw slumps(RTSs)caused by the thawing of ground ice on permafrost slopes have dramatically increased and become a common permafrost hazard across the Northern Hemisphere during previous ***,a gap remains in our comprehensive understanding of the spatial controlling factors,including the climate and terrain,that are conducive to these RTSs at a global *** machine learning methodologies,we mapped the current and future RTSs susceptibility distributions by incorporating a range of environmental factors and RTSs *** identified freezing-degree days and maximum summer rainfall as the primary environmental factors affecting RTSs *** final ensemble susceptibility map suggests that regions with high to very high susceptibility could constitute(11.6±0.78)%of the Northern Hemisphere's permafrost *** juxtaposed with the current(2000-2020)RTSs susceptibility map,the total area with high to very high susceptibility could witness an increase ranging from(31.7±0.65)%(SSP585)to(51.9±0.73)%(SSP126)by the *** insights gleaned from this study not only offer valuable implications for engineering applications across the Northern Hemisphere,but also provide a long-term insight into the potential change of RTSs in permafrost regions in response to climate change.

关键词： Retrogressive thaw slump Machine learning Susceptibility map Permafrost Northern Hemisphere

Pollutant emissions from biomass burning:A review on emission characteristics,environmental impacts,and research perspectives

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Particuology 2024年第2期85卷 296-309页

作者： Ke Jiang Ran Xing Zhihan luo Wenxuan Huang fan Yi Yatai Men Nan Zhao Zhaofeng Chang jinfeng Zhao Bo Pan Guofeng shen College of Urban and Environmental Sciences Peking UniversityBeijing100871China Beijing Key Lab Plant Resources Research and Development Beijing Technology and Business UniversityBeijing100048China College of Ecology and Environment Zhengzhou UniversityZhengzhou450001China Facultyof Environmental Sciences and Engineering Kunming University of Science and TechnologyYunnan Provincial Key Laboratoryof Soil Carbon Sequestration and Pollution ControlKunming650500China Institute of Carbon Neutrality Peking UniversityBeijing100871China

Biomass is one most abundant resource on the earth providing important energies in support of so-cioeconomic development in many *** of biomass fuels comprises to nearly 10%of the total energy from anthropogenic combustion processes:however,as the burning is usually incomplete,this process yields products of incomplete combustion posing consequently significant impacts on air quality,human health,and climate ***,we analyzed spatiotemporal characteristics in intentional and unintentional biomass burning from different sectors,discussed impacts of biomass burning emissions on indoor and outdoor air quality,and consequent influences on human *** global total con-sumption amount of biomass including both natural and anthropogenic sources was approximately 7900 Tg in 2019,with significantly large regional and sectorial discrepancies among ***,anthropogenic biomass burning amounts increased gradually,but notably in some developing countries like China residential consumption of biomass fuels,as one large sector of biomass use,decreased over *** biomass consumption needs to be accurately *** are relatively rich datasets of pollutant emission factors from biomass burning,including laboratory and field tests,but still large variations exit and contribute substantially to the uncertainty in emission *** pri-mary PM2.5,black carbon and organic carbon emissions from biomass burning were about 51,4.6,and 29 Tg,respectively,contributing to nearly 70%,55%,and 90%of the total emission from all sources,and emissions from the residential sector and open fires are major *** carbon emissions from biomass burning attracts growing interests but available studies adopted different methodologies challenging the comparability of those *** burning emissions polluted not only ambient air but more severely indoor air quality,adversely affecting human *** studies that should be emphasiz

关键词： Biomass burning Carbonaceous aerosol Emission Air quality Human health

Sanhua Tang(三化汤) protects against ischemic stroke by preventing blood-brain barrier injury: a network pharmacology and in vivo experiments

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Journal of Traditional Chinese Medicine 2024年第4期44卷 794-803页

作者： luo Shan YANG fan CHEN Yuanchun ZHAO Ruoxi LIU Haiye GAO Fei MA Wencan GAO Weijuan YU Wentao College of Basic Medicine Hebei University of Chinese Medicine Graduate School Hebei University of Chinese Medicine College of Acupuncture and Massage Hebei University of Chinese Medicine Hebei Key Laboratory of Chinese Medicine Research on Cardio-Cerebrovascular Diseases Hebei International Joint Research Centre for Acupuncture and Moxibustion of Traditional Chinese Medicine

OBJECTIVE: To assess the effect and mechanism of Sanhua Tang(三化汤, SHT) in treating ischemic stroke(IS) through the "Kaitong Xuanfu" theory by using network pharmacology and animal experiments. METHODS: The active ingredients and targets of SHT and IS were screened by public databases such as Traditional Chinese Medicine systems pharmacology, GeneCards, and online mendelian inheritance in man. Visual network topographies were constructed using R, Cytoscape 3.6.0, AutoDockTools, a user-sponsored molecular visualization system on an open-source foundation, and other software to analyze the correlation between targets and active ingredients. The middle cerebral artery occlusion(MCAO) model was established by operation. Animals were divided into the Sham group, MCAO group(M group), aloe-emodin(AE) group(MCAO rats treated with aloe-emodin), SHT at low dosage(SL group)(MCAO rats treated with SL), SHT at medium dosage(SM group), and SHT at high dosage(SH group). 2,3,5-triphenyl tetrazolium chloride staining was used to detect the volume of cerebral infarction; Nissl staining was used to observe the morphology of neuronal cells; transmission electron microscopy was used to observe the integrity of the blood-brain barrier(BBB); enzymelinked immunosorbent assay was used to detect the content of interleukin-6(IL-6), IL-10, tumor necrosis factor α(TNF-α) in serum. Western blot was used to detect the expression of vascular endothelial growth factor A(VEGFA) protein in the cerebral ischemic penumbra. RESULTS: Using network pharmacology and molecular docking validation, four active ingredients(lignan, naringenin, aloe-rhodopsin, and β-sitosterol), seven target proteins(protein kinase b 1, IL-6, TNF, VEGFA, TP53, jun proto-oncogene, and cysteinyl aspartate specific proteinase 3), and inflammatory signaling pathways were identified. Animal experiments showed that the SH and AE groups had fewer neurological deficits, reduced brain infarct volumes, decreased serum inflammatory factor l

关键词： Sanhua Tang blood-brain barrier inflammatory reactions ischemic stroke network pharmacology

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Harnessing antimicrobial peptide-coupled photosensitizer to combat drug-resistant biofilm infections through enhanced photodynamic therapy

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Acta Pharmaceutica Sinica B 2024年第4期14卷 1759-1771页

作者： Duoyang fan Xiaohui Liu Yueming Ren Ziheng luo Yanbing Li Jie Dong Seraphine VWegner Fei Chen Wenbin Zeng Xiangya School of Pharmaceutical Sciences Central South UniversityChangsha 410013China Hunan Key Laboratory of Diagnostic and Therapeutic Drug Research for Chronic Diseases Central South UniversityChangsha 410013China Sir William Dunn School of Pathology University of OxfordOxford OX13REUK Xiangya Hospital of Central South University Changsha 410013China Institute of Physiological Chemistry and Pathobiochemistry University of MünsterMünster 48149Germany

Bacterial biofilm-associated infection was one of the most serious threats to human health. However, effective drugs for drug-resistance bacteria or biofilms remain rarely reported. Here, we propose an innovative strategy to develop a multifunctional antimicrobial agent with broad-spectrum antibacterial activity by coupling photosensitizers (PSs) with antimicrobial peptides (AMPs). This strategy capitalizes on the ability of PSs to generate reactive oxygen species (ROS) and the membrane-targeting property of AMPs (KRWWKWIRW, a peptide screened by an artificial neural network), synergistically enhancing the antimicrobial activity. In addition, unlike conventional aggregation-caused quenching (ACQ) photosensitizers, aggregation-induced emission (AIE) PSs show stronger fluorescence emission in the aggregated state to help visualize the antibacterial mechanism. In vitro antibacterial experiments demonstrated the excellent killing effects of the developed agent against both Gram-positive (G^(+)) and Gram-negative (G^(–)) bacteria. The bacterial-aggregations induced ability enhanced the photoactivatable antibacterial activity against G^(–) bacteria. Notably, it exhibited a significant effect on destroying MRSA biofilms. Moreover, it also showed remarkable efficacy in treating wound infections in mice in vivo. This multifunctional antimicrobial agent holds significant potential in addressing the challenges posed by bacterial biofilm-associated infections and drug-resistant bacteria.

关键词： Photodynamic therapy Antimicrobial peptides Multidrug-resistant bacteria Aggregation-induced emission Anti-biofilm

Influences of chemical reactions on polysulfide reduction reaction process on promotor surface in Li-S batteries

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Nano Research 2024年第4期17卷 2712-2718页

作者： Yufeng luo Zhenhan fang Zixin Hong Shaorong Duan Haitao Liu Hengcai Wu Qunqing Li Yuegang Zhang Shoushan fan Wenhui Duan Jiaping Wang Tsinghua-Foxconn Nanotechnology Research Center Tsinghua UniversityBeijing 100084China Department of Physics Tsinghua UniversityBeijing 100084China Laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing 100088China Frontier Science Center for Quantum Information Tsinghua UniversityBeijing 100084China

Polar promotors have been proven effective in catalyzing the polysulfide(PS)reduction reaction(PSRR)process in lithium-sulfur(Li-S)***,the promotor surface tends to be poisoned due to the accumulation of insoluble discharging products of lithium disulfide(Li_(2)S_(2))and lithium sulfide(Li_(2)S)during Li-S battery ***,we investigate the detailed PSRR mechanism on the surface of manganese sulfides(MnS)as a representative promoter by performing in-situ Raman mapping *** catalytic ability of MnS enables thorough electrochemical reduction of PSs to Li_(2)S_(2) and Li_(2)S on the MnS *** generated Li_(2)S_(2) and Li_(2)S then adsorb the dissolved PSs via chemical reactions among sulfur species during the subsequent PSRR *** phenomenon mitigates promotor poisoning and continuously improves the reversible ***,the assembled Li-S cell demonstrates excellent electrochemical performance after introducing a conductive interlayer containing a thin piece of carbon nanotube film and MnS promotors.

关键词： promotors polysulfides chemical reactions catalytic ability in-situ Raman measurements