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Unique double-layer solid electrolyte interphase formed with fluorinated ether-based electrolytes for high-voltage lithium metal batteries

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Journal of Energy Chemistry 2024年第1期88卷 532-542,I0012页

作者： Ruo wang Jiawei Li Bing Han Qingrong wang Ruohong Ke Tong Zhang Xiaohu Ao Guangzhao Zhang Zhongbo {2. {2. Qian Fangfang Pan Iseult Lynch Jun wang Yonghong Deng Department of Materials Science&Engineering School of Innovation and EntrepreneurshipSouthern University of Science and TechnologyShenzhen 518055GuangdongChina school of Geography Earth and Environmental SciencesUniversity of BirminghamEdgbastonBirmingham B152TTUK Key Laboratory of Marine Environmental Corrosion and Bio-Fouling Institute of OceanologyChinese Academy of SciencesQingdao 266071ShandongChina Shenzhen CAPCHEM Technology Co. Ltd.Shenzhen 518118GuangdongChina CALB Group Co. Ltd.Changzhou 213200JiangsuChina

Li metal batteries using high-voltage layered oxides cathodes are of particular interest due to their high energy ***,they suffer from short lifespan and extreme safety concerns,which are attributed to the degradation of layered oxides and the decomposition of electrolyte at high voltage,as well as the high reactivity of metallic *** key is the development of stable electrolytes against both highvoltage cathodes and Li with the formation of robust interphase films on the ***,we report a highly fluorinated ether,1,1,1-trifluoro-2.[(2.2.2.trifluoroethoxy)methoxy]ethane(TTME),as a cosolvent,which not only functions as a diluent forming a localized high concentration electrolyte(LHCE),but also participates in the construction of the inner solvation *** TTME-based electrolyte is stable itself at high voltage and induces the formation of a unique double-layer solid electrolyte interphase(SEI)film,which is embodied as one layer rich in crystalline structural components for enhanced mechanical strength and another amorphous layer with a higher concentration of organic components for enhanced *** Li||Cu cells display a noticeably high Coulombic efficiency of 99.2.%after 300 cycles and Li symmetric cells maintain stable cycling more than 32.0 h at 0.5 mA/cm^(2. and 1.0m Ah/cm^(2..In addition,lithium metal cells using LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2. and Li CoO_(2. cathodes(both loadings~3.0 m Ah/cm^(2.)realize capacity retentions of>85%over 2.0 cycles with a charge cut-off voltage of 4.4 V and 90%for 170 cycles with a charge cut-off voltage of 4.5 V,*** study offers a bifunctional ether-based electrolyte solvent beneficial for high-voltage Li metal batteries.

关键词： Lithium metal batteries High-voltage layered oxides Fluorinated ether-based electrolytes Solid electrolyte interphase Cathode electrolyte interphase

Memristive feature and mechanism induced by laser-doping in defect-free 2. semiconductor materials

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Journal of Semiconductors 2024年第7期45卷 85-91页

作者： Xiaoshan Du shu wang Qiaoxuan Zhang Shengyao Chen Fengyou Yang Zhenzhou {2. Zhengwei Fan Lijun Ma Lei wang Lena Du Zhongchang wang Cong wang Bing Chen Qian {2. College of Electronic and Information Engineering Shandong University of Science and TechnologyQingdao 266590China National Center for Nanoscience and Technology&university of chinese Academy of Sciences Beijing 100190China Hebei university of Water Resources and Electric Engineering Electrical Automation Department Cangzhou 061001China The MOE Key Laboratory of Weak-Light Nonlinear Photonics and International Sino-Slovenian Join Re-search Center on Liquid Crystal Pho-tonics TEDA Institute of Applied Physics and School of PhysicsNankai UniversityTianjin 300457China College of mathematics and Physics Shandong Advanced Optoelectronic Materials and Technologies Engineering LaboratoryQingdao Uni-versity of Science and TechnologyQingdao 266061China Department of Physics Capital Normal UniversityBeijing 100048China Department of Advanced Materials and Computing International Iberian Nanotechnology Laboratory(INL)4715-330 BragaPortugal College of mathematics and Physics Beijing University of Chemical TechnologyBeijing 100029China

Memristors as non-volatile memory devices have gained numerous attentions owing to their advantages in storage,in-memory computing, synaptic applications, etc. In recent years, two-dimensional(2.) materials with moderate defects have been discovered to exist memristive feature. However, it is very difficult to obtain moderate defect degree in 2. materials, and studied on modulation means and mechanism becomes urgent and essential. In this work, we realized memristive feature with a bipolar switching and a configurable on/off ratio in a two-terminal MoS_(2. device(on/off ratio ~100), for the first time, from absent to present using laser-modulation to few-layer defect-free MoS_(2.(about 10 layers), and its retention time in both high resistance state and low resistance state can reach 2.10^(4) s. The mechanism of the laser-induced memristive feature has been cleared by dynamic Monte Carlo simulations and first-principles calculations. Furthermore, we verified the universality of the laser-modulation by investigating other 2. materials of TMDs. Our work will open a route to modulate and optimize the performance of 2. semiconductor memristive devices.

关键词： 2.-material memristor laser doping laser direct writing memristive mechanism

Inhibition of Defect-Induced Ice Nucleation, Propagation, and Adhesion by Bioinspired Self-Healing Anti-Icing Coatings

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Research 2024年第1期2023卷 237-246页

作者： shu Tian Ruiqi Li Xinmeng liu Jiancheng {2. Junyu Yu Sijia Xu Yunqing Tian Jing Yang Lei Zhang Department of Biochemical Engineering Frontier Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering(MOE)School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300350China Binzhou Institute of Technology Weiqiao-UCAS Science and Technology ParkBinzhou CityShandong Province 256606China

Anti-icing coatings on outdoor infrastructures inevitably suffer from mechanical injuries in numerous icing scenarios such as hailstorms,sandstorms,impacts of foreign objects,and icing–deicing ***,the mechanisms of surface-defect-induced icing are *** the defects,water molecules exhibit stronger adsorption and the heat transfer rate increases,accelerating the condensation of water vapor as well as ice nucleation and ***,the ice–defect interlocking structure increases the ice adhesion ***,a self-healing(at−2.℃)antifreeze-protein(AFP)-inspired anti-icing coating is *** coating is based on a design that mimics the ice-binding and non-ice-binding sites in *** enables the coating to markedly inhibit ice nucleation(nucleation temperature2..4℃),prevent ice propagation(propagation rate2./s),and reduce ice adhesion on the surface(adhesion strength2.℃,as a result of multiple dynamic bonds in its structure,to inhibit defect-induced icing *** healed coating sustains high anti-icing and deicing performance even under various extreme *** work reveals the in-depth mechanism of defect-induced ice formation as well as adhesion,and proposes a self-healing anti-icing coating for outdoor infrastructures.

关键词： coating defect clarified

Analysis of the local discontinuous Galerkin method for the drift-diffusion model of semiconductor devices

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Science china mathematics 2016年第1期59卷 115-140页

作者： liu yunxian {2. chi-wang school of mathematics Shandong University Division of Applied mathematics Brown University

We consider the drift-diffusion （DD） model of one dimensional semiconductor devices, which is a system involving not only first derivative convection terms but also second derivative diffusion terms and a coupled Poisson potential equation. Optimal error estimates are obtained for both the semi-discrete and fully discrete local discontinuous Galerkin （LDG） schemes with smooth solutions. In the fully discrete scheme, we couple the implicit-explicit （IMEX） time discretization with the LDG spatial diseretization, in order to allow larger time steps and to save computational cost. The main technical difficulty in the analysis is to treat the inter-element jump terms which arise from the discontinuous nature of the numerical method and the nonlinearity and coupling of the models. A simulation is also performed to validate the analysis.

关键词： local discontinuous Galerkin method semi-discrete implicit-explicit scheme error estimate semi- conductor

Modulating p-type doping of two-dimensional material palladium diselenide

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Nano Research 2024年第4期17卷 3232-3244页

作者： Jiali Yang Yu liu En-Yang wang Jinbo Pang Shirong Huang Thomas Gemming Jin{2.n Bi Alicja Bachmatiuk Hao Jia {2.-Xian Hu Chongyun Jiang Hong liu Gianaurelio Cuniberti Weijia Zhou Mark H Rümmeli Institute for Advanced Interdisciplinary Research(iAIR) University of JinanJinan 250022China Institute for Materials Chemistry Leibniz Institute for Solid State and Materials Research Dresden(IFW Dresden)20 Helmholtz StrasseDresden 01069Germany State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China College of Energy Soochow Institute for Energy and Materials Innovations Soochow UniversitySuzhou 215006China Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow UniversitySuzhou 215006China school of Integrated Circuits University of Chinese Academy of SciencesBeijing 101408China Institute of Microelectronics of Tianjin Binhai New Area Tianjin 300451China Institute of Microelectronics Chinese Academy of SciencesBeijing 100029China Lukasiewicz Research Network PORT Polish Center for Technology DevelopmentStablowicka 147Wroclaw 54-066Poland school of mathematics and Physics University of Science and Technology BeijingBeijing 100083China College of electronic information and optical engineering Nankai UniversityTianjin 300350China Centre of Polymer and Carbon Materials Polish Academy of SciencesM.Curie Sklodowskiej 34Zabrze 41-819Poland Center for Energy and Environmental Technologies VŠB-Technical University of Ostrava17.Listopadu 15Ostrava 70833Czech Republic State Key Laboratory of Crystal Materials Center of Bio&Micro/Nano Functional MaterialsShandong UniversityJinan 250100China Dresden Center for Computational Materials Science Technische Universität DresdenDresden 01062Germany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität DresdenDresden 01062Germany Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresden 01069Germany Center for Advancing Electronics Dresden Technische Universität DresdenDresden 01069Germany

The van der Waals heterostructures have evolved as novel materials for complementing the Si-based semiconductor ***-10 noble metal dichalcogenides(e.g.,PtS_(2.,PtSe_(2.,PdS_(2.,and PdSe_(2.)have been listed into two-dimensional(2.)materials toolkit to assemble van der Waals *** them,PdSe_(2. demonstrates advantages of high stability in air,high mobility,and wide tunable ***,the regulation of p-type doping of PdSe_(2. remains unsolved problem prior to fabricating p–n junction as a fundamental platform of semiconductor ***,a quantitative method for the controllable doping of PdSe_(2. is yet to be *** this study,the doping level of PdSe_(2. was correlated with the concentration of Lewis acids,for example,SnCl_(4),used for *** the transfer characteristics,the threshold voltage(the gate voltage corresponding to the minimum drain current)increased after SnCl_(4) soaking ***_(2. transistors were soaked in SnCl_(4) solutions with five different *** threshold voltages from the as-obtained transfer curves were extracted for linear fitting to the threshold voltage versus doping concentration correlation *** study provides in-depth insights into the controllable p-type doping of PdSe_(2..It may also push forward the research of the regulation of conductivity behaviors of 2. materials.

关键词： two-dimensional(2.)materials Lewis acid treatment p-type doping field-effect transistors transfer characteristic

Photon counting technique as a potential tool in micro-defect detection of epoxy insulation pull rod in gas-insulated switchgears

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High Voltage 2024年第2期9卷 267-274页

作者： Xianhao Fan shu Niu Hanhua Luo Jizhong Liang Fang liu Wenqiang Li Weidong liu Wensheng Gao Yulong Huang Chuanyang Li Jinliang He school of Electrical Engineering Tsinghua UniversityBeijingChina Electric Power Research Institute Shangxi Power Grid CorporationTaiyuanShanxiChina shandong Taikai Electrical Insulation Co. Ltd.TaianShandongChina

The micro-defects in epoxy-based insulation materials generate a local high electric field which results in continuous degradation,seriously endangering the insulation system of gas-insulated switchgears.A highly sensitive detection technique is reported for micro-defects of insulation pull rods based on the photon counting(PC)*** re-sults demonstrated that for an epoxy-based insulation pull rod,the photons released during electroluminescence and ionisation at 2.kV,which is less than the partial discharge inception voltage,can be clearly *** findings presented a strong correlation between photon counts and defect *** has been conducted to elucidate the mechanism behind defect-induced PC,employing the amplification of ionising luminescence through electric field distortion induced by micro defects and the augmentation of electroluminescence through the aggregation of trap *** this regard,the authors verified that PC can serve as a potential tool in the detection of micro-insulation defects,which also has huge potential in online insulation condition monitoring.

关键词： technique. insulation defect

The IDD Transcription Factors:Their Functions in Plant Development and Environmental Response

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Phyton-International Journal of Experimental Botany 2024年第1期93卷 63-79页

作者： Jing liu Defeng shu Zilong Tan Mei Ma Huanhuan Yang Ning Guo Shipeng Li Dayong Cui school of Life Sciences Qilu Normal UniversityJinan250200China school of Life Sciences Shandong Normal UniversityJinan250014China

INDETERMINATE-DOMAIN proteins(IDDs)are a plant-specific transcription factor family characterized by a conserved ID domain with four zinc finger *** studies have demonstrated that IDDs coordinate a diversity of physiological processes and functions in plant growth and development,including floral transition,plant architecture,seed and root development,and hormone *** this review,we especially summarized the latest knowledge on the functions and working models of IDD members in Arabidopsis,rice,and maize,particularly focusing on their role in the regulatory network of biotic and abiotic environmental responses,such as gravity,temperature,water,and *** these mechanisms underlying the function of IDD proteins in these processes is important for improving crop yields by manipulating their ***,the review offers valuable insights into the functions and mechanisms of IDD proteins in plants,providing a foundation for further research and potential applications in agriculture.

关键词： INDETERMINATE DOMAIN flowering time root development shoot gravitropism plant immunity hormonal signaling environmental responses

Gamma/Hadron Separation Method for the HADAR Experiment

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Research in Astronomy and Astrophysics 2024年第3期24卷 70-74页

作者： Yang-Zhao Ren Tian-Lu Chen You-Liang Feng Dan-Zeng Luo-Bu Yi-Qing Guo Cheng liu Qi Gao Mao-Yuan liu Xiang-Li Qian Ya-Ping {2. Zi-Hao Zhang Xin-Long Li Qing-Yuan Hou Heng-Jiao liu Qing-Qian Zhou Shan-Jie shu The Key Laboratory of Cosmic Rays(Tibet university) Ministry of EducationLhasa 850000China Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of Sciences university of chinese Academy of Sciences school of Intelligent Engineering Shandong Management University

Ground-based arrays of imaging atmospheric Cherenkov telescopes(IACTs)are the most sensitiveγ-ray detectors for energies of approximately 100 Ge V and *** such IACT is the High Altitude Detection of Astronomical Radiation(HADAR)experiment,which uses a large aperture refractive water lens system to capture atmospheric Cherenkov photons(i.e.,the imaging atmospheric Cherenkov technique).The telescope array has a low threshold energy and large field of view,and can continuously scan the area of the sky being observed,which is conducive to monitoring and promptly responding to transient *** process ofγ-hadron separation is essential in very-high-energy(>30 Ge V)γ-ray astronomy and is a key factor for the successful utilization of *** this study,Monte Carlo simulations were carried out to model the response of cosmic rays within the HADAR *** analyzing the Hillas parameters and the distance between the event core and the telescope,the distinction between air showers initiated byγ-rays and those initiated by cosmic rays was ***,a Quality Factor was introduced to assess the telescope’s ability to suppress the background and to provide a more effective characterization of its performance.

关键词： astroparticle physics-telescopes-methods data analysis

Genetic diversity of the endangered species Rosa rugosa *** china and implications for conservation strategies

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Journal of Systematics and Evolution 2009年第6期47卷 515-524页

作者： ~1Ji-Hong YANG ~1shu-Ping ZHANG ~2.ian liu ~1Wen ZHAI ~(1,2.Ren-Qing {2.~* 1(school of Life Sciences,{2. university,jinan 2.0100,china) 2.Institute of Environment Research,{2. university,jinan 2.0100,china) (Institute of Environment Research Shandong University Jinan 250100 China)

Rosa rugosa *** one of the dominant and important shrub species in estuary dunes and shingle beaches of northern ***,its area of distribution,the number of populations,and the size of each population have decreased rapidly in the past two decades because of habitat degradation and *** amplified polymorphic DNA markers were used to determine the genetic diversity of four remaining large natural populations of *** and to discuss an effective conservation strategy for this endangered species in *** genetic variations were detected in *** populations in *** mean percentage of polymorphic loci(P%) within four local populations was 57.99%,with the P%of the total population being 75.30%.Mean Shannon’s information index(H0) was 0.2.2.,whereas total H0was *** genetic differentiation among populations was 0.1878, which indicates that most genetic diversity occurs within *** Tumenjiang(TMJ) showed the highest genetic diversity(P%= 66.2.%;H0= 0.3117) and contained two exclusive *** Changshandao (CSD) showed higher genetic diversity(P%= 59.04%;H0= 0.3065).Populations TMJ and CSD contained 95.33% and 99.33%,respectively,of loci with moderate to high frequency(P>0.05) of the total *** results indicate that populations TMJ and CSD should be given priority for in situ conservation and regarded as seed or propagule sources for ex situ *** results of the present study also suggest that *** in china has become endangered as a result of human actions rather than genetic depression of populations;thus,human interference should be absolutely forbidden in *** habitats.

关键词： china genetic diversity in situ conservation random amplified polymorphic DNA(RAPD) Rosa rugosa