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Heavy metal stress strengthens the stability and complexity of microbial molecular ecological networks in Sanyang wetland sediments

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Journal of Oceanology and Limnology 2025年第1期43卷 103-118页

作者： Shengwei WU Huixi ZOU Nan LI Xiufeng yan Wen liu College of Life and Environmental Science Wenzhou UniversityWenzhou 325035China Institute for Eco-environmental Research of Sanyang Wetland Wenzhou UniversityWenzhou 325035China Key Laboratory of Soil Contamination Bioremediation of Zhejiang Province School of Environmental&Resource SciencesZhejiang Agriculture and Forestry UniversityHangzhou 311300China

Pollution from heavy metals(HMs)(Cd,As,Cr,and Ni,etc.)has become a serious environmental issue in urban wetland ecosystems with more and more *** studies conducted in agricultural soils,rivers,and lakes demonstrated that microbial communities exhibit a response to HM ***,little is known about the response of microbial communities to HM pollution in urban wetland *** examined how heavy metals affect the stability of the microbial networks in the sediments of Sanyang wetland,Wenzhou,*** environmental parameters,including HMs,TC(total carbon),TN(total nitrogen),TP(total phosphorus),S,and pH,varied profoundly between moderately and heavily polluted areas in shaping microbial ***,the microbial community composition in moderately polluted sites correlated significantly(P<0.05)with Ni,Cu,Cd and TP,whereas in heavily polluted sites,they correlated significantly with Cd,TN,TP,and *** show that the heavily polluted sites demonstrated more intricate and more stable microbial networks than those of the moderately polluted *** heavily polluted sites exhibited higher values for various network parameters including total nodes,total links,average degree,average clustering coefficient,connectance,relative modularity,robustness,and ***,the structural equation modeling analysis demonstrated a positive correlation between the stability of microbial networks and Cd,TN,TP,and S in heavily polluted ***,in moderately polluted sites,the correlation was positively linked to Cd,Ni,and sediment *** implies that Cd could potentially play a crucial role in affecting the stability of microbial *** study shall enhance our comprehension of microbial co-occurrence patterns in urban wetland ecosystems and offer insights into the ways in which microbial communities respond to environmental factors in varying levels of HM pollution.

关键词： heavy metal(HM) urban wetland microbial networks network stability

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Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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Journal of Energy Chemistry 2025年第1期100卷 730-738页

作者： Peng zheng Wang Zhou Ying Mo Biao zheng Miaomiao Han Qin Zhong Wenwen yang Peng Gao Lezhi yang Jilei liu College of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean EnergyHunan Province Key Laboratory for Advanced Carbon Materials and Applied TechnologyHunan UniversityChangsha 410082HunanChina Greater Bay Area Institute for Innovation Hunan UniversityGuangzhou 511300GuangdongChina Changsha Research Institute of Mining&Metallurgy Co. LTD.Changsha 410017HunanChina

Hard carbon (HC) has been considered as promising anode material for sodium-ion batteries (SIBs).The optimization of hard carbon’s microstructure and solid electrolyte interface (SEI) property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectroscopy/electrochemical impedance spectroscopy (FTIR/EIS) and X-ray photoelectron spectroscopy (XPS) analysis demonstrate the presence of more BC3and less B–C–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping content exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： Hard carbon Sodium-ion batteries Boron doping Pore structure Electrode/electrolyte interphases

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Shenlian Extract Protects against Ultrafine Particulate Matter-Aggravated Myocardial Ischemic Injury by Inhibiting Inflammation and Cell Apoptosis

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Biomedical and Environmental Sciences 2025年第2期38卷 206-218页

作者： Shuiqing Qu yan Liang Shuoqiu deng Yu Li Yue Dai Chengcheng liu Tuo liu Luqi Wang Lina Chen Yujie Li Institute of Chinese Materia Medica China Academy of Chinese Medical SciencesBeijing 100700China Artemisinin Research Center China Academy of Chinese Medical SciencesBeijing 100700China

Objective Emerging evidence suggests that exposure to ultrafine particulate matter(UPM,aerodynamic diameter<0.1μm)is associated with adverse cardiovascular *** studies have found that Shenlian(SL)extract possesses anti-inflammatory and antiapoptotic properties and has a promising protective effect at all stages of the atherosclerotic disease *** this study,we aimed to investigated whether SL improves UPM-aggravated myocardial ischemic injury by inhibiting inflammation and cell *** We established a mouse model of MI+*** measurement,measurement of myocardialinfarct size,biochemical analysis,enzyme-linked immunosorbent assay(ELISA),histopathological analysis,Transferase dUTP Nick End Labeling(TUNEL),Western blotting(WB),Polymerase Chain Reaction(PCR)and so on were used to explore the anti-inflammatory and antiapoptotic effects of SL in vivo and in *** SL treatment can attenuate UPM-induced cardiac dysfunction by improving left ventricular ejection fraction,fractional shortening,and decreasing cardiac infarction *** significantly reduced the levels of myocardial enzymes and attenuated UPM-induced morphological ***,SL significantly reduced expression levels of the inflammatory cytokines IL-6,TNF-α,and *** further increased the infiltration of macrophages in myocardial tissue,whereas SL intervention reversed this *** also triggered myocardial apoptosis,which was markedly attenuated by SL *** results of in vitro experiments revealed that SL prevented cell damage caused by exposure to UPM combined with hypoxia by reducing the expression of the inflammatory factor NF-κB and inhibiting apoptosis in H9c2 *** Overall,both in vivo and in vitro experiments demonstrated that SL attenuated UPMaggravated myocardial ischemic injury by inhibiting inflammation and cell *** mechanisms were related to the downregulation of macrophages infiltrating heart tiss

关键词： Ultrafine particulate matter Shenlian extract Inflammation Apoptosis Macrophage

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Boosting cationic and anionic redox activity of Li-rich layered oxide cathodes via Li/Ni disordered regulation

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Journal of Energy Chemistry 2025年第1期100卷 533-543页

作者： Zewen liu Zhen Wu Hao Wang Xudong Zhang Yuanzhen Chen Yongning liu Shengwu Guo Shenghua Chen yanli Nan yan liu State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina School of Materials Science and Engineering Xi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina Hefei Advanced Computing Center Operation Management Corp Ltd Hefei 230088AnhuiChina Network Information Center Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Lithium-rich layered oxides (LLOs) are increasingly recognized as promising cathode materials for nextgeneration high-energy-density lithium-ion batteries (LIBs).However,they suffer from voltage decay and low initial Coulombic efficiency (ICE) due to severe structural degradation caused by irreversible O ***,we introduce a three-in-one strategy of increasing Ni and Mn content,along with Li/Ni disordering and TM–O covalency regulation to boost cationic and anionic redox activity simultaneously and thus enhance the electrochemical activity of *** target material,Li_(1.2)Ni_(0.168)Mn_(0.558)Co_(0.074)O_(2)(L1),exhibits an improved ICE of 87.2%and specific capacity of 293.2 mA h g^(-1)and minimal voltage decay of less than 0.53 m V cycle-1over 300 cycles at 1C,compared to Li_(1.2)Ni_(0.13)Mn_(0.54)Co_(0.13)O_(2)(Ls)(274.4 mA h g^(-1)for initial capacity,73.8%for ICE and voltage decay of 0.84 mV/cycle over 300 cycles at 1C).Theoretical calculations reveal that the density of states (DOS) area near the Fermi energy level for L1 is larger than that of Ls,indicating higher anionic and cationic redox reactivity than ***,L1 exhibits increased O-vacancy formation energy due to higher Li/Ni disordering of 4.76%(quantified by X-ray diffraction Rietveld refinement) and enhanced TM–O covalency,making lattice O release more difficult and thus improving electrochemical *** increased Li/Ni disordering also leads to more Ni^(2+)presence in the Li layer,which acts as a pillar during Li+de-embedding,improving structural *** research not only presents a viable approach to designing low-Co LLOs with enhanced capacity and ICE but also contributes significantly to the fundamental understanding of structural regulation in high-performance LIB cathodes.

关键词： Low-Co Li-rich layered oxides Li/Ni disordering TM-O covalency Cationic and anionic redox activity

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Polarization variable terahertz metasurface along the propagation path

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Fundamental Research 2025年第1期5卷 124-131页

作者： Jitao Li Jingyu liu Zhen Yue Jie Li Chenglong zheng Fan yang Hui Li Yating Zhang yan Zhang Jianquan Yao Key Laboratory of Opto-Electronics Information Technology(Tianjin University) Ministry of EducationSchool of Precision Instruments and Opto-Electronics EngineeringTianjin UniversityTianjin 300072China Beijing Key Laboratory for Metamaterials and Devices Key Laboratory of Terahertz OptoelectronicsMinistry of Educationand Beijing Advanced Innovation Center for Imaging TechnologyDepartment of PhysicsCapital Normal UniversityBeijing 100048China

Conventional metasurfaces for terahertz polarization are limited to performing lateral(in the x-y plane)polarization control of the output *** such cases,the polarization state remains unchanged in each output plane along the propagation ***,we propose a terahertz polarization metasurface that operates longitudinally(i.e.,along the z-axis direction of propagation),which modifies the polarization state of each output plane throughout the propagation *** designed metasurface can control the phase delays of the left-handed and right-handed circularly polarized(LCP and RCP)components of the incident terahertz *** enables the LCP beam and RCP beam to converge to the z-axis through distinct paths,creating a Bessel *** proposed design achieved a linearly polarized terahertz wave including both LCP and RCP components with a precise phase differenceΔφat each point within a certain range along the ***Δφvaries as the propagation distance,resulting in a rotated linearly polarized output wave along the propagation path,while the rotation angle ranges from 0 toπ.Based on the variable property of longitudinal polarization,we propose an application concept of dielectric refractive index sensing,in which an additional medium is placed in the terahertz propagation path and the unknown refractive index is determined by detecting the rotation angle of the output polarization ***,the device might find potential applications in variable media excitation,terahertz communication,and terahertz radar ranging.

关键词： Terahertz Metasurface Propagation path Polarization manipulation Longitudinal polarization Refractive index sensing

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Secure Fine-Grained Multi-Keyword Ciphertext Search Supporting Cloud-Edge-End Collaboration in IoT

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Chinese Journal of Electronics 2025年第1期34卷 266-281页

作者： Kaifa zheng Ziyu Zhou Jianwei liu Beiyuan Yu School of Cyber Science and Technology Beihang University

The massive terminals access the Internet of things(IoT) through edge nodes, bringing forth new security and privacy challenges in ciphertext search and data sharing. Meanwhile, existing ciphertext search schemes often overlook lightweight computing paradigms and pay little attention to the search requirements of multiple data owners(DOs)/data users(DUs). To address these issues, we propose a secure fine-grained multi-keyword ciphertext search scheme with cloud-edge-end collaboration computing(SFMS-CC). This SFMS-CC scheme focuses on the efficiency of end users and employs a cloud-edge-end collaborative computing paradigm, effectively offloading the incremental overhead from terminals and achieving low-cost constant overhead for the first time on the DO/DU side. Furthermore, based on public-key cryptography, a ciphertext search framework supporting multi-keyword is presented systematically. Each user is assigned an exclusive search Tok to enhance the user experience. Additionally, by integrating attribute-based encryption, a multi-DOs/multi-DUs model is constructed, seamlessly embedding entity private keys and public keys into encryption, search, decryption, and other steps, ensuring high privacy and security of this scheme. Security analysis demonstrates that the SFMS-CC scheme withstands choose plaintext attack, providing privacy-preserving for outsourced data and user information. Simulation results indicate that the SFMS-CC scheme is efficient and feasible in practice.

关键词： Cloud computing Privacy Simulation Scalability Collaboration Public key cryptography User experience Encryption Internet of Things Standards

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A comprehensive review of deactivation and modification of selective catalytic reaction catalysts installed in cement kilns

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Journal of Environmental Sciences 2025年第2期148卷 451-467页

作者： yang zheng Yi Xing Guoliang Li Jiajia Gao Rui Li Qi liu Tao Yue School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

After the ultralow emission transformation of coal-fired power plants,cement production became China’s leading industrial emission source of nitrogen *** gas dust contents at the outlet of cement kiln preheaters were as high as 80-100 g/m^(3),and the calcium oxide content in the dust exceeded 60%.Commercial V_(2)O_(5)(-WO3)/TiO_(2) catalysts suitable for coal-fired flue gas suffer from alkaline earth metal Ca poisoning of cement kiln flue *** studies have also identified the poisoning of cement kiln selective catalytic reaction(SCR)catalysts by the heavy metals lead and *** of the poisoning process is the primary basis for analyzing the catalytic *** review summarizes and analyzes the SCR catalytic mechanism and chronicles the research progress concerning this poisoning *** on the catalytic and toxification mechanisms,it can be inferred that improving the anti-poisoning performance of a catalyst enhances its acidity,surface redox performance-active catalytic sites,and shell layer *** data provide support in guiding engineering practice and reducing operating costs of SCR ***,future research directions for SCR denitrification catalysts in the cement industry are *** study provides critical support for the development and optimization of poisoning-resistant SCR denitrification catalysts.

关键词： Cement Flue Gas NH_(3)-SCR CaO Poisoning Mechanism Anti-poisoning Modification

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Supramolecular Ion Channel with Controlled K+/Na+Transport Behaviors

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Chemical Research in Chinese Universities 2025年第1期41卷 95-100页

作者： HE Lei LUO Yichen ZHANG yang yan Tengfei liu Junqiu College of Material Chemistry and Chemical EngineeringKey Laboratory of Organosilicon Chemistry and Material Technology of Ministry of EducationKey Laboratory of Organosilicon Material Technology of Zhejiang ProvinceHangzhou Normal UniversityHangzhou310036P.R.China

Dysfunction of ion channels,often caused by mutations in natural proteins,can lead to various *** artificial analogs have shown great promise to substitute the abnormal ***,we report a supramolecular potassium channel that forms through the self-assembly of pyrene-crown ether conjugated by intermolecularπ-π*** self-assembled dimer of this channel was optimized and calculated to have a binding energy of−27.4 kcal/mol(1 kcal=4.18 kJ).Evidence for the formation of an active ion channel by PC5 was confirmed using a planar lipid bilayer(BLM)workstation,while no such activity was observed for *** K+/Na+selectivity was reversed in the reduced form,R-PC5,due to the elimination of the planar structure of PC5,resulting in R-PC5 functioning as a Na+***,incorporating the pyrene group facilitates imaging in living cells,providing a potentially viable method for investigating the behaviors of artificial ion channels in living systems.

关键词： Crown ether Pyrene Ion transport Self-assembly

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Magnetically-responsive phase change thermal storage materials:Mechanisms,advances,and beyond

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Journal of Energy Chemistry 2025年第2期101卷 485-510页

作者： yan Gao yang Li Jinjie Lin Panpan liu Xiao Chen Ge Wang Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory of Function Materials for Molecule & Structure Construction School of Materials Science and Engineering University of Science and Technology Beijing School of Physics and Astronomy Beijing Normal University Shunde Graduate School University of Science and Technology Beijing

Rapid advances in thermal management technology and the increasing need for multi-energy conversion have placed stringent energy efficiency requirements on next-generation shape-stable composite phase change materials(PCMs).Magnetically-responsive phase change thermal storage materials are considered an emerging concept for energy storage systems,enabling PCMs to perform unprecedented functions(such as green energy utilization,magnetic thermotherapy,drug release,etc.).The combination of multifunctional magnetic nanomaterials and PCMs is a milestone in the creation of advanced multifunctional composite ***,a timely and comprehensive review of composite PCMs based on magnetic nanoparticle modification is still ***,we furnish an exhaustive exposition elucidating the cutting-edge advancements in magnetically responsive composite *** delve deeply into the multifarious roles assumed by distinct nanoparticles within composite PCMs of varying dimensions,meticulously scrutinizing the intricate interplay between their architectures and thermophysical ***,we prognosticate future research trajectories,delineate alternative stratagems,and illuminate prospective *** review is intended to stimulate broader academic interest in interdisciplinary fields and provide valuable insights into the development of next-generation magnetically-responsive composite PCMs.

关键词： Magnetic nanoparticles Magnetic-thermal conversion Phase change materials Response mechanism Thermal energy storage

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Revealing and predicting the long-term biomechanical response of orthokeratology by developing a patient-specific computational model

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Science China(Physics,Mechanics & Astronomy) 2025年第1期68卷 152-164页

作者： Yifeng Li Zhuoran yang Ziming yan Huibin Shi Zhanli liu Kaijie Wang Department of Engineering Mechanics School of Aerospace EngineeringTsinghua UniversityBeijing 100084China Beijing Tongren Eye Center Beijing Tongren HospitalCapital Medical UniversityBeijing Ophthalmology&Visual Sciences Key LabBeijing 100730China

Orthokeratology(OK)is widely used for effective myopia correction and ***,the incomplete understanding of its biomechanical mechanisms makes OK lens fitting rely heavily on clinician judgment,complicating accurate predictions of treatment *** this paper,we performed clinical experiments and numerical analysis to study corneal deformation modes and long-term changes in central corneal *** experiments were conducted on 194 Chinese myopic patients under OK treatment for 3 *** on the experimental data,a patient-specific computational biomechanical model for OK was established and ***,the anisotropic mechanical properties of the cornea were incorporated into the model to describe the significant difference between its shear modulus(29.5 kPa)and tensile modulus(768.4 kPa).Additionally,a viscohyperelastic material model with a prolonged corneal relaxation time of 5.6 h was developed to capture the long-term deformation *** results show that corneal thickness reduction in OK is primarily due to out-of-plane shear deformation,influenced by the cornea’s low shear *** the extended corneal relaxation time is crucial for predicting long-term biomechanical *** computational model effectively captures long-term changes in central corneal thickness,potentially improving OK lens fitting accuracy.

关键词： orthokeratology computational biomechanical model long-term viscoelasticity myopia correction

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