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Rational modulation of fluorophosphate cathode by anionic groups to reduce the polarization behavior for fast-charging sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 509-521页

作者： Xinyuan Wang Fan zhang Xingyu Zhou Qian Wang Changyu liu Yangyang liu Hui Wang Xiaojie liu Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education College of Chemistry & Materials Science Northwest University

Na3V2（PO4）2O2F （VP） is recognized as a promising cathode material for sodium-ion batteries due to its stable structural framework and high specific *** functional theory （DFT） and finite element simulations show that incorporating SO42-into VP decreases its band gap,lowers the migration energy barrier,and ensures a uniform Na+concentration gradient and stress distribution during charge and discharge ***,the average Na+diffusion coefficient of Na3V2（PO4）1.95（SO4）0.05O2F（VPS-1） is roughly double that of VP,leading to enhanced rate capability (80 C,75.5 mAh g-1) and cycling stability (111.0 mAh g-1capacity after 1000 cycles at 10 C current density) for ***-1 exhibits outstanding fast-charging capabilities,achieving an 80%state of charge in just 8.1 *** assembled VPS-1//SbSn/NPC full cell demonstrated stable cycling over 200 cycles at a high 5 C current,maintaining an average coulombic efficiency of 95.35%.

关键词： Anionic group modulation Polarization behavior Fast-charging Sodium-ion battery Fluorophosphate Cathode

Broadband and perfect terahertz absorber based on multilayer metamaterial with cross-ring patterned structures

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Optoelectronics Letters 2025年第1期21卷 1-6页

作者： wen Jin liu Zhanzhi WU Zhengwei PAN Yu zhang Ying School of Science Xi'an Shiyou University Shaanxi Key Laboratory of Measurement and Control Technology for Oil and Gas Wells

Broadband and perfect terahertz absorber based on multilayer metamaterial using cross-ring patterned structures is proposed and investigated. The structure of the absorber is double absorption layers consisting of a chromium cross ring and eight isosceles right triangles. The unique structure of the double absorbing layers excites the electric dipole multimode resonance, giving rise to high absorption performance. Meanwhile, the influence of construal parameters on absorber behavior is also discussed. The numerical results show that the absorption achieves over 90% ranging from 2.45 THz to 6.25 THz and 99% absorption in the range of 3.7—5.3 THz. The realization of broadband and perfect absorber is described using the impedance matching principle. It is obviously found that the absorber is insensitive to the high angle of incidence for both transverse electric(TE) and transverse magnetic(TM) polarizations. Compared with the former reports, this absorber has remarkable improved absorption efficiency and smaller period. The terahertz absorber may be found applications in the fields of energy capture and thermal detection.

关键词： Metamaterials

Remote Sensing CO,CO_2 in Vehicle Emissions Based on TDLAS

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光机电信息 2007年第5期24卷 25-30页

作者： WANG Tie-dong liu wen-qing zhang Yu-jun liu Jian-guo DONG Feng-zhong WANG Min WANG Xiao-mei XU Min Key Laboratory of Environment Optics and Technology Anhui Institute of Optics and Fine Mechanics Chinese Academy of SciencesHefei 230031China

Knowing the quantity of pollutants that the vehicle fleet is emitting to the air has become a vital problem in almost every major city in China. Finding and fixing gross polluters is therefore very important to control the urban air quality and protect the human health and the environment. Remote sensing is an important advance in the technology of on-road vehicle emissions testing because it is fast, mobile, and unobtrusive. This on-road vehicle emissions remote system is designed to measure the carbon monoxide, carbon dioxide and opacity from the vehicles's tailpipe based on the Tunable Diode Laser Absorption Spectroscopy (TDLAS). There are several advantages of this system such as compact design and easy of use. The measurement principle and optical layout of the instrument has been described in this paper. Field testing at Beijing and Hefei were conducted over one year, more than 6 000 vehicles were tested. This vehicle emissions remote system has been shown to be able to measure CO,CO2 and opacity from individual at highway speeds. In parallel, the plate license, speed, acceleration and length of vehicle are recognised by computer so that the owners of vehicles exceeding the permissible level of emissions can be identified.

关键词：车辆排放一氧化碳排放二氧化碳排放遥感 TDLAS

Visualization of the protective role of estrogen against female liver fibrosis via an ER viscosity NIR fluorescent probe

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Science China Chemistry 2025年第1期 360-368页

作者： Zheng liu Changyu zhang Zipeng Li Wanying Ma Jia liu Xiang Xia Ning Xu wen Sun Jianjun Du Jiangli Fan Xiaojun Peng State Key Laboratory of Fine Chemicals Dalian University of Technology Ningbo Institute of Dalian University of Technology

Endoplasmic reticulum(ER) viscosity has emerged as a new potential biomarker for hepatic fibrosis(HF). Herein, we report the first ER-targeting viscosity-responsive near-infrared(NIR) fluorescent probe HBT-PP for investigations of HF *** twisted intramolecular charge transfer(TICT) and the excited state intramolecular proton transfer(ESIPT) are combined to endow HBT-PP with the selective response towards viscosity(～62-fold) and a super large stokes shift(～320 nm). HBT-PP mainly targets organelle ER and is able to image the drug-or alcohol-induced viscosity elevation in living cells. Significantly,HBT-PP was successfully applied to visualize the gender difference in HF and the protective role of estrogen in restraining HF progression. Of note, after 10 min of stain with HBT-PP, HF lesions showed a stage-based response, indicating the potential of this probe in fast and early diagnosis of HF. These results clearly demonstrated the promising application of HBT-PP as a new tool for exploring ER viscosity-involved physiological and pathological processes.

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3维数据的置信区间及异常数据的修复

计算机集成制造系统 2005年第4期11卷 597-600页

作者：刘章文任天怡古天祥电子科技大学自动化工程学院四川成都610054 中国工程物理研究院应用电子学研究所四川绵阳621900

3维测量是逆向工程设计的数据来源,为此提出了用弦矢量法确定3 维数据的置信区间,并对异常数据进行修复。利用3维曲面上某点相邻的点,求出该点的两个互相垂直的弦矢量,由此,曲面上的一个矩形区域的数据就构成了两个弦矢量阵列。对不等... 详细信息

3维测量是逆向工程设计的数据来源,为此提出了用弦矢量法确定3 维数据的置信区间,并对异常数据进行修复。利用3维曲面上某点相邻的点,求出该点的两个互相垂直的弦矢量,由此,曲面上的一个矩形区域的数据就构成了两个弦矢量阵列。对不等间距的弦矢量阵列进行了校正。对两个等效弦矢量阵列进行概率统计分析,即可确定该测量数据的置信区间。根据该置信区间对异常数据进行了修正。最后对两个目标实物的测量数据进行了分析,结果表明该方法对异常数据的修复是非常有效的。

关键词：置信区间弦矢量异常数据 3维测量

基于31个省份事件史分析的河长制创新与扩散的影响因素

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中国环境科学 2021年第6期41卷 2956-2963页

作者：梅正午刘文璋孙玉栋中国人民大学公共管理学院北京100872

利用事件史分析(EHA)模型对河长制政策2010~2016年在省级层面的扩散进行实证研究,结果表明:水污染越是严重的地区,越倾向于采纳河长制,平均而言,人均水污染排放量每增加一个单位,一个省份河长制政策得到采纳的优势会增加30.2%;财政自给... 详细信息

利用事件史分析(EHA)模型对河长制政策2010~2016年在省级层面的扩散进行实证研究,结果表明:水污染越是严重的地区,越倾向于采纳河长制,平均而言,人均水污染排放量每增加一个单位,一个省份河长制政策得到采纳的优势会增加30.2%;财政自给率在水污染严重程度与河长制采纳之间具有负向调节效应,即面临严重的环境污染,财政自给率高的省份不太倾向于采纳河长制,而财政自给率低的省份则更加倾向于采纳河长制;河长制政策采纳具有明显的政治周期性,在党代会召开的当年,省政府更加倾向于采纳河长制;邻近省份的政策采纳并不会对河长制的横向扩散产生显著影响.

关键词：河长制创新扩散事件史分析

基于声全息法的水下复杂圆柱壳体远场辐射声场计算及试验验证

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船舶力学 2017年第Z1期21卷 638-645页

作者：刘文章严斌吴文伟中国船舶科学研究中心船舶振动噪声重点实验室江苏无锡214082

针对水下圆柱壳体结构,采用声全息技术建立了由近场声预报远场辐射噪声的方法.在波数域内对近场声与远场辐射噪声的关系展开分析,建立了结合近场声信息提高远场辐射噪声特征分析及评估精度的工程实用化方法.通过加肋圆柱壳的算例验证了... 详细信息

针对水下圆柱壳体结构,采用声全息技术建立了由近场声预报远场辐射噪声的方法.在波数域内对近场声与远场辐射噪声的关系展开分析,建立了结合近场声信息提高远场辐射噪声特征分析及评估精度的工程实用化方法.通过加肋圆柱壳的算例验证了方法的正确性,为方法的实际应用提供理论指导.结合模型试验的结果对方法进行了进一步的对比验证.

关键词：声全息法圆柱壳体水下辐射噪声远场辐射噪声试验验证

Ammonia pyrolysis oxidation excited by nanosecond pulsed discharge:Global/fluid models hybrid solution

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Journal of Energy Chemistry 2025年第1期100卷 385-396页

作者： Mingming zhang Hanyu Wu Qi Chen Jiaxin Yang Bonan liu School of Mechanical Electronic and Control Engineering Beijing Jiaotong University China University of Petroleum

The kinetic characteristics of plasma-assisted oxidative pyrolysis of ammonia are studied by using the global/fluid models hybrid solution ***,the stable products of plasma-assisted oxidative pyrolysis of ammonia are *** results show that the consumption of NH3/O2and the production of N2/H2change linearly with the increase of voltage,which indicates the decoupling of nonequilibrium molecular excitation and oxidative pyrolysis of ammonia at low ***,the detailed reaction kinetics mechanism of ammonia oxidative pyrolysis stimulated by a nanosecond pulse voltage at low pressure and room temperature is *** on the reaction path analysis,the simplified mechanism is *** detailed and simplified mechanism simulation results are compared with experimental data to verify the accuracy of the simplified ***,based on the simplified mechanism,the fluid model of ammonia oxidative pyrolysis stimulated by the nanosecond pulse plasma is established to study the pre-sheath/sheath behavior and the resultant consumption and formation of key *** results show that the generation,development,and propagation of the pre-sheath have a great influence on the formation and consumption of *** consumption of NH3by the cathode pre-sheath is greater than that by the anode pre-sheath,but the opposite is true for OH and O（1S）.However,within the sheath,almost all reactions do not ***,by changing the parameters of nanosecond pulse power supply voltage,it is found that the electron number density,electron current density,and applied peak voltages are not the direct reasons for the structural changes of the sheath and ***,the discharge interval has little effect on the sheath structure and gas mixture *** research results of this paper not only help to understand the kinetic promotion of non-equilibrium excitation in the process of oxidative pyrolysis but also help to explore th

关键词： Nanosecond pulsed discharge Ammonia Oxidative pyrolysis Fluid model Global model

The Study on Breast Shape by Age Group Based on 3D Anthropometric Survey

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The Study on Breast Shape by Age Group Based on 3D Anthropom...